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Creation of ferroelectric relaxor superlattices with symmetry braking and brain mimetic memory

Research Project

Project/Area Number 16360154
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Electronic materials/Electric materials
Research InstitutionThe University of Tokyo (2006)
Osaka University (2004-2005)

Principal Investigator

TABATA Hitoshi  The University of Tokyo, Department of Electronic Engineering, Professor (00263319)

Co-Investigator(Kenkyū-buntansha) 佐伯 洋昌  大阪大学, 産業科学研究所, 助手 (20362626)
Project Period (FY) 2004 – 2006
Project Status Completed (Fiscal Year 2006)
Budget Amount *help
¥14,500,000 (Direct Cost: ¥14,500,000)
Fiscal Year 2006: ¥2,800,000 (Direct Cost: ¥2,800,000)
Fiscal Year 2005: ¥2,600,000 (Direct Cost: ¥2,600,000)
Fiscal Year 2004: ¥9,100,000 (Direct Cost: ¥9,100,000)
Keywordsrelaxor / artificial superlattices / spinglass / spinel / garnet / 精密結晶構造解析 / MEM / 秩序-無秩序 / 双極子グラス
Research Abstract

Superlattices of transition metal oxides have been formed by a laser Molecular Beam Epitaxy (MBE) technique connected with RHEED monitoring system. The superlattices of magnetics have been constructed on SrTiO_3(100), (110) and (111) surfaces. These surface selection enables us to control the three dimensional positioning of atoms and spin. In the case of LaCrO_3/LaFeO_3 superlattices on (111) surface, ferromagnetism has been realized for the first time. In the case of LaMnO_3/LaFeO_3 superlattices, on the other hand, spin frustration is expected competing with ferromagnetism of self-doped LaMnO_3 and anti-ferromagnetism of LaFeO_3 on SrTiO_3 (100) surface. Spin glass phase transition (casp shape in magnetization vs. temperature measurements) is observed in the case of LaMnO_3/LaFeO_3 superlattices. It is due to the spin frustration between ferromagnetic couping in LaMnO_3 layer and antiferromagnetic coupling in LaFeO_3 layer.

Report

(4 results)
  • 2006 Annual Research Report   Final Research Report Summary
  • 2005 Annual Research Report
  • 2004 Annual Research Report
  • Research Products

    (67 results)

All 2007 2006 2005 2004

All Journal Article (62 results) Book (3 results) Patent(Industrial Property Rights) (2 results)

  • [Journal Article] Simultaneous control of growth mode and ferromagnetic ordering in Co-doped ZnO layers with Zn polarity2007

    • Author(s)
      H. Matsui
    • Journal Title

      Physical Review B 75

      Pages: 14438-14438

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Co-doped ZnO homoepitaxy : Repeated oxygen-pressure modulated epitaxy2007

    • Author(s)
      H. Matsui
    • Journal Title

      Physica Status Solidi C 3

      Pages: 4106-4109

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Simultaneous control of growth mode and ferromagnetic ordering in Co-doped ZnO layers with Zn polaritv2007

    • Author(s)
      H. Matsui, H. Tabata
    • Journal Title

      Physical Review B 75 014438

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Co-doped ZnO homoepitaxy : Repeated oxygen-pressure modulated epitaxy2007

    • Author(s)
      H. Matsui, H. Tabata
    • Journal Title

      Physica Status Solidi C 3

      Pages: 4106-4109

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Simultaneous control of growth mode and ferromagnetic ordering in Co-doped ZnO layers with Zn polarity2007

    • Author(s)
      H.Matsui
    • Journal Title

      Physical Review B 75

      Pages: 14438-14438

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Co-doped ZnO homoepitaxy : Repeated oxygen-pressure modulated epitaxy2007

    • Author(s)
      H.Matsui
    • Journal Title

      Physica Status Solidi C 3

      Pages: 4106-4109

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Influence of Microstructure on the Complex Permeability of Spinel Type Ni-Zn Ferrite2006

