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Development of resonant soft x-ray small-angle scattering method for observing magnetic texture

Research Project

Project/Area Number 16H05990
Research Category

Grant-in-Aid for Young Scientists (A)

Allocation TypeSingle-year Grants
Research Field Quantum beam science
Research InstitutionNational Institute for Materials Science (2017-2018)
The University of Tokyo (2016)

Principal Investigator

Yamasaki Yuichi  国立研究開発法人物質・材料研究機構, 統合型材料開発・情報基盤部門, 主任研究員 (70571610)

Project Period (FY) 2016-04-01 – 2019-03-31
Project Status Completed (Fiscal Year 2018)
Budget Amount *help
¥16,900,000 (Direct Cost: ¥13,000,000、Indirect Cost: ¥3,900,000)
Fiscal Year 2018: ¥1,820,000 (Direct Cost: ¥1,400,000、Indirect Cost: ¥420,000)
Fiscal Year 2017: ¥3,120,000 (Direct Cost: ¥2,400,000、Indirect Cost: ¥720,000)
Fiscal Year 2016: ¥11,960,000 (Direct Cost: ¥9,200,000、Indirect Cost: ¥2,760,000)
Keywords共鳴X線散乱 / 磁気イメージング / コヒーレント回折イメージング / 磁気スキルミオン / 量子ビーム / 共鳴軟X線散乱 / マルチフェロイクス
Outline of Final Research Achievements

The purpose of this study was to observe nanometer-scale vortex-like magnetic structures called magnetic skyrmions by means of resonant soft x-ray small-angle scattering. Resonant soft x-ray scattering is an element-selective method that can observe the magnetic state by using soft x-rays of energy corresponding to the absorption edge of the target element. Using this method, we observed how magnetic skyrmions are generated and annihilated by an application of external electric field, and how magnetic structures change from magnetic skyrmions to magnetic chiral soliton lattices by tensile strain from the substrate. We also succeeded in reconstructing a real space image element-selectively with a spatial resolution of several tens of nanometers by a phase retrieval algorithm from a diffraction pattern obtained using coherent soft x-rays.

Academic Significance and Societal Importance of the Research Achievements

磁気スキルミオンはトポロジカルに安定な構造であるためスピントロニクスデバイスなどへの応用が期待されている。その特性を理解し性能を向上させるためには、デバイスが駆動している状態で磁気スキルミオンの挙動を観測し解明することが求められる。本研究で確立した共鳴軟X線小角散乱法は、動作状態での磁気スキルミオンを観測するのに適した手法であり、スピントロニクス材料の開発やデバイスのオペランド計測において強力な先端計測手法になり得ることを示せた。

Report

(4 results)
  • 2018 Annual Research Report   Final Research Report ( PDF )
  • 2017 Annual Research Report
  • 2016 Annual Research Report
  • Research Products

    (39 results)

All 2019 2018 2017 2016 Other

All Int'l Joint Research (2 results) Journal Article (13 results) (of which Int'l Joint Research: 3 results,  Peer Reviewed: 12 results,  Open Access: 3 results,  Acknowledgement Compliant: 1 results) Presentation (24 results) (of which Int'l Joint Research: 1 results,  Invited: 23 results)

  • [Int'l Joint Research] ポール・シェラー研究所(PSI)(スイス)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] CELLS, ALBA(スペイン)

    • Related Report
      2018 Annual Research Report
  • [Journal Article] Element-specific soft x-ray spectroscopy, scattering, and imaging studies of the skyrmion-hosting compound Co8Zn8Mn42019

    • Author(s)
      Ukleev V.、Yamasaki Y.、Morikawa D.、Karube K.、Shibata K.、Tokunaga Y.、Okamura Y.、Amemiya K.、Valvidares M.、Nakao H.、Taguchi Y.、Tokura Y.、Arima T.
    • Journal Title

      Physical Review B

      Volume: 99 Issue: 14 Pages: 144408-144408

    • DOI

      10.1103/physrevb.99.144408

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Sparse Phase Retrieval Algorithm for Observing Isolated Magnetic Skyrmions by Coherent Soft X-ray Diffraction Imaging2019

    • Author(s)
      Yokoyama Yuichi、Arima Taka-hisa、Okada Masato、Yamasaki Yuichi
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 88 Issue: 2 Pages: 024009-024009

    • DOI

      10.7566/jpsj.88.024009

    • NAID

      210000135093

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Charge disproportionation of Mn 3d and O 2p electronic states depending on strength of p?d hybridization in (LaMnO3)2(SrMnO3)2 superlattices2018

    • Author(s)
      Nakao Hironori、Tabata Chihiro、Murakami Youichi、Yamasaki Yuichi、Yamada Hiroyuki、Ishihara Sumio、Kawasaki Masashi
    • Journal Title

      Physical Review B

      Volume: 98 Issue: 24 Pages: 245146-245146

    • DOI

      10.1103/physrevb.98.245146

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Tensile-Strain-Dependent Spin States in Epitaxial LaCoO3 Thin Films2018

