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Intelligent Design of Layered Materials Surface for Spintronics

Research Project

Project/Area Number 16J01006
Research Category

Grant-in-Aid for JSPS Fellows

Allocation TypeSingle-year Grants
Section国内
Research Field Thin film/Surface and interfacial physical properties
Research InstitutionAkashi National College of Technology (2017)
Osaka University (2016)

Principal Investigator

Arguelles Elvis Flaviano (2017)  明石工業高等専門学校, その他部局等, 特別研究員(PD) (50816072)

ARGUELLES ELVIS FLAVIANO (2016)  大阪大学, 工学研究科, 特別研究員(DC2)

Project Period (FY) 2016-04-22 – 2018-03-31
Project Status Completed (Fiscal Year 2017)
Budget Amount *help
¥1,700,000 (Direct Cost: ¥1,700,000)
Fiscal Year 2017: ¥800,000 (Direct Cost: ¥800,000)
Fiscal Year 2016: ¥900,000 (Direct Cost: ¥900,000)
Keywordsgraphene / nanosheet / magnetic atom / magnetic exchange / nuclear spin / metal surface / charge carriers / layered oxide / spintronics
Outline of Annual Research Achievements

This year, the adsorption and absorption of magnetic atoms represented by Co on bilayer graphene nanosheets and the second is the interaction of gas molecules on the surface of metal electrodes. It is found that the crystal fields with C3v symmetry split the Co’s 3d orbitals into two doubly degenerate irreducible representations E1 (dxz,dyz) and E2 (dx2-y2,dxy) and a one-dimensional representation A1(d3z2-r2). Further, the estimated magnetic exchange interactions exhibit ferromagnetic exchange coupling between the localized spins of Co.

To model the simplest molecule-surface interactions, H2 adsorption on Pd(210) has been investigated. It is found that H2 is in the molecularly chemisorbed state and the adsorption is characterized by a highly anisotropic potential energy surface. Rotational-vibrational calculations show that two lowest bound state levels belong to J=0 and 1 species, respectively. It is further known that H2 adsorbates drastically affect the electronic properties of the metal surface. Since H2 can practically be separated into two nuclear spin isomers, nuclear spin states interconversion is found to proceed at a very fast rate on Pd(210).This results to a molecule in a different nuclear spin state and a magnetic metal surface.

The accounts of this research have been published to international scientific journals and presented in numerous domestic and international conferences.

Research Progress Status

29年度が最終年度であるため、記入しない。

Strategy for Future Research Activity

29年度が最終年度であるため、記入しない。

Report

(2 results)
  • 2017 Annual Research Report
  • 2016 Annual Research Report
  • Research Products

    (15 results)

All 2018 2017 2016

All Journal Article (4 results) (of which Int'l Joint Research: 4 results,  Peer Reviewed: 4 results,  Open Access: 1 results) Presentation (11 results) (of which Int'l Joint Research: 3 results,  Invited: 3 results)

  • [Journal Article] Rotational state modification and fast ortho-para conversion of H2 trapped within the highly anisotropic potential of Pd(210)2018

    • Author(s)
      Satoshi Ohno, Dmitry Ivanov, Shohei Ogura, Markus Wilde, Elvis Flaviano Arguelles, Wilson Agerico Dino, Hideaki Kasai, Katsuyuki Fukutani
    • Journal Title

      Physical Review B

      Volume: 97 Issue: 8 Pages: 085436-085436

    • DOI

      10.1103/physrevb.97.085436

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Hindered rotation and nuclear spin isomers separation of molecularly chemisorbed H2 on Pd(210)2018

    • Author(s)
      Arguelles Elvis F.、Kasai Hideaki
    • Journal Title

      Journal of Applied Physics

      Volume: 123 Issue: 11 Pages: 115301-115301

    • DOI

      10.1063/1.5021994

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Bound nuclear spin states of H2 in an anisotropic potential induced by a stepped metal surface2018

    • Author(s)
      Arguelles Elvis F.、Kasai Hideaki
    • Journal Title

      Journal of Vacuum Science & Technology A: Vacuum, Surfaces, and Films

      Volume: 36 Issue: 3 Pages: 030601-030601

    • DOI

      10.1116/1.5023158

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Optical control of magnetization dynamics in Gd-Fe-Co films with different compositions2017

    • Author(s)
      Takuo Ohkochi, Hidenori Fujiwara, Masato Kotsugi, Hirokazu Takahashi, Roman Adam, Akira Sekiyama, Tetsuya Nakamura, Arata Tsukamoto, Claus M. Schneider, Hiroto Kuroda, Elvis F. Arguelles, Mamoru Sakaue, Hideaki Kasai, Masakiyo Tsunoda, Shigemasa Suga, and Toyohiko Kinoshita
    • Journal Title

