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High field study of quantum magnets through measurements of magnetoelectric effects

Research Project

Project/Area Number 16K05413
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Condensed matter physics II
Research InstitutionThe University of Tokyo

Principal Investigator

Tokunaga Masashi  東京大学, 物性研究所, 准教授 (50300885)

Project Period (FY) 2016-04-01 – 2019-03-31
Project Status Completed (Fiscal Year 2018)
Budget Amount *help
¥4,550,000 (Direct Cost: ¥3,500,000、Indirect Cost: ¥1,050,000)
Fiscal Year 2018: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Fiscal Year 2017: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Fiscal Year 2016: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Keywordsマルチフェロイクス / 磁性 / 強磁場 / 物性実験
Outline of Final Research Achievements

Multiferroic materials have attracted considerable attentions due to their possible application for magnetoelectric memory devices. BiFeO3 is perhaps the most extensively studied multiferroic material because it exhibits prominent mutiferroic properties at room temperature, In this study, we developed study about non-volatile memory effects in this material, and realized this phenomenon in the ferromagnetic and ferroelectric state. We also clarified microscopic origin for this effect.
In the study of Ba2CuGe2O7, we studied magnetoelectric effects and ultrasound transmission in high magnetic fields. Through these experiments, we clarified field control of hybridization between Cu 3d and O 2p orbitals plays a key role in the magnetoeectric effect even in this quantum spin magnet.

Academic Significance and Societal Importance of the Research Achievements

マルチフェロイック物質における電気磁気効果は、物質の新しい可能性を開くテーマとしてこの20年ほど盛んに研究されてきた。本研究ではこの分野で長年追い求められてきた強磁性と強誘電性の共存状態における電気磁気メモリー効果の実証に成功した。またこの現象の微視的起源である磁性イオンと周囲の配位子イオンとの軌道混成の磁場制御は、単純な理論予測に反してスピンの短い量子スピン系でも観測されている。この現象の代表的物質に対して強磁場下の電気磁気効果と超音波伝導の実験を行うことで、その微視的起源を明らかにした。

Report

(4 results)
  • 2018 Annual Research Report   Final Research Report ( PDF )
  • 2017 Research-status Report
  • 2016 Research-status Report
  • Research Products

    (29 results)

All 2019 2018 2017 2016 Other

All Int'l Joint Research (3 results) Journal Article (7 results) (of which Int'l Joint Research: 4 results,  Peer Reviewed: 7 results,  Acknowledgement Compliant: 1 results) Presentation (19 results) (of which Int'l Joint Research: 6 results,  Invited: 2 results)

  • [Int'l Joint Research] Huazhong University(中国)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] Oak Ridge National Laboratory/NIST Center for Neutron Research(米国)

    • Related Report
      2017 Research-status Report
  • [Int'l Joint Research] Oak Ridge National Laboratory/NIST center for Neutron Research/University of Maryland(米国)

    • Related Report
      2016 Research-status Report
  • [Journal Article] Magnetoelectric behavior from cluster multipoles in square cupolas: Study of Sr(TiO)Cu4(PO4)4 in comparison with Ba and Pb isostructurals2019

    • Author(s)
      Kato Yasuyuki、Kimura Kenta、Miyake Atsushi、Tokunaga Masashi、Matsuo Akira、Kindo Koichi、Akaki Mitsuru、Hagiwara Masayuki、Kimura Shojiro、Kimura Tsuyoshi、Motome Yukitoshi
    • Journal Title

      Physical Review B

      Volume: 99 Issue: 2 Pages: 024415-024415

    • DOI

      10.1103/physrevb.99.024415

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Difference in magnetic and ferroelectric properties between rhombohedral and hexagonal polytypes of AgFeO2: A single-crystal study2019

    • Author(s)
      Terada Noriki、Ikedo Yuta、Sato Hirohiko、Khalyavin Dmitry D.、Manuel Pascal、Orlandi Fabio、Tsujimoto Yoshihiro、Matsushita Yoshitaka、Miyake Atsushi、Matsuo Akira、Tokunaga Masashi、Kindo Koichi
    • Journal Title

      Physical Review B

      Volume: 99 Issue: 6

    • DOI

      10.1103/physrevb.99.064402

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Unusual magnetoelectric memory and polarization reversal in the kagome staircase compound Ni3V2O82018

