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Improvement of formability of wood impregnated with various chemicals using electromagnetic waves aiming at activation of molecule mobility

Research Project

Project/Area Number 16H06122
Research Category

Grant-in-Aid for Young Scientists (A)

Allocation TypeSingle-year Grants
Research Field Material processing/Microstructural control engineering
Research InstitutionNational Institute of Advanced Industrial Science and Technology

Principal Investigator

Tsunehisa Miki  国立研究開発法人産業技術総合研究所, 材料・化学領域, 主任研究員 (20415748)

Project Period (FY) 2016-04-01 – 2020-03-31
Project Status Completed (Fiscal Year 2019)
Budget Amount *help
¥23,530,000 (Direct Cost: ¥18,100,000、Indirect Cost: ¥5,430,000)
Fiscal Year 2019: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Fiscal Year 2018: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Fiscal Year 2017: ¥9,490,000 (Direct Cost: ¥7,300,000、Indirect Cost: ¥2,190,000)
Fiscal Year 2016: ¥10,920,000 (Direct Cost: ¥8,400,000、Indirect Cost: ¥2,520,000)
Keywords木材 / 塑性加工 / 複合材料 / 組織変化 / 電磁波 / 界面 / 誘電加熱 / 物性 / 流動 / 微細構造 / 木材・木質材料 / 流動性 / 誘電特性 / 局所物性 / 熱物性 / 材料科工・処理 / バイオマス / 誘電体物性 / 高分子構造・物性 / 変形能 / 超塑性 / 高周波 / 変形 / 流動成形
Outline of Final Research Achievements

This study aimed at developing novel plastic forming of resin-impregnated wood composites using their fluidity by introducing electromagnetic waves. Especially, feasibility of rapid production process of the plastic forming of those wood product have been experimentally explored. Based on the dielectric properties of resin-impregnated wood, impregnated wood with higher dielectric loss showed a rapid dielectric heating from inside of the material, and meantime, the deformability was improved. A scanning probe microscopy showed the existence of the resin among cellulose microfibril aggregates in the wood cell and intercellular region. These resin might contribute the improvement of cell-cell deformation as well as intra-cell deformations of the impregnated wood.
By this fundamental approach for applying a dielectric heating onto the metal mold system, problems associate with isolation structure and motions of the metal mold parts were addressed.

Academic Significance and Societal Importance of the Research Achievements

本研究で着目した木質流動成形技術は、木質系素材の変形能を利用した賦形技術であり、汎用の塑性加工(鍛造)用金型とプレス装置があれば、自由な形状へバルク状木材を比較的短時間で成形加工できる。さらに樹脂含浸を併用すれば、木材の高強度化や寸法安定化などの機能化も同時に達成できる。この技術を実用化すれば、日本国内に賦存する木質資源から効率的に、且つ、高付加価値で炭素固定に寄与する伐採木材製品へと転換することができ、環境・経済面を両立する技術の創出につながる。この成果は、持続的社会の形成という大目標のなかで、地下資源由来技術に取って代わることのできる地上木質資源の工業的利活用の促進に大きく貢献できる。

Report

(5 results)
  • 2019 Annual Research Report   Final Research Report ( PDF )
  • 2018 Annual Research Report
  • 2017 Annual Research Report
  • 2016 Annual Research Report
  • Research Products

    (19 results)

All 2020 2019 2018 2017 Other

All Int'l Joint Research (1 results) Journal Article (12 results) (of which Peer Reviewed: 12 results,  Open Access: 7 results) Presentation (5 results) (of which Int'l Joint Research: 2 results,  Invited: 3 results) Patent(Industrial Property Rights) (1 results) (of which Overseas: 1 results)

  • [Int'l Joint Research] Empa/ETH(スイス)

    • Related Report
      2019 Annual Research Report
  • [Journal Article] Influence of Electron-beam Irradiation on Plastic Flow Deformation of Wood2020

    • Author(s)
      Sugino Hideaki、Tanaka Soichi、Kasamatsu Yuga、Okubayashi Satoko、Seki Masako、Miki Tsunehisa、Umemura Kenji、Kanayama Kozo
    • Journal Title

      Mokuzai Gakkaishi

      Volume: 66 Issue: 2 Pages: 59-66

    • DOI

      10.2488/jwrs.66.59

    • NAID

      130007837005

    • ISSN
      0021-4795, 1880-7577
    • Year and Date
      2020-04-25
    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Variable temperature solid-state NMR spectral and relaxation analyses of the impregnation of polyethylene glycol (PEG) into coniferous wood2019

    • Author(s)
      Nishida Masakazu、Tanaka Tomoko、Miki Tsunehisa、Shigematsu Ichinori、Kanayama Kozo
    • Journal Title

      RSC Advances

      Volume: 9 Issue: 27 Pages: 15657-15667

    • DOI

      10.1039/c9ra01848d

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Integrated analysis of modified Japanese cypress using solid-state NMR spectra and nuclear magnetic relaxation times2019

    • Author(s)
      Nishida Masakazu、Tanaka Tomoko、Miki Tsunehisa、Hayakawa Yoshio、Kanayama Kozo
    • Journal Title

      Cellulose

      Volume: 26 Issue: 6 Pages: 3625-3642

    • DOI

      10.1007/s10570-019-02330-2

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Effects of resin content and precompression treatment on bulk bamboo extrusion2019

