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Strange metamagnetism and magnetic transitions of TbCu_2Ge_2

Research Project

Project/Area Number 16540323
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Condensed matter physics II
Research InstitutionYamaguchi University

Principal Investigator

SHIGEOKA Toru  Yamaguchi University, Faculty of Science, Professor, 理学部, 教授 (50167441)

Co-Investigator(Kenkyū-buntansha) UWATOKO Yoshiya  University of Tokyo, Institute for Solid State Physics, Associate Professor, 物性研究所, 助教授 (40213524)
Project Period (FY) 2004 – 2005
Project Status Completed (Fiscal Year 2005)
Budget Amount *help
¥3,600,000 (Direct Cost: ¥3,600,000)
Fiscal Year 2005: ¥1,600,000 (Direct Cost: ¥1,600,000)
Fiscal Year 2004: ¥2,000,000 (Direct Cost: ¥2,000,000)
KeywordsTbCu2Ge2 / rare earth compound / metamagnetism / antiferromagnetism / magnetization process / magnetic susceptibility / 比熱
Research Abstract

The tetragonal ternary compound TbCu_2Ge_2 shows a strange metamagnetic transition ; a metamagnetic transition, which appears in the hard magnetization [001] process, persists up to about 30 K above TN. This study has been carried out in order to understand the mechanism of this metamagnetic transition.
1.Single crystal Growth :
Some single crystal compounds have been grown to study physical properties and Neutron diffraction. The crystals are, however, too large mosaic to use the neutron diffraction. An attempt to growth a good crystal is now in progress.
2.Electrical resistivity :
Two anomalies are observed at TN=12.3 K and Tt=9 K in the temperature dependence of electrical resistivity. The way of transition shows the second order transition at TN and the first order one at Tt. No anomaly has been observed around 30 K where a broad peak appears in the magnetic susceptibility along the c-axis vs. temperature curve.
3.TbCu_2Si_2 single crystal :
The isomorphs single crystal compound TbCu_2Si_2 has been grown to study the magnetic properties. The comparison between those of the Ge and Si compound may lead better understanding for this strange metamagnetic transition. The magnetic behaviors of the Si compound is very similar to those of the Ge compound. The difference between Si and Ge does not affect the magnetic properties.
4.Analysis for Crystalline electric field effects
The CEF effects are very important for understanding the magnetic behaviors. From results of the magnetic susceptibility, magnetization and specific heart, the analysis is progress.

Report

(3 results)
  • 2005 Annual Research Report   Final Research Report Summary
  • 2004 Annual Research Report
  • Research Products

    (24 results)

All 2006 2005 2004

All Journal Article (24 results)

  • [Journal Article] Novel magnetization processes of NdCu_2Si_2 singje crystal.2006

    • Author(s)
      T.Shigeoka
    • Journal Title

      Journal of Alloys and Compounds 408-412

      Pages: 88-91

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Magnetocaloric and structural Properties of SmMn_2Ge_22006

    • Author(s)
      K.Koyama
    • Journal Title

      Journal of Alloys and Compounds 408-412

      Pages: 118-121

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Annual Research Report 2005 Final Research Report Summary
  • [Journal Article] Novel magnetization processes of NdCu_2Si_2 single crystal2006

    • Author(s)
      T.Shigeoka, K.Hirata, Y.Uwatoko
    • Journal Title

      Journal of Alloys and Compounds 408-411

      Pages: 88-91

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Magnetocaloric and Structural Properties of SmMn_2Ge_22006

    • Author(s)
      K.Koyama, S.Miura, H.Okada, T.Shigeoka, S.Fujita, K.Fukamichi, K.Watanabe
    • Journal Title

      Journal of Alloys and Compounds 408-411

      Pages: 88-91

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Novel magnetization processes of NdCu_2Si_2 single crystal.2006

    • Author(s)
      T.Shigeoka
    • Journal Title

      Journal of Alloys and Compounds 408-412

      Pages: 88-91

    • Related Report
      2005 Annual Research Report
  • [Journal Article] High-field X-ray Diffraction Measurement of SmMn_2Ge_2.2005

    • Author(s)
      S.Miura
    • Journal Title

      Japanese Journal of Applied Physics 44

      Pages: 1258-1259

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Annual Research Report 2005 Final Research Report Summary
  • [Journal Article] Magnetic phase transitions in PrCu_2Ge_22005

    • Author(s)
      T.Shigeoka
    • Journal Title

      Physica B 359-361

      Pages: 923-925

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Annual Research Report 2005 Final Research Report Summary
  • [Journal Article] High-field X-ray Diffraction Measurement of SmMn_2Ge_22005

