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Design methodology for gas-liquid-solid catalytic reactor focused on transport phenomena in micro-space and its application to C1 chemistry

Research Project

Project/Area Number 15K18263
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeMulti-year Fund
Research Field Reaction engineering/Process system
Research InstitutionNational Institute of Advanced Industrial Science and Technology

Principal Investigator

FUKUDA Takashi  国立研究開発法人産業技術総合研究所, 材料・化学領域, 研究員 (50734969)

Project Period (FY) 2015-04-01 – 2018-03-31
Project Status Completed (Fiscal Year 2017)
Budget Amount *help
¥4,030,000 (Direct Cost: ¥3,100,000、Indirect Cost: ¥930,000)
Fiscal Year 2017: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2016: ¥1,300,000 (Direct Cost: ¥1,000,000、Indirect Cost: ¥300,000)
Fiscal Year 2015: ¥1,820,000 (Direct Cost: ¥1,400,000、Indirect Cost: ¥420,000)
Keywordsマイクロリアクター / 反応器設計 / プレート型反応器 / メタン改質 / 混相流 / 炭素析出 / 低圧力損失 / 熱交換性能 / スラグ流 / CFD計算 / 触媒反応 / マイクロリアクタ
Outline of Final Research Achievements

The micro chemical process recently attracts attentions in manufacture of high value-added products. Since the micro-space gives an excellent contact efficiency, the advantages of the microreactor have been frequently applied to multiphase reaction systems. On the other hand, the reaction's complexity has hindered its dissemination. Thus author set the purpose of this research as to provide simple design guidelines. And author clarified and generalized the influence of reaction rate and mass transfer rate on reaction performance in a catalytic wall plate reactor (CWPR) for methane reforming, which is the basic reaction for a dispersed chemical production and C1 chemistry. CWPR is divided into the gas phase and the solid catalytic phase, and by consideration of this analogy, author confirms a suggestion that the proposed design guideline has validity even in a design of a complex gas-liquid-solid catalytic reaction system.

Report

(5 results)
  • 2017 Annual Research Report   Final Research Report ( PDF )
  • 2016 Research-status Report
  • 2015 Research-status Report
  • Products Report
  • Research Products

    (19 results)

All 2023 2018 2017 2016

All Journal Article (2 results) (of which Peer Reviewed: 2 results,  Open Access: 1 results,  Acknowledgement Compliant: 1 results) Presentation (11 results) (of which Int'l Joint Research: 2 results,  Invited: 1 results) Book (3 results) Patent(Industrial Property Rights) (3 results)

  • [Journal Article] Development of a Newly Catalytic Plate-type Reactor and Its Evaluation of Methane Conversion and Pressure Drop in Dry Reforming of Methane2017

    • Author(s)
      Takashi Fukuda, Hajime Kawanami, Akira Miyazawa
    • Journal Title

      JOURNAL OF CHEMICAL ENGINEERING OF JAPAN

      Volume: 50 Issue: 8 Pages: 657-665

    • DOI

      10.1252/jcej.16we342

    • NAID

      130005988457

    • ISSN
      0021-9592, 1881-1299
    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Development of a newly catalytic plate-type reactor and its evaluation of methane conversion and pressure drop in dry reforming of methane2017

    • Author(s)
      Takashi Fukuda, Hajime Kawanami, Akira Miyazawa
    • Journal Title

      Journal of Chemical Engineering of Japan

      Volume: 印刷中

    • NAID

      130005988457

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Presentation] 種々の酸化剤によるメタン改質反応への影響2018

    • Author(s)
      福田 貴史, 原田 亮, 川波 肇, 宮沢 哲
    • Organizer
      化学工学第83回年会
    • Related Report
      2017 Annual Research Report
  • [Presentation] プレート型反応器を用いたメタン改質の検討(3) -水蒸気改質への展開-2017

    • Author(s)
      福田 貴史、川波 肇、宮沢 哲
    • Organizer
      化学工学会第82年会
    • Place of Presentation
      芝浦工業大学(東京都港区)
    • Year and Date
      2017-03-06
    • Related Report
      2016 Research-status Report
  • [Presentation] マイクロリアクターによるメタン改質時の流路閉塞制御技術2017

    • Author(s)
      福田 貴史
    • Organizer
      化学工学会関西支部主催マイクロプロセス最前線シリーズ
    • Related Report
      2017 Annual Research Report
  • [Presentation] 資源循環を目指した化学装置開発 ~新規メタン改質器~2017

