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Enhancement of tritium isotope separation by using packings packed with materials coated with adsorption

Research Project

Project/Area Number 15K14281
Research Category

Grant-in-Aid for Challenging Exploratory Research

Allocation TypeMulti-year Fund
Research Field Nuclear fusion studies
Research InstitutionKyushu University

Principal Investigator

Fukada Satoshi  九州大学, 総合理工学研究院, 教授 (50117230)

Project Period (FY) 2015-04-01 – 2018-03-31
Project Status Completed (Fiscal Year 2017)
Budget Amount *help
¥3,770,000 (Direct Cost: ¥2,900,000、Indirect Cost: ¥870,000)
Fiscal Year 2017: ¥650,000 (Direct Cost: ¥500,000、Indirect Cost: ¥150,000)
Fiscal Year 2016: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2015: ¥2,210,000 (Direct Cost: ¥1,700,000、Indirect Cost: ¥510,000)
Keywordsトリチウム / 蒸留 / 吸着 / 同位体分離係数 / 同位体交換 / ヒートポンプ / トリチウム水 / 同位体分離 / 気液分散
Outline of Final Research Achievements

We performed isotope separation using water distillation towers packed with materials coated with adsorptive zeolite under reduced pressure to detritiate radioactive tritium water. The method had defects of lower isotope separation factor although distillation is preferable for detritiation of a large amount of water because of no use of catalytic materials, Therefore, it needs a large amount of energy to detritiate it for applications to tritium processing. In the present study, we propose a new isotope separation method for deuterium or tritium using water distillation towers packed with materials coated with zeolite showing higher separation factor in meso-porous part. We have performed isotope separation experiment using radioactive tritium or deuterium, and results are presented in English journals after severe reviewing and also in several international patents. Our results will be helpful for detritiation processes in the future fusion reactor also in Fukushima 1F wastewater.

Report

(4 results)
  • 2017 Annual Research Report   Final Research Report ( PDF )
  • 2016 Research-status Report
  • 2015 Research-status Report
  • Research Products

    (31 results)

All 2018 2017 2016 2015

All Journal Article (14 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 14 results,  Open Access: 10 results,  Acknowledgement Compliant: 2 results) Presentation (13 results) (of which Int'l Joint Research: 9 results,  Invited: 5 results) Patent(Industrial Property Rights) (4 results)

  • [Journal Article] Tritium water distillation assisted with adsorption and isotopic exchange2017

    • Author(s)
      Yoshiaki Miho, Satoshi Fukada, Tomohiro Motomura, Satoru Hirano, Jyunji Mizutani
    • Journal Title

      Fusion Science and Technology

      Volume: 71 Issue: 3 Pages: 726-732

    • DOI

      10.1080/15361055.2017.1291235

    • Related Report
      2017 Annual Research Report 2016 Research-status Report
    • Peer Reviewed
  • [Journal Article] Transient Behavior in Water Distillation Tower for Tritium Separation and Its Long-time Operation Test Results2017

    • Author(s)
      Yoshiaki Miho, Satoshi Fukada, Mitsuki Arimoto, Takaho Takeuchi, Tomohiro Motomura, Junji Mizutani and Satoru Hirano
    • Journal Title

      Journal of Power and Energy Engineering

      Volume: 5 Issue: 03 Pages: 1-17

    • DOI

      10.4236/jpee.2017.53001

    • Related Report
      2017 Annual Research Report 2016 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] Disposal procedure for contaminated surface of tritium handling facility in the decommissioning operation2017

    • Author(s)
      Toshiharu Takeishi, Kazuya Furuichi, Kazunari Katayama, Ryotaro Yamamoto, Yoshiya Kawabata, Satoshi Fukada
    • Journal Title

      Fusion Engineering and Design

      Volume: 128 Pages: 231-234

    • DOI

      10.1016/j.fusengdes.2017.04.013

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Measurement of tritium in tungsten deposition layer by imaging plate technique after exposure to gaseous tritium2017

    • Author(s)
      M. Noguchi, K. Katayama, Y. Torikaia, N. Ashikawa, A. Taguchi, S. Fukada
    • Journal Title

      Fusion Engineering and Design

      Volume: 124 Pages: 257-261

    • DOI

      10.1016/j.fusengdes.2017.04.076

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Estimation of Tritium Permeation Rate to Cooling Water in Fusion DEMO Condition2017

    • Author(s)
      Kazunari Katayama, Youji Someya, Kenji Tobita, Hirofumi Nakamura, Hisashi Tanigawa, Makoto Nakamura, Nobuyuki Asakura, Kazuo Hoshino, Takumi Chikada, Yuji Hatano, Satoshi Fukada
    • Journal Title

      Fusion Science and Technology

      Volume: 71 Issue: 3 Pages: 261-267

    • DOI

      10.1080/15361055.2017.1288423

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Direct decomposition processing of tritiated methane by helium RF plasma2017

