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Exploration of pseudogap in organic superconductors by pump probe spectroscopy

Research Project

Project/Area Number 15K17685
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeMulti-year Fund
Research Field Condensed matter physics II
Research InstitutionHokkaido University

Principal Investigator

Tsuchiya Satoshi  北海道大学, 工学研究院, 助教 (80597633)

Project Period (FY) 2015-04-01 – 2018-03-31
Project Status Completed (Fiscal Year 2017)
Budget Amount *help
¥4,160,000 (Direct Cost: ¥3,200,000、Indirect Cost: ¥960,000)
Fiscal Year 2017: ¥650,000 (Direct Cost: ¥500,000、Indirect Cost: ¥150,000)
Fiscal Year 2016: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Fiscal Year 2015: ¥2,080,000 (Direct Cost: ¥1,600,000、Indirect Cost: ¥480,000)
Keywords有機分子結晶 / 擬ギャップ / ポンププローブ分光 / 時間分解分光 / 有機超伝導体 / 超伝導ゆらぎ
Outline of Final Research Achievements

In this study, we carried out the pump probe spectroscopy in organic molecular superconductors, which have different electron correlation, to investigate the pseudgap (PG) and its relationship with superconductivity (SC) in terms of electron correlation. As a result, we find that the PG responses are observed at 70-80 K, which are much higher than the SC transition temperature (Tc) of 10-13 K. Moreover, their temperature dependences are different from each compound, indicating that the electron correlation plays crucial role for emergence of the PG. On the other hand, below Tc, the SC responses are observed in addition to the PG responses. This implies that PG and SC are coexisted below Tc. From the measurements under rapid cooling conditions, we reveal that a structural ordering of molecules affects the PG response.

Report

(4 results)
  • 2017 Annual Research Report   Final Research Report ( PDF )
  • 2016 Research-status Report
  • 2015 Research-status Report
  • Research Products

    (21 results)

All 2018 2017 2016 2015 Other

All Int'l Joint Research (1 results) Journal Article (4 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 4 results,  Open Access: 1 results,  Acknowledgement Compliant: 3 results) Presentation (16 results) (of which Int'l Joint Research: 6 results,  Invited: 4 results)

  • [Int'l Joint Research] ヨゼフステファン研究所(スロベニア)

    • Related Report
      2017 Annual Research Report
  • [Journal Article] Photoinduced phase separation with local structural ordering in organic molecular conductors2017

    • Author(s)
      S. Tsuchiya, K. Nakagawa, J. Yamada, H. Taniguchi, and Y. Toda
    • Journal Title

      Phys. Rev. B

      Volume: 96 Issue: 13 Pages: 1343111-6

    • DOI

      10.1103/physrevb.96.134311

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Carrier Relaxation Dynamics in the Organic Superconductor κ-(BEDT-TTF)2Cu(NCS)2 Under Pressure2016

    • Author(s)
      S. Tsuchiya, K. Nakagawa, J. Yamada and Y. Toda
    • Journal Title

      Journal of Superconductivity and Novel Magnetism

      Volume: 29 Issue: 12 Pages: 3751-4

    • DOI

      10.1007/s10948-016-3751-4

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Pump- and Probe-polarization Analyses of Ultrafast Carrier Dynamics in Organic Superconductors2016

    • Author(s)
      K. Nakagawa, S. Tsuchiya, J. Yamada, Y. Toda
    • Journal Title

      Journal of Superconductivity and Novel Magnetism

      Volume: 29 Issue: 12 Pages: 3741-6

    • DOI

      10.1007/s10948-016-3741-6

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Development of an optical time-resolved measurement system under high-pressure and low-temperature with a piston-cylinder pressure cell2016

    • Author(s)
      Satoshi Tsuchiya, Yohei Kino, Koichi Nakagawa, Daisuke Nakagawa, Jun-ichi Yamada, and Yasunori Toda
    • Journal Title

      Review of Scientific Instruments

      Volume: 87 Issue: 4

    • DOI

      10.1063/1.4945303

    • NAID

      120005740334

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Presentation] 重水素化ドナーを含んだ有機超伝導体k-(ET)2Cu[N(CN)2]Brにおける光励起キャリアダイナミクスの温度特性2018

    • Author(s)
      中川紘一、土屋聡、山田順一、戸田泰則
    • Organizer
      第73回日本物理学会年次大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 偏光時間分解分光測定を用いたモット臨界近傍の有機超伝導体における超伝導ゆらぎの探索2018

    • Author(s)
      中川紘一、土屋聡、谷口弘三、戸田泰則
    • Organizer
      第53回応用物理学会北海道支部/第14回日本光学会北海道地区合同学術講演会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 急冷した有機超伝導体における光励起準粒子ダイナミクス2018

    • Author(s)
      佐藤貴裕、土屋聡、山田順一、戸田泰則
    • Organizer
      第53回応用物理学会北海道支部/第14回日本光学会北海道地区合同学術講演会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Fluctuating Superconductivity in Partially Deuterated k-(ET)2[N(CN)2]Br Studied by Polarized Time-Resolved Spectroscopy2017

    • Author(s)
      K. Nakagawa, S. Tsuchiya, H. Taniguchi, Y. Toda
    • Organizer
      12th International Symposium on Crystalline Organic Metals, Superconductors and Magnets
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Effect of rapid cooling on photo-induced carrier dynamics in k-(BEDT-TTF)2X (X = Cu[N(CN)2]Br and Cu(NCS)2)2017

