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Mechanism of the High-Tc superconductivity in iron chalcogenide ultrathin films

Research Project

Project/Area Number 15K13354
Research Category

Grant-in-Aid for Challenging Exploratory Research

Allocation TypeMulti-year Fund
Research Field Thin film/Surface and interfacial physical properties
Research InstitutionTohoku University

Principal Investigator

Shiogai Junichi  東北大学, 金属材料研究所, 助教 (30734066)

Project Period (FY) 2015-04-01 – 2017-03-31
Project Status Completed (Fiscal Year 2016)
Budget Amount *help
¥3,900,000 (Direct Cost: ¥3,000,000、Indirect Cost: ¥900,000)
Fiscal Year 2016: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Fiscal Year 2015: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Keywords電気二重層トランジスタ / 鉄系超伝導 / 層状物質 / セレン化鉄 / 高温超伝導
Outline of Final Research Achievements

Layered superconductor FeSe exhibits superconducting transition temperature (Tc) at 8 K in bulk form. Recent spectroscopic measurements have revealed that Tc is significantly increased to 60 K in single monolayer form. However, ex-situ electrical transport properties has not clearly addressed so far possibly due to degradation in air. In this study, we fabricated electric-double-layer transistors based on FeSe thick films and established the method to etch the FeSe film down to monolayer using electrochemical reaction. This electrochemical etching method allows to investigate dependence of superconducting properties on film thickness, oxide substrates, and electric field. From systematic electrical transport measurements in FeSe electric-double-layer transistors, we found that the charge balance in a specific band structure plays an important role to induce the high temperature superconductivity.

Report

(3 results)
  • 2016 Annual Research Report   Final Research Report ( PDF )
  • 2015 Research-status Report
  • Research Products

    (15 results)

All 2017 2016 2015

All Journal Article (3 results) (of which Peer Reviewed: 3 results,  Acknowledgement Compliant: 1 results) Presentation (12 results) (of which Int'l Joint Research: 6 results,  Invited: 5 results)

  • [Journal Article] Unified trend of superconducting transition temperature versus Hall coefficient for ultrathin FeSe films prepared on different oxide substrates2017

    • Author(s)
      Junichi Shiogai, Tomoki Miyakawa, Yukihiro Ito, Tsutomu Nojima, and Atsushi Tsukazaki
    • Journal Title

      Phys. Rev. B

      Volume: 95 Issue: 11 Pages: 115101-115101

    • DOI

      10.1103/physrevb.95.115101

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Electrochemical-Etching Approach to Achieving Ultrathin FeSe Films2016

    • Author(s)
      塩貝 純一, 野島 勉, 塚﨑 敦
    • Journal Title

      Hyomen Kagaku

      Volume: 37 Issue: 11 Pages: 541-546

    • DOI

      10.1380/jsssj.37.541

    • NAID

      130005284288

    • ISSN
      0388-5321, 1881-4743
    • Related Report
      2016 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Electric-field-induced superconductivity in electrochemically etched ultrathin FeSe films on SrTiO3 and MgO2016

    • Author(s)
      J. Shiogai, Y. Ito, T. Mitsuhashi, T. Nojima, A. Tsukazaki
    • Journal Title

      Nature Physics

      Volume: 12 Issue: 3 Pages: 42-42

    • DOI

      10.1088/0022-3727/49/3/03lt01

    • Related Report
      2015 Research-status Report
    • Peer Reviewed
  • [Presentation] 電気化学エッチングを用いたFeSe薄膜高温超伝導2017

    • Author(s)
      塩貝純一、宮川智樹、伊藤恭太、野島勉、塚﨑敦
    • Organizer
      日本物理学会・第72回年次大会
    • Place of Presentation
      大阪大学(大阪府豊中市)
    • Year and Date
      2017-03-19
    • Related Report
      2016 Annual Research Report
    • Invited
  • [Presentation] A universal relationship of superconducting transition temperature and Hall coefficient in etching-induced superconductivity in FeSe electric double layer transistors2017

    • Author(s)
      J. Shiogai, T. Miyakawa, T. Nojima, and A. Tsukazaki
    • Organizer
      CEMS-QPEC Symposium on Emergent Quantum Materials
    • Place of Presentation
      東京大学(東京都文京区)
    • Year and Date
      2017-01-19
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Electrochemical etching induced high temperature superconductivity in FeSe electric double layer transistors2016

