• Search Research Projects
  • Search Researchers
  • How to Use
  1. Back to previous page

Low-temperature sintering of alumina aiming for novel LTCC devices featuring high thermal conductivity and its application to non-shrinkage firing technology

Research Project

Project/Area Number 15K06514
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Material processing/Microstructural control engineering
Research InstitutionUbe National College of Technology

Principal Investigator

Shigeno Koichi  宇部工業高等専門学校, 物質工学科, 准教授 (60707131)

Co-Investigator(Kenkyū-buntansha) 吉田 政司  宇部工業高等専門学校, 機械工学科, 教授 (10370024)
徳永 仁夫  鹿児島工業高等専門学校, 機械工学科, 准教授 (70435460)
Research Collaborator Fujimori Hirotaka  
Kan Akinori  
Project Period (FY) 2015-04-01 – 2019-03-31
Project Status Completed (Fiscal Year 2018)
Budget Amount *help
¥5,070,000 (Direct Cost: ¥3,900,000、Indirect Cost: ¥1,170,000)
Fiscal Year 2017: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2016: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2015: ¥3,250,000 (Direct Cost: ¥2,500,000、Indirect Cost: ¥750,000)
Keywordsアルミナ / セラミックス / 焼結助剤 / 低温焼結化 / LTCC(低温同時焼成セラミックス) / 高熱伝導 / 誘電体 / 無収縮焼成 / 凍結乾燥
Outline of Final Research Achievements

Our previous studies have been intended to develop novel sintering additives that can allow alumina to be well sintered at a low temperature with a small quantity. We successfully invented low temperature co-fired alumina featuring high density and thermal conductivity at 900 °C.
In this study, the dielectric properties of the materials were improved while maintaining the high thermal conductivity of 17 W/mK and the low temperature sintering below the melting point of silver by improving the additive composition and the firing atmosphere. In addition, in this system, it was found that a well sintered body can be almost obtained even below the liquid phase generation temperature (solid-state-activated-sintering). Furthermore, the powder synthesis by the freeze-drying method was examined, and a compact sintered body with a relative density of approximately 95 % was successfully obtained even by non-shrinkage firing in the x-y direction at the firing temperature of 950 °C.

Academic Significance and Societal Importance of the Research Achievements

本研究における社会的意義は、開発した低温同時焼成アルミナが小型化と高放熱性を両立できることにある。今まで個々に製造していたデバイスを1パッケージ内に収めることができるため、放熱性の必要な箇所において付加価値の高いデバイスとしての効果が見込まれる。また、本研究における学術的意義は、焼結メカニズム解明のためのアプローチにあり、他のセラミックスにも有効に活かされると考えられる。

Report

(5 results)
  • 2018 Annual Research Report   Final Research Report ( PDF )
  • 2017 Research-status Report
  • 2016 Research-status Report
  • 2015 Research-status Report
  • Research Products

    (31 results)

All 2019 2018 2017 2016 2015 Other

All Journal Article (5 results) (of which Peer Reviewed: 5 results,  Acknowledgement Compliant: 4 results) Presentation (22 results) (of which Int'l Joint Research: 7 results,  Invited: 1 results) Remarks (3 results) Patent(Industrial Property Rights) (1 results)

  • [Journal Article] Improvement in Dielectric Properties of Low Temperature Sintered Alumina Containing a Small Quantity of a CuO-Nb2O5 Additive by Substitution of Titanium Dioxide2018

    • Author(s)
      Koichi Shigeno, Shinji Kaneko, Tomoya Yamane, Junya Shimokawa and Hirotaka Fujimori
    • Journal Title

      Journal of the Japan Society of Powder and Powder Metallurgy

      Volume: -

    • NAID

      130007412255

    • Related Report
      2017 Research-status Report
    • Peer Reviewed
  • [Journal Article] Effects of Firing Atmosphere on Low Temperature Sintering of Al2O3 with a Small Quantity of CuO-TiO2-Nb2O5-Ag2O Additives2017

    • Author(s)
      Koichi Shigeno, Takumi Nagata and Hirotaka Fujimori
    • Journal Title

      AIP Conference Proceedings

      Volume: -

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Improvement of Sintering Performances and Dielectric Properties of Oriented TiO2 Ceramics Using Sintering Additives2016

    • Author(s)
      Koichi Shigeno and Hirotaka Fujimori
    • Journal Title

      Trans. Mat. Res. Soc. Japan

      Volume: 41 Pages: 337-340

    • NAID

      130005172419

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Improvement in the Low-Temperature Sintering Performances and Characteristics of Alumina with CuO-TiO2-Nb2O5 Additive by Controlling the Firing Atmosphere2016

    • Author(s)
      Koichi Shigeno, Eisaku Kojima and Hirotaka Fujimori
    • Journal Title

      Journal of the Japan Society of Powder and Powder Metallurgy

      Volume: 63

    • NAID

      130005164625

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Effects of Chemical Compositions on Electrical Properties of Low Temperature Co-fired Alumina Ceramics with Built-in Silver Electrodes2016

