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Microscopic studies of anglesite formation under sulfuric acid condition using positronium

Research Project

Project/Area Number 16K05394
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Condensed matter physics I
Research InstitutionTokyo Gakugei University

Principal Investigator

NAKATA Masataka  東京学芸大学, 教育学部, 教授 (80180305)

Research Collaborator SATO Kiminori  
Project Period (FY) 2016-04-01 – 2019-03-31
Project Status Completed (Fiscal Year 2018)
Budget Amount *help
¥4,680,000 (Direct Cost: ¥3,600,000、Indirect Cost: ¥1,080,000)
Fiscal Year 2018: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2017: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2016: ¥2,730,000 (Direct Cost: ¥2,100,000、Indirect Cost: ¥630,000)
Keywords硫酸鉛鉱 / 方鉛鉱 / 硫酸酸性環境 / 硫酸塩ナノ鉱物 / 物質移行 / ナノ空間 / ポジトロニウム / オングストローム空間 / 粒子線 / X線 / 岩石・鉱物・鉱床学
Outline of Final Research Achievements

The formation mechanism of anglesite from galena under sulfuric acid condition was investigated by field emission scanning electron microscopy (FE-SEM), X-ray diffraction (XRD), and a series of positron annihilation experiments. Nanovoids dominantly surrounded by surfer atoms were found in grain boundaries among galena and anglesite nanocrystals upon the formation of anglesite nanocrystals. The concentration of nanovoid increases with increasing the degree of anglesite formation.

Academic Significance and Societal Importance of the Research Achievements

本研究で得られた結果は,硫酸酸性環境中の硫酸塩ナノ鉱物形成に粒界中のナノボイドが関与していることを示唆しており,このことは学術的に意義がある。さらなるデータの蓄積により,硫酸酸性環境下で硫酸塩ナノ鉱物形成メカニズムを説明するモデルの構築が期待される。実現すれば,環境への鉛溶出抑制技術に貢献するだけでなく,地質環境中の物質移行モデルの高精度化にも結びつくため,社会的貢献度も高い。

Report

(4 results)
  • 2018 Annual Research Report   Final Research Report ( PDF )
  • 2017 Research-status Report
  • 2016 Research-status Report
  • Research Products

    (5 results)

All 2017 2016

All Journal Article (5 results) (of which Peer Reviewed: 5 results,  Open Access: 2 results,  Acknowledgement Compliant: 3 results)

  • [Journal Article] 埼玉県吉見丘陵の凝灰質岩表面におけるタン礬の形成2017

    • Author(s)
      直井良太,中田正隆,小室光世
    • Journal Title

      資源地質

      Volume: 67 Pages: 103-110

    • Related Report
      2017 Research-status Report
    • Peer Reviewed
  • [Journal Article] (Au,Ag)Te2 Minerals from Epithermal Gold Deposits in Japan2017

    • Author(s)
      Kosei Komuro and Masataka Nakata
    • Journal Title

      Resource Geology

      Volume: 67 Issue: 1 Pages: 22-34

    • DOI

      10.1111/rge.12115

    • Related Report
      2017 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] Cesium diffusion through angstrom-scale open spaces in clay minerals2017

    • Author(s)
      K.Fujimoto, K.Sato, M.Nakata
    • Journal Title

      Journal of Physical Society of Japan

      Volume: 86 Issue: 3 Pages: 034901-1

    • DOI

      10.7566/jpsj.86.034901

    • NAID

      40021129840

    • Related Report
      2017 Research-status Report 2016 Research-status Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] 鉄重石-CaCl2水溶液間における水熱反応実験2016

    • Author(s)
      田村維都江,中田正隆,小室光世
    • Journal Title

      資源地質

      Volume: 61(2) Pages: 81-88

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] 硫化ナトリウム水溶液と反応させた白鉛鉱に見られる交代組織:130°Cから170°Cにおける実験的研究2016

    • Author(s)
      田村維都江,中田正隆,小室光世
    • Journal Title

      資源地質

      Volume: 61(1) Pages: 1-6

    • NAID

      130007434866

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant

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Published: 2016-04-21   Modified: 2020-03-30  

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