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Fabrication of Catalyst Nanoparticles by an Innovative Multiphase AC Arc

Research Project

Project/Area Number 15K18265
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeMulti-year Fund
Research Field Reaction engineering/Process system
Research InstitutionKyushu University

Principal Investigator

Tanaka Manabu  九州大学, 工学研究院, 助教 (10707152)

Project Period (FY) 2015-04-01 – 2018-03-31
Project Status Completed (Fiscal Year 2017)
Budget Amount *help
¥4,160,000 (Direct Cost: ¥3,200,000、Indirect Cost: ¥960,000)
Fiscal Year 2017: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Fiscal Year 2016: ¥1,300,000 (Direct Cost: ¥1,000,000、Indirect Cost: ¥300,000)
Fiscal Year 2015: ¥1,690,000 (Direct Cost: ¥1,300,000、Indirect Cost: ¥390,000)
Keywords熱プラズマ / 交流アーク / 交流放電 / 多相交流 / ナノ粒子 / 高速度カメラ / ダイオード整流 / 電極消耗 / 多相交流アーク / 金属酸窒化物ナノ粒子 / 高速度可視化 / ナノ粒子前駆体 / 交流電極消耗 / 酸化物ナノ粒子 / 可視化 / ナノ粒子合成
Outline of Final Research Achievements

Fundamental phenomena in a multiphase AC arc as an attractive thermal plasma source has been successfully understood on the basis of a high-speed visualization technique. Optical band-pass filter and the high-speed camera was combined to visualize nanoparticle precursor in thermal plasmas. In the present work, metal oxide nanoparticles such as aluminum oxide and titanium oxide and metal nitride nanoparticles were successfully synthesized. Moreover, their oxide molecular which are precursor of the nanoparticles and temperature field of the multiphase AC arc were visualized. In addition, an innovative generating system of AC arc system has been developed to improve electrode erosion characteristics in the multiphase AC arc on the basis of the understanding of the electrode erosion mechanism in the thermal plasma. Electrode erosion was drastically reduced by new generating system due to the diode-rectification.

Report

(4 results)
  • 2017 Annual Research Report   Final Research Report ( PDF )
  • 2016 Research-status Report
  • 2015 Research-status Report
  • Research Products

    (32 results)

All 2018 2017 2016 2015 Other

All Journal Article (7 results) (of which Peer Reviewed: 7 results,  Open Access: 1 results,  Acknowledgement Compliant: 1 results) Presentation (22 results) (of which Int'l Joint Research: 11 results,  Invited: 1 results) Remarks (2 results) Patent(Industrial Property Rights) (1 results)

  • [Journal Article] Effects of Driving Frequency on Temperature Characteristics in Multiphase AC Arc2018

    • Author(s)
      Takafumi Okuma, Hiroki Maruyama, Manabu Tanaka, Takayuki Watanabe, Hisao Nagai, Takeshi Koiwasaki, and Hiroshi Nasu
    • Journal Title

      IEEE Transactions on Plasma Science

      Volume: 印刷中

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Investigation of Temperature Characteristics of Multiphase AC Arc by High-Speed Visualization2017

    • Author(s)
      Manabu Tanaka, Tomoyuki Imatsuji, Taro Hashizume, Takayuki Watanabe, Hisao Nagai, Takeshi Koiwasaki, and Takafumi Okuma
    • Journal Title

      Journal of Fluid Science and Technology

      Volume: 12 Pages: 17-00131

    • NAID

      130006897041

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Diode-rectified Multiphase AC Arc for Improvement of Electrode Erosion Characteristics2017

    • Author(s)
      Manabu Tanaka, Taro Hashizume, Koki Saga, Tsugio Matsuura, and Takayuki Watanabe
    • Journal Title

      Journal of Physics D: Applied Physics

      Volume: 50 Issue: 46 Pages: 4656044-4656044

    • DOI

      10.1088/1361-6463/aa8cac

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Effect of Arc Current on Droplet Ejection from Tungsten-Based Electrode in Multiphase AC Arc2017

    • Author(s)
      Taro Hashizume, Manabu Tanaka, and Takayuki Watanabe
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 56 Issue: 5 Pages: 056101-056101

    • DOI

      10.7567/jjap.56.056101

    • NAID

      210000147734

    • Related Report
      2017 Annual Research Report 2016 Research-status Report
    • Peer Reviewed
  • [Journal Article] Synthesis of Lithium Metal Oxide Nanoparticles by Induction Thermal Plasmas2016

    • Author(s)
      Manabu Tanaka, Takuya Kageyama, Hirotaka Sone, Shuhei Yoshida, Daisuke Okamoto and Takayuki Watanabe
    • Journal Title

      Nanomaterials

      Volume: 6 Issue: 4 Pages: 60-60

    • DOI

      10.3390/nano6040060

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] Investigation of Erosion Mechanism of Tungsten-Based Electrode in Multi-Phase AC Arc by High-Speed Visualization of Electrode Phenomena2016

