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STM study of large magnetic anisotropy in single Fe atoms on atomically-flat MgO substrate

Research Project

Project/Area Number 15K13357
Research Category

Grant-in-Aid for Challenging Exploratory Research

Allocation TypeMulti-year Fund
Research Field Thin film/Surface and interfacial physical properties
Research InstitutionChiba University

Principal Investigator

Yamada Toyokazu  千葉大学, 大学院融合科学研究科, 准教授 (10383548)

Project Period (FY) 2015-04-01 – 2017-03-31
Project Status Completed (Fiscal Year 2016)
Budget Amount *help
¥4,030,000 (Direct Cost: ¥3,100,000、Indirect Cost: ¥930,000)
Fiscal Year 2016: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2015: ¥2,990,000 (Direct Cost: ¥2,300,000、Indirect Cost: ¥690,000)
Keywordsスピントロニクス / 磁気異方性 / STM / 表面界面物性 / 酸化物 / 走査プローブ顕微鏡
Outline of Final Research Achievements

We have studied magnetic anisotropy of single Fe atoms on MgO substrate by means of homu-built UHV-STM setup. Fe(001)-whisker was used as a substrate. To prevent surface/interface roughness, Fe(001) surface was first coated by an ordered one monolayer (1x1) oxygen film by introducing 1L oxygen at 300 K with subsequent annealing at 850 K. 1 ML Mg was deposited on the Fe(001)-p(1x1)O, and with subsequent oxidization and annealing, we succeeded to obtain an atomically-flat MgO single monolayer film with a gap of ~6 eV. One monolayer Fe film deposited on this MgO film showed LDOS peaks around the Fermi energy (no gap). Next, we tried to deposit single Fe atoms on the MgO substrate. However, suddenly pressure in the STM chamber became bad. We spent almost six months to find and fix problems, Thus, we still need time to measure magnetic anisotropy of single Fe atoms on the MgO films.

Report

(3 results)
  • 2016 Annual Research Report   Final Research Report ( PDF )
  • 2015 Research-status Report
  • Research Products

    (22 results)

All 2017 2016 2015 Other

All Journal Article (6 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 6 results,  Acknowledgement Compliant: 5 results,  Open Access: 1 results) Presentation (14 results) (of which Int'l Joint Research: 8 results,  Invited: 7 results) Book (1 results) Remarks (1 results)

  • [Journal Article] スピン偏極STMの発展の歴史と今後の課題2017

    • Author(s)
      山田豊和
    • Journal Title

      日本真空学会誌

      Volume: 60

    • NAID

      130006900152

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Temperature control of the growth of iron oxide nanoislands on Fe(001)2016

    • Author(s)
      Toyo Kazu Yamada, Yuki Sakaguchi, Lukas Gerhard, and Wulf Wulfhekel
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 55 Issue: 8S1 Pages: 08NB14-08NB14

    • DOI

      10.7567/jjap.55.08nb14

    • NAID

      210000146981

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Role of π-d hybridization in 300-K organic-magnetic interface: metal-free phthalocyanine single molecules on bcc Fe(001)-whisker2016

    • Author(s)
      T. K. Yamada, Y. Yamagishi, S. Nakashima, Y. Kitaoka, and K. Nakamura
    • Journal Title

      Phys. Rev. B

      Volume: 94 Issue: 19 Pages: 195437-195437

    • DOI

      10.1103/physrevb.94.195437

    • NAID

      130006710390

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Electron-bombarded <110>-oriented tungsten tips for stable tunneling electron emission2016

    • Author(s)
      T. K. Yamada, T. Abe, N. M. K. Nazriq, and T. Irisawa
    • Journal Title

      Review of Scientific Instruments

      Volume: 87 Issue: 3 Pages: 033703-033703

    • DOI

      10.1063/1.4943074

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Temperature control of the growth of iron-oxide nano-islands on Fe(001)2016

    • Author(s)
      Toyo Kazu Yamada, Yuki Sakaguchi, Lukas Gerhard, and Wulf Wulfhekel
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: accepted

    • NAID

      210000146981

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] ]Method for Controlling Electrical Properties of Single-Layer Graphene Nanoribbons via Adsorbed Planar Molecular Nanoparticles2015

    • Author(s)
      Hirofumi Tanaka, Ryo Arima, Minoru Fukumori, Daisuke Tanaka, Ryota Negishi, Yoshihiro Kobayashi, Seiya Kasai, Toyo Kazu Yamada and Takuji Ogawa
    • Journal Title

      Scientific Reports

      Volume: 5 Issue: 1 Pages: 12341-12341

    • DOI

      10.1038/srep12341

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Presentation] スピン偏極STM によるFe 単原子膜中のスキルミオン観察2017

    • Author(s)
      山口貴之,ウルフ ウルフヘケル,山田豊和
    • Organizer
      第64回応用物理学会春季学術講演会
    • Place of Presentation
      横浜パシフィコ
    • Related Report
      2016 Annual Research Report
  • [Presentation] Fe(001)上の鉄酸化物ナノ島成長の温度制御2017

