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Atmospheric Distribution, Diffusion, Reaction and Risk Assessment of Hazardous Organic Aerosols in East Asia

Research Project

Project/Area Number 16H05625
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section海外学術
Research Field Environmental impact assessment
Research InstitutionKyoto University

Principal Investigator

Kameda Takayuki  京都大学, エネルギー科学研究科, 准教授 (50398426)

Co-Investigator(Kenkyū-buntansha) 大浦 健  名城大学, 農学部, 教授 (60315851)
Project Period (FY) 2016-04-01 – 2019-03-31
Project Status Completed (Fiscal Year 2018)
Budget Amount *help
¥16,380,000 (Direct Cost: ¥12,600,000、Indirect Cost: ¥3,780,000)
Fiscal Year 2018: ¥4,680,000 (Direct Cost: ¥3,600,000、Indirect Cost: ¥1,080,000)
Fiscal Year 2017: ¥5,590,000 (Direct Cost: ¥4,300,000、Indirect Cost: ¥1,290,000)
Fiscal Year 2016: ¥6,110,000 (Direct Cost: ¥4,700,000、Indirect Cost: ¥1,410,000)
Keywords大気汚染 / PAH / 東アジア / 二次生成 / 黄砂 / PAH
Outline of Final Research Achievements

Air pollutants discharged by energy consumption have an effect on the environment and have a close relation with health hazard to human, so that thorough management is required. Recently, it has been reported that polycyclic aromatic compounds observed at high concentrations in China, which is suffering from serious air pollution, are not only produced by incomplete combustion of fossil fuels, but also secondarily produced in the atmosphere. In order to take effective measures against air pollution caused by these sources, it is necessary to clarify the contribution rate of each source. In this study, we selected Shenyang City, Liaoning Province, China, where air pollution is serious, as an observation site, and estimated the source of polycyclic aromatic compounds and their contribution rate.

Academic Significance and Societal Importance of the Research Achievements

本研究では多環芳香族化合物の発生源寄与の季節変動を明らかにし,各発生源への平均寄与率を算出した.発生源解析を行った結果,多環芳香族化合物は石炭燃焼と自動車排出のほか,バイオマス燃焼,大気内二次生成の寄与が無視できないことがわかった.今まで発生源情報が少ない多環芳香族化合物に関して,多成分間相関関係とレセプターモデルによる解析を使って,その発生源寄与率を明らかにすることができた.

Report

(4 results)
  • 2018 Annual Research Report   Final Research Report ( PDF )
  • 2017 Annual Research Report
  • 2016 Annual Research Report
  • Research Products

    (40 results)

All 2019 2018 2017 2016

All Journal Article (16 results) (of which Int'l Joint Research: 6 results,  Peer Reviewed: 15 results,  Open Access: 6 results) Presentation (22 results) (of which Int'l Joint Research: 3 results,  Invited: 4 results) Book (2 results)

  • [Journal Article] 多環芳香族化合物の大気内二次生成2018

    • Author(s)
      亀田 貴之
    • Journal Title

      大気化学研究

      Volume: 39

    • NAID

      120006636642

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] 大気環境中の化学反応によって生成する有害化学物質2018

    • Author(s)
      亀田 貴之
    • Journal Title

      第31回環境工学連合講演会講演論文集

      Volume: 31 Pages: 13-16

    • NAID

      120006705810

    • Related Report
      2018 Annual Research Report
    • Open Access
  • [Journal Article] Distributions and multiple sources of chlorinated polycyclic aromatic hydrocarbons in the air over Japan2018

    • Author(s)
      T. Ohura, T. Suhara, Y. Kamiya, F. Ikemori, S. Kageyama, D. Nakajima
    • Journal Title

      Sci. Total Environ.

      Volume: 649 Pages: 364-371

    • DOI

      10.1016/j.scitotenv.2018.08.302

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Spatial distribution and exposure risks of ambient chlorinated polycyclic aromatic hydrocarbons in Tokyo Bay area and network approach to source impacts2018

    • Author(s)
      Takeshi Ohura, Yuichi Horii, Nobuyoshi Yamashita
    • Journal Title

      Environmental Pollution

      Volume: 232 Pages: 367-374

    • DOI

      10.1016/j.envpol.2017.09.037

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Determination of Particle-Associated PAH Derivatives (ClPAHs, NPAHs, OPAHs) in Ambient Air and Automobile Exhaust by Gas Chromatography/Mass Spectrometry with Negative Chemical Ionization2017

