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Development of time resolved THz-STM

Research Project

Project/Area Number 16H05982
Research Category

Grant-in-Aid for Young Scientists (A)

Allocation TypeSingle-year Grants
Research Field Thin film/Surface and interfacial physical properties
Research InstitutionUniversity of Tsukuba

Principal Investigator

Yoshida Shoji  筑波大学, 数理物質系, 准教授 (90447227)

Project Period (FY) 2016-04-01 – 2020-03-31
Project Status Completed (Fiscal Year 2019)
Budget Amount *help
¥26,260,000 (Direct Cost: ¥20,200,000、Indirect Cost: ¥6,060,000)
Fiscal Year 2019: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Fiscal Year 2018: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Fiscal Year 2017: ¥3,770,000 (Direct Cost: ¥2,900,000、Indirect Cost: ¥870,000)
Fiscal Year 2016: ¥19,630,000 (Direct Cost: ¥15,100,000、Indirect Cost: ¥4,530,000)
Keywords走査プローブ顕微鏡 / テラヘルツ / 超高速分光 / 表面科学 / 走査トンネル顕微鏡 / 時間分解計測 / 超高速
Outline of Final Research Achievements

In this study, we have developed a novel time-resolved microscopy - THz-STM. We have achieved time-resolved measurement with extremely high signal to noise ratio by using a highly intense and high repetition rate THz pulse, which was generated using high power femtosecond pulse laser.
We have applied the technique to probe the ultrafast dynamics of various materials. For example, we have succeeded in measuring ultrafast carrier relaxation and ultrafast metal-insulator transition in two dimensional layered materials, and we have captured electron motion in an organic semiconductor. We have demonstrated sub-ps time resolution and atomic spatial resolution of the method from the above results.

Academic Significance and Societal Importance of the Research Achievements

本研究で開発した時間分解THz-STMを用いて、超高速領域での光励起キャリアダイナミクスや電子状態の変化を原子レベルで捉えることに成功した。サブps時間分解能、原子分解能を両立した時間分解計測による表面ダイナミクスのイメージングが可能となり、今後様々な試料の光応答・ダイナミクスを原子・分子のスケールで解明できるようになると期待される。

Report

(5 results)
  • 2019 Annual Research Report   Final Research Report ( PDF )
  • 2018 Annual Research Report
  • 2017 Annual Research Report
  • 2016 Annual Research Report
  • Research Products

    (28 results)

All 2019 2018 2017 2016

All Journal Article (18 results) (of which Int'l Joint Research: 3 results,  Peer Reviewed: 18 results,  Open Access: 9 results,  Acknowledgement Compliant: 4 results) Presentation (10 results) (of which Int'l Joint Research: 4 results,  Invited: 3 results)

  • [Journal Article] Surface-mediated effect on electron spin dynamics probed by optical-pump-probe scanning tunneling microscopy2019

    • Author(s)
      Zi-han Wang, Cheul-hyun Yoon, Shoji Yoshida, Yusuke Arashida, Osamu Takeuchi, Yuzo Ohno and Hidemi Shigekawa
    • Journal Title

      Physical Chemistry Chemical Physics

      Volume: 21 Issue: 14 Pages: 7256-7260

    • DOI

      10.1039/c8cp07786j

    • Related Report
      2019 Annual Research Report 2018 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Externally triggerable optical pump-probe scanning tunneling microscopy2019

    • Author(s)
      Hiroyuki Mogi, Wang Zihan, Kikuchi Ryusei, Cheul-hyun Yoon, Shoji Yoshida, Osamu Takeuchi, and Hidemi Shigekawa
    • Journal Title

      Appl. Phys. Express

      Volume: 12、2 Issue: 2 Pages: 025005-025005

    • DOI

      10.7567/1882-0786/aaf8b2

    • NAID

      210000135565

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Subcycle Transient Scanning Tunneling Spectroscopy with Visualization of Enhanced Terahertz Near Field2019

    • Author(s)
      Yoshida Shoji、Hirori Hideki、Tachizaki Takehiro、Yoshioka Katsumasa、Arashida Yusuke、Wang Zi-Han、Sanari Yasuyuki、Takeuchi Osamu、Kanemitsu Yoshihiko、Shigekawa Hidemi
    • Journal Title

      ACS Photonics

      Volume: 6 Issue: 6 Pages: 1356-1364

    • DOI

      10.1021/acsphotonics.9b00266

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Continuous Heteroepitaxy of Two-Dimensional Heterostructures Based on Layered Chalcogenides2019

    • Author(s)
      Kobayashi Yu、Yoshida Shoji、Maruyama Mina、Mogi Hiroyuki、Murase Kota、Maniwa Yutaka、Takeuchi Osamu、Okada Susumu、Shigekawa Hidemi、Miyata Yasumitsu
    • Journal Title

      ACS Nano

      Volume: 13 Issue: 7 Pages: 7527-7535

    • DOI

      10.1021/acsnano.8b07991

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] New delay-time modulation scheme for optical pump?probe scanning tunneling microscopy (OPP-STM) with minimized light-intensity modulation2019

