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Ultrafast dynamics and resonance effects in photoemission from surfaces

Research Project

Project/Area Number 16K05393
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Condensed matter physics I
Research InstitutionChiba University

Principal Investigator

Krueger Peter  千葉大学, 大学院工学研究院, 教授 (30706362)

Project Period (FY) 2016-04-01 – 2020-03-31
Project Status Discontinued (Fiscal Year 2019)
Budget Amount *help
¥4,680,000 (Direct Cost: ¥3,600,000、Indirect Cost: ¥1,080,000)
Fiscal Year 2019: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2018: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Fiscal Year 2017: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2016: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Keywords光物性 / 表面 / 界面 / 表面・界面 / 表面・界面物性
Outline of Final Research Achievements

In this project we have made good progress in the understanding of the photoemission process for (1) time delay and (2) resonance effect upon core-level excitation. (1) By directly comparing the solution of the time-dependent Schroedinger equation with a multiple scattering calculation in a one-dimensional model, we have shown how Wigner delay theory can be generalized from atoms to solids. Second, we have explained the oscillations of the time delay as a function of energy, observed in photoemission from Cu, by ab initio calculations [Optica 4, 1492]. (2) We have developed a theory and computer code for angle-resolved photoemission/photoelectron diffraction at core-level resonances of 3d metals by combining atomic multiplet theory and multiple scattering [J.Phys.Soc.Jpn 87, 061007]. We have fully reproduced the experimental resonant photoemission spectra of Ni(111), and have explained the recent, first observation of the Daimon effect in resonant photoelectron diffraction.

Academic Significance and Societal Importance of the Research Achievements

超高速原子・電子現象の研究は、物質の基本的な動的過程を理解する上で非常に重要なテーマである。 本プロジェクトでは、そのような超高速過程の一つである1フェムト秒以下で起こる表面からの光電子放出遅延現象についての理論的考察に進展が見られた。さらに、共鳴光電子回折の正確な理論を初めて開発した。この手法により、低消費電力電子デバイスの実現が期待されるスピントロニクス材料の磁気的・電子的状態を調べることができる。

Report

(4 results)
  • 2019 Final Research Report ( PDF )
  • 2018 Annual Research Report
  • 2017 Research-status Report
  • 2016 Research-status Report
  • Research Products

    (24 results)

All 2019 2018 2017 2016

All Journal Article (11 results) (of which Int'l Joint Research: 5 results,  Peer Reviewed: 11 results,  Open Access: 4 results) Presentation (13 results) (of which Int'l Joint Research: 5 results,  Invited: 3 results)

  • [Journal Article] Ab initio calculation of ligand field multiplet parameters for transition metal L-edge spectra2019

    • Author(s)
      Peter Krueger,
    • Journal Title

      Radiat. Phys. Chem.

      Volume: in press Pages: 108051-108051

    • DOI

      10.1016/j.radphyschem.2018.11.005

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Polarization dependent X-ray absorption near-edge spectra of boron nitride nanotubes2019

    • Author(s)
      Peter Krueger, Yuya Maekawa, Adam Hitchcock and Carla Bittencourt
    • Journal Title

      Radiat. Phys. Chem.

      Volume: in press Pages: 108129-108129

    • DOI

      10.1016/j.radphyschem.2019.01.014

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Obtaining the highest molecular orbital peak of organic matter from photoelectron yield spectra2019

    • Author(s)
      Shohei Tadano, Yasuo Nakayama, Hiroumi Kinjo, Hisao Ishii and Peter Krueger
    • Journal Title

      Phys. Rev. Applied

      Volume: 11 Issue: 5 Pages: 054081-054081

    • DOI

      10.1103/physrevapplied.11.054081

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Simple model of the ground state and spin-orbital excitations of free and adsorbed Fe(II) phthalocyanine molecules2018

    • Author(s)
      C. R. Natoli, P. Krueger, Y. Yoshimoto, J. Bartolome and F. Bartolome
    • Journal Title

      Phys. Rev. B

      Volume: 98 Issue: 19 Pages: 195108-195108

    • DOI

      10.1103/physrevb.98.195108

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Direct Observation of Room-Temperature Stable Magnetism in LaAlO3/SrTiO3 Heterostructures2018

    • Author(s)
      M. Yang, J. Zhou, T. C. Asmara, P. Krueger, X. J. Yu, X. Wang, C. Sanchez -Hanke, Y. P. Feng, T. Venkatesan and A. Rusydi
    • Journal Title

      ACS Appl. Mater. Interfaces

      Volume: 10 Issue: 11 Pages: 9774-9781

    • DOI

      10.1021/acsami.7b12945

    • Related Report
      2017 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Photoelectron diffraction from valence states of oriented molecules2018

    • Author(s)
      P. Krueger
    • Journal Title

      J. Phys. Soc. Japan

      Volume: 87 Issue: 6 Pages: 061007-061007

    • DOI

      10.7566/jpsj.87.061007

    • Related Report
      2017 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] A One-Dimensional Model for Photoemission Calculations from Plane-Wave Band Structure Codes2018

    • Author(s)
      R. Ono and P. Krueger
    • Journal Title

      e-Journal of Surface Science and Nanotechnology

      Volume: 16 Issue: 0 Pages: 49-52

    • DOI

      10.1380/ejssnt.2018.49

    • NAID

      130006594522

    • ISSN
      1348-0391
    • Related Report
      2017 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] Multiple scattering approach to photoemission from the highest occupied molecular orbital of pentacene2017

