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Ultrafast infrared absorption spectroscopy by using single-cycle mid-infrared pulse

Research Project

Project/Area Number 15K17475
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeMulti-year Fund
Research Field Optical engineering, Photon science
Research InstitutionInstitute for Molecular Science

Principal Investigator

shirai Hideto  分子科学研究所, 分子制御レーザー開発研究センター, 特任助教 (30726237)

Project Period (FY) 2015-04-01 – 2017-03-31
Project Status Completed (Fiscal Year 2016)
Budget Amount *help
¥4,290,000 (Direct Cost: ¥3,300,000、Indirect Cost: ¥990,000)
Fiscal Year 2016: ¥2,080,000 (Direct Cost: ¥1,600,000、Indirect Cost: ¥480,000)
Fiscal Year 2015: ¥2,210,000 (Direct Cost: ¥1,700,000、Indirect Cost: ¥510,000)
Keywords超短光パルス / 赤外吸収分光 / 非線形光学 / 赤外分光 / 超高速分光
Outline of Final Research Achievements

We report novel MIR spectroscopy, which is the combination of an ultra-broadband MIR coherent light source and the chirped-pulse up-conversion (CPU) technique. Moreover, attenuated total reflectance spectroscopy connected with the CPU technique for observing the chemical reaction dynamics of liquid samples on real-time. We succeeded in observation of the changes of absorption spectra of liquids samples in the region from 200 to 5500 cm-1 with 1 ms time resolution by using the novel MIR spectroscopy. We believe that this unique system is useful for advanced studies of biological tissues.

Report

(3 results)
  • 2016 Annual Research Report   Final Research Report ( PDF )
  • 2015 Research-status Report
  • Research Products

    (13 results)

All 2017 2016 2015 Other

All Int'l Joint Research (2 results) Journal Article (4 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 4 results,  Open Access: 4 results,  Acknowledgement Compliant: 4 results) Presentation (7 results) (of which Int'l Joint Research: 3 results,  Invited: 1 results)

  • [Int'l Joint Research] 国立交通大学(台湾)

    • Related Report
      2016 Annual Research Report
  • [Int'l Joint Research] National Chiao Tung University(Taiwan)

    • Related Report
      2015 Research-status Report
  • [Journal Article] Ultrafast carrier dynamics in Ge by ultra-broadband mid-infrared probe spectroscopy2017

    • Author(s)
      T. -T. Teh, H. Shirai, C. -M. Tu, T. Fuji, T. Kobayashi, and C. -W. Luo
    • Journal Title

      Scientific Reports

      Volume: 7 Issue: 1 Pages: 1-10

    • DOI

      10.1038/srep40492

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Ultrabroadband Midinfrared Pump-Probe Spectroscopy Using Chirped-Pulse Up-conversion in Gases2015

    • Author(s)
      Hideto Shirai, Tien-Tien Yeh, Yutaka Nomura, Chih-Wei Luo, and Takao Fuji
    • Journal Title

      Physcal Review Applied

      Volume: 3 Issue: 5 Pages: 051002-051002

    • DOI

      10.1103/physrevapplied.3.051002

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Generation and Characterization of Phase-Stable Sub-Single- Cycle Pulses at 3000 cm^{-1}2015

    • Author(s)
      Takao Fuji, Yutaka Nomura, and Hideto Shirai
    • Journal Title

      IEEE JOURNAL OF SELECTED TOPICS IN QUANTUM ELECTRONICS

      Volume: 21 Issue: 5 Pages: 8700612-8700612

    • DOI

      10.1109/jstqe.2015.2426415

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Ultrabroadband mid-infrared spectroscopy with four-wave difference frequency generation2015

    • Author(s)
      Takao Fuji, Hideto Shirai, and Yutaka Nomura
    • Journal Title

      Journal of optics

      Volume: 17 Issue: 9 Pages: 094004-094004

    • DOI

      10.1088/2040-8978/17/9/094004

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Presentation] 超広帯域コヒーレント赤外光を用いた化学反応ダイナミクスの観測2017

    • Author(s)
      白井英登、野村雄高、古谷裕司、藤貴夫
    • Organizer
      レーザー学会学術講演会37回年次大会
    • Place of Presentation
      徳島大学常三島キャンパス、徳島県、徳島市
    • Year and Date
      2017-01-07
    • Related Report
      2016 Annual Research Report
  • [Presentation] Self-Referenced Waveform Measurement of Few-Cycle Mid-Infrared Pulses2016

    • Author(s)
      H. Shirai, Y. Nomura, and T. Fuji
    • Organizer
      20th Interbational Conference on Ultrafast Phenomena
    • Place of Presentation
      Santa Fe, New Mexico United State
    • Year and Date
      2016-07-17
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Observation of Electric Field of Few-Cycle Mid-Infrared Pulse by Self-Referencing2016

    • Author(s)
      Hideto Shirai, Yutaka Nomura, Takao Fuji
    • Organizer
      Ultrafast Phenomena 2016
    • Place of Presentation
      Santa Fe Community Convention Center, Santa Fe, New Mexico, USA
    • Year and Date
      2016-06-17
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] 超短中赤外光パルスを用いた新規分光法の開発と応用2016

    • Author(s)
      白井英登
    • Organizer
      日本分光学会 先端レーザー分光部会
    • Place of Presentation
      東京工業大学大岡山キャンパス本館(東京都目黒区大岡山2-12-1)
    • Year and Date
      2016-03-10
    • Related Report
      2015 Research-status Report
    • Invited
  • [Presentation] 自己参照でのサブサイクル中赤外光パルスの 電場波形計測2016

    • Author(s)
      白井英登, 野村雄高, 藤貴夫
    • Organizer
      レーザー学会
    • Place of Presentation
      名城大学天白キャンパス(愛知県名古屋市天白区塩釜口1-501)
    • Year and Date
      2016-01-09
    • Related Report
      2015 Research-status Report
  • [Presentation] Ultrabroadband Mid-Infrared Pump-Probe Spectroscopy using Chirped-Pulse Upconversion2015

    • Author(s)
      Hideto Shirai, Tien-Tien Yeh, Yutaka Nomura, Chih-Wei Luo, Takao Fuji
    • Organizer
      CLEO2015
    • Place of Presentation
      San Jose Convention Center San Jose, USA
    • Year and Date
      2015-05-10
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] 気体を用いたチャープパルス上方変換による 超広帯域中赤外ポンプ・プローブ分光2015

    • Author(s)
      白井英登
    • Organizer
      国際光年記念シンポジウム
    • Place of Presentation
      東京大学安田講堂(東京都文京区本郷7-3-1)
    • Year and Date
      2015-04-21
    • Related Report
      2015 Research-status Report

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Published: 2015-04-16   Modified: 2022-03-01  

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