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Detection of higher-order spin and orbital degrees of freedom through novel polarized neutron scattering techniques

Research Project

Project/Area Number 16H04007
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Condensed matter physics II
Research InstitutionTohoku University

Principal Investigator

Nambu Yusuke  東北大学, 金属材料研究所, 准教授 (60579803)

Project Period (FY) 2016-04-01 – 2019-03-31
Project Status Completed (Fiscal Year 2018)
Budget Amount *help
¥18,330,000 (Direct Cost: ¥14,100,000、Indirect Cost: ¥4,230,000)
Fiscal Year 2018: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Fiscal Year 2017: ¥5,590,000 (Direct Cost: ¥4,300,000、Indirect Cost: ¥1,290,000)
Fiscal Year 2016: ¥11,570,000 (Direct Cost: ¥8,900,000、Indirect Cost: ¥2,670,000)
Keywords物性実験 / 中性子散乱 / 鉄系超伝導 / フラストレート磁性 / スピントロニクス / 偏極中性子散乱
Outline of Final Research Achievements

We have conducted the following research topics. (1) In iron-based ladder compound BaFe2Se3 which shows superconductivity under pressures, an orbital order is elucidated. Polar state is identified in BaFe2Se3 through a detailed determination of the space group. Dynamical magnetism in these compounds is examined by combining neutrons and muons, and characteristic timescale of spin fluctuations spanning eight orders in magnitude is quantitatively measured. (2) For the triangular antiferromagnet NiGa2S4, magnetic quadrupole correlation was clarified from neutron and Raman scattering experiments. We also elucidated the vector chirality-driven anomaly at 8.5 K through polarized neutron scattering. (3) We discovered the magnon polarization in the spintronics material Y3Fe5O12.

Academic Significance and Societal Importance of the Research Achievements

磁気四重極子、カイラリティ、軌道揺らぎ等の高次スピン自由度および軌道自由度に基づく物性は磁性研究の分野で注目されており、実験的証拠は蓄積されているものの、その直接検出が待望されてきた。例えば、中性子散乱は二点相関関数を検出するため、磁気散乱で観測できるのはスピンスピン相関のみに限られる。それゆえスピン自由度が担う相関と素励起の観測には威力を発揮してきたが、高次スピン自由度および軌道自由度については現行の手法では傍証しか得ることしかできなかった。本研究で得られた新しい中性子散乱手法とその他の実験による観測は電子の新奇自由度の理解を深め、他の自由度への波及効果という点でも意義深いと考えられる。

Report

(4 results)
  • 2018 Annual Research Report   Final Research Report ( PDF )
  • 2017 Annual Research Report
  • 2016 Annual Research Report
  • Research Products

    (55 results)

All 2019 2018 2017 2016 Other

All Int'l Joint Research (6 results) Journal Article (7 results) (of which Int'l Joint Research: 3 results,  Peer Reviewed: 7 results,  Acknowledgement Compliant: 2 results) Presentation (37 results) (of which Int'l Joint Research: 10 results,  Invited: 12 results) Remarks (5 results)

  • [Int'l Joint Research] ANSTO(オーストラリア)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] Institut Laue-Langevin(フランス)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] Oak Ridge National Laboratory/NIST(米国)

    • Related Report
      2017 Annual Research Report
  • [Int'l Joint Research] ANSTO(オーストラリア)

    • Related Report
      2017 Annual Research Report
  • [Int'l Joint Research] Oak Ridge National Laboratory/NIST(米国)

    • Related Report
      2016 Annual Research Report
  • [Int'l Joint Research] ANSTO(オーストラリア)

    • Related Report
      2016 Annual Research Report
  • [Journal Article] 梯子型鉄系化合物BaFe2S3における圧力誘起超伝導2019

    • Author(s)
      山内徹, 平田靖透, 高橋博樹, 南部雄亮, 佐藤卓, 大串研也
    • Journal Title

      固体物理

      Volume: 54 Pages: 27-42

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] High-pressure electrical resistivity studies for Ba1-xCsxFe2Se32017

    • Author(s)
      Kawashima C、Soeda H、Takahashi H、Hawai T、Nambu Y、Sato T J、Hirata Y、Ohgushi K
    • Journal Title

      Journal of Physics: Conference Series

      Volume: 950 Pages: 042031-042031

    • DOI

      10.1088/1742-6596/950/4/042031

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Thermal stability and irreversibility of skyrmion-lattice phases in Cu2OSeO32017

    • Author(s)
      K. Makino, J. D. Reim, D. Higashi, D. Okuyama, T. J. Sato, Y. Nambu, E. P. Gilbert, N. Booth, S. Seki, Y. Tokura
    • Journal Title

