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Investigation of thermal conductivity mechanism controlled by magnetic field and its application to novel thermoelectric devices

Research Project

Project/Area Number 15K14170
Research Category

Grant-in-Aid for Challenging Exploratory Research

Allocation TypeMulti-year Fund
Research Field Structural/Functional materials
Research InstitutionJapan Synchrotron Radiation Research Institute

Principal Investigator

Satoshi Tsutsui  公益財団法人高輝度光科学研究センター, 利用研究促進部門, 主幹研究員 (70360823)

Co-Investigator(Kenkyū-buntansha) 鬼丸 孝博  広島大学, 先端物質科学研究科, 准教授 (50444708)
Co-Investigator(Renkei-kenkyūsha) Yoshio Kobayashi  電気通信大学, 情報理工学系研究科, 教授 (30221245)
Research Collaborator Goh Swee K.  the Chinese University of Hong Kong
Project Period (FY) 2015-04-01 – 2017-03-31
Project Status Completed (Fiscal Year 2016)
Budget Amount *help
¥3,900,000 (Direct Cost: ¥3,000,000、Indirect Cost: ¥900,000)
Fiscal Year 2016: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Fiscal Year 2015: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Keywordsカゴ状物質 / ゲスト原子 / フォノン / 熱伝導度 / 磁性 / ラットリング / メスバウアー効果 / 非調和フォノン / 部分フォノン状態密度測定 / 核共鳴非弾性散乱 / クラスレート化合物 / 熱伝導
Outline of Final Research Achievements

This study has been focused on cage-structured compounds expected to be a candidate of thermoelectric materials. Particularly, we have investigated cage-structured compounds having a magnetic guest atom, which is important for thermal insulation, in order to reveal relationships between thermal insulation and magnetic properties in cage-structured compounds. One of the important obtained in the present work is the fact that guest atomic motions in type-I clathrates, which correlate with thermal insulation, are more sensitive to number of their carriers than their ferromagnetic ordering.

Report

(3 results)
  • 2016 Annual Research Report   Final Research Report ( PDF )
  • 2015 Research-status Report
  • Research Products

    (19 results)

All 2017 2016 2015 Other

All Int'l Joint Research (1 results) Journal Article (7 results) (of which Int'l Joint Research: 4 results,  Peer Reviewed: 7 results,  Open Access: 3 results,  Acknowledgement Compliant: 3 results) Presentation (11 results) (of which Int'l Joint Research: 4 results,  Invited: 4 results)

  • [Int'l Joint Research] The Chinese University of Hong Kon(China)

    • Related Report
      2016 Annual Research Report
  • [Journal Article] Second-order Structural Transition in (Ca0.5Sr0.5)3Rh4Sn132017

    • Author(s)
      Y. W. Cheung, Y. J. Hu, S. K. Goh, K. Kaneko, S. Tsutsui, P. W. Logg, F. M. Grousch, H. Kanagawa, Y. Tanioku, M. Imai, T. Matsumoto, K. Yoshimura
    • Journal Title

      J. Phys. Conf. Ser.

      Volume: 807 Pages: 0320021-4

    • DOI

      10.1088/1742-6596/807/3/032002

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Structural, Magnetic, and Superconducting Properties of Caged Compounds ROs2Zn20 (R = La, Ce, Pr, and Nd)2017

    • Author(s)
      K. Wakiya, T. Onimaru, K. T. Matsumoto, Y. Yamane, N. Nagasawa, K. Umeo, S. Kittaka, T. Sakakibara, Y. Matsushita, and T. Takabatake
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 86 Issue: 3 Pages: 034707-034707

    • DOI

      10.7566/jpsj.86.034707

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Synchrotron Radiation Mossbauer Spectroscopy using 149Sm Nuclei2016

    • Author(s)
      Satoshi Tsutsui, Ryo Masuda, Yasuhiro Kobayashi, Yoshitaka Yoda, Kota Mizuuchi, Yusei Shimizu, Hiroyuki Hidaka, Tatsuya Yanagisawa, Hiroshi Amitsuka, Fumitoshi Iga, and Makoto Seto
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 85 Issue: 8 Pages: 083704-083704

    • DOI

      10.7566/jpsj.85.083704

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Mixed valence state (SmxLa1-x)Tr2Al202016

    • Author(s)
      Akira Yamada, Ryuji Higashinaka, Kengo Fushiya, Takuya Asano, Tatsuma D. Matsuda, Masaichiro Mizumaki, Satoshi Tsutsui, Kiyofumi Nitta, Toshiaki Ina, Tomoya Uruga and Yuji Aoki
    • Journal Title

      J. Phys.: Conf. Ser.

      Volume: 683 Pages: 0120201-6

    • DOI

      10.1088/1742-6596/683/1/012020

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Effect of Ga Substitution on the Γ3 Doublet Ground State in PrIr2Zn202016

    • Author(s)
      T. Onimaru, K. Uenishi, Y. Yamane, K. Wakiya, K. T. Matsumoto, K. Umeo and T. Takabatake
    • Journal Title

      J. Phys.: Conf. Series

      Volume: 683 Pages: 012011-012011

    • DOI

      10.1088/1742-6596/683/1/012011

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Long-time variation in magnetic structure of CeIr3Si2: Observation of a nucleation-and-growth process of magnetic domains2016

    • Author(s)
      K. Motoya, M. Hagihara, T. Takabatake, M. Matsuda
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 85 Issue: 4 Pages: 043601-043601