    • Author(s)
      Kazunari Katayama, Satoshi Fukada
    • Journal Title

      Fusion Science and Technology

      Volume: 71 Issue: 3 Pages: 426-431

    • DOI

      10.1080/15361055.2017.1293412

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] Study on transfer behavior of hydrogen isotopes from fluidized Li to Y for Li blanket2017

    • Author(s)
      Y. Yamasaki, S. Fukada, K. Hiyane, K. Katayama
    • Journal Title

      Fusion Science and Technology

      Volume: 71 Issue: 4 Pages: 501-506

    • DOI

      10.1080/15361055.2017.1291028

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] Review of recent japanese activities on tritium accountability in fusion reactors2016

    • Author(s)
      Fukada, S., Oya, Y., Hatano, Y.
    • Journal Title

      Fusion Engineering and Design

      Volume: 113 Pages: 231-235

    • DOI

      10.1016/j.fusengdes.2016.08.029

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] Tritium permeation behavior through pyrolytic carbon in tritium production using high-temperature gas-cooled reactor for fusion reactors2016

    • Author(s)
      Hiroki Ushida , Kazunai Katayama , Hideaki Matsuura , R. Yamamoto , Satoshi Fukada , Minoru Goto , Shigeaki Nakagawa
    • Journal Title

      Nuclear Materials and Energy

      Volume: 9 Pages: 524-528

    • DOI

      10.1016/j.nme.2016.09.004

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Low tritium partial pressure permeation system for mass transport measurement in lead lithium eutectic2016

    • Author(s)
      R.J. Pawelko, M. Shimada, K. Katayama, S. Fukada, P.W. Humrickhouse, T. Terai
    • Journal Title

      Fusion Engineering and Design

      Volume: 102 Pages: 8-13

    • DOI

      10.1016/j.fusengdes.2015.11.005

    • Related Report
      2016 Research-status Report 2015 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Correlation of rates of tritium migration through porous concret2015

    • Author(s)
      Satoshi Fukada, K. Katayama, T. Takeishi, Y. Edao, Y. Kawamura, T. Yamanishi
    • Journal Title

      Fusion Science and Technology

      Volume: 67 Issue: 2 Pages: 339-342

    • DOI

      10.13182/fst14-t25

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] Measurement of tritium penetration through concrete material covered by various paints coating2015

    • Author(s)
      Y. Edao, Y. Kawamura, R. Kurata, S. Fukada, T. Takeishi, T. Hayashi and T. Yamanishi
    • Journal Title

      Fusion Science and Technology

      Volume: 67 Issue: 2 Pages: 320-323

    • DOI

      10.13182/fst14-t20

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] Tritium desorption behavior from soil exposed to tritiated water2015

    • Author(s)
      Kazuya Furuichi, Kazunari Katayama, Hiroyuki Date, Toshiharu Takeishi, Satoshi Fukada
    • Journal Title

      Fusion Science and Technology

      Volume: 68 Issue: 2 Pages: 458-464

    • DOI

      10.13182/fst14-969

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] Percolation Behavior of Tritiated Water Into a Soil Packed Bed2015

    • Author(s)
      Takuya Honda, Kazunari Katayama, Keiichiro Uehara, Toshiharu Takeishi, Satoshi Fukada
    • Journal Title

      Fusion Science and Technology

      Volume: 67 Issue: 2 Pages: 382-385

    • DOI

      10.13182/fst14-t34

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Presentation] 吸着蒸留法を利用したトリチウム水除染の研究2018

    • Author(s)
      深田智、三保嘉明、大宅諒、片山一成
    • Organizer
      第12回核融合エネルギー連合講演会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 核融合炉二次冷却材としての超臨界CO2におけるトリチウム挙動研究のための実験設備の構築2018

    • Author(s)
      片山一成、芦川直子、中村博文、相良明男、石山新太郎、森大輔、深田 智
    • Organizer
      第12回核融合エネルギー連合講演会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Tritium separation performance of adsorption/exchange distillation tower packed with structured packing2017

    • Author(s)
      Satoshi Fukada, Yoshiaki Miho, Kazunari Katayama
    • Organizer
      2nd Asia-Pacific Symposium on Tritium Science, Sep. 5-8, (2017)
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Recent R&D results on Fusion Nuclear Technology for DEMO reactor in Japan2016

    • Author(s)
      Toshihiko Yamanishi, Satoshi Fukada
    • Organizer
      The 22nd ANS Topical meeting on the Technology of Fusion Energy, TOFE 2016
    • Place of Presentation
      フィラデルフィア, PA, USA
    • Year and Date
      2016-08-22
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Experiment on tritium recovery from liquid blanket materials2016