    • Author(s)
      Liu Y. J.、Wang J. F.、He Z. Z.、Lu C. L.、Xia Z. C.、Ouyang Z. W.、Liu C. B.、Chen R.、Matsuo A.、Kohama Y.、Kindo K.、Tokunaga M.
    • Journal Title

      Physical Review B

      Volume: 97 Issue: 17 Pages: 1744291-1744296

    • DOI

      10.1103/physrevb.97.174429

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Magnetic structural unit with convex geometry: A building block hosting an exchange-striction-driven magnetoelectric coupling2018

    • Author(s)
      Kenta Kimura, Yasuyuki Kato, Kunihiko Yamauchi, Atsushi Miyake, Masashi Tokunaga, Akira Matsuo, Koichi Kindo, Mitsuru Akaki, Masayuki Hagiwara, Shojiro Kimura, Masayuki Toyoda, Yukitoshi Motome, and Tsuyoshi Kimura
    • Journal Title

      Phys. Rev. Mater.

      Volume: 2 Issue: 10 Pages: 104415-104415

    • DOI

      10.1103/physrevmaterials.2.104415

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] 室温マルチフェロイック物質ビスマスフェライトの電気磁気効果2018

    • Author(s)
      河智史朗、 三宅厚志、 徳永将史、 伊藤利充
    • Journal Title

      固体物理

      Volume: 53 Pages: 61-70

    • NAID

      40021480888

    • Related Report
      2017 Research-status Report
    • Peer Reviewed
  • [Journal Article] Successive field-induced transitions in BiFeO3 around room temperature2017

    • Author(s)
      Kawachi Shiro、Miyake Atsushi、Ito Toshimitsu、Dissanayake Sachith E.、Matsuda Masaaki、Ratcliff William、Xu Zhijun、Zhao Yang、Miyahara Shin、Furukawa Nobuo、Tokunaga Masashi
    • Journal Title

      Physical Review Materials

      Volume: 1 Issue: 2

    • DOI

      10.1103/physrevmaterials.1.024408

    • NAID

      130006710196

    • Related Report
      2017 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Magnetoelectric Behavior from the S=1/2 Asymmetric Square Cupolas2017

    • Author(s)
      Y. Kato, K. Kimura, A. Miyake, M. Tokunaga, A. Matsuo, K. Kindo, M. Akaki, M. Hagiwara, M. Sera, T. Kimura, and Y. Motome
    • Journal Title

      Phys. Rev. Lett

      Volume: 118 Issue: 10 Pages: 1076011-5

    • DOI

      10.1103/physrevlett.118.107601

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Presentation] パルス磁場中での誘電率測定2019

    • Author(s)
      三宅厚志, 木村健太, 三田村裕幸, 木村剛, 徳永将史
    • Organizer
      日本物理学会第74回年次大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] BiFeO3における傾角反強磁性相の新奇電気分極2019

    • Author(s)
      河智史朗, 木下雄斗, 三宅厚志, 伊藤利充, 宮原慎, 山浦淳一, 徳永将史
    • Organizer
      日本物理学会第74回年次大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] パルス強磁場下超音波計測によるBa2CuGe2O7の四極子-歪み相互作用2019

    • Author(s)
      栗原綾佑, 三宅厚志, 徳永将史, 赤木暢, 萩原政幸, 桑原英樹
    • Organizer
      日本物理学会第74回年次大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Magnetic and electric control of chiral spin texture in multiferroic BiFeO32018

    • Author(s)
      M. Tokunaga
    • Organizer
      Research in High Magnetic Field 2018
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 極性キラル磁性体Ni2InSbO6における磁気相図2017

    • Author(s)
      荒木勇介、阿部伸行、佐藤樹、木村尚次郎、徳永将史、徳永祐介、有馬孝尚
    • Organizer
      日本物理学会第72回年次大会
    • Place of Presentation
      大阪大学(大阪府・豊中市)
    • Year and Date
      2017-03-17
    • Related Report
      2016 Research-status Report
  • [Presentation] BiFeO3の室温付近における磁場誘起逐次相転移2017

    • Author(s)
      河智史朗、三宅厚志、伊藤利充、松田雅昌、宮原慎、古川信夫、徳永将史
    • Organizer
      日本物理学会第72回年次大会
    • Place of Presentation
      大阪大学(大阪府・豊中市)
    • Year and Date
      2017-03-17
    • Related Report
      2016 Research-status Report
  • [Presentation] 室温マルチフェロイックBiFeO3単結晶の磁気ドメインの性質2017