      Physical Review B

      Volume: 95 Issue: 13

    • DOI

      10.1103/physrevb.95.134412

    • Related Report
      2017 Annual Research Report 2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Impact of minute-time-scale kinetics on the stabilization of the skyrmion-lattice in Cu2OSeO32017

    • Author(s)
      J. D. Reim, K. Makino, D. Higashi, Y. Nambu, D. Okuyama, T. J Sato, E. P. Gilbert, N. Booth, S. Seki
    • Journal Title

      J. Phys.: Conf. Ser.

      Volume: 828 Pages: 012004-012004

    • DOI

      10.1088/1742-6596/828/1/012004

    • Related Report
      2017 Annual Research Report 2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Development of a polarized 3He neutron spin filter for POLANO at J-PARC2017

    • Author(s)
      T. Ino, M. Ohkawara, K. Ohoyama, T. Yokoo, S. Itoh, Y. Nambu, M. Fujita, H. Kira, H. Hayashida, K. Hiroi, K. Sakai, T. Oku, and K. Kakurai
    • Journal Title

      Journal of Physics: Conference Series

      Volume: 862 Pages: 012011-012011

    • DOI

      10.1088/1742-6596/862/1/012011

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Pressure-Induced Metallization in Iron-Based Ladder Compounds Ba1-xCsxFe2Se32017

    • Author(s)
      T.Hawai, C.Kawashima, K.Ohgushi, K.Matsubayashi, Y.Nambu, Y.Uwatoko, T.J.Sato, H.Takahashi
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 86 Issue: 2 Pages: 024701-024701

    • DOI

      10.7566/jpsj.86.024701

    • NAID

      210000134262

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Magnetic Reversal of Electric Polarization with Fixed Chirality of Magnetic Structure in a Chiral-Lattice Helimagnet MnSb2O62016

    • Author(s)
      M. Kinoshita, S. Seki, T. J. Sato, Y. Nambu, T. Hong, M. Matsuda, H. B. Cao, S.Ishiwata, and Y. Tokura
    • Journal Title

      Phys. Rev. Lett.

      Volume: 117 Issue: 4 Pages: 047201-047201

    • DOI

      10.1103/physrevlett.117.047201

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Presentation] Helicity of magnon modes in YIG2019

    • Author(s)
      Y. Nambu
    • Organizer
      The 17th Japan-Korea Meeting on Neutron Science
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Role of magnon mode helicity in the spin current2019

    • Author(s)
      Y. Nambu
    • Organizer
      53rd REIMEI International Workshop “New excitations in spintronics”
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 複合アニオン化ペロブスカイトPb3Fe2O5F2における結晶場変化によるスピンフロップ2019

    • Author(s)
      南部雄亮、岡研吾、越智正之
    • Organizer
      日本物理学会第74回年次大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 量子ビームを用いたスピンの時空間相関の研究2019

    • Author(s)
      南部雄亮
    • Organizer
      日本物理学会第74回年次大会
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] ミュオンで視た鉄系梯子型物質およびMajumdar-Ghosh系物質の動的磁性2019

    • Author(s)
      南部雄亮、鈴木謙介、岡部博孝、幸田章宏、門野良典
    • Organizer
      2018年度量子ビームサイエンスフェスタ
    • Related Report
      2018 Annual Research Report
  • [Presentation] マグノンモードヘリシティがスピン流に与える影響2019

    • Author(s)
      南部雄亮、川本陽、沖野夕貴、藤田全基、加倉井和久
    • Organizer
      2018年度量子ビームサイエンスフェスタ
    • Related Report
      2018 Annual Research Report
  • [Presentation] 三角格子反強磁性体NiGa2S4のパルス強磁場ESR2019

    • Author(s)
      鳴海康雄、佐藤和樹、南部雄亮、川本陽、水戸陵人、赤木暢、萩原政幸
    • Organizer
      日本物理学会第74回年次大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Kinetics of the magnetic skyrmion lattice in MnSi under direct/alternating electric current2019

    • Author(s)
      D. Okuyama, M. Bleue, Q. Ye, N. Nagaosa, A. Kikkawa, Y. Taguchi, Y. Tokura, J.D. Reim, Y. Nambu, T.J. Sato
    • Organizer
      The 2nd Symposium for World Leading Research Centers -Materials Science and Spintronics-
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 中性子非弾性散乱実験に備えたTb3Fe5O12の単結晶試料育成2019

    • Author(s)
      川本陽、吉川貴史、藤田全基、南部雄亮
    • Organizer
      2018年度量子ビームサイエンスフェスタ
    • Related Report
      2018 Annual Research Report
  • [Presentation] 熱ホール効果を示すTb3Ga5O12のフォノンと結晶場2019

    • Author(s)
      森道康、藤田全基、南部雄亮、河村聖子、古府麻衣子、中島健次、C. Urlich、O.P. Sushkov
    • Organizer
      日本物理学会第74回年次大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 磁性体における偏極中性子散乱研究 -定常炉・核破砕炉の相補利用を見据えて2018