    • Author(s)
      Takeuchi Osamu、Mogi Hiroyuki、Wang Zi-Han、Yoon Cheul Hyun、Taninaka Atsushi、Yoshida Shoji、Shigekawa Hidemi
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 58 Issue: SI Pages: SIIA12-SIIA12

    • DOI

      10.7567/1347-4065/ab1255

    • NAID

      210000156640

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Subcycle mid-infrared coherent transients at 4??MHz repetition rate applicable to light-wave-driven scanning tunneling microscopy2019

    • Author(s)
      Yoshioka Katsumasa、Igarashi Ippo、Yoshida Shoji、Arashida Yusuke、Katayama Ikufumi、Takeda Jun、Shigekawa Hidemi
    • Journal Title

      Optics Letters

      Volume: 44 Issue: 21 Pages: 5350-5350

    • DOI

      10.1364/ol.44.005350

    • NAID

      120006773346

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Development of laser-combined scanning multiprobe spectroscopy and application to analysis of WSe2/MoSe2 in-plane heterostructure2019

    • Author(s)
      Hiroyuki Mogi, Zi-Han Wang, Takafumi Banba, Yuhei Takaguchi, Naohiko Endo, Shoji Yoshida, Atsushi Taninaka, Haruhiro Oigawa, Yasumitsu Miyata, Osamu Takeuchi, and Hidemi Shigekawa
    • Journal Title

      Appl. Phys. Express

      Volume: 12 Issue: 4 Pages: 045002-045002

    • DOI

      10.7567/1882-0786/ab09b9

    • NAID

      120007128101

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Evolution of local conductance pathways in a single-molecule junction studied by three-dimensional dynamic probe method2019

    • Author(s)
      Atsushi Taninaka, Shoji Yoshida, Yoshihiro Sugita, Osamu Takeuchi, and Hidemi Shigekawa
    • Journal Title

      Nanoscale

      Volume: 11 Issue: 13 Pages: 5951-5959

    • DOI

      10.1039/c9nr00717b

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Laser-combined Scanning Tunneling Microscopy and Its Applications2018

    • Author(s)
      Hidemi Shigekawa and Shoji Yoshida
    • Journal Title

      Association of Asia Pacific Physical Societies

      Volume: 28 Pages: 9-18

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Externally triggerable optical pump-probe scanning tunneling microscopy2018

    • Author(s)
      Hiroyuki Mogi, Wang Zihan, Kikuchi Ryusei, Cheul-hyun Yoon, Shoji Yoshida, Osamu Takeuchi, and Hidemi Shigekawa
    • Journal Title

      Applied Physics Express

      Volume: 12 Issue: 1-2 Pages: 025005-025005

    • DOI

      10.1016/j.ijpharm.2007.07.014

    • NAID

      210000135565

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] The effect of nitrogen lone-pair interaction on the conduction in a single-molecule junction with amine-Au bonding2018

    • Author(s)
      Yoshihiro Sugita, Atsushi Taninaka, Shoji Yoshida, Osamu Takeuchi, and Hidemi Shigekawa
    • Journal Title

      Scientific Reports

      Volume: 8 Issue: 1 Pages: 5222-5222

    • DOI

      10.1038/s41598-018-22893-7

    • NAID

      120007134252

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Scanning tunneling microscopy/spectroscopy on MoS2 embedded nanowire formed in CVD-grown Mo1_xWxS2 alloy2017

    • Author(s)
      H. Mogi, Y. Kobayashi, A. Taninaka, R. Sakurada, T. Takeuchi, S. Yoshida1, O. Takeuchi, Y. Miyata, H. Shigekawa
    • Journal Title

      Jpn. J. Appl. Phys.

      Volume: 56 Issue: 8S1 Pages: 1-4

    • DOI

      10.7567/jjap.56.08lb06

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Modulation of the Local Density of States of Carbon Nanotubes by Encapsulation of Europium Nanowires As Observed by Scanning Tunneling Microscopy and Spectroscopy2017

    • Author(s)
      Nakanishi Terunobu、Kitaura Ryo、Kawai Takazumi、Okada Susumu、Yoshida Shoji、Takeuchi Osamu、Shigekawa Hidemi、Shinohara Hisanori
    • Journal Title

      The Journal of Physical Chemistry C

      Volume: 121 Issue: 33 Pages: 18195-18201

    • DOI

      10.1021/acs.jpcc.7b04047

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Attractive Interaction between Mn Atoms on GaAs(110) Surface Observed by Scanning Tunneling Microscopy2016

    • Author(s)
      A. Taninaka, S. Yoshida, K. Kanazawa, E. Hayaki, O. Takeuchi, and H. Shigekawa
    • Journal Title

      Nanoscale

      Volume: 2016, 8 Issue: 24 Pages: 12118-12122

    • DOI

      10.1039/c6nr02190e

    • NAID

      120007135303

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Temperature dependence of Peierls-Hubbard Phase Transition in [Pd(cptn)2Br]Br2 Studied by Scanning Tunneling Microscopy2016

    • Author(s)
      Y. Hosomi, S. Yoshida, A. Taninaka, T. Yoshida, S. Takaishi, O. Takeuchi, M. Yamashita, and H. Shigekawa
    • Journal Title

      Jpn. J. Appl. Phys.

