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Generation of superheavy element atomic beams and its application to extreme chemistry of superheavy elements

Research Project

Project/Area Number 16H02130
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field Quantum beam science
Research InstitutionJapan Atomic Energy Agency

Principal Investigator

Nagame Yuichiro  国立研究開発法人日本原子力研究開発機構, 原子力科学研究部門 原子力科学研究所 先端基礎研究センター, 研究嘱託 (80354885)

Co-Investigator(Kenkyū-buntansha) 塚田 和明  国立研究開発法人日本原子力研究開発機構, 原子力科学研究部門 原子力科学研究所 先端基礎研究センター, 研究主席 (30343916)
佐藤 哲也  国立研究開発法人日本原子力研究開発機構, 原子力科学研究部門 原子力科学研究所 先端基礎研究センター, 研究副主幹 (40370382)
Chiera Nadine  国立研究開発法人日本原子力研究開発機構, 原子力科学研究部門 原子力科学研究所 先端基礎研究センター, 博士研究員 (00807498)
豊嶋 厚史  国立研究開発法人日本原子力研究開発機構, 原子力科学研究部門 先端基礎研究センター, 研究副主幹 (40414578)
Project Period (FY) 2016-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2020)
Budget Amount *help
¥40,950,000 (Direct Cost: ¥31,500,000、Indirect Cost: ¥9,450,000)
Fiscal Year 2020: ¥3,640,000 (Direct Cost: ¥2,800,000、Indirect Cost: ¥840,000)
Fiscal Year 2019: ¥3,640,000 (Direct Cost: ¥2,800,000、Indirect Cost: ¥840,000)
Fiscal Year 2018: ¥8,840,000 (Direct Cost: ¥6,800,000、Indirect Cost: ¥2,040,000)
Fiscal Year 2017: ¥8,840,000 (Direct Cost: ¥6,800,000、Indirect Cost: ¥2,040,000)
Fiscal Year 2016: ¥15,990,000 (Direct Cost: ¥12,300,000、Indirect Cost: ¥3,690,000)
Keywords超重元素 / 超重元素ビーム / シングルアトム / 相対論効果 / 表面電離 / イオン化エネルギー / 迅速ガスクロマトグラフ / 吸着エンタルピー / 超重原子ビーム / 価電子構造 / 超重分子の形成 / イオンビーム / 分子形成反応 / 真空クロマトグラフ / アエロダイナミックレンズ / Extreme Chemistry
Outline of Final Research Achievements

We have developed a high intensity ion beam extraction technique using a surface ionization source and succeeded in measuring the first ionization energies of heavy actinide elements. The adsorption behavior of the lawrencium (Lr) atom on a metallic Ta surface was also investigated by modifying a cylindrical metal ion source as a chromatographic column. Interesting results were obtained that the adsorption mainly involves electrons different from the valence electrons in the ground state. The volatile compound of dubnium (Db) was successfully synthesized and chemically separated, and the volatile species was determined. The influence of relativistic effects on the formation of the Db compound was also suggested. A high-temperature nozzle-type and an electron recombination-type atomic beam generator were constructed and both them successfully extracted an atomic beam. However, it was found that further improvement is needed for the application to superheavy elements.

Academic Significance and Societal Importance of the Research Achievements

量子ビーム技術の高度化を進めることで重アクチノイド元素の第一イオン化エネルギー測定を可能にした。この結果、元素周期表でのアクチノイド系列がローレンシウムで終了することを初めて実験的に検証した。また、重い元素で特徴的な原子核と電子との強い相互作用を、化合物形成という観点から明らかにした。これらの成果は、元素の周期表全体を理解するという化学の基本的課題に貢献したといえる。さらにシングルアトムスケールでの実験が要求される超重元素領域の化学、「極限の化学」という新しい研究領域を開拓している。

Report

(6 results)
  • 2020 Annual Research Report   Final Research Report ( PDF )
  • 2019 Annual Research Report
  • 2018 Annual Research Report
  • 2017 Annual Research Report
  • 2016 Annual Research Report
  • Research Products

    (97 results)

All 2021 2020 2019 2018 2017 2016 Other

All Int'l Joint Research (15 results) Journal Article (18 results) (of which Int'l Joint Research: 15 results,  Peer Reviewed: 18 results,  Open Access: 5 results) Presentation (63 results) (of which Int'l Joint Research: 37 results,  Invited: 22 results) Book (1 results)

  • [Int'l Joint Research] 重イオン研究所(GSI)/Johannes Gutenberg-University Mainz(ドイツ)

    • Related Report
      2020 Annual Research Report
  • [Int'l Joint Research] Paul Scherrer Institute (PSI)(スイス)

    • Related Report
      2020 Annual Research Report
  • [Int'l Joint Research] University of Groningen(オランダ)

