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Creation of organic-inorganic hybrid environmental load-reducting materials using photoinduced reducing ability

Research Project

Project/Area Number 16H02987
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Environmental conscious materials and recycle
Research InstitutionIbaraki University (2018)
Meiji University (2016-2017)

Principal Investigator

MUNETOSHI SAKAI  茨城大学, 研究・産学官連携機構, 准教授 (00392928)

Co-Investigator(Kenkyū-buntansha) 相澤 守  明治大学, 理工学部, 専任教授 (10255713)
池上 啓太  山陽小野田市立山口東京理科大学, 工学部, 准教授 (60372786)
Kalousek Vit  山陽小野田市立山口東京理科大学, 工学部, 助教 (00749773)
Project Period (FY) 2016-04-01 – 2019-03-31
Project Status Completed (Fiscal Year 2018)
Budget Amount *help
¥17,940,000 (Direct Cost: ¥13,800,000、Indirect Cost: ¥4,140,000)
Fiscal Year 2018: ¥4,680,000 (Direct Cost: ¥3,600,000、Indirect Cost: ¥1,080,000)
Fiscal Year 2017: ¥4,940,000 (Direct Cost: ¥3,800,000、Indirect Cost: ¥1,140,000)
Fiscal Year 2016: ¥8,320,000 (Direct Cost: ¥6,400,000、Indirect Cost: ¥1,920,000)
Keywords表面・界面物性 / 新エネルギー / 複合材料・物性 / ナノ材料 / 光触媒 / 人工光合成 / メソ孔・多孔体 / キャリア寿命
Outline of Final Research Achievements

To increase the performance of photo-induced reduction catalyst contributing to green technology, it was investigated to combine nano-particles with different functions; carbon dioxide adsorption materials and photo-induced reduction catalyst. In this research, K-Al composite oxide and strontium titanate was used respectively. In addition, the relationship between "photocatalytic reduction ability" and "carrier life time" was considered from the measurement results using the "microwave photoconductivity decay method". In the future, we will advance the elucidation of the phenomenon at the related phase interface in more detail.

Academic Significance and Societal Importance of the Research Achievements

太陽光利用を想定した大気中CO2の光触媒還元固定化は人工光合成型反応として注目されいるが、メタンやメタノールのようなより付加価値の高い炭化水素への物質変換が高効率で実現するためには、CO2の活性化過程を促進する高機能光触媒の開発が望まれる。これに対し、物理化学的な視点から性能向上に取り組み、電子寿命と光触媒活性の間の学理の追求を深め、関連する相界面の現象メカニズム解明できることに意義を有する。

Report

(4 results)
  • 2018 Annual Research Report   Final Research Report ( PDF )
  • 2017 Annual Research Report
  • 2016 Annual Research Report
  • Research Products

    (29 results)

All 2019 2018 2017 2016 Other

All Journal Article (15 results) (of which Peer Reviewed: 15 results,  Open Access: 3 results,  Acknowledgement Compliant: 1 results) Presentation (7 results) (of which Int'l Joint Research: 3 results) Book (3 results) Remarks (4 results)

  • [Journal Article] Carbon dioxide adsorption properties of K-Al-Fe?based oxides prepared from a porous polymer monolith template2019

    • Author(s)
      Ikeue Keita、Suzuki Masashige、Yoshimoto Daisuke、Usukawa Ryutaro、Sakai Munetoshi、Vagvala Tarun Chand、Kalousek Vit
    • Journal Title

      Journal of Solid State Chemistry

      Volume: 274 Pages: 75-80

    • DOI

      10.1016/j.jssc.2019.03.013

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] 均一沈殿法によるウィスカー/繊維状リン酸カルシウムの合成と応用2019

    • Author(s)
      板谷清司、林 英子、相澤 守
    • Journal Title

      無機マテリアル

      Volume: 26 Pages: 54-64

    • NAID

      40021829078

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Bioresorbability of chelate-setting calcium-phosphate cement hybridized with gelatin particles using a porcine tibial defect model2018

    • Author(s)
      KIMINAMI Keishi、NAGATA Kohei、KONISHI Toshiisa、MIZUMOTO Minori、HONDA Michiyo、NAKANO Kazuaki、NAGAYA Masaki、ARIMURA Hidetoshi、NAGASHIMA Hiroshi、AIZAWA Mamoru
    • Journal Title

      Journal of the Ceramic Society of Japan

      Volume: 126 Issue: 2 Pages: 71-78

    • DOI

      10.2109/jcersj2.17197

    • NAID

      130006329683

    • ISSN
      1348-6535, 1882-0743
    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Synthesis and characterization of metal-diaminobipyridine complexes as low-cost co-catalysts for photo-sensitized hydrogen evolution2018