      Volume: 55 Issue: 8S1 Pages: 08NB16-08NB16

    • DOI

      10.7567/jjap.55.08nb16

    • NAID

      120007129519

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Modulation of electrical potential and conductivity in an atomic-layer semiconductor heterojunction2016

    • Author(s)
      Y. Kobayashi, S. Yoshida, R. Sakurada, K. Takashima, T. Yamamoto, T. Saito, S. Konabe, T. Taniguchi, K. Watanabe, Y. Maniwa, O. Takeuchi, H. Shigekawa, Y. Miyata
    • Journal Title

      Sci. Rep.

      Volume: 6 Issue: 1 Pages: 31223-31223

    • DOI

      10.1038/srep31223

    • NAID

      120007129481

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Real-space coherent manipulation of electrons in a single tunnel junction by single-cycle terahertz fields2016

    • Author(s)
      K. Yoshioka, I. Katayama, Y. Minami, M. Kitajima, S. Yoshida, H. Shigekawa, and J. Takeda
    • Journal Title

      Nature Photonics

      Volume: 10 Issue: 12 Pages: 762-765

    • DOI

      10.1038/nphoton.2016.205

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Revealing conformational dynamics in single-molecule junction by site- and angle-resolved dynamic probe method2016

    • Author(s)
      S. Yoshida, A. Taninaka, Y. Sugita, T. Katayama, O. Takeuchi, and H. Shigekawa
    • Journal Title

      ACS Nano

      Volume: 2016, 10 Issue: 12 Pages: 11211-11218

    • DOI

      10.1021/acsnano.6b06278

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Presentation] sub-ps Snapshot of Electron Dynamics in an Organic Thin Film Captured by THz-STM2019

    • Author(s)
      S. Yoshida, Y. Arashida, H. Hirori, T. Tachizaki, H. Ueno, I. Igarashi, Y. Shinomiya, O.Takeuchi, and H. Shigekawa
    • Organizer
      27th International Colloquium on Scanning Probe Microscopy
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 時間分解THz-STMによる光誘起ダイナミクスの計測2019

    • Author(s)
      吉田昭二, 廣理英基, 立崎武弘, 嵐田雄介, 吉岡克将, 四ノ宮慶保, 上野寛輝, 五十嵐一歩, 武内修, 重川秀実
    • Organizer
      日本表面真空学会学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Ultrafast photo-induced dynamics probed by time resolved THz-STM2018

    • Author(s)
      S. Yoshida, H. Hirori, T. Tachizaki, O. Takeuchi, H. Shigekawa
    • Organizer
      2018 International Conference on Nanoscience + Technology
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Revealing the conformational dynamics in a single-molecule junction by site- and angle resolved dynamic probe method2018

    • Author(s)
      S. Yoshida, T. Atsushi, Y. Sugita, O. Takeuchi, H. Shigekawa
    • Organizer
      2018 International Conference on Nanoscience + Technology
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Ultrafast dynamics at surfaces probed by time resolved THz-STM2018

    • Author(s)
      Shoji Yoshida, Hideki Hirori, Takehiro Tachizaki, Satoki Nagai, Yoshiyasu Shinomiya, Hiroki Ueno, Osamu Takeuchi and Hidemi Shigekawa
    • Organizer
      14th International Conference on Atomically Controlled Surfaces, Interfaces and Nanostructures
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 時間分解 THz-STM による光誘起ダイナミクスの計測2018

    • Author(s)
      吉田昭二
    • Organizer
      2018年日本真空表面学会学術講演会
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] 時間分解STMの開発と光励起ダイナミクス計測2018

    • Author(s)
      吉田昭二
    • Organizer
      第2回日本表面科学会プローブ顕微鏡研究部会 合同シンポジウム
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] MoS2単原子層中Reドーパントの局所電子状態のSTM/STS計測2018

    • Author(s)
      吉田昭二、吉村真太郎、竹内高広、本田周太、植田暁子、武内修、宮田耕充、重川秀実
    • Organizer
      第65回応用物理学会春季学術講演会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 高強度THzパルスを用いた時間分解STMの開発2017

    • Author(s)
      廣理英基、吉田昭二、立崎武弘、長井聡紀、重川秀実
    • Organizer
      2017年 第64回応用物理学会春季学術講演会
    • Place of Presentation
      パシフィコ横浜、神奈川県、横浜市
    • Year and Date
      2017-03-14
    • Related Report
      2016 Annual Research Report
  • [Presentation] 時間分解走査トンネル顕微鏡の開発と展望2016

    • Author(s)
      吉田 昭二, Zi-han Wang, 武内 修, 重川 秀実
    • Organizer
      2016年 第77回応用物理学会秋季学術講演会
    • Place of Presentation
      朱鷺メッセ、新潟市、新潟県
    • Year and Date
      2016-09-13
    • Related Report
      2016 Annual Research Report
    • Invited

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Published: 2016-04-21   Modified: 2021-02-19  

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