    • Author(s)
      Yuta Kamiya, Takayuki Kameda, Takeshi Ohura and Susumu Tohno
    • Journal Title

      Polycyclic Aromatic Compounds

      Volume: 37 Issue: 2-3 Pages: 128-140

    • DOI

      10.1080/10406638.2016.1202290

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Chlorinated polycyclic aromatic hydrocarbons in surface sediment from Maowei Sea, Guangxi, China: occurrence, distribution, and source apportionment2017

    • Author(s)
      Y. Wang, R. Liao, W. Liu, K. Kannan, T. Ohura, M. Wu, J. Ma
    • Journal Title

      Environ. Sci. Pollut. Res.

      Volume: 24 Issue: 19 Pages: 16241-16252

    • DOI

      10.1007/s11356-017-9193-0

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Atmospheric behaviors of particulate-bound polycyclic aromatic hydrocarbons and nitropolycyclic aromatic hydrocarbons in Beijing, China from 2004 to 20102017

    • Author(s)
      N. Tang, G. Suzuki, H. Morisaki, T. Tokuda, X. Yang, L. Zhao, J. Lin, T. Kameda, A. Toriba, K. Hayakawa
    • Journal Title

      Atmos. Environ.

      Volume: 152 Pages: 354-361

    • DOI

      10.1016/j.atmosenv.2016.12.056

    • NAID

      120005982986

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Size distribution of chlorinated polycyclic aromatic hydrocarbons in atmospheric particles2017

    • Author(s)
      K. Kakimoto, H. Nagayoshi, Y. Konishi, K. Kajimura, T. Ohura, T. Nakano, M. Hata, M. Furuuchi, N. Tang, K. Hayakawa, A. Toriba
    • Journal Title

      Arch. Environ. Contam. Toxicol.

      Volume: 72 Issue: 1 Pages: 58-64

    • DOI

      10.1007/s00244-016-0327-z

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Estimation of rate constants for gas-phase reactions of chrysene, benz[a]anthracene, and benzanthrone with OH and NO3 radicals via a relative rate method in CCl4 liquid phase-system2016

    • Author(s)
      Takayuki Kameda, Kohei Asano, Hiroshi Bandow, Kazuichi Hayakawa
    • Journal Title

      Polycyclic Aromatic Compounds

      Volume: 印刷中 Issue: 2-3 Pages: 101-105

    • DOI

      10.1080/10406638.2016.1159583

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Simultaneous determination of polycyclic aromatic hydrocarbon quinones by gas chromatography-tandem mass spectrometry, following a one-pot reductive trimethysilyl derivatization2016

    • Author(s)
      A. Toriba, C. Homma, M. Kita, W. Uozaki, Y. Boongla, W. Orakij, N. Tang, T. Kameda, K. Hayakawa
    • Journal Title

      J. Chromatogr. A

      Volume: 1459 Pages: 89-100

    • DOI

      10.1016/j.chroma.2016.06.034

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Polycyclic Aromatic Hydrocarbons in Surface Water of the Southeastern Japan Sea2016

    • Author(s)
      K. Hayakawa, F. Makino, M. Yasuma, S. Yoshita, Y. Chondo, A. Toriba, T. Kameda, C-S. Hong, N. Tang, M. Kumagai, H. Nakase, C. Kinoshita, T. Kawanishi, Z. Zhou, W. Qing, V. Mishukov, P. Tishchenko, V. Lobanov, T. Chizhova, Y. Konoudryasho
    • Journal Title

      Chemical and Pharmaceutical Bulletin

      Volume: 64 Issue: 6 Pages: 625-631

    • DOI

      10.1248/cpb.c16-00063

    • NAID

      130005154410

    • ISSN
      0009-2363, 1347-5223
    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Nitro-PAH exposures of occupationally-exposed traffic workers and associated urinary 1-nitropyrene metabolite concentrations2016

    • Author(s)
      J.P. Miller-Schulze, M. Paulsen, T. Kameda, A. Toriba, K. Hayakawa, B. Cassidy, L. Naeher, M.A. Villalobos, C.D. Simpson
    • Journal Title

      J. Environ. Sci.

      Volume: 49 Pages: 213-221

    • DOI

      10.1016/j.jes.2016.06.007

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Source apportionment of chlorinated polycyclic aromatic hydrocarbons associated with ambient particles in a Japanese megacity2016

    • Author(s)
      Y. Kamiya, A. Iijima, F. Ikemori, T. Okuda, T. Ohura
    • Journal Title

      Sci. Rep.