    • Author(s)
      Seki Masako、Yashima Yuko、Miki Tsunehisa、Kiryu Tomoaki、Tanaka Soichi、Kanayama Kozo
    • Journal Title

      International Journal of Material Forming

      Volume: - Issue: 3 Pages: 331-339

    • DOI

      10.1007/s12289-019-01497-0

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Influence of pulsive pressure waves on liquid penetration into wood in semi-opened container2019

    • Author(s)
      Tanaka Soichi、Seki Masako、Miki Tsunehisa、Umemura Kenji、Kanayama Kozo
    • Journal Title

      Journal of Wood Science

      Volume: 65 Issue: 1

    • DOI

      10.1186/s10086-019-1832-2

    • NAID

      120006898050

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Influence on Wood Color of Relative Humidity in Conditioning Process of Dye-Aqueous Solution Impregnated Wood2018

    • Author(s)
      田中聡一、杉野秀明、関雅子、三木恒久、梅村研二、金山公三
    • Journal Title

      Journal of the Society of Materials Science, Japan

      Volume: 67 Issue: 8 Pages: 767-772

    • DOI

      10.2472/jsms.67.767

    • NAID

      130007437250

    • ISSN
      0514-5163, 1880-7488
    • Year and Date
      2018-08-15
    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Instrumental analyses of nanostructures and interactions with bound water of superheated steam treated plant materials2018

    • Author(s)
      M. Nishida, T. Tanaka, T. Miki, T. Ito, K. Kanayama
    • Journal Title

      Industrial Crops and Products

      Volume: 114 Pages: 1-13

    • DOI

      10.1016/j.indcrop.2018.01.072

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Visualization of solute diffusion into cell walls in solution-impregnated wood under varying relative humidity using time-of-flight secondary ion mass spectrometry2018

    • Author(s)
      P. Zheng, D. Aoki, M. Seki, T. Miki, S. Tanaka, K. Kanayama, Y. Matsushita & K. Fukushima
    • Journal Title

      Scientific Reports

      Volume: 8 Issue: 1 Pages: 9819-9819

    • DOI

      10.1038/s41598-018-28230-2

    • NAID

      120006489936

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] 木質系材料を用いた塑性加工技術2018

    • Author(s)
      三木 恒久
    • Journal Title

      ぷらすとす

      Volume: 1 Pages: 20-25

    • NAID

      130007802458

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Instrumental analyses of nanostructures and interactions with water molecules of biomass constituents of Japanese cypress2017

    • Author(s)
      Nishida Masakazu、Tanaka Tomoko、Miki Tsunehisa、Hayakawa Yoshio、Kanayama Kozo
    • Journal Title

      Cellulose

      Volume: 24 Issue: 12 Pages: 5295-5312

    • DOI

      10.1007/s10570-017-1507-3

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Solute diffusion into cell walls in solution-impregnated wood under conditioning process IV: effect of temperature on solute diffusivity2017

    • Author(s)
      Tanaka Soichi、Seki Masako、Miki Tsunehisa、Umemura Kenji、Kanayama Kozo
    • Journal Title

      Journal of Wood Science

      Volume: 63 Issue: 6 Pages: 644-651

    • DOI

      10.1007/s10086-017-1658-8

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Integrated analysis of solid-state NMR spectra and nuclear magnetic relaxation times for the phenol formaldehyde (PF) resin impregnation process into soft wood2017

    • Author(s)
      Nishida Masakazu、Tanaka Tomoko、Miki Tsunehisa、Hayakawa Yoshio、Kanayama Kozo
    • Journal Title

      RSC Advances

      Volume: 7 Issue: 86 Pages: 54532-54541

    • DOI

      10.1039/c7ra11295e

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Presentation] Fluidity of Bulk Bamboo Impregnated with Phenol Formaldehyde (PF) Resin2018

    • Author(s)
      M. Seki, Y. Yashima, T. Kiryu, T. Miki, S. Tanaka, K. Kanayama
    • Organizer
      2018 Joint Convention SWST & JWRS
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Esterification of Solid Wood for Plastic Forming Process2018

    • Author(s)
      Y. Enomoto, M. Abe, T. Miki, M. Seki
    • Organizer
      2018 Joint Convention SWST & JWRS
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 快適なモビリティ空間に資する木質素材の利用を考える2018

    • Author(s)
      三木恒久
    • Organizer
      日本塑性加工学会関西支部 平成 30 年度 関西支部 若手技術交流会 (兼 関西支部 第 36 回先端塑性加工技術コロキウム)
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] 木質系材料の高信頼性・高付加価値化を実現する三次元成形加工技術2017

    • Author(s)
      三木恒久
    • Organizer
      科学技術振興機構(JST)新技術説明会
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] 木質バイオマス素材の固相流動現象による成形技術(流動成形の開発)2017

    • Author(s)
      三木 恒久
    • Organizer
      京都大学生存圏研究所 第217回定例オープンセミナー
    • Place of Presentation
      京都大学生存圏研究所
    • Related Report
      2016 Annual Research Report
    • Invited
  • [Patent(Industrial Property Rights)] 改質木材とその製造方法並びにその成形体2018

    • Inventor(s)
      榎本有希子、三木恒久、関雅子
    • Industrial Property Rights Holder
      榎本有希子、三木恒久、関雅子
    • Industrial Property Rights Type
      特許
    • Filing Date
      2018
    • Related Report
      2018 Annual Research Report
    • Overseas

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Published: 2016-04-21   Modified: 2021-02-19  

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