• Search Research Projects
  • Search Researchers
  • How to Use
  1. Back to previous page

Adsorption of trace uranium on iron oxides: reconstruction of water chemistry from ancient lakes in Baikal catchment area.

Research Project

Project/Area Number 15K21019
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeMulti-year Fund
Research Field Petrology/Mineralogy/Economic geology
Geochemistry/Cosmochemistry
Research InstitutionKanazawa University

Principal Investigator

Fukushi Keisuke  金沢大学, 環日本海域環境研究センター, 准教授 (90444207)

Project Period (FY) 2015-04-01 – 2018-03-31
Project Status Completed (Fiscal Year 2017)
Budget Amount *help
¥4,160,000 (Direct Cost: ¥3,200,000、Indirect Cost: ¥960,000)
Fiscal Year 2016: ¥2,080,000 (Direct Cost: ¥1,600,000、Indirect Cost: ¥480,000)
Fiscal Year 2015: ¥2,080,000 (Direct Cost: ¥1,600,000、Indirect Cost: ¥480,000)
Keywordsウラン / 鉄酸化物 / 吸着 / 表面錯体モデリング / フブスグル湖 / 水質 / pH / フェリハイドライト / 古水質復元 / 水質復元 / ウラニル
Outline of Final Research Achievements

Uranium concentrations in the sediments core obtained from Lake Hovsgol located in the catchment area of Baikal lake are varied with the core depth depending on the glacial - inter glacial periods. Because the uranium in the sediments was originated from the adsorption process of dissolved uranium onto iron oxide in the lake, the concentration of uranium in the sediments is expected to reflect the changes of water chemistry derived from the climatic change. In present study, the adsorption behavior of trace uranium was examined by adsorption experiments and modeled quantitatively. Results showed that the most important factor affecting the uranium concentrations in the sediments was pH. The adsorption modeling suggested that the pH of lake Hovsgol during the glacial periods, when the uranium concentrations in the sediments were extremely low, exceeded 9.5.

Report

(4 results)
  • 2017 Annual Research Report   Final Research Report ( PDF )
  • 2016 Research-status Report
  • 2015 Research-status Report
  • Research Products

    (25 results)

All 2018 2017 2016 2015

All Journal Article (11 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 9 results,  Open Access: 3 results,  Acknowledgement Compliant: 3 results) Presentation (14 results) (of which Int'l Joint Research: 2 results,  Invited: 4 results)

  • [Journal Article] Amorphous silica-promoted lysine dimerization: A thermodynamic prediction2018

    • Author(s)
      Kitadai N., Nishiuchi K., Nishii A., Fukushi K.
    • Journal Title

      Origin of Life and Evolution of Biospheres

      Volume: 48 Issue: 1 Pages: 23-34

    • DOI

      10.1007/s11084-017-9548-z

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Speciation of Magnesium in monohydrocalcite: XANES, ab initio and geochemical modeling.2017

    • Author(s)
      K. Fukushi, Y. Suzuki, J. Kawano, T. Ohno, M. Ogawa, T. Yaji, and Y. Takahashi,
    • Journal Title

      Geochimica et Cosmochimica Acta

      Volume: 213 Pages: 457-474

    • DOI

      10.1016/j.gca.2017.06.040

    • NAID

      130006198607

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Introduction to the Special Issue “Rock Weathering from Nanoscale to Global Scale: 2. Macroscopic Weathering and Applied Studies”2017

    • Author(s)
      MATSUOKA Norikazu、OGUCHI Chiaki T.、FUKUSHI Keisuke、MATSUSHI Yuki、YOKOYAMA Tadashi
    • Journal Title

      Journal of Geography (Chigaku Zasshi)

      Volume: 126 Issue: 4 Pages: 409-411

    • DOI

      10.5026/jgeography.126.409

    • NAID

      130006105209

    • ISSN
      0022-135X, 1884-0884
    • Related Report
      2017 Annual Research Report
  • [Journal Article] Introduction to the Special Issue “Rock Weathering from Nanoscale to Global Scale: 1. Microscopic Weathering and Basic Studies”2017