    • Author(s)
      S. T. Mahmuda
    • Journal Title

      J. Magnetism & Magnetic Materials 305

      Pages: 269-274

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Stranski-Krastanov growth in Mg0.37Zn0.63O/ZnO heteroepitaxy : Self-organized nanodots and local composition separation2006

    • Author(s)
      H. Matsui
    • Journal Title

      Appl. Phys. Lett. 89

      Pages: 91909-91909

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Novel DNA Nano-Patterning Design Method Utilizing Poly-L-Lysine Patterning by Nanoimprint Lithography2006

    • Author(s)
      T. Ohtake
    • Journal Title

      J. Nanosci. Nanotechnol. 6

      Pages: 2187-2190

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Correlation of self-organized surface nanostructures and anisotropic electron transport in nonpolar ZnO (10-10) homoepitaxy2006

    • Author(s)
      H. Matsui
    • Journal Title

      J. Appl. Phys. 99

      Pages: 124307-124307

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Dielectric and ferroelectric properties of c-axiis oriented strontium bismuth tantalate thin films applied transverse electric fields2006

    • Author(s)
      K. Kotani
    • Journal Title

      J. Appl. Phys. 99

      Pages: 124106-124106

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Modification of Temperature Dependence of Dielectric Properties by Symmetry-Controlled Superlattices Thin Films of BaZr_xTi_<1-x>O_32006

    • Author(s)
      T. Kawahara
    • Journal Title

      Jpn. J. Appl. Phys. 45

      Pages: 4484-4488

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Critical thickness and lattice relaxation of Mg-rich strained Mg_<0.37>Zn_<0.63>O (0001) layers towards multi-quantum-wells2006

    • Author(s)
      H. Matsui
    • Journal Title

      J. Appl. Phys. 99

      Pages: 24902-24902

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] 酸化亜鉛半導体薄膜の光・電子・磁気機能-極性・非極性の観点から-2006

    • Author(s)
      松井裕章
    • Journal Title

      応用物理 75

      Pages: 1211-1217

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] 酸化物半導体ZnO薄膜の成長表面と格子欠陥2006

    • Author(s)
      松井裕章
    • Journal Title

      表面科学 27

      Pages: 708-714

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] 強誘電体薄膜BaZrxTil-xO3の超格子による温度特性の制御2006

    • Author(s)
      河原敏男
    • Journal Title

      超音波TECHNO 9-10

      Pages: 31-34

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Influence of Microstructure on the Complex Permeability of Sninel Tyne, Ni-Zn Ferrite2006

    • Author(s)
      S. T. Mahmuda Hosain, H. Tabata
    • Journal Title

      J. Magnetism & Magnetic Materials 305

      Pages: 269-274

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Stranski-Krastanov growth in Mg0.37Zn0.63O/ZnO heteroepitaxy : Self-organized nanodots and local composition separation2006

    • Author(s)
      H. Matsui, H. Tabata
    • Journal Title

      Appl. Phys. Lett. 89, 091909

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Novel DNA Nano-Patterning Design Method Utilizing Poly-L-Lysine Patterning bv Nanoimprint Lithography2006

    • Author(s)
      T. Ohtake, H. Tabata
    • Journal Title

      J. Nanosci. Nanotechnol. 6

      Pages: 2187-2190

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Correlation of self-organized surface nanostructures and anisotropic electron transport in nonpolar ZnO (10-10) homoepitaxv2006

    • Author(s)
      H. Matsui, H. Tabata
    • Journal Title

      J. Appl. Phys. 99, 124307

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Dielectric and ferroelectric properties of c-axis oriented strontium bismuth tantalate thin films applied transverse electric fields2006

    • Author(s)
      K. Kotani, A. Fujimori, H. Tabata
    • Journal Title

      J. Appl. Phys. 99, 124106

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Modification of Temperature Dependence of Dielectric Properties by Symmetry-Controlled Superlattices Thin Films of BaZr_xTi_1-xO_32006

    • Author(s)
      T. Kawahara, H. Tabata
    • Journal Title

      Jpn. J. Appl. Phys. 45

      Pages: 4484-4488

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Critical thickness and lattice relaxation of Mg-rich strained Mg_0.37Zn0.63O(0001)layers towards multi-quantum-wells2006