    • Author(s)
      Manabu Tanaka, Taro Hashizume, Tomoyuki Imatsuji, Yushi Nawata, and Takayuki Watanabe
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 55 Issue: 7S2 Pages: 07LC01-07LC01

    • DOI

      10.7567/jjap.55.07lc01

    • Related Report
      2016 Research-status Report
    • Peer Reviewed
  • [Journal Article] Investigation of erosion mechanism of tungsten-based electrode in multiphase AC arc by high-speed visualization of electrode phenomena2016

    • Author(s)
      Manabu Tanaka, Taro Hashizume, Tomoyuki Imatsuji, Yushi Nawata, and Takayuki Watanabe
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 印刷中

    • NAID

      210000146865

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Presentation] Improvement of Electrode Erosion Characteristics in Diode-Rectified Multiphase AC Arc2017

    • Author(s)
      Manabu Tanaka, Taro Hashizume, Tsugio Matsuura, and Takayuki Watanabe
    • Organizer
      23rd International Symposium on Plasma Chemistry
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] High-speed visualization of erosion phenomena of tungsten-based electrode in multiphase AC arc2017

    • Author(s)
      Taro Hashizume, Manabu Tanaka, and Takayuki Watanabe
    • Organizer
      23rd International Symposium on Plasma Chemistry
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] High-speed visualization of fluctuation phenomena in multiphase AC arc2017

    • Author(s)
      Manabu Tanaka, Tomoyuki Imatsuji, Taro Hashizume, Takayuki Watanabe, Hisao Nagai, Takeshi Koiwasaki, and Takafumi Okuma
    • Organizer
      The 9th JSME-KSME Thermal and Fluids Engineering Conference
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 多相交流アークを用いた酸化物ナノ粒子生成プロセス中の前駆体蒸気の動的挙動2017

    • Author(s)
      田中学,縄田祐志,斎藤佑樹,橋詰太郎,渡辺隆行
    • Organizer
      化学工学会 第49回秋季大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 高速度カメラを用いた多相交流アークにおける電極現象の可視化2017

    • Author(s)
      田中学,橋詰太郎,渡辺隆行
    • Organizer
      化学工学会 第83年会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 高速度カメラと二波長分光光学系を用いた多相交流アークの電極消耗現象の可視化2017

    • Author(s)
      田中学,橋詰太郎,渡辺隆行
    • Organizer
      高速度イメージングとフォトニクスに関する総合シンポジウム2017
    • Related Report
      2017 Annual Research Report
  • [Presentation] 熱プラズマ中のAl2O3ナノ粒子前駆体の可視化2017

    • Author(s)
      齋藤裕樹,縄田祐志,橋詰太郎,田中学,渡辺隆行
    • Organizer
      高速度イメージングとフォトニクスに関する総合シンポジウム2017
    • Related Report
      2017 Annual Research Report
  • [Presentation] Investigation of Electrode Erosion Mechanism by High-Speed Camera Visualization of Electrode Phenomena in Multiphase AC Arc2017

    • Author(s)
      Manabu Tanaka, Taro Hashizume, Takayuki Watanabe
    • Organizer
      Plasma Conference 2017
    • Related Report
      2017 Annual Research Report
  • [Presentation] ナノ粒子合成に用いる直流窒素アークの陰極消耗機構2017

    • Author(s)
      田中学,吉田匡希,佐倉直喜,渡辺隆行
    • Organizer
      第33回 九州・山口プラズマ研究会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Dynamic Behaviour of Metal Oxide Vapors in Multiphase AC Arc during Oxide Nanoparticle Fabrication Process2016

    • Author(s)
      M. Tanaka, Y. Nawata, T. Imatsuji, and T. Watanabe
    • Organizer
      第26回日本MRS年次大会
    • Place of Presentation
      横浜市開港記念会館
    • Year and Date
      2016-12-19
    • Related Report
      2016 Research-status Report
    • Invited
  • [Presentation] Investigation of Temperature Fluctuation Phenomena in Multiphase AC Arc by High-Speed Camera with Bandpass Filter Optics2016

    • Author(s)
      Manabu Tanaka, Tomoyuki Imatsuji, Yushi Nawata, Taro Hashizume, and Takayuki Watanabe
    • Organizer
      31st International Congress of High-speed Imaging and Photonics
    • Place of Presentation
      Osaka, Japan
    • Year and Date
      2016-11-07
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research
  • [Presentation] Influence of Doped-Metal Oxide on Tungsten-Based Electrode Evaporation in Multiphase AC Arc2016

    • Author(s)
      Taro Hashizume, Seiya Nagao, Manabu Tanaka, and Takayuki Watanabe
    • Organizer
      10th International Conference on Trends in Welding Research
    • Place of Presentation
      Hitotsubashi Hall, Tokyo, Japan
    • Year and Date
      2016-10-11
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research
  • [Presentation] Investigation of Temperature Charactersitcs in Multi-Phase AC Arc by High-Speed Visualization2016