    • Author(s)
      Chand Vagvala Tarun、Ooyabe Takashi、Sakai Munetoshi、Funasako Yusuke、Inokuchi Makoto、Kurashige Wataru、Negishi Yuichi、Kalousek Vit、Ikeue Keita
    • Journal Title

      Inorganica Chimica Acta

      Volume: 482 Pages: 821-829

    • DOI

      10.1016/j.ica.2018.07.022

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Comparative study of the dynamic hydrophobicity of fluoroalkylsilane coatings tilted at acute and obtuse angles2018

    • Author(s)
      Y. Higashino, H. Takahashi, M. Sakai, T. Isobe, S. Matsushita, A. Nakajima
    • Journal Title

      J. Coatings Tech. Res.

      Volume: 印刷中 Issue: 4 Pages: 891-898

    • DOI

      10.1007/s11998-018-0064-5

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] 最近の撥水技術と水ハーベスタ2018

    • Author(s)
      酒井宗寿, 中島 章.
    • Journal Title

      セラミックス

      Volume: 53, 2 Pages: 99-103

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Sliding of water/glycerol mixture droplets on hydrophobic solid?liquid bulk composites using Ti plates with a fibrous TiO2 layer2017

    • Author(s)
      Takahashi Hirokazu、Higashino Yuta、Sakai Munetoshi、Isobe Toshihiro、Matsushita Sachiko、Nakajima Akira
    • Journal Title

      J. Mater. Sci.

      Volume: 53 Issue: 2 Pages: 1157-1166

    • DOI

      10.1007/s10853-017-1582-8

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] FABRICATION OF POTASSIUM-SUBSTITUTED HYDROXYAPATITE CERAMICS VIA ULTRASONIC SPRAY-PYROLYSIS ROUTE2017

    • Author(s)
      T. Yokota, M. Honda, M. Aizawa.
    • Journal Title

      Phosphorus Research Bulletin

      Volume: 33 Issue: 0 Pages: 35-40

    • DOI

      10.3363/prb.33.35

    • NAID

      130006250615

    • ISSN
      0918-4783, 1882-2363
    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Preparation and characterization of β-tricalcium phosphate powders with high solubility for chelate-setting calcium-phosphate cements.2017

    • Author(s)
      K. Nagata, T. Konishi, M. Honda, M. Aizawa.
    • Journal Title

      Key Engineering Materials

      Volume: 758 Pages: 194-198

    • DOI

      10.4028/www.scientific.net/kem.758.194

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Low-cost Ni-complex/graphitic carbon nitride photocatalyst for hydrogen evolution2017

    • Author(s)
      V. Kalousek, K. Kikuta, T. C. Vagvala, K. Ikeue
    • Journal Title

      Materials Letters

      Volume: 199 Pages: 65-67

    • DOI

      10.1016/j.matlet.2017.04.043

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Al-based mixed oxides as high-capacity carbon dioxide adsorbents2017

    • Author(s)
      Keita Ikeue, Masashige Suzuki, Munetoshi Sakai, Tarun Chand Vagvala, Vit Kalousek
    • Journal Title

      Chemical Physics Letters

      Volume: 677 Pages: 55-59

    • DOI

      10.1016/j.cplett.2017.03.087

    • Related Report
      2017 Annual Research Report 2016 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Droplet viscosity effects on dynamic hydrophobicity of a solid/liquid bulk composite prepared from porous glass2017

    • Author(s)
      K. Yokoyama, M. Sakai, T. Isobe, S. Matsushita, A. Nakajima
    • Journal Title

      J. Mater. Sci.

      Volume: 52 Issue: 1 Pages: 595-604

    • DOI

      10.1007/s10853-016-0356-z

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Recent Topics on Dynamic Hydrophobicity of Solid Surfaces2017

    • Author(s)
      酒井宗寿・中島章
    • Journal Title

      Journal of the Japan Society of Colour Material

      Volume: 90 Issue: 1 Pages: 15-22

    • DOI

      10.4011/shikizai.90.15

    • NAID

      130006770623

    • ISSN
      0010-180X, 1883-2199
    • Related Report
      2016 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Fabrication of chelate-setting B-tricalcium phosphate cements with enhanced bioresorbability and their materials properties2017

    • Author(s)
      K. Nagata, T. Konishi, M. Honda, M. Aizawa
    • Journal Title

      Key Engineering Materials

      Volume: 720 Pages: 157-161

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed
  • [Journal Article] New Applications of Surface Technology by Using Super Hydrophobic / Hydrophilic Coating2016

