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Self-assembled integration technologies of silicon quantum dots toward future NeoSilicon quantum information devices

Research Project

Project/Area Number 16206030
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field Electronic materials/Electric materials
Research InstitutionTokyo Institute of Technology

Principal Investigator

ODA Shunri  Quantum Nanoelectronics Research Center, Professor, 量子ナノエレクトロニクス研究センター, 教授 (50126314)

Co-Investigator(Kenkyū-buntansha) MIZUTA Hiroshi  Tokyo Institute of Technology, Department of Physical Electronics, Associate Professor, 大学院理工学研究科, 助教授 (90372458)
TSUCHIYA Yoshishige  Quantum Nanoelectronics Research Center, Assistant Professor, 量子ナノエレクトロニクス研究センター, 助手 (80334506)
Project Period (FY) 2004 – 2006
Project Status Completed (Fiscal Year 2006)
Budget Amount *help
¥50,440,000 (Direct Cost: ¥38,800,000、Indirect Cost: ¥11,640,000)
Fiscal Year 2006: ¥12,350,000 (Direct Cost: ¥9,500,000、Indirect Cost: ¥2,850,000)
Fiscal Year 2005: ¥12,090,000 (Direct Cost: ¥9,300,000、Indirect Cost: ¥2,790,000)
Fiscal Year 2004: ¥26,000,000 (Direct Cost: ¥20,000,000、Indirect Cost: ¥6,000,000)
KeywordsNanocrystalline silicon / Nanodots integration / Dispersion solution / Langmuir-Blodgett (LB) technique / Quantum information device / Lateral capillary meniscus force / Double nc-Si dots charge qubit / Charge polarization detection / 2重nc-Si量子ドット / RF-SET / メニスカス相互作用
Research Abstract

Nanocrystalline Si dots with a diameter of -8 nm were fabricated by using pulsed gas VHF plasma process and deposited on the substrate. We have successfully prepared the nc-Si dot dispersion solution by immersing the deposited wafer into alcohols with ultra sonic treatment. We then dropped a small volume of the solution onto other substrates and dried it. During the evaporation of alcohols the nc-Si dots were assembled in the solution via the lateral capillary meniscus force. Two-dimensional assembly of the dots was obtained by this method. Furthermore, we developped a new bottom-up technique for high-density assembly of the nc-Si quantum dots based on the Langmuir-Blodgett (LB) technique. We found that the solvent consists of chloroform (CHCl_3) and HMDS ([(CH_3)_3Si]_2NH) was suitable to the LB method for nc-Si. High density assembly of dots was obtained by using the LB method.
We examined the assembly of the nc-Si dots on the silicon-on-insulator substrates with nanoscale patterning and succeeded in making the nc-Si dots cluster bridging between the nano-electrodes with a gap of as small as 20 nm. Combining the top-down nanolithography and bottom-up self-assembly may provide a new method to fabricate nanoscale Si structures for the future quantum information device applications. We also tried to integrate of nc-Si quantum dots with the single electron transistor (SET) A resist hole was prepared in the narrow region between the SET island and gate electrodes using the electron beam lithography. After the nc-Si deposition and lift-off processes, we observed that nc-Si QDs contacted directly to the substrate only in the resist hole area. From the equivalent circuit simulation and 3D capacitance analysis, we found that nc-Si QDs help to shift the Coulomb oscillation peak lines effectively and subtle charge polarization can be sensed as their remarkable shift.

Report

(4 results)
  • 2006 Annual Research Report   Final Research Report Summary
  • 2005 Annual Research Report
  • 2004 Annual Research Report
  • Research Products

    (48 results)

All 2007 2006 2005 2004

All Journal Article (44 results) Book (4 results)

  • [Journal Article] Charge Storage and Electron/Light Emission Properties of Silicon Nanocrystals2007

    • Author(s)
      S.Oda, S.Y.Huang, M.A.Salem, D.Hippo, H.Mizuta
    • Journal Title

      Physica E 38

      Pages: 59-63

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] New Design Concept and Fabrication Process for Three-Dimensional Silicon Photonic Crystal Structures2007

    • Author(s)
      D.Hippo, K.Urakawa, Y.Kawata, Y.Tsuchiya, H.Mizuta, N.Koshida, S.Oda
    • Journal Title

      Japanese Journal of Applied Physics 46・2

      Pages: 633-637

    • NAID

      10018545174

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Design and Analysis of Functional NEMS-gate MOSFETs and SETs2007

    • Author(s)
      B.Pruvost, H.Mizuta, S.Oda
    • Journal Title

      IEEE Transactions on Nanotechnology 6・2

      Pages: 218-224

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Three-dimensional numerical analysis of switching properties of high-speed and non-volatile nanoelectromechanical memory2007

