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Direct observation of spin electronic states of novel Rashba and topological materials with small multi-domains

Research Project

Project/Area Number 16H02114
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field Thin film/Surface and interfacial physical properties
Research InstitutionHiroshima University

Principal Investigator

OKUDA TAICHI  広島大学, 放射光科学研究センター, 教授 (80313120)

Project Period (FY) 2016-04-01 – 2020-03-31
Project Status Completed (Fiscal Year 2019)
Budget Amount *help
¥42,250,000 (Direct Cost: ¥32,500,000、Indirect Cost: ¥9,750,000)
Fiscal Year 2019: ¥4,940,000 (Direct Cost: ¥3,800,000、Indirect Cost: ¥1,140,000)
Fiscal Year 2018: ¥5,590,000 (Direct Cost: ¥4,300,000、Indirect Cost: ¥1,290,000)
Fiscal Year 2017: ¥15,990,000 (Direct Cost: ¥12,300,000、Indirect Cost: ¥3,690,000)
Fiscal Year 2016: ¥15,730,000 (Direct Cost: ¥12,100,000、Indirect Cost: ¥3,630,000)
Keywords新奇トポロジカル物質 / 局所スピン / スピントロニクス / マイクロフォーカスレーザー / 多チャンネルスピン分解光電子分光 / トポロジカル / ラシュバ / スピン分解光電子分光 / レーザー / 多チャンネルスピン検出 / レーザー光電子分光 / 新規ラシュバ物質 / トポロジカル絶縁体 / ラシュバ効果 / マルチチャンネル / レーザー光 / 光電子分光 / 表面・界面物性 / スピンエレクトロニクス / 低速電子回折スピン検出器 / マルチチャンネル検出 / レーザーマイクロビーム / ハーフメタル / 微小ドメイン
Outline of Final Research Achievements

Recently, it has been theoretically predicted that there can be a local spin polarization state, which is induced by spin-orbit interaction and local symmetry breaking, even in materials possessing centrosymmetry. However, in such materials, there must be the site which is possessing opposite spin-polarization, it is necessary to do site selective measurement to observe the local spin-polarized electronic states experimentally. In order to investigate the electronic state of such novel spin-polarized materials, in this study, we have developed a new spin- and angle-resolved photoelectron spectroscopy system utilizing the focused laser beam (~10 micron) as the excitation light. Since the intensity of the focused beam is low and spin-polarized photoemission measurement is inefficient, we have also developed a multi-channel spin- detector which can improve the measurement efficiency more than 1000 times higher than the normal single channel spin detector.

Academic Significance and Societal Importance of the Research Achievements

トポロジカル絶縁体に代表されるトポロジカル物質は、非磁性体であるがスピン偏極した電子状態を有し、電場などによってそのスピンを制御することができる可能性があるため次世代スピントロニクスデバイスのキーマテリアルとして注目されている。本研究では局所構造にスピン偏極電子状態を有することが理論的に予想されていた新奇スピン偏極物質のスピン電子状態を探るために、レーザー光をミクロンサイズに集光するとともに高効率多チャンネルスピン検出器を開発して、サイト選択的に効率よくスピン電子状態観測を可能とするシステムを構築した。実験的に新奇スピン偏極物質の物性が観測可能となり、将来のスピントロニクス実現へ貢献した。

Report

(5 results)
  • 2019 Annual Research Report   Final Research Report ( PDF )
  • 2018 Annual Research Report
  • 2017 Annual Research Report
  • 2016 Annual Research Report
  • Research Products

    (29 results)

All 2020 2019 2018 2017 2016 Other

All Int'l Joint Research (2 results) Journal Article (3 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 3 results) Presentation (24 results) (of which Int'l Joint Research: 14 results,  Invited: 14 results)

  • [Int'l Joint Research] 中国科学院(中国)

    • Related Report
      2017 Annual Research Report
  • [Int'l Joint Research] 中国科学院(中国)

    • Related Report
      2016 Annual Research Report
  • [Journal Article] Electronic and spin structure of the wide-band-gap topological insulator: Nearly stoichiometric Bi2Te2S2018