    • Author(s)
      H. Matsui, H. Tabata
    • Journal Title

      J. Appl. Phys. 99 024902

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Modification of Temperature Dependence of Dielectric Properties by Symmetry-Controlled Superlattices Thin Films of BaZr_xTi_<1-x>O_32006

    • Author(s)
      T.Kawahara
    • Journal Title

      Jpn. J. Appl. Phys. 45

      Pages: 4484-4488

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Critical thickness and lattice relaxation of Mg-rich strained Mg_<0.37>Zn_<0.63>O(0001) layers towards multi-quantum-wells2006

    • Author(s)
      H.Matsui
    • Journal Title

      J.Appl. Phys. 99

      Pages: 24902-24902

    • Related Report
      2006 Annual Research Report
  • [Journal Article] 酸化亜鉛半導体薄膜の光・電子・磁気機能 -極性・非極性の観点から-2006

    • Author(s)
      松井裕章
    • Journal Title

      応用物理 75

      Pages: 1211-1217

    • Related Report
      2006 Annual Research Report
  • [Journal Article] 酸化物半導体ZnO薄膜の成長表面と格子欠陥2006

    • Author(s)
      松井 裕章
    • Journal Title

      表面科学 27

      Pages: 708-714

    • Related Report
      2006 Annual Research Report
  • [Journal Article] 強誘電体薄膜BaZrxTil-xO3の超格子による温度特性の制御2006

    • Author(s)
      河原 敏男
    • Journal Title

      超音波TECHNO 9-10

      Pages: 31-34

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Influence of Microstructure on the Complex Permeability of Spinel Type Ni-Zn Ferrite2006

    • Author(s)
      S.T.Mahmuda
    • Journal Title

      J. Magnetism & Magnetic Materials 305

      Pages: 269-274

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Stranski-Krastanov growth in Mg0.37Zn0.63O/ZnO heteroepitaxy : Self-organized nanodots and local composition separation2006

    • Author(s)
      H.Matsui
    • Journal Title

      Appl. Phys. Lett. 89

      Pages: 91909-91909

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Correlation of self-organized surface nanostructures and anisotropic electron transport in nonpolar ZnO (10-10) homoepitaxy2006

    • Author(s)
      H.Matsui
    • Journal Title

      J. Appl. Phys. 99

      Pages: 124307-124307

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Dielectric and ferroelectric properties of c-axis oriented strontium bismuth tantalate thin films applied transverse electric fields2006

    • Author(s)
      K.Kotani
    • Journal Title

      J. Appl. Phys. 99

      Pages: 124106-124106

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Critical thickness and lattice relaxation of Mg-rich strained Mg_<0.37>Zn_<0.63>O (0001) layers towards multi-quantum-wells2006

    • Author(s)
      H.Matsui
    • Journal Title

      J.Appl.Phys. 99

      Pages: 24902-24902

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Characterization of magnetic components in the diluted magnetic semiconductor Zn_<1-x>Co_xO by x-ray magnetic circular dichroism2005

    • Author(s)
      M.Kobayashi
    • Journal Title

      Phys.Rev.B 72

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Self-organized nanostripe arrays on ZnO (10-10) surfaces formed during laser molecular-beam-epitaxy growth2005

    • Author(s)
      H.Matsui
    • Journal Title

      Appl.Phys.Lett. 87

      Pages: 143109-143109

    • Related Report
      2005 Annual Research Report
  • [Journal Article] SEM Observation of Collagen Fibrils Secreted from the Body Surface of Osteoblasts on a CO_3apatite-collagen Sponge2005

    • Author(s)
      I.Hirata
    • Journal Title

      Dent.Mater.J. 24

      Pages: 460-464

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Epitaxial growth and characteristics of N-doped anatase TiO_2 films grown using a free-radical nitrogen oxide source2005