      Applied Physics Express

      Volume: 10 Issue: 10 Pages: 1030021-4

    • DOI

      10.7567/apex.10.103002

    • NAID

      210000135995

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Presentation] H2 Adsorption on Pd(210): Nuclear Spin Isomer Separation and Conversion2017

    • Author(s)
      Elvis F. Arguelles, Wilson Agerico Dino, Hideaki Kasai
    • Organizer
      64th Japan Society of Applied Physics Conference
    • Place of Presentation
      Pacifico Yokohama, Yokohama, Japan
    • Year and Date
      2017-03-14
    • Related Report
      2016 Annual Research Report
  • [Presentation] Hindered Rotation and Ortho-Para Conversion of H2 on Pd(210) Surface2017

    • Author(s)
      Elvis F. Arguelles, Wilson Agerico Dino, Hideaki Kasai
    • Organizer
      Symposium of Surface Science and Nanotechnology, 25th Anniversary of SSJ Kansai
    • Place of Presentation
      Kyoto International Community House, Kyoto, Japan
    • Year and Date
      2017-01-24
    • Related Report
      2016 Annual Research Report
  • [Presentation] H2 Adsorption on Pd(210) Surface: Nuclear Spin Species Separation and Conversion2017

    • Author(s)
      Elvis F. Arguelles, Wilson Agerico Dino, Hideaki Kasai
    • Organizer
      The International Symposium of “Recent Trends in Analysis and Techniques of Functional Materials”
    • Place of Presentation
      Osaka University, Osaka, Japan
    • Year and Date
      2017-01-18
    • Related Report
      2016 Annual Research Report
    • Invited
  • [Presentation] Interstital impurity induced magnetism on lead oxide surface2017

    • Author(s)
      Arguelles E F, Amino S, Aspera S, Nakanishi H, Kasai H, Dino W A
    • Organizer
      European Conference on Surface Science (ECOSS33)
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Nuclear bound states of H2 on a stepped metal surface2017

    • Author(s)
      Arguelles E F, Kasai H, Fukutani K, Yajima A, Nakayama K, Yamashita S, Dino W A
    • Organizer
      European Conference on Surface Science (ECOSS33)
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Bound nuclear spin states of H2 on a stepped metal surface2017

    • Author(s)
      Elvis F. Arguelles, Hiroshi Nakanishi, Hideaki Kasai, Katsuyuki Fukutani, Wilson Agerico Dino
    • Organizer
      9th Asian Computational Materials Design (CMD Asia) Workshop
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] H2 nuclear spin isomer transition on a stepped metal surface2017

    • Author(s)
      Elvis F. Arguelles, Hiroshi Nakanishi, Hideaki Kasai, Katsuyuki Fukutani, Wilson Agerico Dino
    • Organizer
      2017 Fall Meeting, Japan Physical Society (JPS)
    • Related Report
      2017 Annual Research Report
  • [Presentation] Interstitial impurity-induced magnetism in a layered oxide surface2017

    • Author(s)
      E. Arguelles S. Amino, S. Aspera, H. Nakanishi and H. Kasai
    • Organizer
      78th Japan Society of Applied Physics (JSAP) Autumn Meeting
    • Related Report
      2017 Annual Research Report
  • [Presentation] Nuclear Spin Separation and Conversion of H2 on Stepped Metal Surface2016

    • Author(s)
      Elvis F. Arguelles, Wilson Agerico Dino, Hideaki Kasai
    • Organizer
      8th Asian Computational Materials Design (CMD) Workshop
    • Place of Presentation
      De La Salle University, Manila, Philippines
    • Year and Date
      2016-09-21
    • Related Report
      2016 Annual Research Report
    • Invited
  • [Presentation] Nuclear Spin States of H2 Adsorbed on Pd(210) Surface2016

    • Author(s)
      Elvis F. Arguelles, Wilson Agerico Dino, Hideaki Kasai
    • Organizer
      Japan Physical Society Conference, Autumn Meeting
    • Place of Presentation
      Kanazawa University, Kanazawa, Japan
    • Year and Date
      2016-09-13
    • Related Report
      2016 Annual Research Report
  • [Presentation] Revisiting H2 Adsorption on Pd(210): Nuclear Spin States Separation and Conversion2016

    • Author(s)
      Elvis F. Arguelles, Wilson Agerico Dino, Hideaki Kasai
    • Organizer
      32nd European Conference on Surface Science (ECOSS 32)
    • Place of Presentation
      Grenoble, France
    • Year and Date
      2016-08-28
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research

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Published: 2016-05-17   Modified: 2024-03-26  

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