    • Related Report
      2020 Annual Research Report
  • [Int'l Joint Research] Johannes Gutenberg Universitaet Mainz/重イオン研究所(GSI)(ドイツ)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] Paul Scherrer Institute (PSI)(スイス)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] Johannes Gutenberg Universitaet Mainz/重イオン研究所(GSI)/Friedrich-Schiller Universitaet(ドイツ)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] Paul Scherrer Institute (PSI)(スイス)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] University of Groningen(オランダ)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] Tel Aviv University(イスラエル)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] Johannes Gutenberg-Universitaet Mainz/重イオン研究所(GSI)/Friedrich-Schiller-Universitaet(ドイツ)

    • Related Report
      2017 Annual Research Report
  • [Int'l Joint Research] Paul Scherrer Institute (PSI)/CERN(スイス)

    • Related Report
      2017 Annual Research Report
  • [Int'l Joint Research] University of Groningen(オランダ)

    • Related Report
      2017 Annual Research Report
  • [Int'l Joint Research] Tel Aviv University(イスラエル)

    • Related Report
      2017 Annual Research Report
  • [Int'l Joint Research] Johannes Gutenberg-Universitaet Mainz/重イオン研究所(GSI)(ドイツ)

    • Related Report
      2016 Annual Research Report
  • [Int'l Joint Research] Paul Scherrer Institute (PSI)/CERN(スイス)

    • Related Report
      2016 Annual Research Report
  • [Journal Article] Gas phase synthesis of 4d transition metal carbonyl complexes with thermalized fission fragments in single-atom reactions2021

    • Author(s)
      M. Goetz, S. Goetz, J. V. Kratz, J. Ballof, Ch. E. Duellmann, K. Eberhardt, C. Mokry, D. Renisch, J. Runke, T. K.. Sato, P. Thoerle-Pospiech, N. Trautmann, and A. Yakushev
    • Journal Title

      Radiochim. Acta

      Volume: 109 Issue: 3 Pages: 153-165

    • DOI

      10.1515/ract-2020-0052

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] First online operation of TRIGA-TRAP2020

    • Author(s)
      J. Grund, M. Asai, K. Blaum, M. Block, S. Chenmarev, Ch. E. Duellmann, K. Eberhardt, S. Lohse, Y. Nagame, Sz. Nagy, P. Naubereit, J. J. W. van de Laar, F. Schneider, T. K. Sato, N. Sato. D. Simonovski, K. Tsukada, and K. Wendt
    • Journal Title

      Nucl. Instrum. Methods in Phys. Res. A

      Volume: 972 Pages: 164013-164013

    • DOI

      10.1016/j.nima.2020.164013

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Production of Bh266 in the Cm248(Na23,5n)Bh266 reaction and its decay properties2020

    • Author(s)
      Haba H.他(Shigekawa Y. 19番目)
    • Journal Title

      Physical Review C

      Volume: 102 Issue: 2 Pages: 024625-024625

    • DOI

      10.1103/physrevc.102.024625

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] New excited 2+ and 3- two-proton states in 21084Po126 populated by two-proton transfer2020

    • Author(s)
      E. Dupont, A. Astier, C. M. Petrache, B.F. Lv, I. Deloncle, J. Kiener, R. Orlandi, H. Makii, K. Nishio, K. Hirose, M. Asai, T. K. Sato, K. Tsukada, Y. Ito, K. R. Kean, R. Yanagihara, G. Scamps
    • Journal Title

      Phys. Rev. C

      Volume: 101 Issue: 1

    • DOI

      10.1103/physrevc.101.014309

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Measurement of fission-fragment mass distributions in the multinucleon transfer channels of the 18O + 237Np reaction2020

    • Author(s)
      M. J. Vermeulen, K. Nishio, K. Hirose, K. R. Kean, H. Makii, R. Orlandi, K. Tsukada, I. Tsekhanovich, A. N. Andreyev, S. Ishizaki, M. Okubayashi, S. Tanaka, and Y. Aritomo
    • Journal Title

      Phys. Rev. C

      Volume: 102 Issue: 5

    • DOI

      10.1103/physrevc.102.054610

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Size Distribution of Droplets in a Two Liquid-phase Mixture Compared between Liquid Spraying and Mechanical Stirring2019

    • Author(s)
      T. Shimogouchi, H. Naganawa, T. Nagano, B. Grambow, and Y. Nagame
    • Journal Title

      Analytical Sciences

      Volume: 35 Issue: 9 Pages: 955-960

    • DOI

      10.2116/analsci.18P508

    • NAID

      130007705244

    • ISSN
      0910-6340, 1348-2246
    • Year and Date
      2019-09-10
    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Optimization of an isothermal gas-chromatographic setup for the chemical exploration of dubnium (Db, Z = 105) oxychlorides2019

    • Author(s)
      N. M. Chiera, T. K. Sato, T. Tomitsuka, M. Asai, Y. Ito, K. Shirai, H. Suzuki, K. Tokoi, A. Toyoshima, K. Tsukada, and Y. Nagame
    • Journal Title