    • Author(s)
      T.Nagami, H.Mizuta, N.Momo, Y.Tsuchiya, S.Saito, T.Arai, T.Shimada, S.Oda
    • Journal Title

      IEEE Transactions on Electron Devices 54・5

      Pages: 1132-1139

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Integration of tunnel-coupled double nanocrystalline silicon quantum dots with a multiple gate single-electron transistor2007

    • Author(s)
      Y.Kawata, M.Khalafalla, K.Usami, Y.Tsuchiya, H.Mizuta, S.Oda
    • Journal Title

      Japanese Journal of Applied Physics 46(印刷中)

    • NAID

      40015465565

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Charge Storage and Electron/Light Emission Properties of / Silicon Nanocrystals2007

    • Author(s)
      S.Oda, S.Y.Huang, M.A.Salem, D.Hippo, H.Mizuta
    • Journal Title

      Physica E 38

      Pages: 59-63

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] New Design Concept and Fabrication Process for Three-Dimensional Silicon Photonic Crystal Structures2007

    • Author(s)
      D.Hippo, K.Urakawa, Y.Kawata, Y.Tsuchiya, H.Mizuta, N Koshida, S.Oda
    • Journal Title

      Japanese Journal of Applied Physics 46 (2)

      Pages: 633-637

    • NAID

      10018545174

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Design and Analysis of Functional NEMS-gate MOSFETs and SETs2007

    • Author(s)
      B.Pruvost, H.Mizuta, S.Oda
    • Journal Title

      IEEE Transactions on Nanotechnology 6 (2)

      Pages: 218-224

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Three-dimensional numerical analysis of switching properties of high-speed and non-volatile nanoelectromechanical memory2007

    • Author(s)
      T.Nagami, H.Mizuta, N.Momo, Y.Tsuchiya, S.Saito, T.Arai, T.Shimada, S.Oda
    • Journal Title

      IEEE Transactions on Electron Devices 54 (5)

      Pages: 1132-1139

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Integration of tunnel-coupled double nanocrystalline silicon quantum dots with a multiple gate single-electron transistor2007

    • Author(s)
      Y.Kawata, M.Khalafalla, K Usami, Y.Tsuchiya, H.Mizuta, S.Oda
    • Journal Title

      Japanese Journal of Applied Physics 46(in press)

    • NAID

      40015465565

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Charge Storage and Electron/Light Emission Properties of Silicon Nanocrystals,2007

    • Author(s)
      S.Oda, S.Y.Huang, M.A.Salem, D.Hippo, H.Mizuta
    • Journal Title

      Physica E (in press)

    • Related Report
      2006 Annual Research Report
  • [Journal Article] New Design Concept and Fabrication Process for Three-Dimensional Silicon Photonic Crystal Structures,2007

    • Author(s)
      D.Hippo, K.Urakawa, Y.Kawata, Y.Tsuchiya, H.Mizuta, N.Koshida, S.Oda
    • Journal Title

      Jpn. J. Appl. Phys. 46(2)

      Pages: 633-637

    • NAID

      10018545174

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Design and Analysis of Functional NEMS-gate MOSFETs and SETs,2007

    • Author(s)
      B.Pruvost, H.Mizuta, S.Oda
    • Journal Title

      IEEE Trans on Nanotechnology Vol.6, No.2

      Pages: 218-224

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Observation and Analysis of Tunneling Properties of a Single Spherical Nanocrystalline Silicon Quantum Dot2006

    • Author(s)
      A.Surawijaya, H.Mizuta, S.Oda
    • Journal Title

      Japanese Journal of Applied Physics 87・4B

      Pages: 3638-3641

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] High-Density Assembly of Nanocrystalline Silicon Quantum Dots2006

    • Author(s)
      A.Tanaka, Y.Tsuchiya, K.Usami, H.Mizuta, S.Oda
    • Journal Title

      Current Applied Physics 6・3

      Pages: 344-347

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Observation of Interdot Coupling Phenomena in Nanocrystalline Silicon Point-Contact Structures2006

    • Author(s)
      M.Khalafalla, H.Mizuta, Z.A.K.Durrani, H.Ahmed, S.Oda
    • Journal Title

      Current Applied Physics 6・3

      Pages: 536-540

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Hopping conduction in size-controlled Si nanocrystals2006

    • Author(s)
      M.A.Rafiq, Y.Tsuchiya, H.Mizuta, S.Oda, S.Uno, Z.A.K.Durrani, W.I.Milne
    • Journal Title

      Journal of Applied Physics 100

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Nano-electro-mechanical nonvolatile memory device incorporating nanocrystalline Si dots2006

    • Author(s)
      Y.Tsuchiya, K.Takai, N.Momo, T.Nagami, S.Yamaguchi, T.Shimada, H.Mizuta, S.Oda
    • Journal Title

