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Observation of a superconducting gap in a magnetic-field-induced two-dimensional organic superconductor by multi-frequency ESR spectroscopy

Research Project

Project/Area Number 16340106
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Condensed matter physics II
Research InstitutionKobe University

Principal Investigator

OHTA Hitoshi  Kobe University, Organization of Advanced Science and Technology, Molecular Photoscience Research Center, Professor (70194173)

Co-Investigator(Kenkyū-buntansha) OKUBO Susumu  Kobe University, Organization of Advanced Science and Technology, Molecular Photoscience Research Center Assistant, Professor (80283901)
Project Period (FY) 2004 – 2007
Project Status Completed (Fiscal Year 2007)
Budget Amount *help
¥16,580,000 (Direct Cost: ¥16,100,000、Indirect Cost: ¥480,000)
Fiscal Year 2007: ¥2,080,000 (Direct Cost: ¥1,600,000、Indirect Cost: ¥480,000)
Fiscal Year 2006: ¥5,000,000 (Direct Cost: ¥5,000,000)
Fiscal Year 2005: ¥6,600,000 (Direct Cost: ¥6,600,000)
Fiscal Year 2004: ¥2,900,000 (Direct Cost: ¥2,900,000)
Keywordsorganic conductor / magnetic-field-induced superconductivity / ESR spectroscopy / high magnetic field / sunperconducting gap / international collaboration / USA
Research Abstract

Magneto-optical measurements of field-induced superconductor λ-(BETS)_2FeCl_4 have been performed at 1.4 K using the 33 T water cooling magnet at NHMFL, Florida, USA. The Backward traveling wave oscillators (BWO) are used as the light sources, and the InSb hot electron bolometer is used as a detector. The rotational sample holder which is developed for this measurement, is used to enable the angular dependence measurement. Firstly we performed the measurement with one needle like single crystal without a mask but we were not able to detect the signal. Therefore, we set several needle like single crystals parallel to each other with a mask and let the light transmit through the spacing between samples. It turned out to be very difficult to apply the magnetic field parallel to the c-axes of all samples and we were not able to eliminate ESR signals completely. As a result, we observed unusual frequency dependence where the transmission aound 8 T became stronger as the frequency increased. Moreover, the transmission above 8T became very small and no significant change was observed within the S/N limit above 20, T where the field-induced superconductivity was expected. As, however the organic superconductor is in the clean limit and the Drude tail is smaller than the superconducting gap, there is a possibility that it is difficult to estimate the superconducting gap by the frequency dependence measurements because the transmission difference between the superconducting state and the metal state is small. On the other hand, in order to understand the very unusual increase of transmission around 8 T in the high frequency region, the discussion at the high field international conference, which will be held in Tallin this summer, is planned.

Report

(5 results)
  • 2007 Annual Research Report   Final Research Report Summary
  • 2006 Annual Research Report
  • 2005 Annual Research Report
  • 2004 Annual Research Report
  • Research Products

    (20 results)

All 2008 2007 2006 2005 2004

All Journal Article (17 results) (of which Peer Reviewed: 5 results) Presentation (3 results)

  • [Journal Article] 多重極限高周波ESRの開発とスピン凝縮系の研究2008

    • Author(s)
      太田 仁
    • Journal Title

      電子スピンサイエンス Vol.6(Spring)

      Pages: 45-54

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Low-temperature Fermi surface of the organic conductor β'-(BEDT-TTF) (TCNQ)_<(1-x)>(F1-TCNQ)_x (x=0,0.05) from magnetooptical measurements2007

    • Author(s)
      M. Kimata
    • Journal Title

      Phys. Rev. B 第75巻

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Low-temperature Fermi surface of the organic conductor β"-(BEDT-TTF)(TCNQ)(1-x)(F1-TCNQ)x(x=0,0.05) from magnetooptical measurements2007

    • Author(s)
      M, Kimata, Y, Oshima, H, Ohta, K, Koyama, M, Motokawa, H, M, Yamamoto, R, Kato
    • Journal Title

      Phys. Rev 75

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Low-temperature Fermi surface of the organic conductor β"-(BEDT-TTF)(TCNQ)_<(1-x)>(F1-TCNQ)_x(x=0,0.05)from magnetooptical measurements2007

    • Author(s)
      M. Kimata
    • Journal Title

      Phys. Rev. B 第75巻

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Fermi surface study of organic conductors using a magneto-optical measurement under high magnetic fields2006

    • Author(s)
      M. Kimata
    • Journal Title

      J. Phys.: Conf. Series 第51巻

      Pages: 359-362

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Fermi surface study of organic conductors using a magneto-optical measurement under high magnetic fields2006