    • Author(s)
      Yokoyama Y.、Yamasaki Y.、Taguchi M.、Hirata Y.、Takubo K.、Miyawaki J.、Harada Y.、Asakura D.、Fujioka J.、Nakamura M.、Daimon H.、Kawasaki M.、Tokura Y.、Wadati H.
    • Journal Title

      Physical Review Letters

      Volume: 120 Issue: 20 Pages: 206402-206402

    • DOI

      10.1103/physrevlett.120.206402

    • NAID

      120006490174

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Commensurate versus incommensurate charge ordering near the superconducting dome in Ir1-xPtxTe2 revealed by resonant x-ray scattering2018

    • Author(s)
      Takubo K.、Yamamoto K.、Hirata Y.、Wadati H.、Mizokawa T.、Sutarto R.、He F.、Ishii K.、Yamasaki Y.、Nakao H.、Murakami Y.、Matsuo G.、Ishii H.、Kobayashi M.、Kudo K.、Nohara M.
    • Journal Title

      Physical Review B

      Volume: 97 Issue: 20 Pages: 1-9

    • DOI

      10.1103/physrevb.97.205142

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Coherent Resonant Soft X-ray Scattering Study of Magnetic Textures in FeGe2018

    • Author(s)
      V. Ukleev, Y. Yamasaki, D. Morikawa, N. Kanazawa, Y. Okamura, H. Nakao, Y. Tokura, and T. Arima
    • Journal Title

      Quantum Beam Sci.

      Volume: 2 Issue: 1 Pages: 3-3

    • DOI

      10.3390/qubs2010003

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Thickness dependence and dimensionality effects on charge and magnetic orderings in La1/3Sr2/3FeO3 thin films2018

    • Author(s)
      K. Yamamoto, Y. Hirata, M. Horio, Y. Yokoyama, K. Takubo, M. Minohara, H. Kumigashira, Y. Yamasaki, H. Nakao, Y. Murakami, A. Fujimori, and H. Wadati
    • Journal Title

      Phys. Rev. B

      Volume: 97 Issue: 7 Pages: 75134-75134

    • DOI

      10.1103/physrevb.97.075134

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Emergence and magnetic-field variation of chiral-soliton lattice and skyrmion lattice in the strained helimagnet Cu2OSeO32017

    • Author(s)
      Y. Okamura, Y. Yamasaki, D. Morikawa, T. Honda, V. Ukleev, H. Nakao, Y. Murakami, K. Shibata, F. Kagawa, S. Seki, T. Arima, and Y. Tokura
    • Journal Title

      Phys. Rev. B

      Volume: 96 Issue: 17 Pages: 174417-174417

    • DOI

      10.1103/physrevb.96.174417

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] High-pressure synthesis of an unusual antiferromagnetic metal CaCoO3 with GdFeO3-type perovskite structure.2017

    • Author(s)
      T. Osaka, H. Takahashi, H. Sagayama, Y. Yamasaki, S. Ishiwata
    • Journal Title

      PHYSICAL REVIEW B.

      Volume: 95 Issue: 22 Pages: 224440-224440

    • DOI

      10.1103/physrevb.95.224440

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Spin State of Co3+ in LaCo1-xRhxO3 Studied Using X-ray Absorption Spectroscopy2017

    • Author(s)
      T. Sudayama, H. Nakao, Y. Yamasaki, Y. Murakami, S. Asai, R. Okazaki, Y. Yasui, and I. Terasaki
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 86 Issue: 9 Pages: 94701-94701

    • DOI

      10.7566/jpsj.86.094701

    • NAID

      210000134503

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Role of commensurability of spin order for optical magnetoelectric effect with electromagnons in multiferroic YMn2O5.2017

    • Author(s)
      R. Masuda, Y. Kaneko, Y. Yamasaki, Y. Tokura, Y. Takahashi
    • Journal Title

      PHYSICAL REVIEW B.

      Volume: 96 Issue: 4 Pages: 41117-41117

    • DOI

      10.1103/physrevb.96.041117

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] 共鳴軟X線回折法の新展開2017

    • Author(s)
      山崎裕一、中尾裕則
    • Journal Title

      日本放射光学会誌

      Volume: 30 Pages: 3-12

    • NAID

      40021076126

    • Related Report
      2016 Annual Research Report
  • [Journal Article] Directional electric-field induced transformation from skyrmion lattice to distinct helices in multiferroic Cu 2OSeO 32017

    • Author(s)
      Y. Okamura, Y. Yamasaki, D. Morikawa, T. Honda, V. Ukleev, H. Nakao, Y. Murakami, K. Shibata, F. Kagawa, S. Seki, T. Arima , and Y. Tokura
    • Journal Title

      Physical Review B

      Volume: 印刷中

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Presentation] コヒーレント軟X線回折とスパース位相回復法による磁気イメージング2019