    • Author(s)
      福田 貴史
    • Organizer
      JPIJS北海道・東北地区講演会
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] Methane reforming in a catalytic plate reactor for high-throughput production2017

    • Author(s)
      T. Fukuda, H. Kawanami, and A. Miyazawa
    • Organizer
      17th Congress of Asian-Pacific Confederation of Chemical Engineering, Proceedings (17th APCChE)
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Methane reforming in a catalytic plate reactor for high-throughput production2016

    • Author(s)
      Takashi Fukuda, Hajime Kawanami, Akira Miyazawa
    • Organizer
      The 14th International Conference on Microreaction Technology
    • Place of Presentation
      Beijing, China
    • Year and Date
      2016-09-12
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research
  • [Presentation] プレート型反応器を用いたメタン改質の検討(2) -濃厚ドライガスの改質-2016

    • Author(s)
      福田 貴史、川波 肇、宮沢 哲
    • Organizer
      化学工学会第48回秋季大会
    • Place of Presentation
      徳島大学(徳島県徳島市)
    • Year and Date
      2016-09-06
    • Related Report
      2016 Research-status Report
  • [Presentation] プレート型反応器を用いたメタン改質の検討2016

    • Author(s)
      福田 貴史、川波 肇、宮沢 哲
    • Organizer
      化学工学会第81年会
    • Place of Presentation
      関西大学 (吹田市)
    • Year and Date
      2016-03-15
    • Related Report
      2015 Research-status Report
  • [Presentation] 気液スラグ流を用いたガス吸収操作設計論2016

    • Author(s)
      正木 理恵、福田 貴史、牧 泰輔、前 一廣
    • Organizer
      化学工学会第81年会
    • Place of Presentation
      関西大学 (吹田市)
    • Year and Date
      2016-03-14
    • Related Report
      2015 Research-status Report
  • [Presentation] プレート型反応器を用いたメタン改質の効率化2016

    • Author(s)
      福田 貴史、川波 肇、宮沢 哲
    • Organizer
      第24回Clayteamセミナー
    • Place of Presentation
      TKPガーデンシティ仙台 (仙台市)
    • Year and Date
      2016-02-18
    • Related Report
      2015 Research-status Report
  • [Presentation] プレート型反応器を用いたメタン改質の効率化2016

    • Author(s)
      福田 貴史、川波 肇、宮沢 哲
    • Organizer
      平成27年度 産総研 材料・化学シンポジウム
    • Place of Presentation
      つくば国際会議場 (つくば市)
    • Year and Date
      2016-02-05
    • Related Report
      2015 Research-status Report
  • [Book] ケミカルエンジニヤリング 63 巻 2 号2018

    • Author(s)
      福田貴史
    • Publisher
      株式会社 化学工業社
    • Related Report
      2017 Annual Research Report
  • [Book] 化学工学 80 巻 4 号 (分担執筆:TOPICS [493])2017

    • Author(s)
      深井 潤、依田 智、垣内田 洋、高橋 和雄、菅野 勉、上田 祐樹、中尾 正喜、森田 真樹、松野 孝充、高橋 勝六、久保田 隆、梅田 富雄、田多 康裕、今井 裕之、福田 貴史、島田 直樹
    • Total Pages
      44
    • Publisher
      公益社団法人 化学工学会
    • Related Report
      2016 Research-status Report
  • [Book] 化学工学 第80巻第4号2016

    • Author(s)
      公益社団法人 化学工学会
    • Total Pages
      44
    • Publisher
      公益社団法人 化学工学会
    • Related Report
      2015 Research-status Report
  • [Patent(Industrial Property Rights)] 積層型反応器2023

    • Inventor(s)
      福田 貴史、原田 亮、宮沢 哲
    • Industrial Property Rights Holder
      国立研究開発法人産業技術総合研究所
    • Industrial Property Rights Type
      特許
    • Acquisition Date
      2023
    • Related Report
      Products Report
  • [Patent(Industrial Property Rights)] 積層型反応器2023

    • Inventor(s)
      福田 貴史、原田 亮、宮沢 哲
    • Industrial Property Rights Holder
      国立研究開発法人産業技術総合研究所
    • Industrial Property Rights Type
      特許
    • Acquisition Date
      2023
    • Related Report
      Products Report
  • [Patent(Industrial Property Rights)] プレート型反応器2016

    • Inventor(s)
      福田貴史
    • Industrial Property Rights Holder
      福田貴史
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      2016-029292
    • Filing Date
      2016-02-18
    • Related Report
      2015 Research-status Report

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Published: 2015-04-16   Modified: 2024-03-28  

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