    • Author(s)
      MATSUOKA Norikazu、OGUCHI Chiaki T.、FUKUSHI Keisuke、MATSUSHI Yuki、YOKOYAMA Tadashi
    • Journal Title

      Journal of Geography (Chigaku Zasshi)

      Volume: 126 Issue: 3 Pages: 267-269

    • DOI

      10.5026/jgeography.126.267

    • NAID

      130005893326

    • ISSN
      0022-135X, 1884-0884
    • Related Report
      2017 Annual Research Report
  • [Journal Article] Modelling Sorption Processes of Trace Elements by Earth Surface Materials2017

    • Author(s)
      福士圭介
    • Journal Title

      Journal of Geography (Chigaku Zasshi)

      Volume: 126 Issue: 3 Pages: 325-341

    • DOI

      10.5026/jgeography.126.325

    • NAID

      130005893333

    • ISSN
      0022-135X, 1884-0884
    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] 地球表層物質による微量元素とり込み過程とそのモデル化2017

    • Author(s)
      福士圭介
    • Journal Title

      地学雑誌

      Volume: 印刷中

    • NAID

      130005893333

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Glycine polymerization on oxide minerals2017

    • Author(s)
      Kitadai, N., Oonishi H., Umemoto K., Usui T., Fukushi K. and Nakashima S.
    • Journal Title

      Origins of Life and Evolution of Biospheres

      Volume: 印刷中 Issue: 2 Pages: 123-143

    • DOI

      10.1007/s11084-016-9516-z

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Predictive model for Pb(II) adsorption on soil minerals (oxides and low-crystalline aluminum silicate) consistent with spectroscopic evidence2016

    • Author(s)
      Usiyama, T. and Fukushi, K.
    • Journal Title

      Geochimica et Cosmochimica Acta

      Volume: 190 Pages: 134-155

    • DOI

      10.1016/j.gca.2016.06.022

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] High-temperature hydrothermal activities around suboceanic Moho: an example from diopsidite and anorthosite in Wadi Fizh, Oman ophiolite2016

    • Author(s)
      Akizawa, N., Tamura, A., Fukushi, K., Yamamoto, J., Mizukami, T., Python, M. and Arai S.
    • Journal Title

      Lithos

      Volume: 263 Pages: 66-87

    • DOI

      10.1016/j.lithos.2016.07.012

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Arsenate sorption on monohydrocalcite by coprecipitation during transformation to aragonite2016

    • Author(s)
      Fukushi K, Sakai M, Munemoto T, Yokoyama Y and Takahashi Y
    • Journal Title

      Journal of Hazardous Materials

      Volume: 304 Pages: 110-117

    • DOI

      10.1016/j.jhazmat.2015.10.019

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] Prediction of intrinsic cesium desorption from Na-smectite in mixed cation solutions2015

    • Author(s)
      Fukushi K and Fukiage T
    • Journal Title

      Environmental Science and Technology

      Volume: 49 Issue: 17 Pages: 10398-10404

    • DOI

      10.1021/acs.est.5b01884

    • Related Report
      2015 Research-status Report
    • Peer Reviewed
  • [Presentation] 堆積物中の吸着重元素分布を利用した水質復元:鉄酸化物による微量ウラン吸着の表面錯体モデリング2017

    • Author(s)
      小林ゆい・牛山智樹・福士圭介・坂口綾・長谷部徳子
    • Organizer
      地球惑星科学連合2017年大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 鉄酸化物による微量ウラン吸着の表面錯体モデリング:微量元素の吸着挙動 を利用した古水質復元2017

    • Author(s)
      小林ゆい・福士圭介
    • Organizer
      日本地球化学会第64回年会
    • Related Report
      2017 Annual Research Report
  • [Presentation] モノハイドロカルサイトと共存するMgの存在状態:XANES, 第一原理計算と地球化学モデリング2017

    • Author(s)
      福士圭介・鈴木雄真・松宮春奈・川野潤・大野剛・小川雅裕・家路豊成・高橋嘉夫
    • Organizer
      日本地球化学会第64回年会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 金属酸化物への微量亜鉛吸着の表面錯体モデリング2017