      Journal of Applied Physics 100

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Observation and Analysis of Tunneling Properties of a Single Spherical Nanocrystalline Silicon Quantum Dot2006

    • Author(s)
      A.Surawijaya, H.Mizuta, S.Oda
    • Journal Title

      Japanese Journal of Applied Physics 45 (4B)

      Pages: 3638-3641

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] High-Density Assembly of Nanocrystalline Silicon Quantum' Dots2006

    • Author(s)
      A.Tanaka, Y.Tsuchiya, K.Usami, H.Mizuta, S.Oda
    • Journal Title

      Current Applied Physics 6 (3)

      Pages: 344-347

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Observation of Interdot Coupling Phenomena in Nanocrystalline Silicon Point-Contact Structures2006

    • Author(s)
      M.Khalafalla, H.Mizuta, Z.A..K.Durrani, H.Ahmed, S Oda
    • Journal Title

      Current Applied Physics 6 (3)

      Pages: 536-540

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Nano-electro-mechanical nonvolatile memory device incorporating nanocrystalline Si dots2006

    • Author(s)
      Y.Tsuchiya, K Takai, N.Momo, T.Nagami, S.Yamaguchi, T.Shimada, H.Mizuta, S.Oda
    • Journal Title

      Journal of Applied Physics 100

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Observation and Analysis of Tunneling Properties of a Single Spherical Nanocrystalline Silicon Quantum Dot,2006

    • Author(s)
      A.Surawijaya, H.Mizuta, S.Oda
    • Journal Title

      Jpn. J. Appl. Phys. Vol.87 No.4B

      Pages: 3638-3641

    • Related Report
      2006 Annual Research Report
  • [Journal Article] High-Density Assembly of Nanocrystalline Silicon Quantum Dots,2006

    • Author(s)
      A.Tanaka, Y.Tsuchiya, K.Usami, H.Mizuta, S.Oda
    • Journal Title

      Current Appl. Phys. Vol.6, No.3

      Pages: 344-347

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Observation of Interdot Coupling Phenomena in Nanocrystalline Silicon Point-Contact Structures,2006

    • Author(s)
      M.Khalafalla, H.Mizuta, Z.A.K.Durrani, H.Ahmed, S.Oda
    • Journal Title

      Current Appl. Phys. Vol.6, No.3

      Pages: 536-540

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Hopping conduction in size-controlled Si nanocrystals,2006

    • Author(s)
      M.A.Rafiq, Y.Tsuchiya, H.Mizuta, S.Oda, S.Uno, Z.A.K.Darrani, W.I.Milne
    • Journal Title

      J. Appl. Phys. Vol.100

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Nano-electro-mechanical nonvolatile memory device incorporating nanocrystalline Si dot,2006

    • Author(s)
      Y.Tsuchiya, K.Takai, N.Nomo, T.Nagami, S.Yamaguchi, T.Shimada, H.Mizuta, S.Oda
    • Journal Title

      J. Appl. Phys. Vol.100

    • Related Report
      2006 Annual Research Report
  • [Journal Article] In situ real-time spectroscopic ellipsometry study of HfO_2 thin films grown by using the pulsed-source MOCVD2005

    • Author(s)
      Y.D.Zheng, H.Mizuta, Y.Tsuchiya, M.Endo, D.Sato, S.Oda
    • Journal Title

      Journal of Applied Physics 97

      Pages: 23527-23527

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Quasiballistic Electron Emission from Planarized Nanocrystalline-Si Cold Cathode2005

    • Author(s)
      Y.Tsuchiya, T.Nakatsukasa, H.Mizuta, S.Oda, A.Kojima, N.Koshida
    • Journal Title

      Materials Research Society Symposium Proceedings 832

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Atomic force microscope current-imaging study for current density through nanocrystalline silicon dots embedded in SiO_22005

    • Author(s)
      M.A.Salem, H.Mizuta, S.Oda, Y.Fu, M.Willander
    • Journal Title

      Japanese Journal of Applied Physics 44

    • NAID

      10014420424

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary 2004 Annual Research Report
  • [Journal Article] Charge injection and trapping in silicon nanocrystals2005

    • Author(s)
      M.A.Rafiq, Y.Tsuchiya, H.Mizuta, S.Oda, S.Uno, Z.A.K.Durrani, W.I.Milne
    • Journal Title

      Applied Physics Letters 87

      Pages: 182101-182101

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary 2005 Annual Research Report
  • [Journal Article] Charge storage in nitrided nanocrystalline silicon dots2005