    • Author(s)
      M, Kimata, H, Ohta, K, Koyama, M, Motokawa, R, Kondo, S, Kagoshima, H, Tanaka, M, Tokumoto, H, Kobayashi, A, Kobayashi
    • Journal Title

      J. Phys: Conf. Series 51

      Pages: 359-362

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Detailed Fermi Surface Topology of the Quasi-One-Dimensional Conducto (DMET)_2I_32006

    • Author(s)
      M.Kimata
    • Journal Title

      J. Low Temp. Phys 第142巻

      Pages: 523-526

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Fermi surface study of organic conductors using a magneto-optical measurement under high magnetic fields2006

    • Author(s)
      M.Kimata
    • Journal Title

      J. Phys. : Conf. Series 第51巻

      Pages: 359-362

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Low-temperature Fermi surface of the organic conductor β"-(BEDT-TTF) (TCNQ)_<(1-x)> (F1-TCNQ)_x (x=0, 0.05) from magnetooptical measurements2006

    • Author(s)
      M.Kimata
    • Journal Title

      Phys. Rev. B 第75巻

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Development of the High Field Magneto-optical Measurement System with a Rotational Cavity for the Study of Organic Conductors2006

    • Author(s)
      M.Kimata
    • Journal Title

      High magnetic Fields in Semiconductor Physics(Yong-Jie Wang, Lloyd Engel and N.Bonesteel Eds.)(World Scientific, Singapore)

      Pages: 355-358

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Development and Applications of Magnetooptical Measurement System Equipped with a Rotational Resonant Cavity in the Millimeter-Wave Region2005

    • Author(s)
      M. Kimata
    • Journal Title

      Jpn. J. Appl. Phys. 第44巻

      Pages: 4930-4934

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Development and Applications of Magnetooptical Measurement System Equipped with a Rotational Resonant Cavity in the Millimeter-Wave Region2005

    • Author(s)
      M, Kimata, K, Koyama, H, Ohra, Y, Oshima, M, Motokawa, H, Nishikawa, K, Kikuchi, I, Ikemoto
    • Journal Title

      Jpn.J.Appl.Phys 44(7A)

      Pages: 4930-4934

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Development and Applications of Magnetooptical Measurement System Equipped with a Rotational Resonant Cavity in the Millimeter-Wave Region2005

    • Author(s)
      M.Kimata
    • Journal Title

      Jpn.J.Appl.Phys. 第44巻・7A号

      Pages: 4930-4934

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Fermi Surface Study of β"-(BEDT-TTF)(TCNQ) by Magnetooptical Measurements2005

    • Author(s)
      M.Kimata
    • Journal Title

      Synthetic Metals 第153巻

      Pages: 369-372

    • Related Report
      2005 Annual Research Report
  • [Journal Article] MAGNETO-OPTICAL MEASUREMENT OF ORGANIC CONDUCTOR USING ROTATIONAL CAVITY SYSTEM2005

    • Author(s)
      H.Ohta
    • Journal Title

      Int.J.IRMMW 第26巻・11号

      Pages: 1525-1530

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Magnetooptical measurements of β"-(BEDT-TTF)(TCNQ)2004

    • Author(s)
      木俣 基
    • Journal Title

      Physica B 346-347巻

      Pages: 382-386

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Observation of high-order quasi-one-dimensional periodic orbit resonance in (DMET)_2I_3 and its Fermi surface2004

    • Author(s)
      大島 勇吾
    • Journal Title

      Physica B 346-347巻

      Pages: 387-391

    • Related Report
      2004 Annual Research Report
  • [Presentation] EtMe_3P[Pd(dmit)_2]_2の強磁場ESR測定2007

    • Author(s)
      吉田喬久
    • Organizer
      日本物理学会
    • Place of Presentation
      北海道大学
    • Year and Date
      2007-09-22
    • Related Report
      2007 Annual Research Report
  • [Presentation] Magnetooptical and ESR Studies of Organic Conductors under High Magnetic Field and High Pressure2005

    • Author(s)
      H. Ohta
    • Organizer
      International Symposium on Molecular Conductors
    • Place of Presentation
      湘南国際村,葉山
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Magnetooptical and ESR Studies of Organic Conductors under High magnetic Field and High Pressure2005

    • Author(s)
      Hitoshi, Ohta, Motoi, Kimata, Takahiro, Sakurai, Susumu, Okuho, Yoshiya, Uwatoko, Keiichi, Koyama, Mitsuhiro, Motokawa, Eiji, Ohmichi, Toshihito, Osada
    • Organizer
      International Symposium on Molecular Conductors
    • Place of Presentation
      Hayama, Japan
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary

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Published: 2004-04-01   Modified: 2020-05-15  

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