    • Author(s)
      米健太郎・小林ゆい・福士圭介
    • Organizer
      第61回粘土科学討論会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 土壌鉱物による微量元素吸着挙動の予測2017

    • Author(s)
      福士圭介
    • Organizer
      2017年度土壌物理学会大会
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] Adsorption of trace amount of uranium on iron oxide: Toward the quantitative reconstruction of past water qualities of an ancient lakes in the Baikal catchment area2016

    • Author(s)
      Fukushi, K., Kobayashi, Y. and Ushiyama, T.
    • Organizer
      Present Earth Surface Processes and Historical Environmental Changes in East Asia,
    • Place of Presentation
      Nago, Okinawa
    • Year and Date
      2016-10-14
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research
  • [Presentation] モノハイドロカルサイトと共存するマグネシウムの存在状態2016

    • Author(s)
      福士圭介・鈴木雄真・大野剛・小川雅裕・家路豊成・高橋嘉夫
    • Organizer
      日本鉱物科学会2016年度年会
    • Place of Presentation
      金沢大学
    • Year and Date
      2016-09-24
    • Related Report
      2016 Research-status Report
  • [Presentation] 鉱物-水界面の地球化学2016

    • Author(s)
      福士圭介
    • Organizer
      鉱物科学若手の会
    • Place of Presentation
      金沢大学
    • Year and Date
      2016-09-23
    • Related Report
      2016 Research-status Report
    • Invited
  • [Presentation] 鉄酸化物による微量ウラン吸着挙動:バイカル集水域古代湖の水質変動復元に向けて2016

    • Author(s)
      小林ゆい・牛山智樹・福士圭介
    • Organizer
      日本地球化学会第63回年会
    • Place of Presentation
      大阪市立大学
    • Year and Date
      2016-09-14
    • Related Report
      2016 Research-status Report
  • [Presentation] モノハイドロカルサイトと共存するMgの存在状態2015

    • Author(s)
      鈴木雄真・福士圭介・大野剛 ・小川雅裕・ 山川庸芝明・高橋嘉夫
    • Organizer
      日本鉱物科学会2015年年会
    • Place of Presentation
      東京大学
    • Year and Date
      2015-09-25
    • Related Report
      2015 Research-status Report
  • [Presentation] 土壌鉱物への鉛吸着の予測モデル:鉄酸化物不在下での鉛のfate2015

    • Author(s)
      牛山智樹・福士圭介
    • Organizer
      日本地球化学会第62回年会
    • Place of Presentation
      横浜国立大学
    • Year and Date
      2015-09-16
    • Related Report
      2015 Research-status Report
  • [Presentation] Water chemistries and sediment mineralogies of some salt lakes (Olgoi, Boon Tsagaan and Orog) in Mongolia2015

    • Author(s)
      Imai, E. Fukushi, K. Katsuta N. Davaadorj, D. Tanaka, Y. Hasebe, N. and Kashiwaya, K.
    • Organizer
      Present Earth Surface Processes and Histrical Environmental Changes in East Asia
    • Place of Presentation
      台北・台湾
    • Year and Date
      2015-09-04
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] イオン吸着のモデリング2015

    • Author(s)
      福士圭介
    • Organizer
      第59回粘土科学討論会
    • Place of Presentation
      山口大学
    • Year and Date
      2015-09-02
    • Related Report
      2015 Research-status Report
    • Invited
  • [Presentation] モノハイドロカルサイト(CaCO3.H2O)の生成条件:バイカル集水域古代湖の水質変動復元に向けて2015

    • Author(s)
      福士圭介・西山理沙・鈴木雄真・福本寛人・宗本隆志
    • Organizer
      地球惑星科学連合2015年大会
    • Place of Presentation
      千葉幕張メッセ
    • Year and Date
      2015-05-25
    • Related Report
      2015 Research-status Report
    • Invited

URL: 

Published: 2015-04-16   Modified: 2019-03-29  

Information User Guide FAQ News Terms of Use Attribution of KAKENHI

Powered by NII kakenhi