    • Author(s)
      S.Huang, S.Oda
    • Journal Title

      Applied Physics Letters 87

      Pages: 173107-173107

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary 2005 Annual Research Report
  • [Journal Article] In situ real-time spectroscopic ellipsometry study of HfO_2 thin films grown by using the pulsed-source MOCVD2005

    • Author(s)
      Y.D.Zheng, H Mizuta, Y.Tsuchiya, M.Endo, D.Sato, S.Oda
    • Journal Title

      journal of Applied Physics 97

      Pages: 23527-23527

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Atomic force microscope current-imaging study for current density through nanocrystalline silicon dots embedded in SiO22005

    • Author(s)
      M.A.Salem, H.Mizuta, S.Oda, Y.Fu, M.Willander
    • Journal Title

      Japanese Journal of Applied Physics 44 (2)

    • NAID

      210000059690

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Charge injection and trapping in silicon naNo.crystals2005

    • Author(s)
      M.A.Rafiq, Y.Tsuchiya, H.Mizuta, S.Oda, S.Uno, Z.A.K.Durrani, W.I.Milne
    • Journal Title

      Applied Physics Letters 87

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Charge storage in nitrided naNo.crystalline silicon dots2005

    • Author(s)
      S.Huang, S.Oda
    • Journal Title

      Applied Physics Letters 87 (17)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] In situ real-time spectroscopic ellipsometry study of HfO2 thin films grown by using the pulsed-source MOCVD2005

    • Author(s)
      Y.D.Zheng, H.Mizuta, Y.Tsuchiya, M.Endo, D.Sato, S.Oda
    • Journal Title

      Journal of Applied Physics 97

      Pages: 23527-23527

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Atomic force microscope current-imaging study for current density through nanocrystalline silicon dots embedded in SiO22005

    • Author(s)
      M.A.Salem, H.Mizuta, S.Oda, Y.Fu, M.Willander
    • Journal Title

      Japanese Journal of Applied Physics 44

    • NAID

      210000059690

    • Related Report
      2005 Annual Research Report
  • [Journal Article] High-Density Assembly of Nanocrystalline Silicon Quantum Dot2005

    • Author(s)
      A.Tanaka, G.Yamahata, Y.Tsuchiya, K.Usami, H.Mizuta, S.Oda
    • Journal Title

      Current Applied Physics (発表予定)(to be published)

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Probing electron charging in nanocrystalline Si dots using Kelvin probe force microscopy2004

    • Author(s)
      M.A.Salem, H.Mizuta, S.Oda
    • Journal Title

      Applied Physics Letters 85

      Pages: 3262-3262

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary 2004 Annual Research Report
  • [Journal Article] Probing electron charging in nanocrystalline Si dots using Kelvin Probe Force Microscopy2004

    • Author(s)
      M.A.Salem, H.Mizuta, S.Oda
    • Journal Title

      Applied Physics Letters 85 (15)

      Pages: 3262-3264

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Nanocrystalline silicon dot displacement using speed-controlled tapping-mode atomic force microscopy2004

    • Author(s)
      S.Kanjanachuchai, Y.Tsuchiya, K.Usami, S.Oda
    • Journal Title

      Microelectronic Engineering 73-74

      Pages: 615-615

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Towards long-term retention-time single-electron-memory devices based on nitrided nanocrystalline silicon dots2004

    • Author(s)
      S.Huang, K.Arai, K.Usami, S.Oda
    • Journal Title

      IEEE Trans. Nanotechnology 3

      Pages: 210-210

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Coherent states in a coupled quantum dot nanocrystalline silicon transistor2004

    • Author(s)
      M.Khalafalla, H.Mizuta, Z.A.K.Durrani
    • Journal Title

      Applied Physics Letters 85

      Pages: 2262-2262

    • Related Report
      2004 Annual Research Report
  • [Book] Handbook of Semiconductor : Nanostructures and Nanodevices2006

    • Author(s)
      S-Y.Huang, H.Mizuta, S.Oda
    • Total Pages
      63
    • Publisher
      American Scientific Publishers
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Annual Research Report 2006 Final Research Report Summary
  • [Book] Silicon Nanoelectronics2005

    • Author(s)
      S.Oda, D.Ferry
    • Total Pages
      328
    • Publisher
      ISBN 0824726332, CRC Press
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Book] Future Integrated Systems2005

    • Author(s)
      S.Oda, D.F.Moore
    • Total Pages
      65
    • Publisher
      ISBN 0 9535142 1 8, MTP, Cambridge
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary 2005 Annual Research Report
  • [Book] Silicon Nanoelectronics2005

    • Author(s)
      S.Oda, D.Ferry
    • Total Pages
      328
    • Publisher
      ISBN O824726332, CRC Press
    • Related Report
      2005 Annual Research Report

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Published: 2004-04-01   Modified: 2016-04-21  

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