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EVALUATION OF TRTIUM INVENTORY IN LOW-ACTIVATED FUSION MATERIALS BASED ON IRRADIATION EXPERIMENTS

Research Project

Project/Area Number 16360458
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Nuclear fusion studies
Research InstitutionKYOTO UNIVERSITY

Principal Investigator

TAKAGI Ikuji  Kyoto University, Graduate School of Engineering, Associate Professor, 工学研究科, 助教授 (20206717)

Co-Investigator(Kenkyū-buntansha) MORIYAMA Hirotake  Kyoto University, Graduate School of Engineering, Professor, 工学研究科, 教授 (90127150)
MORITANI Kimikazu  Kyoto University, Graduate School of Engineering, Assistant Professor, 工学研究科, 助手 (50111943)
AKIYOSHI Masafumi  Kyoto University, Graduate School of Engineering, Assistant Professor, 工学研究科, 助手 (70378793)
Project Period (FY) 2004 – 2006
Project Status Completed (Fiscal Year 2006)
Budget Amount *help
¥8,500,000 (Direct Cost: ¥8,500,000)
Fiscal Year 2006: ¥3,300,000 (Direct Cost: ¥3,300,000)
Fiscal Year 2005: ¥2,800,000 (Direct Cost: ¥2,800,000)
Fiscal Year 2004: ¥2,400,000 (Direct Cost: ¥2,400,000)
KeywordsTRITIUM INVENTORY / RADIATION DAMAGE / HYDROGEN TRAPPING / ION BEAM ANALYSIS / LOW ACTIVATION / VANADIUM / COPPER / DEFECT / アルミニウム / 鉄 / 低放射化 / 回復
Research Abstract

Tritium inventory in low-activated materials such as vanadium, copper, aluminum and iron has been experimentally studied using ion beam techniques. Samples were irradiated with energetic helium or hydrogen ions and simultaneously charged with deuterium atoms from plasma. Deuterium was representative of tritium. Deuterium depth profiles in the samples were observed by nuclear reaction analysis.
Irradiation to vanadium yielded much amount of traps for hydrogen isotopes and the deuterium inventory significantly increased. As the traps were annihilated around 500 K, lower than fusion operating temperatures, the traps would not affect the tritium inventory. As vanadium is exothermic for hydrogen dissociation, dissolved tritium would mainly contribute to the inventory. Vanadium alloy of V-Cr-Ti showed the same characteristics as vanadium.
Two types of the traps were produced in copper by the irradiation. One was considered to be vacancies and the other interstitial loops. Both the traps were n … More ot annihilated at 673 K, which indicated that the traps much increased the tritium inventory of copper tubes in the cooling system. As copper is endothermic for hydrogen dissociation, trapped tritium would mainly contribute to the inventory.
No traps were observed in aluminum, which was heavily irradiated by helium ions. It is expected that the tritium inventory in aluminum is very low at any operating conditions of the fusion reactor.
As for vanadium, the deuterium concentration in iron significantly increased due to the trap produced by irradiation. The trap was considered to be vacancy which was annihilated around 500 K. Iron is a candidate for low-inventory materials.
In the experiments, parameters such as the diffusion 'coefficient, the trap density, the equilibrium constant for trapping and de-trapping and trap production rate have been quantitatively determined. Knowing the reactor conditions such as the damage rate and the incident fuel particle flux, the tritium inventory can be evaluated with these parameters. Less

Report

(4 results)
  • 2006 Annual Research Report   Final Research Report Summary
  • 2005 Annual Research Report
  • 2004 Annual Research Report
  • Research Products

    (18 results)

All 2007 2006 2005 2004 Other

All Journal Article (18 results)

  • [Journal Article] Characteristics of traps for hydrogen in helium-irradiated copper2007

    • Author(s)
      I.Takagi
    • Journal Title

      Journal of Nuclear Materials (in press)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Annual Research Report 2006 Final Research Report Summary
  • [Journal Article] Production and annihilation of deuterium traps in He-irradiated vanadium2007

    • Author(s)
      I.Takagi
    • Journal Title

      Journal of Nuclear Materials 363-365

      Pages: 955-959

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] PRODUCTION AND ANNIHILATION OF DEUTERIUM TRAPS IN He-IRRADIATED VANADIUM2007