      J. Radioanal. Nucl. Chem. 320, 633-642 (2019)

      Volume: 320 Issue: 3 Pages: 633-642

    • DOI

      10.1007/s10967-019-06505-w

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] α-decay properties of 200,202Fr2019

    • Author(s)
      L. Ghys, A. N. Andreyev, M. Huyse, P. Van Duppen, S. Antalic, A. Barzakh, L. Capponi, T. E. Cocolios, J. Cubiss, X. Derkx, H. De Witte, J. Elseviers, F. P. Hessberger, Z. Kalaninova, U. Koester, J. F. W. Lane, V. Liberati, S. Mitsuoka, Y. Nagame, et al.
    • Journal Title

      Phys. Rev. C

      Volume: 100 Issue: 5

    • DOI

      10.1103/physrevc.100.054310

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Nuclear and chemical characterization of heavy actinides2019

    • Author(s)
      Y. Nagame
    • Journal Title

      Radiochim. Acta

      Volume: 107 Issue: 9-11 Pages: 803-819

    • DOI

      10.1515/ract-2019-3133

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] From SRAFAP to ARCA and AIDA- developments and implementation of automated aqueous-phase rapid chemistry apparatuses for heavy actinides and transactinides2019

    • Author(s)
      M. Schaedel and Y. Nagame
    • Journal Title

      Radiochim. Acta

      Volume: 107 Issue: 7 Pages: 561-585

    • DOI

      10.1515/ract-2019-3103

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Formation and thermochemical properties of oxychlorides of niobium (Nb) and tantalum (Ta): Towards the gas-phase investigation of dubnium (Db) oxychloride2019

    • Author(s)
      N. M. Chiera, T. K. Sato, T. Tomitsuka, M. Asai, H. Suzuki, K. Tokoi, A. Toyoshima, K. Tsukada, and Y. Nagame
    • Journal Title

      Inorg. Chim. Acta

      Volume: 486 Pages: 361-366

    • DOI

      10.1016/j.ica.2018.10.032

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Online chemical adsorption studies of Hg, Tl, and Pb on SiO2 and Au surfaces in preparation for chemical investigations on Cn, Nh, and Fl at TASCA2018

    • Author(s)
      L. Lens, A. Yakushev, Ch. E. Duelllmann, M. Asai, J. Ballof, M. Block, H. M. David, J. Despotopulos, A. Di Nitto, K. Eberhardt, J. Even, Y. Nagame 他
    • Journal Title

      Radiochim. Acta

      Volume: 106 Issue: 12 Pages: 949-962

    • DOI

      10.1515/ract-2017-2914

    • NAID

      120007188903

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] First ionization potentials of Fm, Md, No, and Lr: Verification of filling-up of 5f electrons and confirmation of the actinide series2018

    • Author(s)
      T. K. Sato, M. Asai, A. Borschevsky, R. Beerwerth, Y. Kaneya, H. Makii, A. Mitsukai, Y. Nagame 他
    • Journal Title

      J. Am. Chem. Soc.

      Volume: 140 Issue: 44 Pages: 14609-14613

    • DOI

      10.1021/jacs.8b09068

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Extraction behavior of Mo and W from H2SO4 and HF/HCl solutions into toluene with Aliquat336: Sulfate and fluoride complex formation of Mo and W towards chemical studies of seaborgium (Sg)2018

    • Author(s)
      A. Toyoshima, A. Mitsukai, K. Tsukada, K. Ooe, H. Haba, Y. Komori, M. Murakami, Y. Kaneya, D. Sato, M. Asai, T. K. Sato, and Y. Nagame
    • Journal Title

      J. Raioanal. Nucl. Chem.

      Volume: 317 Issue: 1 Pages: 421-430

    • DOI

      10.1007/s10967-018-5882-5

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] First ionization potential of the heaviest actinide lawrencium, element 1032016

    • Author(s)
      T. K. Sato, M. Asai, A. Borschevsky, T. Stora, N. Sato, Y. Kaneya, K. Tsukada, Ch. E. Duellmann, K. Eberhardt, E. Eliav, S. Ichikawa, U. Kaldor, J. V. Kratz, S. Miyashita, Y. Nagame, K. Ooe, A. Osa, D. Renish, J. Runke, M. Schaedel, P. Thoerle-Pospiech, A. Toyoshima, and N. Trautmann
    • Journal Title

      Eur. Phys. J Web of Conferences

      Volume: 131

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Complex chemistry with complex compounds2016

    • Author(s)
      R. Eichler, M. Asai, H. Brand, N. M. Chiera, A. Di Nitto, R. Dressler, Ch. E. Duellmann, J. Even, F. Fangli, M Goetz, H. Haba, W. Hartmann, E. Jaeger, D. Kaji, J. Kanaya, Y. Kaneya, J. Khuyabaatar, B. Kindler, Y. Komori, B. Kraus, J. V. Kratz, Y. Nagame et al.
    • Journal Title

      Eur. Phys. J Web of Conferences

      Volume: 131

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Chemical properties of rutherfordium (Rf) and dubnium (Db) in the aqueous phase2016

