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High resolution spectroscopy of multi-electron photoexcitation resonances in a static electric field

Research Project

Project/Area Number 16540362
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field 原子・分子・量子エレクトロニクス・プラズマ
Research InstitutionHigh Energy Accelerator Research Organization

Principal Investigator

AZUMA Yoshiro  High Energy Accelerator Research Organization, Institute of Materials Structure Science, Associate Professor (50270393)

Project Period (FY) 2004 – 2005
Project Status Completed (Fiscal Year 2005)
Budget Amount *help
¥3,700,000 (Direct Cost: ¥3,700,000)
Fiscal Year 2005: ¥1,600,000 (Direct Cost: ¥1,600,000)
Fiscal Year 2004: ¥2,100,000 (Direct Cost: ¥2,100,000)
Keywordssynchrotron radiation / two electron excitation / metastable atom / 多電子効果 / 光励起
Research Abstract

Helium is the simplest neutral atom with electron-electron correlation. Helium double photoexcitation is the most typical of electron correlation effects, transcending the independent electron approximation, and thus becomes an important theme for atomic physics with synchrotron radiation. Unlike the Stark effect of hydrogen like atoms, the system dominated by electron correlation and the effect of static electric field on the decay process is opening up new directions in the theoretical studies of many electron effects. In the future, studies of two electron excitations and three electron excitation with other rare gases and the lithium atom should provide new fertile ground for research.
An important aspect of the experimental methodology of this research is the fluorescence detection and metastable atoms detection utilizing the time structure of the signal obtained during single-bunch operation of synchrotron radiation In order to fully utilize the time structure of the signal, modifications to the apparatus including the supersonic expansion chamber were implemented. They resulted in the greater target dnsity and improved directionality, which enabled the previously difficult fluorescence and metastable atoms detection. Our data indicates strong distortion of the ion yield spectra over the region of N equal to approximately 6, which indicate the emergence of normally forbidden transitions. These all stand out very clearly in the spectra of alternative decay modes including fluorescence and metastables.
In addition to the helium data, we obtained preliminary data of the fluorescence from hydrogen molecules which indicate that extension of our methodology to molecules shoud be pursued.

Report

(3 results)
  • 2005 Annual Research Report   Final Research Report Summary
  • 2004 Annual Research Report
  • Research Products

    (9 results)

All 2006 2004 Other

All Journal Article (7 results) (of which Peer Reviewed: 3 results) Presentation (2 results)

  • [Journal Article] Photoionization of He in the 3lnl' doubly excited state energy region : angular distribution of the fluorescence from the residual ion He+(2p)2P2006

    • Author(s)
      Y.Azuma, et al.
    • Journal Title

      Journal of Physics B 39

      Pages: 4819-4824

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Apparatus for measuring static electric field effects in photoexcitation experiments of gas-phase atoms and molecules.2004

    • Author(s)
      J.R.Harries, Y.Azuma
    • Journal Title

      Review of Scientific Instruments 75-11

      Pages: 4406-4412

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Experimental determination of the lifetimes of the 2(1,0)'2pnd' doubly excited states of helium by detection of VUV fluorescence2004

    • Author(s)
      Y.Azuma, et al.
    • Journal Title

      Journal of Physics B 37

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Apparatus for measuring static electric field effects in photoexcitation experiments of gas-phase atoms and molecules2004

    • Author(s)
      J.R.Harries, Y.Azuma
    • Journal Title

      Review of Scientific Instruments 75-11

      Pages: 4406-4412

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Apparatus for measuring static electric field effects in photoexcitation experiments of gas-phase atoms and molecules2004

    • Author(s)
      James R.Harries
    • Journal Title

      Review of Scientific Instruments 75-11

      Pages: 4406-4406

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Experimental determination of the lifetimes of the 2(1,0) ‘2pnd' doubly excited states of helium by detection of VUV fluorescence2004

    • Author(s)
      James R.Harries
    • Journal Title

      Journal of Physics B 37

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Photoionization of He in the 31nl' doubly excited state energy region : angular distribution of the fluorescence from the residual ion He+(2p)2P

    • Author(s)
      Y.Azuma, et al.
    • Journal Title

      Journal of Physics B 39

      Pages: 4819-4824

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Presentation] Double photoexcitation of helium in a strong static electric field2004

    • Author(s)
      Yoshiro Azuma
    • Organizer
      The 14^<th> International Conference on Vacuum Ultraviolet Physics(invited)
    • Place of Presentation
      Cairns, Australia
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Presentation] Double photoexcitation of helium in a strong static electric field2004

    • Author(s)
      Yoshiro Azuma
    • Organizer
      The 14^<th> International Conference on Vacuum Ultraviolet Physics
    • Place of Presentation
      Cairns, Australia
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary

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Published: 2004-04-01   Modified: 2016-04-21  

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