    • Author(s)
      I.TAKAGI
    • Journal Title

      JOURNAL OF NUCLEAR MATERIALS 363-365

      Pages: 955-959

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Production and annihilation of deuterium traps in He-irradiated vanadium2007

    • Author(s)
      I.Takagi
    • Journal Title

      Journal of Nuclear Materials (in press)

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Experiments on deuterium trapping in helium-irradiated copper2006

    • Author(s)
      I.Takagi
    • Journal Title

      Fusion Engineering and Design 81

      Pages: 785-789

    • NAID

      130007026151

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Annual Research Report 2006 Final Research Report Summary 2005 Annual Research Report
  • [Journal Article] EXPERIMENTS ON DEUTERIUM TRAPPING IN HELIUM-IRRADIATED COPPER2006

    • Author(s)
      I.TAKAGI
    • Journal Title

      FUSION ENGINEERING AND DESIGN 81

      Pages: 785-789

    • NAID

      130007026151

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Deuterium trapping near vanadium surface bombarded with hydrogen ions2005

    • Author(s)
      I.Takagi
    • Journal Title

      Nuclear Instruments and Methods B232

      Pages: 327-332

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] TOF measurement of eV energy hydrogen atoms reflected by stainless steel surface2005

    • Author(s)
      M.Akiyoshi, I.Takagi
    • Journal Title

      Nuclear Instruments and Methods B232

      Pages: 173-177

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] DEUTERIUM TRAPPING NEAR VANADIUM SURFACE BOMBARDED WITH HYDROGEN IONS2005

    • Author(s)
      I.TAKAGI
    • Journal Title

      NUCLEAR INSTRUMENTS AND METHODS B232

      Pages: 327-332

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] TOF MEASUREMENT OF eV ENERGY HYDROGEN ATOMS REFLECTED BY STAINLESS STEEL SURFACE2005

    • Author(s)
      M.AKIYOSHI, I.TAKAGI
    • Journal Title

      NUCLEAR INSTRUMENTS AND METHODS B232

      Pages: 173-177

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Deuterium trapping near vanadium surface bombarded with hydrogen ions2005

    • Author(s)
      I.Takagi
    • Journal Title

      Nuclear Instruments and Methods in Physics Research B 232

      Pages: 327-332

    • Related Report
      2005 Annual Research Report
  • [Journal Article] TOF measurement of eV energy hydrogen atoms reflected by stainless-steel surface2005

    • Author(s)
      M.Akiyoshi, I.Takagi
    • Journal Title

      Nuclear Instruments and Methods in Physics Research B 232

      Pages: 173-177

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Deuterium trapping near vanadium surface bombarded with hydrogen ions2005

    • Author(s)
      I.Takagi
    • Journal Title

      Nuclear Instruments and Methods in Physics Research B (発表予定)

    • Related Report
      2004 Annual Research Report
  • [Journal Article] TOF measurement of eV energy hydrogen atoms reflected by stainless-steel surface2005

    • Author(s)
      M.Akiyoshi, I.Takagi
    • Journal Title

      Nuclear Instruments and Methods in Physics Research B (発表予定)

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Potential energy diagram for hydrogen near vanadium surface2004

    • Author(s)
      I.Takagi
    • Journal Title

      Journal of Nuclear Materials 329-333

      Pages: 434-437

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary 2004 Annual Research Report
  • [Journal Article] POTENTIAL ENERGY DIAGRAM FOR HYDROGEN NEAR VANADIUM SURFACE2004

    • Author(s)
      I.TAKAGI
    • Journal Title

      JOURNAL OF NUCLEAR MATERIALS 329-333

      Pages: 434-437

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Simulated waste glass corrosion in humic acid solution using Rutherford backscattering spectrometry2004

    • Author(s)
      I.Takagi
    • Journal Title

      Journal of Nuclear Science and Technology 41(8)

      Pages: 837-842

    • NAID

      10013169546

    • Related Report
      2004 Annual Research Report
  • [Journal Article] CHARACTERISTICS OF TRAPS FOR HYDROGEN IN HELIUM-IRRADIATED COPPER

    • Author(s)
      I.TAKAGI
    • Journal Title

      JOURNAL OF NUCLEAR MATERIALS (IN PRESS)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary

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Published: 2004-04-01   Modified: 2016-04-21  

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