    • Author(s)
      J. Shiogai, T. Miyakawa, Y. Ito, T. Nojima, and A. Tsukazaki
    • Organizer
      ISS 2016 - 29th International Symposium on Superconductivity
    • Place of Presentation
      東京国際フォーラム(東京都千代田区)
    • Year and Date
      2016-12-14
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Electrochemical approach to achieving ultrathin FeSe using electric double layer transistor 2016 MRS Fall Meeting2016

    • Author(s)
      J. Shiogai, T. Miyakawa, Y. Ito, T. Mitsuhashi, T. Nojima, and A. Tsukazaki
    • Organizer
      2016 MRS Fall Meeting
    • Place of Presentation
      ボストン(米国)
    • Year and Date
      2016-11-28
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Electrochemical etching approach to ultrathin FeSe films using electric double layer transistor2016

    • Author(s)
      J. Shiogai, T. Miyakawa, Y. Ito, T. Nojima and A. Tsukazaki
    • Organizer
      JSPS-EPSRC Tohoku-Cambridge-CNRS Core to Core program Symposium "Two dimensional electronics/spintronics devices"
    • Place of Presentation
      東北大学(宮城県仙台市)
    • Year and Date
      2016-11-17
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] High temperature superconductivity in electrochemically-etched FeSe thin films2016

    • Author(s)
      J. Shiogai, T. Miyakawa, Y. Ito, T. Mitsuhashi, T. Nojima, and A. Tsukazaki
    • Organizer
      International Symposium on Revolutionary Atomic-Layer Materials
    • Place of Presentation
      東北大学(宮城県仙台市)
    • Year and Date
      2016-10-22
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] FeSe EDLTで誘起される超伝導転移のイオン液体依存性2016

    • Author(s)
      宮川智樹、伊藤恭太、塩貝純一、野島勉、松本道生、清水直、岩佐義宏、相田卓三、塚﨑敦
    • Organizer
      日本物理学会・2016年秋季大会
    • Place of Presentation
      金沢大学(石川県金沢市)
    • Year and Date
      2016-09-13
    • Related Report
      2016 Annual Research Report
  • [Presentation] High-Tc Superconductivity at 40 K observed in electrochemically etched FeSe films2016

    • Author(s)
      J. Shiogai, Y. Ito, T. Mitsuhashi, T. Nojima, and A. Tsukazaki
    • Organizer
      ICSM 2016 - The 5th International Conference of Superconductivity and Magnetism
    • Place of Presentation
      フェトヒイェ(トルコ共和国)
    • Year and Date
      2016-04-26
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] FeSe電気二重層トランジスタにおける超伝導転移温度の酸化物基板依存性2016

    • Author(s)
      塩貝 純一, 伊藤 恭太, 三橋 駿貴, 野島 勉, 塚﨑 敦
    • Organizer
      第63回応用物理学会春季学術講演会
    • Place of Presentation
      東工大大岡山キャンパス, 東京
    • Year and Date
      2016-03-19
    • Related Report
      2015 Research-status Report
  • [Presentation] High-Tc superconductivity at 40 K emerged in ultrathin FeSe electric-double-layer transistors2016

    • Author(s)
      J. Shiogai, Y. Ito, T. Mitsuhashi, T. Nojima, and A. Tsukazaki
    • Organizer
      APS March Meeting 2016
    • Place of Presentation
      Baltimore, Maryland, USA
    • Year and Date
      2016-03-18
    • Related Report
      2015 Research-status Report
  • [Presentation] FeSe薄膜電気二重層トランジスタにおけるHall効果測定2015

    • Author(s)
      塩貝 純一, 伊藤 恭太, 三橋 駿貴, 野島 勉, 塚﨑 敦
    • Organizer
      第76回応用物理学会秋季学術講演会
    • Place of Presentation
      名古屋国際会議場, 名古屋
    • Year and Date
      2015-09-13
    • Related Report
      2015 Research-status Report
  • [Presentation] FeSe超薄膜の作製と電気二重層トランジスタ特性の評価2015

    • Author(s)
      伊藤 恭太, 塩貝 純一, 三橋 駿貴, 野島 勉, 塚﨑 敦
    • Organizer
      第76回応用物理学会秋季学術講演会
    • Place of Presentation
      名古屋国際会議場, 名古屋
    • Year and Date
      2015-09-13
    • Related Report
      2015 Research-status Report

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Published: 2015-04-16   Modified: 2018-03-22  

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