    • Author(s)
      T. Sato, S. Tsuchiya, J. Yamada, Y. Toda
    • Organizer
      12th International Symposium on Crystalline Organic Metals, Superconductors and Magnets
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] K. Nakagawa, S. Tsuchiya, H. Taniguchi, Y. Toda, "Photo-induced Carrier Relaxation Dynamics in Mott Insulator k-(BEDT-TTF)2Cu[N(CN)2]Cl Probed by Probe Polarization2017

    • Author(s)
      K. Nakagawa, S. Tsuchiya, H. Taniguchi, Y. Toda
    • Organizer
      6th International Conference on Photoinduced Phase Transitions
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Electron Correlation Effect on Non-equilibrium Phase Separation Studied by Polarized Femtosecond Spectroscopy2016

    • Author(s)
      K. Nakagawa,S. Tsuchiya, J. Yamada, Y. Toda
    • Organizer
      Emallia Conference 2016 Winte
    • Place of Presentation
      Sapporo, Hokkaido
    • Year and Date
      2016-12-19
    • Related Report
      2016 Research-status Report
  • [Presentation] Femtosecond relaxation dynamics in strongly correlated organic superconductors k-(BEDT-TTF)2X (X = Cu[N(CN)2]Br and Cu(NCS)2)2016

    • Author(s)
      S. Tsuchiya, K. Nakagawa, J. Yamada, Y. Toda
    • Organizer
      The EMN meeting on Ultrafast 2016
    • Place of Presentation
      Melbourne, Australia
    • Year and Date
      2016-10-10
    • Related Report
      2016 Research-status Report
    • Invited
  • [Presentation] 偏光時間分解分光を用いたκ-(BEDT-TTF)2X(X=Cu[N(CN)2]Br,Cu(NCS)2)における超伝導ゆらぎの探索2016

    • Author(s)
      中川紘一,土屋聡,山田順一,戸田泰則
    • Organizer
      日本物理学会2016年秋季大会
    • Place of Presentation
      金沢大学 角間キャンパス
    • Year and Date
      2016-09-14
    • Related Report
      2016 Research-status Report
  • [Presentation] Quasiparticle dynamics in the organic superconductors investigated with polarized femtosecond spectroscopy2016

    • Author(s)
      S. Tsuchiya, K. Nakagawa, J. Yamada, Y. Toda
    • Organizer
      International Conference Superstripes 2016
    • Place of Presentation
      Ischia, Italy
    • Year and Date
      2016-06-23
    • Related Report
      2016 Research-status Report
    • Invited
  • [Presentation] Fluctuating Superconductivity in the Strongly Correlated Organic Superconductors in κ-(BEDT-TTF)2X (X = Cu[N(CN)2]Br,Cu(NCS)2) Studied by Polarized Femtosecond Spectroscopy2016

    • Author(s)
      K. Nakagawa, S. Tsuchiya, J. Yamada, Y. Toda
    • Organizer
      International Conference Superstripes 2016
    • Place of Presentation
      Ischia, Italy
    • Year and Date
      2016-06-23
    • Related Report
      2016 Research-status Report
    • Invited
  • [Presentation] Quasiparticle dynamics in the organic superconductors investigated with polarized femtosecond spectroscopy2016

    • Author(s)
      Satoshi Tsuchiya, Koichi Nakagawa, Jun-ichi Yamada, Yasunori Toda
    • Organizer
      Superstripes2016
    • Place of Presentation
      Ischia, Italy
    • Year and Date
      2016-06-23
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Fluctuating Superconductivity in the Strongly Correlated Organic Superconductors in k -(BEDT-TTF)2X (X = Cu[N(CN)2]Br, Cu(NCS)2) Studied by Polarized Femtosecond Spectroscopy2016

    • Author(s)
      Koichi Nakagawa, Satoshi Tsuchiya, Jun-ichi Yamada, Yasunori Toda
    • Organizer
      Superstripes2016
    • Place of Presentation
      Ischia, Italy
    • Year and Date
      2016-06-23
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] 有機超伝導体k-(BEDT-TTF)2X (X=Cu[N(CN)2]Br, Cu(NCS)2)における光励起準粒子緩和の温度特性2016

    • Author(s)
      中川 紘一, 土屋 聡, 山田 順一, 戸田 泰則
    • Organizer
      第51回応用物理学会北海道支部学術講演会
    • Place of Presentation
      北海道大学 札幌市
    • Year and Date
      2016-01-09
    • Related Report
      2015 Research-status Report
  • [Presentation] k-(ET)2Cu(NCS)2におけるポンプ-プローブ時間分解分光2015

    • Author(s)
      土屋聡、中川紘一、山田順一、戸田泰則
    • Organizer
      日本物理学会2015年秋季大会
    • Place of Presentation
      関西大学千里山キャンパス 吹田市
    • Year and Date
      2015-09-16
    • Related Report
      2015 Research-status Report
  • [Presentation] Photo-induced phase separation in metallic phase of the organic compound k-(ET)2Cu(NCS)22015

    • Author(s)
      Satoshi Tsuchiya, Koichi Nakagawa, Jun-ichi Yamada, Yasunori Toda
    • Organizer
      International Symposium of Crystalline Organic Metals, Superconductors and Magnets
    • Place of Presentation
      Bad Gögging, Germany
    • Year and Date
      2015-09-06
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research

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Published: 2015-04-16   Modified: 2020-05-15  

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