    • Author(s)
      酒井宗寿・中島章
    • Journal Title

      Journal of The Surface Finishing Society of Japan

      Volume: 67 Issue: 9 Pages: 467-472

    • DOI

      10.4139/sfj.67.467

    • NAID

      130006094369

    • ISSN
      0915-1869, 1884-3409
    • Related Report
      2016 Annual Research Report
    • Peer Reviewed
  • [Presentation] Comparative study of the dynamic hydrophobicity of fluoroalkylsilane coatings tilted as acute and obtuse angles2018

    • Author(s)
      Y. Higashino, H. Takahashi, M. Sakai, T. Isobe, S. Matsushita, A. Nakajima
    • Organizer
      Water on Materials Surface 2018
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Investigation of low cost metal bipyridyldiamine complexes as co-catalysts for hydrogen evolution from aqueous media2018

    • Author(s)
      T. C. Vagvala, T. Ooyabe, M. Sakai, Y, Funasako, V. Kalousek, K. Ikeue
    • Organizer
      TOCAT8
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 固体/液体複合撥水性材料上での水-グリセリン混合液体の転落2017

    • Author(s)
      高橋 宏和・磯部 敏宏・松下 祥子・中島 章・酒井 宗寿
    • Organizer
      セラミックス協会 年会
    • Place of Presentation
      日本大学 (東京都)
    • Year and Date
      2017-03-18
    • Related Report
      2016 Annual Research Report
  • [Presentation] Fabrication of sodium-substituted hydroxyapatite ceramics via ultrasonic spray-pyrolysis route and their material properties.2017

    • Author(s)
      T. Yokota, R. Ito, Y. Shimizu, M. Honda and M. Aizawa.
    • Organizer
      Bioceramics 29, France, Toulouse, The International Society for Ceramics in Medicine (ISCM), October 25th to 27th.
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] a面を多く露出した水酸アパタイトセラミックスの作製とその評価2016

    • Author(s)
      玉澤成記, 相澤 守
    • Organizer
      日本バイオマテリアル学会 シンポジウム2016
    • Place of Presentation
      福岡市 福岡国際会議場
    • Year and Date
      2016-11-21
    • Related Report
      2016 Annual Research Report
  • [Presentation] 多孔質吸着材上に固定化したSrTiO3ナノ粒子の光触媒特性2016

    • Author(s)
      板井崇晃, 鈴木将成, Vagvala Traun Chand, Kalousek Vit, 池上啓太
    • Organizer
      2016年日本化学会中国四国支部大会
    • Place of Presentation
      香川
    • Year and Date
      2016-11-05
    • Related Report
      2016 Annual Research Report
  • [Presentation] 金属錯体で修飾したカーボンナノチュブ系光触媒による水素発生反応2016

    • Author(s)
      池上啓太, 箱木晃, 井上匡人, 酒井宗寿, VAGVALA, Tarun,, Vit KALOUSEK, 田嶋智之, 高口豊
    • Organizer
      第118回触媒討論会
    • Place of Presentation
      盛岡市
    • Year and Date
      2016-09-21
    • Related Report
      2016 Annual Research Report
  • [Book] 「防汚・防水・防食および撥水親水に関する技術資料集」,第4章 接触角および撥水親水,撥油親油の試験評価:「接触角,液滴流動性の可視化技術とその応用」,第5章 防曇性を付与する表面処理,コーティング技術とその応用 :「酸化チタン・光触媒による表面親水性向上による防曇性向上2018

    • Author(s)
      酒井宗寿, 中島 章.
    • Total Pages
      200
    • Publisher
      技術情報協会
    • Related Report
      2017 Annual Research Report
  • [Book] 超親水・親油性表面の技術 第4章 親水性表面の応用展開・活用事例:「第1 節 親水性表面を活用した流体の流動性制御」2018

    • Author(s)
      酒井宗寿, 中島 章.
    • Total Pages
      200
    • Publisher
      サイエンス&テクノロジー
    • ISBN
      9784864281713
    • Related Report
      2017 Annual Research Report
  • [Book] リンの事典:第1章 リンの化学;1-1 リンとはなにか;リンの性質2017

    • Author(s)
      相澤 守
    • Publisher
      朝倉書店
    • Related Report
      2016 Annual Research Report
  • [Remarks] https://www.facebook.com/munesakai

    • Related Report
      2018 Annual Research Report
  • [Remarks]

    • URL

      https://ja-jp.facebook.com/munesakai

    • Related Report
      2017 Annual Research Report
  • [Remarks]

    • URL

      https://info.ibaraki.ac.jp/Profiles/105/0010451/profile.html

    • Related Report
      2017 Annual Research Report
  • [Remarks] https://ja-jp.facebook.com/munesakai

    • URL

      https://ja-jp.facebook.com/munesakai

    • Related Report
      2016 Annual Research Report

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Published: 2016-04-21   Modified: 2020-03-30  

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