    • Author(s)
      Y. Nagame, J. V. Kratz, and M. Schaedel
    • Journal Title

      Eur. Phys. J Web of Conferences

      Volume: 131

    • NAID

      120006502097

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Beta-delayed fission and α decay of 196At2016

    • Author(s)
      V. L. Truesdale, A. N. Andreyev, L. Ghys, M. Huyse, P. van Duppen, S. Sels, B. Andel, S. Antalic, A. Barzakh, L. Capponi, T. E. Cocolios, X. Derkx, H. De Witte, J. Elseviers, D. V. Fedorov, V. N. Fedosseev, F. P. Hessberger, Z. Kalaninova, U. Koester, J. F. W. Lane, V. Liberati, K. M. Lynch, Y. Nagame, et al.
    • Journal Title

      Phys Rev. C

      Volume: 94 Issue: 3

    • DOI

      10.1103/physrevc.94.034308

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Presentation] 超重元素用EBGPイオン源の開発2021

    • Author(s)
      青木 涼太、佐藤 哲也、大谷 怜、鈴木 颯人、伊藤 由太、浅井 雅人、塚田 和明、永目 諭一郎
    • Organizer
      日本化学会 第101春季年会(2021)
    • Related Report
      2020 Annual Research Report
  • [Presentation] 103番元素ローレンシウムの揮発性研究のための表面電離イオン源モンテカルロシミュレーション2021

    • Author(s)
      佐藤 哲也、Robert Eichler、永目 諭一郎
    • Organizer
      日本化学会 第101春季年会(2021)
    • Related Report
      2020 Annual Research Report
  • [Presentation] 106番元素シーボーギウムオキシ塩化物の揮発性研究に向けた等温ガスクロマトグラフ法の開発2021

    • Author(s)
      大谷 怜、佐藤 哲也、青木 涼太、白井 香里、鈴木 颯人、塚田 和明、浅井 雅人、伊藤 由太、永目 諭一郎
    • Organizer
      日本化学会 第101春季年会(2021)
    • Related Report
      2020 Annual Research Report
  • [Presentation] 超重元素原子線分光に向けた電子再結合法による原子ビームの生成2020

    • Author(s)
      鈴木 颯人, 伊藤 由太, 佐藤 哲也, 青木 涼太, 塚田 和明, 浅井 雅人, 永目 諭一郎
    • Organizer
      日本放射化学会第64回討論会(2020)
    • Related Report
      2020 Annual Research Report
  • [Presentation] 105 番元素ドブニウムオキシ塩化物のオンライン等温ガスクロマトグラフ挙動2020

    • Author(s)
      佐藤 哲也, C.M. Nadine, 富塚 知博, 床井 健運, 鈴木 颯人, 伊藤 由太, 浅井 雅人, 白井 香里, 井上 浩樹, 安達 サディア, 柏原 歩那, 牧井 宏之, 廣瀬 健太郎, 西尾 勝久, 永目 諭一郎, 渡邉 瑛介, 阪間 稔, 後藤 真一
    • Organizer
      日本放射化学会第64回討論会(2020)
    • Related Report
      2020 Annual Research Report
  • [Presentation] Current Status of Atomic/Chemical Studies of Heavy and Trans- Actinide Elements at JAEA2020

    • Author(s)
      T. K. Sato
    • Organizer
      57th Annual Convention of Chemists 2020 & International Conference on Recent Trends in Chemical Sciences (RTCS)
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] First ionization potentials of heavy actinides - based on an atom-at-a-time scale2020

    • Author(s)
      Y. Nagame
    • Organizer
      10th International Conference on Isotopes (10ICI)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] ランタノイドの高温金属表面における吸着エンタルピー測定2020

    • Author(s)
      床井健運、佐藤哲也、菊池 圭、浅井雅人、伊藤由太、鈴木颯人、塚田和明、永目諭一郎
    • Organizer
      日本化学会第100春季年会(2020)
    • Related Report
      2019 Annual Research Report
  • [Presentation] 105 番元素ドブニウムオキシ塩化物のオンライン等温ガスクロマトグラフ挙動2020

    • Author(s)
      佐藤哲也、Chiera Nadine M.、富塚知博、床井健運、鈴木颯人、伊藤由太、浅井雅人、白井香里、井上浩樹、安達サディア、柏原歩那、牧井宏之、廣瀬健太郎、西尾勝久、永目諭一郎、渡邉瑛介、阪間 稔、後藤真一、塚田和明
    • Organizer
      日本化学会第100春季年会(2020)
    • Related Report
      2019 Annual Research Report
  • [Presentation] Chemical studies of the heaviest elements at JAEA2019

    • Author(s)
      Y. Nagame
    • Organizer
      XXI Mendeleev Congress on General and Applied Chemistry
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Chemical characterization of the heaviest elements2019