    • Author(s)
      南部雄亮
    • Organizer
      東京大学物性研究所中性子セミナー
    • Related Report
      2018 Annual Research Report
  • [Presentation] 中性子を用いたスピンダイナミクスの研究2018

    • Author(s)
      南部雄亮
    • Organizer
      第28回日本MRS年次大会
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] MnSiにおける電流中の磁気スキルミオン格子の塑性流動的な振る舞い2018

    • Author(s)
      奥山大輔、M. Bleuel、Q. Ye、P. Butler、永長直人、吉川明子、田口康二郎、十倉好紀、J. D. Reim、東大樹、南部雄亮、佐藤卓
    • Organizer
      日本物理学会2018年秋季大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] MnSiにおける変動電流中の磁気スキルミオン格子のダイナミクス2018

    • Author(s)
      奥山大輔、M. Bleuel、Q. Ye、P. Butler、永長直人、吉川明子、田口康二郎、十倉好紀、J. D. Reim、東大樹、南部雄亮、佐藤卓
    • Organizer
      日本物理学会2018年秋季大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 擬一次元梯子型鉄系化合物BaFe2(Se1-xSx)3における基礎物性測定2018

    • Author(s)
      今泉聖司、青山拓也、佐伯雄大、今井良宗、南部雄亮、Fei Du、上田寛、Maxim Avdeev、大串研也
    • Organizer
      日本物理学会2018年秋季大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] MnSiの定常/変動電流中の磁気スキルミオン格子ダイナミクス2018

    • Author(s)
      奥山大輔、M. Bleuel、永長直人、吉川明子、田口康二郎、十倉好紀、東大樹、J. D. Reim、南部雄亮、佐藤卓
    • Organizer
      日本中性子科学会第18回年会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 磁気スカーミオンの相安定性と電流下挙動2018

    • Author(s)
      奥山大輔、J. Reim、牧野晃也、東大樹、南部雄亮、E. P. Gilbert、N. Booth、M. Bleue、J. Krzywon、P. D. Butler、J. S. White、G. Nagy、M. Bartkowiak、I. Z. Quan、I. Zivkovic、H. M. Ronnow、関真一郎、星野晋太郎、岩崎惇一、永長直人、吉川明子、田口康二郎、十倉好紀、佐藤卓
    • Organizer
      物性研究所短期研究会「量子多体効果が生み出す液晶的電子状態」
    • Related Report
      2018 Annual Research Report
  • [Presentation] Magnetic excitations in YIG: Neutron scattering study2018

    • Author(s)
      Y. Nambu
    • Organizer
      Reimei/GP-Spin/ICC-IMR International Workshop “New Excitations in Spintronics”
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] カイラル磁性絶縁体Cu2OSeO3における磁気スキルミオンの中性子小角散乱2018

    • Author(s)
      南部雄亮
    • Organizer
      2017年度量子ビームサイエンスフェスタ
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] Current Status of the Powder Diffractometer HERMES stationed at the JRR-3 Reactor2018

    • Author(s)
      Y. Nambu, M. Ohkawara, Y. Ikeda, K.M. Suzuki, and M. Fujita
    • Organizer
      Kick-off Symposium for World Leading Research Centers -Materials Science and Spintronics-
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] マルチプローブで視た鉄系梯子型物質の動的磁性2018

    • Author(s)
      南部雄亮、鈴木謙介、羽合孝文、長尾道弘、伊藤晋一、岡部博孝、幸田章宏、門野良典、今泉聖司、橋詰和樹、青山拓也、大串研也
    • Organizer
      2017年度量子ビームサイエンスフェスタ
    • Related Report
      2017 Annual Research Report
  • [Presentation] Magnetic dynamics in the iron-based ladder compound BaFe2Se32017

    • Author(s)
      Y. Nambu, K.M. Suzuki, H. Okabe, A. Koda, R. Kadono, S. Imaizumi, K. Hashizume, T. Aoyama, Y. Imai, and K. Ohgushi
    • Organizer
      The 14th International Conference on Muon Spin Rotation, Relaxation and Resonance
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Dynamical magnetism in the iron-based ladder compound BaFe2Se3 through multi-probe techniques2017

    • Author(s)
      Y. Nambu, K.M. Suzuki, S. Imaizumi, K. Hashizume, T. Aoyama, Y. Imai, and K. Ohgushi
    • Organizer
      28th International Conference on Low Temperature Physics
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 中性子とミュオンでみた鉄系梯子型物質BaFe2Se3の動的磁性2017

    • Author(s)
      南部雄亮、鈴木謙介、羽合孝文、長尾道弘、横尾哲也、伊藤晋一、岡部博孝、幸田章宏、門野良典、今泉聖司、橋詰和樹、青山拓也、今井良宗、大串研也
    • Organizer
      日本物理学会 2017年秋季大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 複合アニオン研究に中性子が貢献できること2017

