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Vacancy-induced ferromagnetism in metal oxides probed by spin-polarized positron annihilation spectroscopy

Research Project

Project/Area Number 15K14135
Research Category

Grant-in-Aid for Challenging Exploratory Research

Allocation TypeMulti-year Fund
Research Field Inorganic materials/Physical properties
Research InstitutionNational Institutes for Quantum and Radiological Science and Technology (2016-2017)
Japan Atomic Energy Agency (2015)

Principal Investigator

Maekawa Masaki  国立研究開発法人量子科学技術研究開発機構, 高崎量子応用研究所 先端機能材料研究部, 主幹研究員(定常) (10354945)

Co-Investigator(Renkei-kenkyūsha) KAWASUSO ATSUO  国立研究開発法人量子科学技術研究開発機構, 高崎量子応用研究所 先端機能材料研究部, 上席研究員 (20354946)
ZHANG HONJYUN  独立行政法人日本原子力研究開発機構, 原子力科学研究部門 先端基礎研究センター, 研究員 (50644374)
Research Collaborator ABE HIROSHI  国立研究開発法人量子科学技術研究開発機構, 高崎量子応用研究所 先端機能材料研究部, 主任研究員 (30354947)
Project Period (FY) 2015-04-01 – 2018-03-31
Project Status Completed (Fiscal Year 2017)
Budget Amount *help
¥2,860,000 (Direct Cost: ¥2,200,000、Indirect Cost: ¥660,000)
Fiscal Year 2017: ¥650,000 (Direct Cost: ¥500,000、Indirect Cost: ¥150,000)
Fiscal Year 2016: ¥650,000 (Direct Cost: ¥500,000、Indirect Cost: ¥150,000)
Fiscal Year 2015: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Keywords陽電子消滅 / スピン偏極陽電子 / 空孔誘起磁性 / 酸化亜鉛 / イオンビーム照射 / d0強磁性 / カチオン原子空孔 / SQUID / イオンビーム
Outline of Final Research Achievements

We investigated the ferromagnetism of Zinc Oxide (ZnO) induced by oxygen implantation by using spin-polarized positron annihilation spectroscopy together with magnetization measurements. The magnetization measurements showed the appearance of ferromagnetism after oxygen implantation. The Magnetic Doppler broadening of annihilation radiation (MDB) spectrum showed asymmetry upon field reversal after oxygen implantation. The obtained MDB spectrum was well-explained with a theoretical calculation considering zinc vacancies. These results suggest the radiation-induced zinc vacancies to be the source of the observed ferromagnetism of ZnO.

Report

(4 results)
  • 2017 Annual Research Report   Final Research Report ( PDF )
  • 2016 Research-status Report
  • 2015 Research-status Report
  • Research Products

    (23 results)

All 2018 2017 2016 2015 Other

All Journal Article (5 results) (of which Peer Reviewed: 4 results) Presentation (17 results) (of which Int'l Joint Research: 4 results,  Invited: 3 results) Remarks (1 results)

  • [Journal Article] スピン偏極陽電子ビームによる空孔誘起磁性の研究2018

    • Author(s)
      前川雅樹
    • Journal Title

      陽電子科学

      Volume: 10 Pages: 29-37

    • NAID

      40021484840

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Vacancy-induced magnetism in GaN film probed by spin-polarized positron beam2018

    • Author(s)
      M. Maekawa, S. Sakai, K. Wada, A. Miyashita and A. Kawasuso
    • Journal Title

      QST Takasaki Annual Report 2016

      Volume: QST M-8 Pages: 131-131

    • NAID

      130006710563

    • Related Report
      2017 Annual Research Report
  • [Journal Article] Vacancy-induced ferromagnetism in ZnO probed by spin-polarized positron annihilation spectroscopy2017

    • Author(s)
      Maekawa Masaki、Abe Hiroshi、Miyashita Atsumi、Sakai Seiji、Yamamoto Shunya、Kawasuso Atsuo
    • Journal Title