    • Author(s)
      Y. Nagame
    • Organizer
      2nd International Conference on Radioanalytical and Nuclear Chemistry (RANC-2019)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] In-situ synthesis of volatile transition metal carbonyl complexws with short-lived radioisotopes2019

    • Author(s)
      M. Goetz, Ch.E. Duemllmann, A. Yakushev, M. Asai, J. Ballof, A. Di Nitto, K. Eberhardt, H. Haba, Y. Kaneya, Y. Komori, J.-V. Kratz, J. Krier, B. Lommel, A. Mitsukai, Y. Nagame, et al.
    • Organizer
      6th International Conference on the Chemistry and Physics of the Transactinide Elements
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Optimizations of the TASCA-COMPACT setup towards chemical studies of nihonium (element 113)2019

    • Author(s)
      L. Lens, A. Yakushev, Ch.E. Duemllmann, M. Asai, M. Block, H. Brand, A. Di Nitto, L. Harkness-Brennan, R.-D. Herzberg, D. Hinde, J. Khuyagbaatar, J.V. Kratz, J. Krier, N. Kurz, M. Laatiaoui, S. Lahiri, B. Lommel, Y. Nagame, et al.
    • Organizer
      6th International Conference on the Chemistry and Physics of the Transactinide Elements
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Establishment of the volatility trend in Group-5 elements via gas-chromatographic experiments with Nb-, Ta-, and Db-oxychlorides2019

    • Author(s)
      N. M. Chiera, T. K. Sato, T. Tomitsuka, M. Asai, Y. Ito, K. Shirai, H. Suzuki, K. Tokoi, A. Toyoshima, K. Tsukada, and Y. Nagame
    • Organizer
      6th International Conference on the Chemistry and Physics of the Transactinide Elements
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Atomic and chemical properties of Lawrencium (Lr, Z = 103) and an outlook to the transactinides2019

    • Author(s)
      T. K. Sato, M. Asai, Y. Kaneya, A. Toyoshima, Y. Ito, K. Tsukada, K. Tokoi, T. Tomohiro, H. Suzuki, H. Makii, A. Osa, Y. Nagame, et al.
    • Organizer
      6th International Conference on the Chemistry and Physics of the Transactinide Elements
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Chemical studies of superheavy elements at a recoil separator, with a focus on Fl2019

    • Author(s)
      A. Yakushev, L. Lens, Ch.E. Duellmann, M. Asai, M. Block, H. Brand, H. M. David, J. Despotopulos, M. Maiti, A. Mistry, Ch. Mokry, K. Moody, Y. Nagame, et al.
    • Organizer
      6th International Conference on the Chemistry and Physics of the Transactinide Elements
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Atomic and chemical properties of the heaviest actinide element, lawrencium (Lr, Z = 103)2019

    • Author(s)
      T. K. Sato
    • Organizer
      XXI Mendeleev Congress on General and Applied Chemistry
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 周期表が書き換わる? ~アクチノイド最後の元素でみつけた周期表のほころび~2019

    • Author(s)
      佐藤哲也
    • Organizer
      日本放射化学会第63回討論会(2019)
    • Related Report
      2019 Annual Research Report
    • Invited
  • [Presentation] 超重元素原子ビーム生成に向けた高温ノズル型低速原子ビーム源の開発2019

    • Author(s)
      富塚知博、佐藤哲也、伊藤由太、床井健運、鈴木颯人、浅井雅人、塚田和明、後藤真一、永目諭一郎
    • Organizer
      日本放射化学会第63回討論会(2019)
    • Related Report
      2019 Annual Research Report
  • [Presentation] 超重元素原子線分光に向けた電子再結合型原子ビーム源の開発2019

    • Author(s)
      鈴木颯人、伊藤由太、佐藤哲也、富塚知博、床井健運、塚田和明、浅井雅人、永目諭一郎
    • Organizer
      日本放射化学会第63回討論会(2019)
    • Related Report
      2019 Annual Research Report
  • [Presentation] アクチノイドの高温金属表面における吸着エンタルピー測定に向けた真空脱離装置の開発2019

    • Author(s)
      床井健運、佐藤哲也、浅井雅人、伊藤由太、鈴木颯人、富塚知博、塚田和明、永目諭一郎
    • Organizer
      日本放射化学会第63回討論会(2019)
    • Related Report
      2019 Annual Research Report
  • [Presentation] 超重核原子線分光のための再結合型低速原子ビーム源の開発2019

    • Author(s)
      伊藤由太, 鈴木颯人, 浅井雅, 永目諭一郎, 西尾勝久, 佐藤哲也, 床井健運, 富塚知博, 塚田和明
    • Organizer
      日本物理学会第74回年次大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 254Es標的を用いた中性子過剰Fm同位体の自発核分裂測定2019

    • Author(s)
      浅井雅人, 塚田和明, 廣瀬健太郎, 豊嶋厚史, 富塚知博, Nadine M. Chiera, 伊藤由太, 牧井宏之, 永目諭一郎 他
    • Organizer
      日本物理学会第74回年次大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 表面電離イオン源内における短寿命核種の吸着脱離挙動の解析に向けたモンテカルロシミュレーション開発2019