    • Author(s)
      山田豊和,坂口雄基
    • Organizer
      第64回応用物理学会春季学術講演会
    • Place of Presentation
      横浜パシフィコ
    • Related Report
      2016 Annual Research Report
  • [Presentation] スピン偏極走査トンネル顕微鏡(SP-STM)2016

    • Author(s)
      山田豊和
    • Organizer
      ナノ学会部会合同シンポジウム
    • Place of Presentation
      グランドパレス川端, 秋田
    • Year and Date
      2016-12-26
    • Related Report
      2016 Annual Research Report
    • Invited
  • [Presentation] STM molecular architecting using single atoms, single molecules, and graphene nanoribbons2016

    • Author(s)
      T. K. Yamada
    • Organizer
      12th International Conference on Nano-Molecular Electronics (ICNME 2016)
    • Place of Presentation
      神戸
    • Year and Date
      2016-12-14
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] STMによるFe/MgO単原子層/Fe(001)-p(1x1)Oの原子・電子構造解明2016

    • Author(s)
      坂口雄基,山田豊和,
    • Organizer
      日本物理学会年次大会
    • Place of Presentation
      東北学院大学
    • Year and Date
      2016-03-19
    • Related Report
      2015 Research-status Report
  • [Presentation] Growth of atomically-flat bcc-Fe/MgO(001) films on Fe(001)-p(1x1)O2016

    • Author(s)
      Toyo Kazu Yamada
    • Organizer
      The First Symposium of Chiral Molecular Science and Technology in Chiba University ‘-Advanced Materials Science, Biology & Nanophotonics in Chiba-‘
    • Place of Presentation
      Chiba Univ.
    • Year and Date
      2016-03-01
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] Opeing talk: spin-polarized STM overview2016

    • Author(s)
      T. K. Yamada
    • Organizer
      6th international conference of spin-polarized scanning tunneling microscopy (SPSTM-6
    • Place of Presentation
      Chiba Univ, Chiba
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] スピン偏極STMによる原子レベルでの磁性探索2016

    • Author(s)
      山田豊和
    • Organizer
      第77回応用物理学会秋季学術講演会STMノーベル賞&AFM発明30周年記念シンポジウム
    • Place of Presentation
      朱鷺メッセ, 新潟
    • Related Report
      2016 Annual Research Report
    • Invited
  • [Presentation] 極限スピン観察と制御:SP-STM2016

    • Author(s)
      山田豊和
    • Organizer
      日本磁気学会第210回研究会
    • Place of Presentation
      中央大学駿河台記念館510号室
    • Related Report
      2016 Annual Research Report
    • Invited
  • [Presentation] Atomically flat MgO monolayer films on Fe(001)-p(1x1)O2016

    • Author(s)
      Yuki Sakaguchi, Lukas Gerhard, Wulf Wulfhekel, and Toyo Kazu Yamada
    • Organizer
      International 2016 Multilayers Metallic on Symposium (MML2016)
    • Place of Presentation
      Uppsala Univ., Uppsala, Sweden
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Atomically-Flat MgO Interfaceon Fe(001)-p(1x1)O2015

    • Author(s)
      Y. Sakaguchi,N.K.M.Nazriq and T.K. Yamada
    • Organizer
      The 23rd International Colloquium on Scanning Probe Microscopy (ICSPM23)
    • Place of Presentation
      Niseko
    • Year and Date
      2015-12-10
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] Control of single molecular electronic states with STM atom manipulation: toward single molecular device2015

    • Author(s)
      Toyo Kazu Yamada
    • Organizer
      2015 International Symposium for Advanced Materials Research (ISAMR 2015)
    • Place of Presentation
      Sun Moon Lake, Taiwan
    • Year and Date
      2015-08-17
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Defect free interface for bcc-MgO/Fe(001): STM/STS study2015

    • Author(s)
      SAKAGUCHI Y., GERHARD L., YAMADA T. K.,
    • Organizer
      International Colloquium on Magnetic Films and Surfaces 2015 (ICMFS2015)
    • Place of Presentation
      Krakow, Poland
    • Year and Date
      2015-07-14
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] Quantitative STM spin-polarization measurements of single molecules on magnetic domains2015

    • Author(s)
      Toyo Kazu Yamada
    • Organizer
      Workshop on “Spins at Surfaces”
    • Place of Presentation
      Univ. of Tokyo
    • Year and Date
      2015-06-09
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research / Invited
  • [Book] Encyclopedia of Surface Analysis, Chapter: Spin-polarized scanning tunneling microscopy (SP-STM)2017

    • Author(s)
      Toyo Kazu Yamada
    • Publisher
      Springer
    • Related Report
      2016 Annual Research Report
  • [Remarks] 山田豊和研究室ホームページ

    • URL

      http://adv.chiba-u.jp/nano/yamada-upload/

    • Related Report
      2016 Annual Research Report 2015 Research-status Report

URL: 

Published: 2015-04-16   Modified: 2018-03-22  

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