      Applied Physics Letters

      Volume: 110 Issue: 17 Pages: 172402-172402

    • DOI

      10.1063/1.4979696

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Vacancy-Induced magnetism in ZnO probed by Spin-Polarized Positron Beam2017

    • Author(s)
      M. Maekawa, H. Abe, S. Sakai and A. Kawasuso
    • Journal Title

      QST-Takasaki annual report 2015

      Volume: QST-M-2 Pages: 60-60

    • Related Report
      2016 Research-status Report
    • Peer Reviewed
  • [Journal Article] Observation of Vacancy-induced Magnetizm by the Spin-polarized Positron Annihilation Spectroscopy2015

    • Author(s)
      M. Maekawa, K. Zhou and A. Kawasuso
    • Journal Title

      JAEA-Review

      Volume: 022 Pages: 134-134

    • Related Report
      2015 Research-status Report
    • Peer Reviewed
  • [Presentation] 前川雅樹、境誠司、和田健、宮下敦巳、河裾厚男2018

    • Author(s)
      スピン偏極陽電子ビームによる窒化ガリウム薄膜の空孔誘起磁性評価
    • Organizer
      日本物理学会第73回年次大会(2018年)
    • Related Report
      2017 Annual Research Report
  • [Presentation] スピン偏極陽電子ビームを用いた窒化ガリウム薄膜の空孔誘起磁性の検2017

    • Author(s)
      前川雅樹、境誠司、和田健、宮下敦巳、河裾厚男
    • Organizer
      日本物理学会 第72回年次大会
    • Place of Presentation
      大阪大学豊中キャンパス(大阪府豊中市)
    • Year and Date
      2017-03-18
    • Related Report
      2016 Research-status Report
  • [Presentation] スピン偏極陽電子ビームを用いた希薄磁性半導体中の空孔誘起磁性評価2017

    • Author(s)
      前川雅樹、阿部浩之、宮下敦己、圓谷史郎、境誠司、山本春也、河裾厚男
    • Organizer
      第 1 回 QST 高崎研シンポジウム
    • Place of Presentation
      高崎量子応用研究所(群馬県高崎市)
    • Year and Date
      2017-01-27
    • Related Report
      2016 Research-status Report
  • [Presentation] スピン偏極陽電子ビームによるイオン照射窒化ガリウム薄膜の空孔局在電子スピンの検出2017

    • Author(s)
      前川雅樹、境誠司、和田健、宮下敦巳、河裾厚男
    • Organizer
      日本物理学会2017年秋季大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Vacancy-induced magnetism in metal oxides or nitrides probed by spin-polarized positron beam2017

    • Author(s)
      M. Maekawa, S. Sakai, K. Wada, A. Miyashita and A. Kawasuso
    • Organizer
      The 8th International Symposium on Surface Science
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] スピン偏極陽電子ビームを用いた希薄磁性半導体中の空孔誘起磁性評価2017

    • Author(s)
      前川雅樹、境誠司、和田健、宮下敦巳、河裾厚男
    • Organizer
      QST高崎サイエンスフェスタ2017
    • Related Report
      2017 Annual Research Report
  • [Presentation] Application of spin-polarized positron spectroscopy to some ferromagnetic systems2017

    • Author(s)
      A. Kawasuso, M. Maekawa, A. Miyashita, H. Abe, S. Sakai, S. Entani, S. Yamamoto, K. Wada , H. Zhang, H. Li, T. Seki, E. Saitoh, K. Takanashi, S. Iida, Y. Nagashima, J. Ieda, G. Bo, S. Maekawa, T. Hyodo, I. Mochizuki, A. Yabuuchi
    • Organizer
      International workshop on computational science 2017
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 前川雅樹、境誠司、圓谷史郎、河裾厚男2016

    • Author(s)
      窒素イオン照射GaN膜の空孔誘起磁性評価
    • Organizer
      平成28年度京都大学原子炉実験所専門研究会「陽電子科学とその理工学への応用」
    • Place of Presentation
      京都大学原子炉実験所(大阪府熊取市)
    • Year and Date
      2016-12-08
    • Related Report
      2016 Research-status Report
  • [Presentation] スピン偏極陽電子ビームを用いたイオン照射酸化亜鉛による空孔誘起磁性効果2016