    • Author(s)
      床井健運, 佐藤哲也, Eichler Robert, 伊藤由太, 富塚知博, 鈴木颯人, 浅井雅人, 塚田和明, 永目諭一郎
    • Organizer
      日本化学会第99春季年会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 電子プラズマを用いた再結合型低速中性原子ビーム源の開発2019

    • Author(s)
      鈴木颯人, 伊藤由太, 佐藤哲也, 冨塚知博, 床井健運, 浅井雅人, 塚田和明, 永目諭一郎
    • Organizer
      日本化学会第99春季年会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 超重元素の価電子構造決定に向けた低速原子ビーム取り出し技術の開発2019

    • Author(s)
      富塚知博, 床井健運, 佐藤哲也, 伊藤由太, 鈴木颯人, 浅井雅人, 塚田和明, 豊嶋厚史, Chiera Nadine M., 後藤真一, 永目諭一郎
    • Organizer
      日本化学会第99春季年会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 5族元素オキシ塩化物のオンライン等温ガスクロマトグラフ挙動2019

    • Author(s)
      佐藤哲也, Chiera Nadine M., 富塚知博, 床井健運, 鈴木颯人, 伊藤由太, 浅井雅人, 塚田和明, 白井香里, 井上浩樹, 安達サディア, 柏原歩那, 永目諭一郎, 後藤真一, 末木啓介
    • Organizer
      日本化学会第99春季年会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Chemical properties of lawrencium (Lr, Z = 103): Adsorption behavior on a tantalum surface2018

    • Author(s)
      Tetsuya K. Sato, Masato Asai, Kazuaki Tsukada, Yusuke Kaneya, Tomohiro Tomitsuka, Atsushi Toyoshima, Akina Mitsukai, Akihiko Osa, Hiroyuki Makii, Kentaro Hirose, Katsuhisa Nishio, Yuichiro Nagame 他
    • Organizer
      18th Radiochemical Conference
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Superheavy Element Chemistry at the gas-filled separator TASCA2018

    • Author(s)
      A. Yakushev, L. Lens, Ch.E. Duellmann, M. Asai, M. Block, H. Brand, H.M. David, J. Despotopulos, A. Di Nitto, K. Eberhardt, U. Forsberg, P. Golubev, M. Goetz, S. Goetz, Y. Nagame 他
    • Organizer
      18th Radiochemical Conference
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Development of an atomic beam apparatus for chemistry of the heaviest elements2018

    • Author(s)
      T. Tomitsuka, K. Tokoi, T. K. Sato, M. Asai, N. M. Chiera, S. Goto, A. Osa, A. Toyoshima, K. Tsukada, and Y. Nagame
    • Organizer
      18th Radiochemical Conference
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Determination of the first ionization potentials of heavy actinides based on an atom-at-a-time scale2018

    • Author(s)
      Y. Nagame
    • Organizer
      4th International Conference on Physics (Physics 2018)
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Liquid-phase chemistry of superheavy elements2018

    • Author(s)
      Y. Nagame
    • Organizer
      The 4th International Conference on Application of Radiotracers and Energetic Beams in Sciences (ARCEBS-18)
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Chemical characterization of the heaviest elements2018

    • Author(s)
      Y. Nagame
    • Organizer
      The 4th International Conference on Application of Radiotracers and Energetic Beams in Sciences (ARCEBS-18)
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Nuclear Structure 20182018

    • Author(s)
      T. K. Sato
    • Organizer
      Measurements of the first ionization potentials of heavy actinides, Fm (Z = 100), Md (Z = 101), No (Z = 102), and Lr (Z = 103)
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] The first ionization potentials of heavy actinides, Fm (Z = 100), Md (Z = 101), No (Z = 102), and Lr (Z = 103)2018

    • Author(s)
      T. K. Sato
    • Organizer
      IX International Symposium on Exotic Nuclei
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Atomic/chemical properties of the heaviest actinide element lawrencium2018

    • Author(s)
      T. K. Sato
    • Organizer
      The 4th International Conference on Application of Radiotracers and Energetic Beams in Sciences (ARCEBS-18)
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 254Es標的を用いて生成する中性子過剰Fm領域核の自発核分裂の測定2018

    • Author(s)
      浅井雅人,塚田和明,廣瀬健太郎,豊嶋厚史,富塚知博,Nadine M. Chiera,伊藤由太,牧井宏之,永目諭一郎 他
    • Organizer
      2018日本放射化学会年会・第62回放射化学討論会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 超重元素を対象とした低速原子ビーム源の開発2018

    • Author(s)
      富塚知博, 床井健運, 佐藤哲也, 伊藤由太, 鈴木颯人, 浅井雅人, 塚田和明, 豊嶋厚史, Nadine M. Chiera, 後藤真一, 永目諭一郎
    • Organizer
      2018日本放射化学会年会・第62回放射化学討論会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 表面電離イオン源内における短寿命同位体の吸着脱離挙動の解析に向けたモンテカルロシミュレーション開発2018