    • Author(s)
      南部雄亮
    • Organizer
      第7回CSJ化学フェスタ2017
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] 中性子を用いた複合アニオン化合物の磁性研究2017

    • Author(s)
      南部雄亮
    • Organizer
      日本磁気学会第215回研究会/第61回化合物新磁性材料専門研究会
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] 研究用原子炉JRR-3の粉末回折計HERMESの現状と結晶・磁気構造解析2017

    • Author(s)
      南部雄亮、大河原学、池田陽一、鈴木謙介、藤田全基
    • Organizer
      第133回金属材料研究所講演会
    • Related Report
      2017 Annual Research Report
  • [Presentation] JRR-3に設置された粉末回折計HERMESの現状2017

    • Author(s)
      南部雄亮、大河原学、池田陽一、鈴木謙介、藤田全基
    • Organizer
      日本中性子科学会第17回年会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Magnetic excitations in YIG revisited2017

    • Author(s)
      Y. Nambu
    • Organizer
      The 37th REIMEI Workshop on Frontiers of Correlated Quantum Matters and Spintronics
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 三角格子反強磁性体NiGa2S4の偏極中性子弾性散乱2017

    • Author(s)
      南部雄亮、Y. Qiu、T.R. Gentile、W.C. Chen、S. Watson、C. Broholm
    • Organizer
      日本物理学会第72回年次大会
    • Related Report
      2016 Annual Research Report
  • [Presentation] 中性子粉末回折装置HERMESの現状―研究用原子炉JRR-3の再稼働に向けて2017

    • Author(s)
      南部雄亮、大河原学、池田陽一、鈴木謙介、藤田全基
    • Organizer
      2016年度量子ビームサイエンスフェスタ
    • Related Report
      2016 Annual Research Report
  • [Presentation] マルチプローブで視た鉄系梯子系BaFe2Se3の磁気揺動2017

    • Author(s)
      南部雄亮、鈴木謙介、羽合孝文、長尾道弘、横尾哲也、伊藤晋一、大串研也
    • Organizer
      2016年度量子ビームサイエンスフェスタ
    • Related Report
      2016 Annual Research Report
  • [Presentation] 中性子でみた鉄系梯子型物質の磁気揺動2016

    • Author(s)
      南部雄亮
    • Organizer
      KEK-S型課題中性子スピンエコー研究会
    • Related Report
      2016 Annual Research Report
    • Invited
  • [Presentation] Magnetism of the triangular antiferromagnet NiGa2S4 and introduction of POLANO2016

    • Author(s)
      Y. Nambu
    • Organizer
      Polarised Neutrons for Condensed Matter Investigations
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 偏極中性子を用いた研究展望とPOLANOの現状2016

    • Author(s)
      南部雄亮
    • Organizer
      Workshop: CROSSroads of Users and J-PARC 第18回「偏極ターゲットと偏極中性子技術開発」
    • Related Report
      2016 Annual Research Report
    • Invited
  • [Presentation] Spin fluctuations on a triangular lattice2016

    • Author(s)
      Y. Nambu
    • Organizer
      Summit of Materials Science
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 研究用原子炉JRR-3の再稼働に向けての中性子粉末回折装置HERMESの取り組み2016

    • Author(s)
      南部雄亮、大河原学、池田陽一、鈴木謙介、藤田全基
    • Organizer
      第10回物性科学領域横断研究会
    • Related Report
      2016 Annual Research Report
  • [Remarks] 物理学専攻 南部 雄亮 准教授 が 第13回(2019年)日本物理学会若手奨励賞 を受賞

    • URL

      http://www.sci.tohoku.ac.jp/news/20190228-10141.html

    • Related Report
      2018 Annual Research Report
  • [Remarks] 南部雄亮 准教授が第13回日本物理学会若手奨励賞(領域3)を受賞しました。

    • URL

      http://www.phys.tohoku.ac.jp/cat_jp/post-2411/

    • Related Report
      2018 Annual Research Report
  • [Remarks] 受賞

    • URL

      http://www.imr.tohoku.ac.jp/ja/news/awards/2019/#aw1103

    • Related Report
      2018 Annual Research Report
  • [Remarks] 若手奨励賞

    • URL

      https://www.jps.or.jp/activities/awards/jusyosya/wakate2019.php#r3

    • Related Report
      2018 Annual Research Report
  • [Remarks] 特別インタビュー物理の「美しさ」に導かれて

    • URL

      http://www.imr.tohoku.ac.jp/kinken-mapping/00-201707.html

    • Related Report
      2017 Annual Research Report

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Published: 2016-04-21   Modified: 2022-05-20  

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