    • DOI

      10.7566/jpsj.85.043601

    • NAID

      210000133881

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Low-energy optical phonon modes in the caged compound LaRu2Zn202015

    • Author(s)
      K. Wakiya, T. Onimaru, S. Tsutsui, T. Hasegawa, K. T. Matsumoto, N. Nagasawa, A. Q. R. Baron, N. Ogita, M. Udagawa, T. Takabatake
    • Journal Title

      Phys. Rev. B

      Volume: 93 Issue: 6

    • DOI

      10.1103/physrevb.93.064105

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Presentation] Sm系重い電子化合物の放射光メスバウアー分光2017

    • Author(s)
      筒井智嗣、中村 仁、小林義男、久保謙哉、依田芳卓、山田 瑛、東中隆二、松田達磨、青木勇二、水牧仁一朗、佐藤英行
    • Organizer
      日本物理学会第72回年会
    • Place of Presentation
      大阪大学豊中キャンパス(大阪府豊中市)
    • Year and Date
      2017-03-17
    • Related Report
      2016 Annual Research Report
  • [Presentation] PrIr2Zn20の非フェルミ液体的挙動に対するZnサイト置換効果2017

    • Author(s)
      山田怜志, 鬼丸孝博, 上西和登, 山根悠, 脇舎和平, 松本圭介, 梅尾和則, 高畠敏郎
    • Organizer
      日本物理学会第72回年会
    • Place of Presentation
      大阪大学 豊中キャンパス(大阪府豊中市)
    • Year and Date
      2017-03-17
    • Related Report
      2016 Annual Research Report
  • [Presentation] Pr希薄系Y1-xPrxIr2Zn20 (x≦0.05)の非フェルミ液体的挙動に対する磁場効果2017

    • Author(s)
      山根悠, 上西和登, 脇舎和平, 松本圭介, 鬼丸孝博, 梅尾和則, 高畠敏郎
    • Organizer
      日本物理学会第72回年会
    • Place of Presentation
      大阪大学 豊中キャンパス(大阪府豊中市)
    • Year and Date
      2017-03-17
    • Related Report
      2016 Annual Research Report
  • [Presentation] 六方晶RRh3(R = Pr, Nd)の強磁性と二形LaRh3の超伝導2017

    • Author(s)
      朴景培, 山根悠, 鬼丸孝博, 梅尾和則, 高畠敏郎
    • Organizer
      日本物理学会第72回年会
    • Place of Presentation
      大阪大学 豊中キャンパス(大阪府豊中市)
    • Year and Date
      2017-03-17
    • Related Report
      2016 Annual Research Report
  • [Presentation] Sm金属間化合物の放射光メスバウアー分光2017

    • Author(s)
      筒井智嗣、依田芳卓、中村 仁、小林義男、久保謙哉
    • Organizer
      第18回メスバウアー分光研究会シンポジウム
    • Place of Presentation
      東京理科大学森戸会館(東京都新宿区)
    • Year and Date
      2017-03-15
    • Related Report
      2016 Annual Research Report
  • [Presentation] Sm金属間化合物における電荷・磁気自由度のプローブとしてのSm-149放射光メスバウアー分光2017

    • Author(s)
      筒井智嗣
    • Organizer
      第5回先進的放射光メスバウアー分光研究会
    • Place of Presentation
      名古屋工業大学(愛知県名古屋市)
    • Related Report
      2016 Annual Research Report
    • Invited
  • [Presentation] Application of Synchrotron Radiation Mossbauer Spectroscopy to Samarium Compounds2016

    • Author(s)
      S. Tsutsui, Y. Kobayashi, Y. Yoda, R. Masuda, K. Mizuuchi, Y. Shimizu, H. Hidaka, T. Yanagisawa, H. Amitsuka, F. Iga and M. Seto
    • Organizer
      Mediterranean Conference on the Applications of the Mossbauer Effect (MECAME2016)
    • Place of Presentation
      Cavtat in Croatia
    • Year and Date
      2016-05-31
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Quadrupole-Driven Non-Fermi Liquid Behaviors in Pr 1-2-20 System2016

    • Author(s)
      T. Onimaru
    • Organizer
      J-Physics: Mini International Workshop: “Physics of Strongly Correlated Electron Systems under Extreme Conditions”
    • Place of Presentation
      神戸大学六甲台キャンパス(兵庫県神戸市)
    • Year and Date
      2016-04-13
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] エネルギー分散型放射光メスバウアー分光のSm化合物への応用2016

    • Author(s)
      筒井智嗣
    • Organizer
      第4回先進的放射光メスバウアー分光のSm化合物への応用
    • Place of Presentation
      名古屋工業大学
    • Year and Date
      2016-03-03
    • Related Report
      2015 Research-status Report
    • Invited
  • [Presentation] Quadrupole-driven exotic phenomena in non-Kramers doublet systems2016

    • Author(s)
      T. Onimaru
    • Organizer
      13th German-Japanese symposium: Effects of Parity Mixing in Correlated Electron Systems
    • Place of Presentation
      北海道札幌市
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Os-2p Magnetic Circular Dichroism of a Heavy Fermion Compound SmOs4Sb122015

    • Author(s)
      Satoshi Tsutsui
    • Organizer
      Application of XAFS to the Study of magnetic materials
    • Place of Presentation
      Max-Planck Institute, Stuttgart
    • Year and Date
      2015-08-30
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research

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Published: 2015-04-16   Modified: 2018-03-22  

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