    • Author(s)
      山崎 裕一
    • Organizer
      2019年顕微ナノ・表面科学・SPM合同シンポジウム
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] コヒーレント軟X線回折による磁気イメージングとスパース位相回復法2019

    • Author(s)
      山崎 裕一
    • Organizer
      2018年度量子ビームサイエンスフェスタ
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] スパース位相回復法によるコヒーレント軟X線回折磁気イメージング2018

    • Author(s)
      山崎裕一
    • Organizer
      日本結晶学会年会シンポジウム
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] 共鳴軟 X 線散乱による磁気スキルミオンの外場制御と実空間観測2018

    • Author(s)
      山崎裕一
    • Organizer
      平成30年度磁性材料研究会
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] スパースモデリングを活用したコヒーレント軟X線回折イメージング2018

    • Author(s)
      山崎裕一
    • Organizer
      東京大学物性研LASORセミナー
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] コヒーレント軟 X 線回折イメージングデータからの磁気構造の情報抽出2018

    • Author(s)
      山崎裕一
    • Organizer
      日本分析化学会第 67 年会特別シンポジウム
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] スパースモデリングを活用したコヒーレント軟X線回折磁気イメージング2018

    • Author(s)
      山崎裕一
    • Organizer
      放射光学会若手研究会「放射光科学Xインフォマティクス」
    • Related Report
      2018 Annual Research Report
  • [Presentation] コヒーレント軟X線回折イメージングとインフォマティクスの融合2018

    • Author(s)
      山崎裕一
    • Organizer
      PF研究会「量子ビームと新規合成手法の融合による酸化物の新機能探索」
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] スパースモデリングを用いたコヒーレント回折イメージング2018

    • Author(s)
      山崎裕一
    • Organizer
      先端ナノデバイス・材料テクノロジー第151委員会
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] スパース位相回復法によるコヒーレント軟X線回折磁気イメージング2018

    • Author(s)
      山崎裕一
    • Organizer
      顕微鏡学会超高分解能研究会
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] スパース位相回復法によるコヒーレント軟X線回折磁気イメージング2018

    • Author(s)
      山崎裕一
    • Organizer
      NIMS MI・計測合同シンポジウム
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] 共鳴軟X線小角散乱による超伝導磁束格子観測の可能性2018

    • Author(s)
      山崎裕一
    • Organizer
      つくば-柏-本郷超伝導かけはしプロジェクトワークショップ
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] スパース位相回復法による磁気イメージング2017

    • Author(s)
      山崎裕一
    • Organizer
      物質・材料研究機構/九州シンクロトロン光研究センター合同シンポジ
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] 共鳴軟X線回折による薄膜試料の電子状態観測2017

    • Author(s)
      山崎裕一
    • Organizer
      2017年応用物理学会秋季学術講演会
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] 共鳴軟X線回折による磁気構造の観察2017

    • Author(s)
      山崎裕一
    • Organizer
      日本物理学会2017年秋季大会
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] スパース位相回復法を用いた磁気イメージング2017

    • Author(s)
      山崎裕一
    • Organizer
      第271回第271回 SPring-8セミナー
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] スパース位相回復法による磁気イメージング2017

    • Author(s)
      山崎裕一
    • Organizer
      第4回放射光連携研究ワークショップ
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] スパース位相回復法を用いた磁気イメージング2017

    • Author(s)
      山崎裕一
    • Organizer
      情報理論を用いた原子・電子構造のインタースケールイメージング~位
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] 共鳴軟X線小角散乱による磁気テクスチャの観測2017

    • Author(s)
      山崎裕一
    • Organizer
      第30回日本放射光学会年会放射光科学合同シンポジウム
    • Related Report
      2017 Annual Research Report 2016 Annual Research Report
    • Invited
  • [Presentation] 共鳴軟X線コヒーレント回折イメージングの現状と展開2017

    • Author(s)
      山崎裕一
    • Organizer
      PF研究会「PF挿入光源ビームラインBL-19の戦略的利用に関する研究会
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] コヒーレント軟X線共鳴回折による磁気イメージング2017

    • Author(s)
      山崎裕一
    • Organizer
      SLiT-Jイメージングエンドステーションに関する ミニワークショップ
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] コヒーレント共鳴軟X線散乱による磁気テクスチャの観測2017

    • Author(s)
      山崎裕一
    • Organizer
      ISSP-Workshop SPring-8 BL07LSUが 照らしだす物質機能の起源
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] 共鳴軟X線回折による表面・界面電子秩序観測の現状と展望2017

    • Author(s)
      山崎裕一
    • Organizer
      科学研究費基盤A研究会「酸化物薄膜界面の異方的磁性とスピン-軌道結
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] Topological spin texture in chiral magnets as seen via small-angle resonant soft x-ray diffraction2016

    • Author(s)
      山崎裕一
    • Organizer
      REXS2016
    • Place of Presentation
      ドイツ ハンブルク
    • Year and Date
      2016-06-13
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited

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Published: 2016-04-21   Modified: 2020-03-30  

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