    • Author(s)
      E. Annese, T. Okuda, E. F. Schwier, H. Iwasawa, K. Shimada, M. Natamane, M. Taniguchi, I. P. Rusinov, S. V. Eremeev, K. A. Kokh, O. E. Tereshchenko, E. V. Chulkov, and A. Kimura
    • Journal Title

      Phys. Rev. B

      Volume: 97 Issue: 20

    • DOI

      10.1103/physrevb.97.205113

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Enhanced surface state protection and band gap in the topological insulator PbBi4Te4S32018

    • Author(s)
      K. Sumida, T. Natsumeda, K. Miyamoto, I. V. Silkin, K. Kuroda, K. Shirai, S. Zhu, K. Taguchi, M. Arita, J. Fujii, A. Varykhalov, O. Rader, V. A. Golyashov, K. A. Kokh, O. E. Tereshchenko, E. V. Chulkov, T. Okuda, and A. Kimura
    • Journal Title

      PHYSICAL REVIEW MATERIALS

      Volume: 2 Issue: 10 Pages: 104201-104201

    • DOI

      10.1103/physrevmaterials.2.104201

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Recent trend of spin-resolved photoemission2017

    • Author(s)
      T. Okuda
    • Journal Title

      Journal of Physics Condensed Matter

      Volume: 29 Issue: 48 Pages: 483001-483001

    • DOI

      10.1088/1361-648x/aa8f28

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Presentation] Investigation of Temperature-induced Topological Phase Transition in TlBiS22020

    • Author(s)
      T. Imai, K. Kato, K. Miyamoto, T. Okuda
    • Organizer
      The 23rd Hiroshima International Symposium on Synchrotron Radiation
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Development of Multi-channel Spin-detector at HiSOR2019

    • Author(s)
      T. Matsuda, K. Miyamoto, A. Kimura, and T. Okuda
    • Organizer
      International Young Researchers Workshop on Synchrotron Radiation Science 2019
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Spin-resolved ARPES: high-efficiency detector and results at HiSOR2019

    • Author(s)
      T. Okuda
    • Organizer
      Inauguration of the Undulator Beamline of the Russian-German Laboratory at BESSY II, Accompanied by a workshop on Spin-resolved Photoemission and Electronic Structure of Quantum and Energy Materials
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] High-efficient spin-resolved photoelectron spectroscopy end-station at Hiroshima Synchrotron Radiation Center2019

    • Author(s)
      T. Okuda
    • Organizer
      Chirality-induced spin selectivity and its related phenomena, The 80th Okazaki Conference
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Hidden spin-polarized states at the interface of layered materials investigated by spin- and angle-resolved photoemission2019

    • Author(s)
      T. Okuda
    • Organizer
      The 17th International Conference on the Formation of Semiconductor Interfaces (ICFSI17)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Hidden Local Spin-polarized Electronic States investigated by Spin- and Angle-resolved Photoelectron Spectroscopy2019

    • Author(s)
      T. Okuda
    • Organizer
      American Vacuum Society 66th International Symposium and Exhibition (AVS66)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] TlBi(S1-xSex)2の温度誘起トポロジカル相転移の光電子分光による研究2019

    • Author(s)
      今井健人, 加藤和貴、Jiahua Chen, 宮本幸司、木村昭夫、奥田太一
    • Organizer
      日本物理学会 2019年秋季大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] TlBiS2およびTlBiSe2における温度誘起トポロジカル相転移の光電子分光による研究2019

    • Author(s)
      今井健人, 加藤和貴、松田旭央、Jiahua Chen, 宮本幸司、木村昭夫、奥田太一
    • Organizer
      日本放射光学会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Recent activities and future prospects of spin- and angle-resolved photoemission spectroscopy at HiSOR2019

    • Author(s)
      T. Okuda
    • Organizer
      1st International Workshop on Momentum Microscopy and Spectroscopy for Materials Science
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Spin-resolved photoelectron spectroscopy at HiSOR, present status and future prospect2019