    • Author(s)
      Manabu Tanaka, Tomoyuki Imatsuji, Taro Hashizume, Takayuki Watanabe, Hisao Nagai, Tsuyoshi Koiwasaki, and Takafumi Okuma
    • Organizer
      13th International Conference on Fluid Dynamics
    • Place of Presentation
      Sendai International Center, Sendai, Japan
    • Year and Date
      2016-10-10
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research
  • [Presentation] ダイオード整流による新規な多相交流アーク発生システムの開発2016

    • Author(s)
      田中学, 佐賀弘基, 橋詰太郎, 今辻智幸, 松浦次雄, 渡辺隆行
    • Organizer
      化学工学会第48回秋季大会
    • Place of Presentation
      徳島大学
    • Year and Date
      2016-09-06
    • Related Report
      2016 Research-status Report
  • [Presentation] Influence of Doped Oxide on Tungsten-Based Electrode Evaporation in Multiphase AC Arc2016

    • Author(s)
      Taro Hashizume, Manabu Tanaka, Seiya Nagao, and Takayuki Watanabe
    • Organizer
      14th High-Tech Plasma Processes
    • Place of Presentation
      Munich, Germany
    • Year and Date
      2016-07-03
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research
  • [Presentation] Diode-Rectified Multiphase AC Arc with Bipolar Electrodes for Degradation of Electrode erosion2016

    • Author(s)
      Manabu Tanaka, Tsugio Matsuura, Taro Hashizume, and Takayuki Watanabe
    • Organizer
      14th High-Tech Plasma Processes
    • Place of Presentation
      Munich, Germany
    • Year and Date
      2016-07-03
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research
  • [Presentation] 高速度カメラを用いた多相交流アーク中のCuOナノ粒子生成過程の解明2015

    • Author(s)
      縄田祐志,田中学,今辻智幸,橋詰太郎,渡辺隆行
    • Organizer
      プラズマ・核融合学会 九州・沖縄・山口支部 第19回支部大会
    • Place of Presentation
      熊本大学
    • Year and Date
      2015-12-19
    • Related Report
      2015 Research-status Report
  • [Presentation] High-Speed Visualization of Evaporation Phenomena from Tungsten Based Electrode in Multi-Phase AC Arc2015

    • Author(s)
      Manabu Tanaka, Taro Hashizume, Tomoyuki Imatsuji, Yushi Nawata, and Takayuki Watanabe
    • Organizer
      9th International Conference on Reactive Plasmas
    • Place of Presentation
      Hawaii Convention Center
    • Year and Date
      2015-10-12
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] 高速度カメラを用いた多相交流アークの電極蒸発現象の可視化2015

    • Author(s)
      田中学,橋詰太郎,今辻智幸,縄田祐志,渡辺隆行
    • Organizer
      化学工学会 第47回秋季大会
    • Place of Presentation
      北海道大学
    • Year and Date
      2015-09-09
    • Related Report
      2015 Research-status Report
  • [Presentation] 電極添加酸化物が多相交流アークにおける液滴飛散現象に与える影響2015

    • Author(s)
      橋詰太郎,田中学,今辻智幸,縄田祐志,渡辺隆行
    • Organizer
      化学工学会 第47回秋季大会
    • Place of Presentation
      北海道大学
    • Year and Date
      2015-09-09
    • Related Report
      2015 Research-status Report
  • [Presentation] Fluctuation Phenomena in Multi-Phase AC Arc for Nanoparticles Fabrication2015

    • Author(s)
      Manabu Tanaka, Tomoyuki Imatsuji, Yushi Nawata, Taro Hashizume and Takayuki Watanabe
    • Organizer
      22nd International Symposium on Plasma Chemistry
    • Place of Presentation
      University of Antwerp
    • Year and Date
      2015-07-05
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] Droplet Ejection Mechanism from Tungsten Electrode in Multi-Phase AC Arc by High-Speed Visualization2015

    • Author(s)
      Taro Hashizume, Manabu Tanaka and Takayuki Watanabe
    • Organizer
      22nd International Symposium on Plasma Chemistry
    • Place of Presentation
      University of Antwerp
    • Year and Date
      2015-07-05
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Remarks] 研究室ホームページ

    • URL

      http://www.chem-eng.kyushu-u.ac.jp/lab5/index.html

    • Related Report
      2017 Annual Research Report
  • [Remarks] 個人ページ

    • URL

      http://hyoka.ofc.kyushu-u.ac.jp/search/details/K005271/index.html

    • Related Report
      2017 Annual Research Report
  • [Patent(Industrial Property Rights)] プラズマ発生装置及び方法並びにこれらを用いた微粒子製造装置及び方法2016

    • Inventor(s)
      田中学,渡邉隆行,橋詰太郎,松浦次雄
    • Industrial Property Rights Holder
      田中学,渡邉隆行,橋詰太郎,松浦次雄
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      2016-203678
    • Filing Date
      2016-10-17
    • Related Report
      2016 Research-status Report

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Published: 2015-04-16   Modified: 2019-03-29  

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