    • Author(s)
      N. Komiya, K. Hatada, F. Ota, P. Krueger, T. Fuijikawa, K. Niki
    • Journal Title

      J. Electron Spectrosc. Related Phenom

      Volume: 220 Pages: 21-24

    • DOI

      10.1016/j.elspec.2017.04.002

    • Related Report
      2017 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Effective mass effect in attosecond electron transport2017

    • Author(s)
      Lamia Kasmi, Matteo Lucchini, Luca Castiglioni, Pavel Kliuiev , Juerg Osterwalder, Matthias Hengsberger, Lukas Gallmann, Peter Krueger and Ursula Keller
    • Journal Title

      Optica

      Volume: 4 Issue: 12 Pages: 1492-1497

    • DOI

      10.1364/optica.4.001492

    • Related Report
      2017 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Gap state imaging and spin-orbit effects in resonant photoelectron diffraction2016

    • Author(s)
      Peter Krueger and Fabiana Da Pieve
    • Journal Title

      Surface and Interface Analysis

      Volume: 48 Issue: 11 Pages: 1169-1174

    • DOI

      10.1002/sia.6182

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] ES2MS: An interface package for passing self-consistent charge density and potential from Electronic Structure codes To Multiple Scattering codes2016

    • Author(s)
      Junqing Xu, Calogero R. Natoli, Peter Krueger, Kuniko Hayakawa, Didier Sebilleau, Li Song, and Keisuke Hatada
    • Journal Title

      Computer Physics Communications

      Volume: 203 Pages: 331-338

    • DOI

      10.1016/j.cpc.2016.02.031

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Presentation] Theoretical advances in angle-resolved photoelectron and resonant Auger electron spectroscopy2019

    • Author(s)
      Peter Krueger
    • Organizer
      The first international Workshop on Momentum Microscopy & Spectroscopy for Materials Science, 分子研, 岡崎, 22-23 February 2019.
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Orbital angular momentum transfer in angle resolved resonant Auger electron emission2019

    • Author(s)
      Godeung Park, Peter Krueger
    • Organizer
      第66回応用物理学会春季学術講演会, 東京, 9-12 March 2019.
    • Related Report
      2018 Annual Research Report
  • [Presentation] X-ray absorption and linear dichroism of individual Boron Nitride nanotubes - experiment and theory2018

    • Author(s)
      前川裕哉, Peter Krueger
    • Organizer
      17th International Conference on X-ray Absorption Fine Structure (XAFS18), Krakow, Poland, 22-27 July 2018.
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Transition metal L-edge spectra with ligand-field multiplet parameters from density functional theory2018

    • Author(s)
      Peter Krueger
    • Organizer
      17th International Conference on X-ray Absorption Fine Structure (XAFS18), Krakow, Poland, 22-27 July 2018.
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] DFTから得られた配位子場の多重項法によるX線吸収理論2018

    • Author(s)
      Peter Krueger, 原田洋樹, 吉本有輝
    • Organizer
      第21回XAFS討論会, 札幌, 3-5 Sep 2018.
    • Related Report
      2018 Annual Research Report
  • [Presentation] 多重散乱理論によるCO on Pt(111)のARPESの理論解析2018

    • Author(s)
      鈴木悠人, Peter Krueger
    • Organizer
      日本物理学会2018年秋季大会, 京都, 9-12 Sep 2018.
    • Related Report
      2018 Annual Research Report
  • [Presentation] Spectroscopies: Theory and Calculations2018

    • Author(s)
      Peter Krueger
    • Organizer
      The 7th International School on Magnetism and Synchrotron Radiation, Mittelwihr, France, 7-12 Oct 2018.
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 平面波基底を用いたARPES強度計算におけるマッチング法2018

    • Author(s)
      小野凌太, Peter Krueger
    • Organizer
      73rd Annual meeting of the Japanese Physical Society
    • Related Report
      2017 Research-status Report
  • [Presentation] 光電子分光におけるウィグナー遅延時間のモデル計算2018

    • Author(s)
      クリューガー ピーター, 小田部祐樹, 但野将平
    • Organizer
      73rd Annual meeting of the Japanese Physical Society
    • Related Report
      2017 Research-status Report
  • [Presentation] 「有機遷移金属分子によるXLD・XMCDの理論研究」2017

    • Author(s)
      ピーター クリューガー
    • Organizer
      ワークショップ:放射光物質構造科学への新展開:X線吸収共鳴現象
    • Related Report
      2017 Research-status Report
    • Invited
  • [Presentation] フラーレン薄膜のARPESの理論解析2017

    • Author(s)
      鈴木悠人、Peter Krueger
    • Organizer
      Autumn meeting of the Japanese Physical Society
    • Related Report
      2017 Research-status Report
  • [Presentation] Final state effects in ARPES from plane-wave band structure methods2017

    • Author(s)
      R. Ono and P. Krueger
    • Organizer
      The 8th International Symposium on Surface Science (ISSS-8)
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research
  • [Presentation] Analysis of angle dependent resonant photoemission of titanium dioxide2016

    • Author(s)
      P. Krueger and S. Moser
    • Organizer
      PLESI16 - Prospects and Limitations of Electronic Structure Imaging by Angle Resolved Photoemission Spectroscopy
    • Place of Presentation
      Dresden, Germany
    • Year and Date
      2016-04-25
    • Related Report
      2016 Research-status Report

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Published: 2016-04-21   Modified: 2021-02-19  

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