    • Author(s)
      床井健運, 佐藤哲也, Robert Eichler, 伊藤由太, 富塚知博, 鈴木颯人, 浅井雅人, 塚田和明, 豊嶋厚史, Nadine M. Chiera, 永目諭一郎
    • Organizer
      2018日本放射化学会年会・第62回放射化学討論会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 電子プラズマを用いた再結合型低速原子ビーム源の開発2018

    • Author(s)
      鈴木颯人,伊藤由太,佐藤哲也,富塚知博,床井健運,浅井雅人,塚田和明,永目諭一郎
    • Organizer
      2018日本放射化学会年会・第62回放射化学討論会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 103番元素ローレンシウム(Lr)のタンタル表面における吸着脱離挙動2017

    • Author(s)
      佐藤 哲也、金谷 佑亮、浅井 雅人、塚田 和明、豊嶋 厚史、水飼 秋菜、長 明彦、牧井 宏之、廣瀬 健太郎、永目 諭一郎、富塚 知博、白井 香里、Christoph Duellmann, Matthias Schaedel, Jens V. Kratz, Thierry Stora, et al.
    • Organizer
      日本化学会 第97春季年会 (2017)
    • Place of Presentation
      慶應義塾大学(神奈川県横浜市)
    • Year and Date
      2017-03-16
    • Related Report
      2016 Annual Research Report
  • [Presentation] First ionization potentials of heavy actinides2017

    • Author(s)
      T.K. Sato
    • Organizer
      Actinides 2017
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Adsorption of lowrencium (Lr) on a metallic tantalum (Ta) surface2017

    • Author(s)
      Y. Kaneya, T. Tomitsuka, T.K. Sato、M. Asai, K. Tsukada, A. Toyoshima, A. Mitsukai, H. Makii, K. Hirose, A. Osa, K. Nishio, Y. Nagame 他
    • Organizer
      Actinides 2017
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Ionization potential measurements of the heaviest actinides2017

    • Author(s)
      T.K. Sato
    • Organizer
      254th American Chemical Society National Meeting, Division of Nuclear Chemistry & Technology
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Redox studies of the heaviest actinides2017

    • Author(s)
      Y. Nagame
    • Organizer
      254th American Chemical Society National Meeting, Division of Nuclear Chemistry & Technology
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 103番元素ローレンシウムの価電子構造決定に向けた低速原子ビーム取り出し技術の開発2017

    • Author(s)
      富塚知博、床井建運、佐藤哲也、浅井雅人、塚田和明、豊嶋厚史、Nadine M. Chiera、鎌田裕生、永目諭一郎、後藤真一
    • Organizer
      2017放射化学会年会・第61回放射化学討論会
    • Related Report
      2017 Annual Research Report
  • [Presentation] First ionization potentials of the heaviest elements2017

    • Author(s)
      Y. Nagame
    • Organizer
      3rd Symposium on Superheavy Elements
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Adsorption behavior of lawrencium on tantalum2017

    • Author(s)
      T.K. Sato
    • Organizer
      3rd Symposium on Superheavy Elements
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Chemistry of the heaviest elements2017

    • Author(s)
      Y. Nagame
    • Organizer
      6th Asia-Pacific Symposium on Radiochemistry
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] First ionization energies of heavy actinides2017

    • Author(s)
      Y. Nagame, T.K. Sato, M. Asai, Y. Kaneya, H. Makii, A. Mitsukai, A. Osa, M. Schaedel, A. Toyoshima, K. Tsukada, 他
    • Organizer
      6th Asia-Pacific Symposium on Radiochemistry
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Adsorption of lawrencium (Z = 103) on a tantalum surface2017

    • Author(s)
      T. Tomitsuka, Y. Kaneya, T.K. Sato, M. Asai, K. Tsukada, A. Toyoshima, A. Mitsukai, H. Makii, K. Hirose, A. Osa, K. Nishio, Y. Nagame 他
    • Organizer
      6th Asia-Pacific Symposium on Radiochemistry
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Recent achievements and future challenges in the heaviest element chemistry2017

    • Author(s)
      Y. Nagame
    • Organizer
      9th Workshop on Chemistry of the Heaviest Elements
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Measurements of the first ionization potentials of heavy actinides2017

    • Author(s)
      T.K. Sato, M. Asai, Y. Kaneya, K. Tsukada, A. Toyoshima, A. Mitsukai, S. Takeda, A. Vascon, M. Sakama, D. Sato, K. Ooe, S. Miyashita, Y. Shigekawa, A. Borschevsky, H. Makii, A. Osa, S. Ichikawa, Y. Nagame 他
    • Organizer
      9th Workshop on Chemistry of the Heaviest Elements
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Adsorption of lawrencium on a metallic tantalum surface at high temperature2017