      Volume: 6 Issue: 1 Pages: 38358-38358

    • DOI

      10.1038/srep38358

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Spatio-temporal distribution, source, and genotoxic potential of polycyclic aromatic hydrocarbons in estuarine and riverine sediments from southern India2016

    • Author(s)
      P. Goswami, T. Ohura, K. S. Guruge, M. Yoshioka, N. Yamanaka, M. Akiba, N. Munuswamy
    • Journal Title

      Ecotoxicol. Environ. Saf.

      Volume: 130 Pages: 113-123

    • DOI

      10.1016/j.ecoenv.2016.04.016

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Local and seasonal variations in concentrations of chlorinated polycyclic aromatic hydrocarbons associated with particles in a Japanese megacity2016

    • Author(s)
      T. Ohura, Y. Kamiya, F. Ikemor
    • Journal Title

      J. Hazard. Mater.

      Volume: 312 Pages: 254-261

    • DOI

      10.1016/j.jhazmat.2016.03.072

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Photochlorination of polycyclic aromatic hydrocarbons in acidic brine solution2016

    • Author(s)
      T. Ohura, M. Miwa
    • Journal Title

      Bull. Environ. Contam. Toxicol.

      Volume: 96 Issue: 4 Pages: 524-529

    • DOI

      10.1007/s00128-015-1723-1

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed
  • [Presentation] 大気輸送中のPAH類の化学反応と毒性の変化2019

    • Author(s)
      亀田 貴之
    • Organizer
      日本薬学会第139年会
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] Passive air sampling of halogenated polycyclic aromatic hydrocarbons in the largest industrial city in Korea: Spatial distributions and source identification2018

    • Author(s)
      Q. T. Vuong, S-J. Kim, T. N. T. Nguyen, T. Q. Phan, T. Ohura, S-D. Choi
    • Organizer
      The 11th Society of Environmental Toxicology and Chemistry;Asia Pacific 2018
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 大気浮遊粒子における高級脂肪酸の粒径別季節変動と発生源解析2018

    • Author(s)
      今井 悠貴,吉野 由梨,池盛 文数,大浦 健
    • Organizer
      第27回環境化学討論会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Orbitrap GC-MSの微量汚染物質分析への活用2018

    • Author(s)
      平林卓真、大浦健
    • Organizer
      第1回中部環境化学セミナー
    • Related Report
      2018 Annual Research Report
  • [Presentation] 大気環境中の化学反応によって生成する有害化学物質2018

    • Author(s)
      亀田 貴之
    • Organizer
      第31回環境工学連合講演会
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] Comprehensive assessment of carbonaceous PM2.5 in Malaysia during haze events influenced by Indonesia peatland fire and non-haze period2018

    • Author(s)
      Kurita, H., Fujii, Yusuke, Tohno, S., Saito, N., Kamiya, Y., Kameda, T., Hitzenberger, R., Haller, T., Ikeda, K., Sakai, N., Sulong, N.A., Latif, M.T., Ohura, T.
    • Organizer
      10th International Aerosol Conference
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] ピレンキノンの大気粒子中濃度と酸化能評価2018

    • Author(s)
      亀田貴之,大久保力斗, 東野 達
    • Organizer
      第35回エアロゾル科学・技術研究討論会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 鉱物エアロゾル上におけるPAHとオゾンとの反応によるPAHキノンの二次生成2018

    • Author(s)
      Gao Yatong, 亀田貴之,Dule, 東野 達
    • Organizer
      第59回大気環境学会年会
    • Related Report
      2018 Annual Research Report
  • [Presentation] DTTアッセイを用いたPAHキノン化合物の評価2018

    • Author(s)
      大久保力斗, 亀田貴之,東野 達
    • Organizer
      第59回大気環境学会年会
    • Related Report
      2018 Annual Research Report
  • [Presentation] PM2.5中多環芳香族炭化水素(PAH, nitro-PAH, oxy-PAH)日内濃度変動の高時間分解能解析2018

    • Author(s)
      亀田貴之,張 子丹,東野 達
    • Organizer
      第59回大気環境学会年会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 鉱物エアロゾル上におけるフェナントレンとオゾンとの反応による9,10-フェナントレンキノンの二次生成2017