    • Author(s)
      T.Okuda
    • Organizer
      22nd Hiroshima International Symposium on Synchrotron Radiation
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Design of multi-channel spin detector at HiSOR2019

    • Author(s)
      T. Matsuda, K. Miyamoto, A. Kimura, T. Okuda
    • Organizer
      23rd Hiroshima International Symposium on Synchrotron Radiation
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] マルチチャンネルスピン検出器の開発(1)2019

    • Author(s)
      松田旭央、宮本幸治、木村昭夫、奥田太一
    • Organizer
      日本物理学会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Recent activities and future prospects of spin- and angle-resolvedphotoemission spectroscopy at HiSOR2019

    • Author(s)
      Taichi Okuda
    • Organizer
      The first international workshop on Momentum Microscopy and Spectroscopy for materials science
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Design of Multi-channel spin detector at HiSOR2019

    • Author(s)
      T. Matsuda, K. Miyamoto, A. Kimura, T. Okuda
    • Organizer
      23rd Hiroshima International Symposium on Synchrotron Radiation
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Exploration of hidden spin polarized electronic states by high-resolution spin-resolved photoemission2018

    • Author(s)
      Taichi Okuda
    • Organizer
      International Workshop on Trends in Advanced Spectroscopy in Materials Science (TASPEC)
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 放射光スピン分解光電子分光の現状と新展開2018

    • Author(s)
      奥田太一
    • Organizer
      日本物理学会第73回年会シンポジウム「シンクロトロン光電子分光が拓く物性研究の新展開」
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] Spin Resolved Photoelectron Spectroscopy for the investigation of hidden spin polarized states2017

    • Author(s)
      Taichi Okuda
    • Organizer
      21th HiSOR symposium
    • Place of Presentation
      広島大学 (広島県)
    • Year and Date
      2017-03-02
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] VLEED型スピン検出器によるスピン分解ARPESの現状2017

    • Author(s)
      奥田太一
    • Organizer
      第4回JASRIワークショップ
    • Place of Presentation
      SPring-8 (兵庫県)
    • Year and Date
      2017-02-22
    • Related Report
      2016 Annual Research Report
    • Invited
  • [Presentation] Exploration of hidden spin polarized electron by high-resolution spin- and angle-resolved photoemission2017

    • Author(s)
      Taichi Okuda
    • Organizer
      Symposium on Surface Science & Nanotechnology 25th Anniversary of SSSJ-Kansai
    • Place of Presentation
      Kyoto International Community House (京都府)
    • Year and Date
      2017-01-24
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] VLEEDスピン検出器によるバルク敏感スピン分解光電子分光の可能性2017

    • Author(s)
      奥田太一
    • Organizer
      SPring-8シンポジウム2017 SPRUCサテライト研究会 「軟X線スピン分解ARPES検討会」
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] HiSORにおけるスピン分解光電子分光現状と展望2017

    • Author(s)
      奥田太一
    • Organizer
      PF研究会「次世代光源で拓かれる光電子分光研究の将来展望」
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] Development of High-resolution Spin- and Angle-resolved Photoelectron Spectrometer Using VLEED Spin Detector and its application2017

    • Author(s)
      奥田太一
    • Organizer
      日韓ワークショップ(釜山大学)
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] スピン分解光電子分光で探る隠されたスピン分裂状態2016

    • Author(s)
      奥田太一
    • Organizer
      UVSORシンポジウム
    • Place of Presentation
      分子化学研究所 (愛知県)
    • Year and Date
      2016-10-29
    • Related Report
      2016 Annual Research Report
    • Invited
  • [Presentation] 高効率スピン分解光電子分光装置の開発と表面スピン電子状態研究2016

    • Author(s)
      奥田太一
    • Organizer
      日本表面科学会九州支部 平成28年度九州表面・真空研究会
    • Place of Presentation
      九州大学 (福岡県)
    • Year and Date
      2016-06-11
    • Related Report
      2016 Annual Research Report
    • Invited

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Published: 2016-04-21   Modified: 2022-08-30  

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