    • Author(s)
      S.Miura, K.Koyama, H.Okada, T.Shigeoka, K.Watanabe
    • Journal Title

      Japanese Journal of Applied Physics 44

      Pages: 1258-1259

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Magnetic phase transitions in PrCu_2Ge_22005

    • Author(s)
      T.Shigeoka, K.Hirata, T.Nakano, Y.Uwatoko
    • Journal Title

      Physica B. 359-361

      Pages: 923-925

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Pulsed-neutron diffraction studies of multi-step Metamagnetism in DyRu_2Si_22004

    • Author(s)
      S.Kawano, M.Takahashi, T.Shigeoka, N.Iwata, M.J.Bull
    • Journal Title

      Physica, B. 346-347

      Pages: 99-103

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Anomalous metamagnetic behavior of TbCu_2Ge_2 single crystal2004

    • Author(s)
      T.Shigeoka, M.Shiraishi, H.Mitamura, Y.Uwatoko, T.Fujiwara, T.Goto
    • Journal Title

      Physica, B. 346-347

      Pages: 112-116

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] High field magnetization in NdCu_2Ge_2 single crystal2004

    • Author(s)
      T.Shigeoka, K.Hirata, H.Mitamura, Y.Uwatoko, T.Goto
    • Journal Title

      Physica, B. 346-347

      Pages: 117-121

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Low-temperature resistivity and magnetization of a CeCo_2Si_2 single crystal2004

    • Author(s)
      G.Nakamoto, A.Fuse, M.Kurisu, T.Shigeoka
    • Journal Title

      Journal of Magnetism and Magnetic Materials 272-276

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Frustration and two-dimensional spin ordering in TbRu_2Si_2, TbRu_2Ge_2 and DyRu_2Si_22004

    • Author(s)
      S.Kawano, B.Lebech, M.Takahashi, T.Shigeoka, N.Iwata, T.Kosugi
    • Journal Title

      Journal of Magnetism and Magnetic Materials 272-276

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Magnetic characteristics of DyCu_2Si_2 single crystal2004

    • Author(s)
      T.Shigeoka, K.Ohishi, M.Fukuhara, M.Hedo, Y.Uwatoko
    • Journal Title

      Journal of Magnetism and Magnetic Materials 272-276

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Polar measurement of metamagnetic process in X-Y tetragonal systems2004

    • Author(s)
      H.Suzuki, D.Gignoux, D.Schmitt, T.Shigeoka, P.C.Canfield, C.Detlefs
    • Journal Title

      Journal of Magnetism and Magnetic Materials 272-276

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] The correlation between the phase transition and valence change of the Yb ionic state induced upon pressurization in YbMn_2Ge_22004

    • Author(s)
      T.Fujiwara, Y.Uwatoko, H.Fujii, K.Koyama, M.Motokawa, T.Shigeoka
    • Journal Title

      Journal of Magnetism and Magnetic Materials 272-276

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Neutron Diffraction Studies of Two-Dimensional Ordering in the Low Temperature Phase in TbRu_2Si_22004

    • Author(s)
      S.Kawano, M.Takahashi, T.Shigeoka, N.Iwata, B.Lebech
    • Journal Title

      Physica B. 350

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Anomalous metamagnetic behavior of TbCu_2Ge_2 single crystal2004

    • Author(s)
      T.Shigeoka
    • Journal Title

      Physica B 346

      Pages: 112-116

    • Related Report
      2004 Annual Research Report
  • [Journal Article] High field magnetization in NdCu_2Ge_2 single crystal2004

    • Author(s)
      T.Shigeoka
    • Journal Title

      Physica B 346

      Pages: 117-121

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Pulsed-neutron diffraction studies of multi-step Metamagnetism in DyRu_2Si_22004

    • Author(s)
      S.Kawano
    • Journal Title

      Physica B 346

      Pages: 99-103

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Magnetic characteristics of DyCu_2Si_2 single crystal2004

    • Author(s)
      T.Shigeoka
    • Journal Title

      Journal of Magnetism and Magnetic Materials 272

      Pages: 429-430

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Polar measurement of metamagnetic process in X-Y tetragonal systems2004

    • Author(s)
      H.Suzuki
    • Journal Title

      Journal of Magnetism and Magnetic Materials 272

      Pages: 459-460

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Frustration and two-dimensional spin ordering in TbRu_2Si_2, TbRu_2Ge_2 and DyRu_2Si_22004

    • Author(s)
      S.Kawano
    • Journal Title

      Journal of Magnetism and Magnetic Materials 272

      Pages: 363-365

    • Related Report
      2004 Annual Research Report

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Published: 2004-04-01   Modified: 2020-05-15  

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