    • Author(s)
      Satoshi Fukada
    • Organizer
      2016 Korea-Japan Tritium workshop
    • Place of Presentation
      ソウル、韓国
    • Year and Date
      2016-06-05
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Overview of Fusion-Related Tritium Research in Japanese Universities2016

    • Author(s)
      Yuji Hatano, Yasuhisa Oya, Satoshi Konishi, Satoshi Fukada, Akio Sagara
    • Organizer
      11th International Conference on Tritium Science & Technology, Tritium 2016
    • Place of Presentation
      チャールストン, SC, USA
    • Year and Date
      2016-04-17
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Estimation of Tritium Permeation Rate to Cooling Water in Fusion DEMO Condition2016

    • Author(s)
      Kazunari Katayama, Youji Someya, Kenji Tobita, Hirofumi Nakamura, Hisashi Tanigawa, Makoto Nakamura, Nobuyuki Asakura, Takumi Chikada, Yuji Hatano, Satoshi Fukada
    • Organizer
      11th International Conference on Tritium Science & Technology, Tritium 2016
    • Place of Presentation
      チャールストン, SC, USA
    • Year and Date
      2016-04-17
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research
  • [Presentation] Tritium water distillation assisted with adsorption and isotopic exchange2016

    • Author(s)
      Satoshi Fukada, Tomohiro Motomura, Satoru Hirano, Jyunji Mizutani, Yoshiaki Miho
    • Organizer
      11th International Conference on Tritium Science & Technology, Tritium 2016
    • Place of Presentation
      チャールストン, SC, USA
    • Year and Date
      2016-04-17
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research
  • [Presentation] 水分吸着性能を有した充填材を含む蒸留塔における同位体分離係数の予測2016

    • Author(s)
      深田智
    • Organizer
      日本原子力学会2016年春の年会
    • Place of Presentation
      仙台市、東北大学
    • Year and Date
      2016-03-26
    • Related Report
      2015 Research-status Report
  • [Presentation] Review of recent Japanese activities on tritium accountability in fusion reactors2015

    • Author(s)
      Satoshi Fukada, Yasuhisa Oya, Yuji Hatano
    • Organizer
      Asia and Pacific Symposium on Tritium Science, APSOT-1
    • Place of Presentation
      Mianyang, Sichuan, China
    • Year and Date
      2015-11-01
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Correlation of multi-component hydrogen isotope mixtures absorbing in or permeating through metals2015

    • Author(s)
      S. Fukada, K. Katayama
    • Organizer
      Asia and Pacific Symposium on Tritium Science, APSOT-1
    • Place of Presentation
      Mianyang, Sichuan, China
    • Year and Date
      2015-11-01
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] 各種金属への水素同位体混合ガス吸収脱離時の同位体効果と同位体分離係数の関係2015

    • Author(s)
      深田智、片山一成
    • Organizer
      日本原子力学会2015年秋の大会
    • Place of Presentation
      静岡市、静岡大学
    • Year and Date
      2015-09-09
    • Related Report
      2015 Research-status Report
  • [Presentation] Separation of tritium in multi-component water and gas heading for detritiation of Fukushima's wastewater2015

    • Author(s)
      Satoshi Fukada
    • Organizer
      2015 Japan Korea Tritium Workshop
    • Place of Presentation
      福岡市,九州大学
    • Year and Date
      2015-06-04
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Patent(Industrial Property Rights)] トリチウム水蒸留装置及びトリチウム水蒸留方法2016

    • Inventor(s)
      平野悟、湯浅升夫、元村智博、水谷淳二、深田智
    • Industrial Property Rights Holder
      平野悟、湯浅升夫、元村智博、水谷淳二、深田智
    • Industrial Property Rights Type
      特許
    • Filing Date
      2016-06-08
    • Related Report
      2016 Research-status Report
  • [Patent(Industrial Property Rights)] 充填材、該充填材を用いた蒸留分離方法及び蒸留分離装置2016

    • Inventor(s)
      水谷淳二、深田智
    • Industrial Property Rights Holder
      水谷淳二、深田智
    • Industrial Property Rights Type
      特許
    • Filing Date
      2016-04-25
    • Related Report
      2016 Research-status Report
  • [Patent(Industrial Property Rights)] 充填材、該充填材を用いた蒸留分離方法および蒸留分離装置2015

    • Inventor(s)
      水谷淳二、深田智
    • Industrial Property Rights Holder
      水谷淳二、深田智
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      2015-090539
    • Filing Date
      2015-04-27
    • Related Report
      2015 Research-status Report
  • [Patent(Industrial Property Rights)] トリチウム水蒸留装置及びトリチウム水蒸留方法2015

    • Inventor(s)
      水谷淳二、深田智
    • Industrial Property Rights Holder
      水谷淳二、深田智
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      2015-115478
    • Filing Date
      2015-06-08
    • Related Report
      2015 Research-status Report

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Published: 2015-04-16   Modified: 2019-03-29  

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