    • Author(s)
      阿部浩之・前川雅樹・宮下敦巳・境誠司・圓谷志郎・山本春也・河裾厚男
    • Organizer
      第53回アイソトープ・放射線研究発表会
    • Place of Presentation
      東京大学(東京都文京区)
    • Year and Date
      2016-07-07
    • Related Report
      2016 Research-status Report
  • [Presentation] Spin-polarized positron annihilation spectroscopy on ferromagnets, surfaces and vacancies2016

    • Author(s)
      A. Kawasuso, H. J. Zhang, H. Li, K. Zhou, M. Maekawa, A. Miyashita, H. Abe, S. Sakai, S. Yamamoto, K. Wada
    • Organizer
      14th International Workshop on Slow Positron Beam Techniques & Applications
    • Place of Presentation
      松江国際会議場(島根県松江市)
    • Year and Date
      2016-05-24
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] スピン偏極陽電子ビームによって明らかにされた酸化亜鉛空孔誘起”d0”強磁性2015

    • Author(s)
      阿部浩之
    • Organizer
      第25回日本MRS年次大会
    • Place of Presentation
      開港記念会館(神奈川県横浜市)
    • Year and Date
      2015-12-08
    • Related Report
      2015 Research-status Report
  • [Presentation] 陽電子で観る表面、界面、原子空孔、スピン2015

    • Author(s)
      前川雅樹、阿部浩之、宮下敦巳、李輝、河裾厚男
    • Organizer
      第31 回PIXE シンポジウム
    • Place of Presentation
      高崎量子応用研究所(群馬県高崎市)
    • Year and Date
      2015-10-28
    • Related Report
      2015 Research-status Report
    • Invited
  • [Presentation] スピン偏極陽電子消滅法によるNi添加ZnO空孔誘起磁性の評価2015

    • Author(s)
      前川 雅樹、周凱、河裾厚男
    • Organizer
      第10回高崎量子応用研究シンポジウム
    • Place of Presentation
      高崎量子応用研究所(群馬県高崎市)
    • Year and Date
      2015-10-08
    • Related Report
      2015 Research-status Report
  • [Presentation] イオンビーム照射で導入された原子空孔に由来する強磁性効果2015

    • Author(s)
      阿部浩之
    • Organizer
      第10回 高崎量子応用研究シンポジウム
    • Place of Presentation
      高崎量子応用研究所(群馬県高崎市)
    • Year and Date
      2015-10-08
    • Related Report
      2015 Research-status Report
  • [Presentation] Spin-Polarized Positron Annihilation Spectroscopy: Present and Future2015

    • Author(s)
      Atsuo Kawasuso
    • Organizer
      17th International Conference on Positron Annihilation
    • Place of Presentation
      Wuhan(China)
    • Year and Date
      2015-09-24
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] スピン偏極陽電子ビームを用いた酸化亜鉛空孔誘起磁性の検出2015

    • Author(s)
      阿部浩之, 前川雅樹, 周凱, 河裾厚男
    • Organizer
      日本物理学会2015年秋季大会
    • Place of Presentation
      関西大学千里山キャンパス(大阪府吹田市)
    • Year and Date
      2015-09-17
    • Related Report
      2015 Research-status Report
  • [Presentation] 金属酸化物の原子空孔誘起強磁性効果の研究2015

    • Author(s)
      河裾厚男、前川雅樹、宮下敦巳、境誠司
    • Organizer
      第52回アイソトープ・放射線研究発表会
    • Place of Presentation
      東京大学弥生講堂(東京都文京区)
    • Year and Date
      2015-07-09
    • Related Report
      2015 Research-status Report
  • [Remarks] 世界に先駆けた技術を用いて、酸化亜鉛に放射線を照射すると強磁性が現れるしくみを解明

    • URL

      http://www.qst.go.jp/information/itemid034-002172.html

    • Related Report
      2017 Annual Research Report

URL: 

Published: 2015-04-16   Modified: 2019-03-29  

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