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A trial of tritium water concentration by freezing and thawing processes

Research Project

Project/Area Number 15K12226
Research Category

Grant-in-Aid for Challenging Exploratory Research

Allocation TypeMulti-year Fund
Research Field Environmental engineering and reduction of environmental burden
Research InstitutionNagaoka University of Technology

Principal Investigator

Kamimura Seiji  長岡技術科学大学, Nagaoka, 教授 (70224673)

Project Period (FY) 2015-04-01 – 2017-03-31
Project Status Completed (Fiscal Year 2016)
Budget Amount *help
¥3,120,000 (Direct Cost: ¥2,400,000、Indirect Cost: ¥720,000)
Fiscal Year 2016: ¥1,300,000 (Direct Cost: ¥1,000,000、Indirect Cost: ¥300,000)
Fiscal Year 2015: ¥1,820,000 (Direct Cost: ¥1,400,000、Indirect Cost: ¥420,000)
KeywordsTritium water / Radiation freezing / Radioactive water / トリチウム水 / 凍結濃縮 / 放射製氷 / 融解分離 / トリチウム / 凍結分離 / 放射冷却 / 汚染水
Outline of Final Research Achievements

In this study, we tried to develop a technique to separate / enrich tritium water, T2O, contained in radioactively contaminated water, using the difference in melting point from pure water H2O. In order to seperate / concentrate D2O from the D2O solution simulating T2O, an experimental apparatus was assembled, which is composed of a radiation cooling unit, an water freezing inner tank and a temperature stabilizing outer tank, and placed in a constant temperature water tank (range of -20 to 80 C, 0.01 C resolution), covered with a thermal insulating lid. Two approaches was made as follow: a freeze concentration method and a melting concentration method. As a result, it was found that the HDO enrichment to the solid phase tended to increase as the temperature of the water tank in the former case, and the maximum enrichment degree was 40% when the water tank temperature was 1.5 C. . In the latter method, the maximum enrichment to solid phase was 13% at 1.4 C.

Report

(3 results)
  • 2016 Annual Research Report   Final Research Report ( PDF )
  • 2015 Research-status Report
  • Research Products

    (2 results)

All 2016

All Presentation (2 results)

  • [Presentation] 放射凍結を応用したトリチウム分離の試行2016

    • Author(s)
      藤岡泰斗,上村靖司
    • Organizer
      日本雪氷学会
    • Place of Presentation
      名古屋
    • Year and Date
      2016-09-28
    • Related Report
      2016 Annual Research Report
  • [Presentation] 赤外分光法による単結晶氷c軸方向の吸収スペクトル測定2016

    • Author(s)
      西間木悠輔,上村靖司,千葉健介
    • Organizer
      日本雪氷学会
    • Place of Presentation
      名古屋
    • Year and Date
      2016-09-28
    • Related Report
      2016 Annual Research Report

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Published: 2015-04-16   Modified: 2018-03-22  

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