    • Author(s)
      H.Matsui
    • Journal Title

      J.Appl.Phys. 97

      Pages: 123511-123511

    • Related Report
      2005 Annual Research Report
  • [Journal Article] DNA Pattering by Nano-imprinting Technique and Its Application for Bio-chips2005

    • Author(s)
      H.Tabata
    • Journal Title

      J.Photopolym.Sci.Technol. 18

      Pages: 519-522

    • Related Report
      2005 Annual Research Report
  • [Journal Article] High-temperature cluster glass state and photomagnetism in Zn- and Ti-substituted NiFe_2O_4 films2005

    • Author(s)
      M.Seki
    • Journal Title

      J.Appl.Phys. 97

      Pages: 83541-83541

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Photocontrol of magnetization in Al-substituted Fe_3O_4 thin films2005

    • Author(s)
      M.Seki
    • Journal Title

      Solid State Commun. 133

      Pages: 791-796

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Photoemission study of poly(dA)-poly(dT) DNA : Experimental and theoretical approach to the electronic density of states2005

    • Author(s)
      H.Wadati
    • Journal Title

      Appl.Phys.Lett. 86

      Pages: 23901-23901

    • Related Report
      2005 Annual Research Report 2004 Annual Research Report
  • [Journal Article] Self-assembly ZnO nanorods by pulsed laser deposition under argon atmosphere2005

    • Author(s)
      S.Choopun
    • Journal Title

      J.Cryst.Growth 274

      Pages: 167-172

    • Related Report
      2005 Annual Research Report 2004 Annual Research Report
  • [Journal Article] DNAナノテクノロジー/半導体トップダウン技術と自己組織化ボトムアップ技術の融合2005

    • Author(s)
      田畑 仁
    • Journal Title

      表面技術 56(12)

      Pages: 892-896

    • Related Report
      2005 Annual Research Report
  • [Journal Article] バイオ関連材料のテラヘルツ分光2005

    • Author(s)
      田畑 仁
    • Journal Title

      光学 34(9)

      Pages: 475-477

    • Related Report
      2005 Annual Research Report
  • [Journal Article] リラクサー強誘電体 -バルク,薄膜,人工格子-2005

    • Author(s)
      田畑 仁
    • Journal Title

      表面科学 26(4)

      Pages: 200-207

    • NAID

      10015506660

    • Related Report
      2005 Annual Research Report
  • [Journal Article] DNAと半導体 ナノテクノロジーと融合2005

    • Author(s)
      田畑 仁
    • Journal Title

      Bio Clinica 20(1)

      Pages: 47-52

    • Related Report
      2005 Annual Research Report
  • [Journal Article] DNAと半導体ナノテクノロジーと融合2005

    • Author(s)
      田畑 仁
    • Journal Title

      Bio Clinica 20・1

      Pages: 47-52

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Characteristics of polarity-controlled ZnO films fabricated using the homoepitaxy technique2004

    • Author(s)
      H.Matsui
    • Journal Title

      J.Vac.Sci.Technol.B 22

      Pages: 2454-2461

    • Related Report
      2004 Annual Research Report
  • [Journal Article] N doping using N_2O and NO sources : From the viewpoint of ZnO2004

    • Author(s)
      H.Matsui
    • Journal Title

      J.Appl.Phys. 95

      Pages: 5882-5888

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Orthorhombic Molybdenum Trioxide Whiskers by Vapor Transport Method2004

    • Author(s)
      S.Choopun
    • Journal Title

      Jpn.J.Appl.Phys. 43

    • Related Report
      2004 Annual Research Report
  • [Journal Article] High-Energy Spectroscopy Study of the Ferromagnetic Diluted Magnetic Semiconductor Zn1-xVxO2004

    • Author(s)
      Y.Ishida
    • Journal Title

      Physica B 351

      Pages: 304-306

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Colossal magnetoresistance in spinel type Zn1-xNixFe2O42004

    • Author(s)
      A.K.M.Akther Hossain
    • Journal Title

      J.Appl.Phys. 96・2

      Pages: 1273-1275

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Immobilization of Probe DNA on Ta_2O_5 Thin Film and Detection of Hybridized Helix DNA by Using IS-FET2004