    • Author(s)
      Koichi Shigeno, Tadashi Asakawa, Yuto Kuraoka and Hirotaka Fujimori
    • Journal Title

      Trans. Mat. Res. Soc. Japan

      Volume: 41 Pages: 121-126

    • NAID

      130005126123

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Presentation] B-Nb-O系助剤添加ガーナイトセラミックスの低温焼結化及び誘電・熱特性の評価2019

    • Author(s)
      末永健太, 中島一, 茂野交市, 藤野智也, 矢野匠真
    • Organizer
      第21回化学工学会学生発表会京都大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Cu-Ti-Nb-Ag-O系助剤添加アルミナセラミックスの無収縮焼成の検討2019

    • Author(s)
      手塚真菜, 茂野交市, 蔵重優果
    • Organizer
      第21回化学工学会学生発表会京都大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Ag-Cu-Ti-Nb-O系新規複合酸化物の合成と解析2019

    • Author(s)
      永田匠, 茂野交市, 川西一平, 藤森宏高
    • Organizer
      第21回化学工学会学生発表会京都大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Cu-Nb-O系助剤によるガーナイトセラミックスの低温焼結化及び誘電・熱特性の評価2018

    • Author(s)
      中島一, 茂野交市, 末永健太, 金子慎嗣, 藤森宏高
    • Organizer
      第28回日本MRS年次大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Ag-Cu-Ti-Nb-O系新規複合酸化物の合成2018

    • Author(s)
      永田匠, 茂野交市, 金子慎嗣, 川西一平, 藤森宏高
    • Organizer
      第20回化学工学会学生発表会東広島大会
    • Related Report
      2017 Research-status Report
  • [Presentation] Cu-Ti-Nb-O系助剤添加アルミナセラミックスの無収縮焼成の検討2018

    • Author(s)
      松野みほ里, 茂野交市, 金子慎嗣, 手塚真菜
    • Organizer
      第20回化学工学会学生発表会東広島大会
    • Related Report
      2017 Research-status Report
  • [Presentation] Improvement in Dielectric Properties of Low Temperature Sintered Alumina Containing a Small Quantity of Cu-Nb-O Additive by Substitution of Titanium Dioxide2017

    • Author(s)
      Shinji Kaneko, Koichi Shigeno, Tomoya Yamane, Junya Shimokawa and Hirotaka Fujimori
    • Organizer
      JSPM International Conference on Powder and Powder Metallurgy -60th Anniversary- (JSPMIC2017)
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research
  • [Presentation] Improvement of Dielectric Properties of Low Temperature Co-fired Alumina Containing a Small Quantity of Additives by Substitution of Titanium Dioxide2017

    • Author(s)
      Koichi Shigeno, Moyuan Li and Hirotaka Fujimori
    • Organizer
      IUMRS-ICAM 2017
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research
  • [Presentation] Development of Low Temperature Co-fired Alumina with a Small Quantity of Sintering Additives2017

    • Author(s)
      Koichi Shigeno and Hirotaka Fujimori
    • Organizer
      The 12th Pacific Rim Conference on Ceramic and Glass Technology (PACRIM12)
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Cu-Ti-Nb-O系助剤添加アルミナの固相活性化焼結2017

    • Author(s)
      金子慎嗣, 茂野交市, 藤森宏高
    • Organizer
      第19回化学工学会学生発表会豊中大会
    • Place of Presentation
      大阪大学
    • Related Report
      2016 Research-status Report
  • [Presentation] 助剤添加アルミナの見かけの拡散係数測定2017

    • Author(s)
      岡部航大, 茂野交市, 金子慎嗣, 藤森宏高
    • Organizer
      第19回化学工学会学生発表会豊中大会
    • Place of Presentation
      大阪大学
    • Related Report
      2016 Research-status Report
  • [Presentation] 酸化チタンの添加によるCu-Nb-O系助剤添加アルミナの誘電特性改善2017

    • Author(s)
      山根那哉, 茂野交市, 下川淳也, 藤森宏高
    • Organizer
      第19回化学工学会学生発表会豊中大会
    • Place of Presentation
      大阪大学
    • Related Report
      2016 Research-status Report
  • [Presentation] 窒素雰囲気におけるCu-Ti-Nb-O系助剤添加アルミナの低温焼結化と誘電特性2017

    • Author(s)
      下川淳也, 茂野交市, 山根那哉, 藤森宏高
    • Organizer
      第19回化学工学会学生発表会豊中大会
    • Place of Presentation
      大阪大学
    • Related Report
      2016 Research-status Report
  • [Presentation] CuO-TiO2-Nb2O5-Ag2O助剤添加アルミナセラミックスの低温焼結挙動及びマイクロ波誘電特性2016