    • Author(s)
      Y. Kaneya, M. Asai, T.K. Sato, T. Tomitsuka, K. Tsukada, A. Toyoshima, A. Mitsukai, H. Makii, K. Hirose, A. Osa, K. Nishio, Y. Nagame 他
    • Organizer
      9th Workshop on Chemistry of the Heaviest Elements
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] First ionization potentials of the heaviest elements2017

    • Author(s)
      Y. Nagame
    • Organizer
      International Conference on Shapes and Symmetries in Nuclei: from Experiment to Theory
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 103番元素ローレンシウム(Lr)のタンタル金属表面における吸着挙動2016

    • Author(s)
      金谷佑亮、佐藤哲也、浅井雅人、塚田和明、豊嶋厚史、水飼秋菜、永目諭一郎、Ch.E. Duellmann, K. Eberhardt, J. Grund, J.V. Kratz, et al.
    • Organizer
      2016日本放射化学会年会・第60回放射化学討論会
    • Place of Presentation
      新潟大学(新潟県新潟市)
    • Year and Date
      2016-09-10
    • Related Report
      2016 Annual Research Report
  • [Presentation] 重アクチノイド元素の第一イオン化エネルギー2016

    • Author(s)
      佐藤哲也、浅井雅人、金谷佑亮、塚田和明、豊嶋厚史、水飼秋菜、武田晋作、阪間稔、佐藤大輔、大江一弘、重川優大、牧井宏之、長明彦、市川進一、永目諭一郎、A. Borschevsky, M. Schaedel, Ch.E. Duellmann, J.V. Kratz, T. Stora et al.
    • Organizer
      2016日本放射化学会年会・第60回放射化学討論会
    • Place of Presentation
      新潟大学(新潟県新潟市)
    • Year and Date
      2016-09-10
    • Related Report
      2016 Annual Research Report
  • [Presentation] フロー抽出装置を用いたフッ化水素酸ーAliquat336系におけるタングステンの溶媒抽出2016

    • Author(s)
      水飼秋菜、豊嶋厚史、小森有希子、羽場宏光、浅井雅人、塚田和明、佐藤哲也、永目諭一郎
    • Organizer
      2016日本放射化学会年会・第60回放射化学討論会
    • Place of Presentation
      新潟大学(新潟県新潟市)
    • Year and Date
      2016-09-10
    • Related Report
      2016 Annual Research Report
  • [Presentation] Chemistry of the heaviest actinides and early transactinides - Experimental achievements and perspectives2016

    • Author(s)
      Y. Nagame
    • Organizer
      9th International Conference on Nuclear and Radiochemistry (NRC9)
    • Place of Presentation
      Helsinki, Finland
    • Year and Date
      2016-08-29
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] First on-line vacuum chromatography experiments with single atoms of Tl on SiO2 and E1132016

    • Author(s)
      P. Steinegger, M. Asai, R. Dressler, R. Eichler, Y. Kaneya, A. Mitsukai, Y. Nagame, D. Piguet, T. K. Sato, M. Schaedel, S. Takeda, A. Toyoshima, K. Tsukada, A. Tuerler and A. Vascon
    • Organizer
      9th International Conference on Nuclear and Radiochemistry (NRC9)
    • Place of Presentation
      Helsinki, Finland
    • Year and Date
      2016-08-29
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Adsorption behavior of Lr on a Ta surface at high temperature2016

    • Author(s)
      Y. Kaneya, M. Asai, Ch. E. Duellmann, K. Eberhardt, R. Eichler, S. Goto, J. Grund, K. Hirose, H. Kamada, Y. Kasamatsu, J. V. Kratz, H. Makii, A. Mitsukai, S. Miyashita, Y. Nagame, et al.
    • Organizer
      9th International Conference on Nuclear and Radiochemistry (NRC9)
    • Place of Presentation
      Helsinki, Finland
    • Year and Date
      2016-08-29
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Chemistry of superheavy elements2016

    • Author(s)
      Y. Nagame
    • Organizer
      The 71st Fujiwara seminar - Shimoda 2016 - International Symposium on Interplay between Hadronic, Nuclear and Atomic Physics
    • Place of Presentation
      下田東急ホテル(静岡県下田市)
    • Year and Date
      2016-07-06
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Chemical properties of Rf and Db in the aqueous phase2016

    • Author(s)
      Y. Nagame
    • Organizer
      Nobel symposium NS 160 “Chemistry and Physics of Heavy and Superheavy Elements”
    • Place of Presentation
      Baeckaskog Castle, Sweden
    • Year and Date
      2016-05-29
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Book] Actinides and Transactinides In "Kirk-Othmer Encyclopedia of Chemical Technology"2020

    • Author(s)
      Y. Nagame, T. K. Sato, and J. V. Kratz
    • Total Pages
      52
    • Publisher
      John Wiley & Sons, Inc.
    • ISBN
      9780471484943
    • Related Report
      2020 Annual Research Report

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Published: 2016-04-21   Modified: 2022-01-27  

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