    • Author(s)
      亀田 貴之,Dule, 東野 達
    • Organizer
      第34回エアロゾル科学・技術研究討論会
    • Related Report
      2017 Annual Research Report
  • [Presentation] インドネシア泥炭火災の影響を受けるマレーシアPM2.5の細胞影響と多環芳香族炭化水素及び誘導体の性状特性2017

    • Author(s)
      斉藤 想,藤井 佑介,神谷 優太,本田 晶子,亀田 貴之,東野 達, 高野 裕久, Mohd Talib Latif,Haryono S. Huboyo,大浦 健
    • Organizer
      第34回エアロゾル科学・技術研究討論会
    • Related Report
      2017 Annual Research Report
  • [Presentation] ポストカラム誘導体化-蛍光検出二次元高速液体クロマトグラフィを用いた大気粒子中9,10-フェナントレンキノンの分析2017

    • Author(s)
      剣崎佑多,亀田 貴之,東野 達
    • Organizer
      第58回大気環境学会年会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 能登半島珠洲および京都における大気中多環芳香族誘導体の通年観測2017

    • Author(s)
      神谷 優太,亀田 貴之,松木 篤,大浦 健,東野 達
    • Organizer
      第58回大気環境学会年会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 鉱物エアロゾル上におけるphenanthreneとO3との不均一反応による9,10-phenanthrenequinoneの二次生成2017

    • Author(s)
      亀田 貴之,Dule, Gao Yatong, 東野 達
    • Organizer
      第58回大気環境学会年会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 多環芳香族炭化水素類の大気粉塵中における粒径分布の解明2017

    • Author(s)
      柿本健作,永吉晴奈,小西良昌,梶村計志,大浦健,畑光彦,古内正美,唐寧,早川和一,鳥羽陽
    • Organizer
      第26回環境化学討論会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 大気微小粒子における塩素化多環芳香族炭 化水素類の発生源解析2017

    • Author(s)
      今井 悠貴,池盛 文数,東海林 完,大浦 健
    • Organizer
      第26回環境化学討論会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Mineral dust aerosols promote the nitration of atmospheric polycyclic aromatic hydrocarbons2016

    • Author(s)
      Takayuki Kameda
    • Organizer
      The 2nd International Workshop on Heterogeneous Kinetics Related to Atmospheric Aerosols
    • Place of Presentation
      つくば国際会議場(つくば市)
    • Year and Date
      2016-11-12
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 鉱物エアロゾル表面における多環芳香族炭化水素の特異的ニトロ化2016

    • Author(s)
      亀田 貴之
    • Organizer
      第57回大気環境学会年会
    • Place of Presentation
      北海道大学(札幌市)
    • Year and Date
      2016-09-07
    • Related Report
      2016 Annual Research Report
  • [Presentation] 能登半島珠洲における多環芳香族炭化水素誘導体の大気内挙動解析2016

    • Author(s)
      神谷優太
    • Organizer
      第57回大気環境学会年会
    • Place of Presentation
      北海道大学(札幌市)
    • Year and Date
      2016-09-07
    • Related Report
      2016 Annual Research Report
  • [Presentation] 海鳥における塩素化多環芳香族類の生体蓄積性2016

    • Author(s)
      大浦 健
    • Organizer
      第25回環境化学討論会
    • Place of Presentation
      朱鷺メッセ(新潟市)
    • Year and Date
      2016-06-08
    • Related Report
      2016 Annual Research Report
  • [Presentation] 黄砂粒子上で二次生成する有害ニトロ化多環芳香族炭化水素2016

    • Author(s)
      亀田 貴之
    • Organizer
      大気環境学会近畿支部 反応と測定部会 2016年度講演会
    • Place of Presentation
      大阪府立大学 I-site なんば(大阪市)
    • Related Report
      2016 Annual Research Report
    • Invited
  • [Book] Polycyclic Aromatic Hydrocarbons - Environmental Behavior and Toxicity in East Asia2018

    • Author(s)
      T. Kameda
    • Total Pages
      274
    • Publisher
      Springer Nature
    • ISBN
      9789811067747
    • Related Report
      2018 Annual Research Report 2017 Annual Research Report
  • [Book] Trans-Boundary Pollution in North-East Asia2018

    • Author(s)
      T. Kameda
    • Total Pages
      287
    • Publisher
      Nova Science Publishers
    • ISBN
      9781536141634
    • Related Report
      2018 Annual Research Report

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Published: 2016-04-21   Modified: 2020-03-30  

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