    • Author(s)
      T.Ohtake
    • Journal Title

      Jpn.J.Appl.Phys. 43

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Structural and multiferroic properties of BiFeO_3 thin films at room temperature2004

    • Author(s)
      K.Y.Yun
    • Journal Title

      J.Appl.Phys. 96・6

      Pages: 3399-3403

    • Related Report
      2004 Annual Research Report
  • [Journal Article] A simple fabrication method of nanogap electrodes for top-contacted geometry : application to porphyrin nanorods and a DNA network2004

    • Author(s)
      Y.Otsuka
    • Journal Title

      Nanotechnology 15

      Pages: 1639-1644

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Sputtering and annealing effect of sapphire substrate for an orientation of lead phthalocyanine films2004

    • Author(s)
      S.Tabuchi
    • Journal Title

      Surface Science 571

      Pages: 117-127

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Direct Deoxyribonucleic Acid Detection Using Ion-Sensitive Field-Effect Transistors Based on Peptide Nucleic Acid2004

    • Author(s)
      T.Uno
    • Journal Title

      Jpn.J.Appl.Phys. 43・12B

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Transparent magnetic semiconductors based on ZnO2004

    • Author(s)
      H.Saeki
    • Journal Title

      J.Phys.: Condens.Matter 16

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Growth and impurities in Zn-polar homoepitaxial ZnO films on (0001) ZnO2004

    • Author(s)
      H.Matsui
    • Journal Title

      Proc.of 10th PASPS

      Pages: 39-42

    • Related Report
      2004 Annual Research Report
  • [Journal Article] MCD and NMR study of transition-metal doped ZnO thin films2004

    • Author(s)
      H.Saeki
    • Journal Title

      Proc.of 10th PASPS

      Pages: 32-34

    • Related Report
      2004 Annual Research Report
  • [Journal Article] DNA自己組織化を利用したナノパターン制御形成〜ボトムアップ半導体ナノテクノロジー〜2004

    • Author(s)
      田畑 仁
    • Journal Title

      SEAJ Journal 92

      Pages: 24-27

    • Related Report
      2004 Annual Research Report
  • [Journal Article] 超伝導材料以外への展開:磁性材料・誘電材料・光学材料2004

    • Author(s)
      田畑 仁
    • Journal Title

      (社)日本応用磁気学会 第136研究会

      Pages: 17-24

    • NAID

      10013116167

    • Related Report
      2004 Annual Research Report
  • [Book] 科学立国日本を築く2006

    • Author(s)
      田畑仁
    • Total Pages
      325
    • Publisher
      日刊工業新聞社
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Book] 科学立国日本を築く2006

    • Author(s)
      田畑 仁
    • Total Pages
      325
    • Publisher
      日刊工業新聞社
    • Related Report
      2006 Annual Research Report
  • [Book] Ferroelectric Thin Films2005

    • Author(s)
      Hitoshi Tabata
    • Total Pages
      248
    • Publisher
      Springer Verlag
    • Related Report
      2005 Annual Research Report
  • [Patent(Industrial Property Rights)] 光触媒作用を有する窒素ドープ酸化チタンとその製造方法2005

    • Inventor(s)
      松井 裕章, 田畑 仁, 溝淵 文章
    • Industrial Property Rights Holder
      住友精化(株), 園田 隆一
    • Industrial Property Number
      2005-034668
    • Filing Date
      2005-02-10
    • Related Report
      2004 Annual Research Report
  • [Patent(Industrial Property Rights)] 自己組織化材料または微粒子を基板上に固定化する方法、および当該方法を用いて作製した基板2004

    • Inventor(s)
      川合 知二, 田畑 仁, 大塚 洋一, 山田 郁彦, 松本 卓他
    • Industrial Property Rights Holder
      (独)科学技術振興機構
    • Industrial Property Number
      2004-381549
    • Filing Date
      2004-12-28
    • Related Report
      2004 Annual Research Report

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Published: 2004-04-01   Modified: 2016-04-21  

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