    • Author(s)
      茂野交市, 蔵岡佑人, 浅川忠, 金子慎嗣, 藤森宏高
    • Organizer
      第26回日本MRS年次大会
    • Place of Presentation
      横浜情報文化センター
    • Year and Date
      2016-12-19
    • Related Report
      2016 Research-status Report
  • [Presentation] CuO-TiO2-Nb2O5助剤添加アルミナセラミックスの低温焼結挙動及びマイクロ波誘電特性2016

    • Author(s)
      茂野交市, 金子慎嗣, 浅川忠, 蔵岡佑人, 藤森宏高
    • Organizer
      第26回日本MRS年次大会
    • Place of Presentation
      万国橋会議センター
    • Year and Date
      2016-12-19
    • Related Report
      2016 Research-status Report
  • [Presentation] Low Temperature Sintering Behavior of Al2O3 Dielectric Ceramic with CuO-TiO2-Nb2O5-Ag2O Additive2016

    • Author(s)
      Koichi Shigeno, Yuto Kuraoka, Tadashi Asakawa and Hirotaka Fujimori
    • Organizer
      The 9th International Conference on Microwave Materials and Their Applications 2016 (MMA 2016)
    • Place of Presentation
      Seoul, Korea
    • Year and Date
      2016-07-03
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research
  • [Presentation] 良好な誘電特性を有する低温同時焼成アルミナの組成開発2016

    • Author(s)
      李墨源, 茂野交市, 藤森宏高
    • Organizer
      第18回化学工学会学生発表会福岡大会
    • Place of Presentation
      福岡大学
    • Year and Date
      2016-03-05
    • Related Report
      2015 Research-status Report
  • [Presentation] 焼成時の酸素分圧が助剤添加アルミナの低温焼結性に及ぼす影響2016

    • Author(s)
      永田匠, 茂野交市, 藤森宏高
    • Organizer
      第18回化学工学会学生発表会福岡大会
    • Place of Presentation
      福岡大学
    • Year and Date
      2016-03-05
    • Related Report
      2015 Research-status Report
  • [Presentation] Effects of Firing Atmosphere on Low Temperature Sintering of Al2O3 with a Small Quantity of CuO-TiO2-Nb2O5-Ag2O Additives2016

    • Author(s)
      Koichi Shigeno, Takumi Nagata and Hirotaka Fujimori
    • Organizer
      The 3rd International Conference of Global Network for Innovative Technology (IGNITE2016)
    • Place of Presentation
      Penang, Malaysia
    • Year and Date
      2016-01-27
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] Low Temperature Sintering Behavior of Al2O3 Dielectric Ceramic with CuO-TiO2-Nb2O5 Additive2015

    • Author(s)
      Koichi Shigeno, Tadashi Asakawa, Yuto Kuraoka and Hirotaka Fujimori
    • Organizer
      2015 Global Research Efforts on Energy and Nanomaterials (GREEN 2015)
    • Place of Presentation
      Sun Moon Lake, Taiwan
    • Year and Date
      2015-12-20
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] Improvement of Low Temperature Sintering Performances and Characteristics of Alumina with CuO-TiO2-Nb2O5 Additives by Control of Firing Atmosphere2015

    • Author(s)
      Koichi Shigeno, Eisaku Kojima and Hirotaka Fujimori
    • Organizer
      3rd International Conference on Powder Metallurgy in Asia (APMA2015)
    • Place of Presentation
      Kyoto, Japan
    • Year and Date
      2015-11-08
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] Cu-Ti-Nb-Ag-O系助剤添加アルミナの低温焼結化に及ぼす焼成雰囲気の影響2015

    • Author(s)
      永田匠, 茂野交市, 濱﨑圭, 李墨源, 藤森宏高
    • Organizer
      第52回化学関連支部合同九州大会
    • Place of Presentation
      北九州国際会議場
    • Year and Date
      2015-06-27
    • Related Report
      2015 Research-status Report
  • [Remarks] 化学工学会学生発表会で物質工学科の学生が優秀賞をダブル受賞

    • URL

      https://www.ube-k.ac.jp/topics/20190302/

    • Related Report
      2018 Annual Research Report
  • [Remarks] 物質工学科の茂野准教授が第66回電気科学技術奨励賞を受賞

    • URL

      http://www.ube-k.ac.jp/topics/20181114/

    • Related Report
      2018 Annual Research Report
  • [Remarks] Ube Kosen student received an award

    • URL

      http://www.ube-k.ac.jp/en/topics/20171106/

    • Related Report
      2017 Research-status Report
  • [Patent(Industrial Property Rights)] 誘電体セラミック材料及び誘電体セラミック組成物2016

    • Inventor(s)
      茂野交市, 藤森宏高
    • Industrial Property Rights Holder
      茂野交市, 藤森宏高
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      2016-150648
    • Filing Date
      2016-07-11
    • Related Report
      2016 Research-status Report

URL: 

Published: 2015-04-16   Modified: 2020-03-30  

Information User Guide FAQ News Terms of Use Attribution of KAKENHI

Powered by NII kakenhi