    • Author(s)
      伊藤利充、尾崎康子、富岡泰秀、松田雅昌、徳永将史、木下雄斗、宮本辰也、貴田徳明、岡本博
    • Organizer
      日本物理学会第72回年次大会
    • Place of Presentation
      大阪大学(大阪府・豊中市)
    • Year and Date
      2017-03-17
    • Related Report
      2016 Research-status Report
  • [Presentation] 正四角台塔系における磁気秩序の多極子分解と電気磁気応答2017

    • Author(s)
      加藤康之、木村健太、三宅厚志、徳永将史、松尾晶、金道浩一、赤木暢、萩原政幸、世良正一、木村剛、求幸年
    • Organizer
      日本物理学会第72回年次大会
    • Place of Presentation
      大阪大学(大阪府・豊中市)
    • Year and Date
      2017-03-17
    • Related Report
      2016 Research-status Report
  • [Presentation] Magnetic and electric control of multiferroic properties in monodomain crystals of BiFeO32017

    • Author(s)
      M. Tokunaga
    • Organizer
      APS March meeting 2017
    • Place of Presentation
      New Orleans, USA
    • Year and Date
      2017-03-13
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Magnetoelectric effects in Ba2CuGe2O7 beyond the saturation field2017

    • Author(s)
      M. Tokunaga, Y. Sato, A. Miyake, M. Akaki, M. Hagiwara, and H. Kuwahara
    • Organizer
      The 9th APCTP Workshop on Multiferroics
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research
  • [Presentation] The magnetoelectric effect in bismuth ferrite around room temperature2017

    • Author(s)
      S. Kawachi, A. Miyake, T. Ito, S. Miyahara, M. Matsuda, W. Ratcliff II, and M. Tokunaga
    • Organizer
      The 9th APCTP Workshop on Multiferroics
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research
  • [Presentation] マルチフェロイックBiFeO3 の新奇磁場誘起相2017

    • Author(s)
      河智史朗、伊藤利充、宮原慎、松田雅昌、三宅厚志、徳永将史
    • Organizer
      強磁場コラボラトリーが拓く未踏計測領域への挑戦と物質・材料科学の最先端
    • Related Report
      2017 Research-status Report
  • [Presentation] Field-induced changes in various properties of BiFeO3 crystals grown by the LD-FZ method2017

    • Author(s)
      S. Kawachi, K. Akiba, A. Miyake, T. Ito, Y. Nakanishi, M. Yoshizawa, and M. Tokunaga
    • Organizer
      SCES2017
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research
  • [Presentation] S=1/2正方晶カイラル反強磁性体A(TiO)Cu4(PO4)4(A = Ba, Sr)の強磁場中物性2016

    • Author(s)
      世良正一、木村健太、赤木暢、萩原政幸、三宅厚志、徳永将史、松尾晶、金道浩一、中野岳仁、野末泰夫、木村剛
    • Organizer
      日本物理学会2016年秋季大会
    • Place of Presentation
      金沢大学(石川県・金沢市)
    • Year and Date
      2016-09-13
    • Related Report
      2016 Research-status Report
  • [Presentation] 反強磁性カイラル正四角台塔系(A(TiO)Cu4(PO4)4(A=Ba, Sr))の磁化曲線と電気磁気効果2016

    • Author(s)
      加藤康之、木村健太、三宅厚志、徳永将史、松尾晶、金道浩一、赤木暢、萩原政幸、世良正一、木村剛、求幸年
    • Organizer
      日本物理学会2016年秋季大会
    • Place of Presentation
      金沢大学(石川県・金沢市)
    • Year and Date
      2016-09-13
    • Related Report
      2016 Research-status Report
  • [Presentation] 強磁場下におけるBa2CuGe2O7の電気磁気効果2016

    • Author(s)
      徳永将史、佐藤由昌、赤木暢、三宅厚志
    • Organizer
      日本物理学会2016年秋季大会
    • Place of Presentation
      金沢大学(石川県・金沢市)
    • Year and Date
      2016-09-13
    • Related Report
      2016 Research-status Report
  • [Presentation] 三方晶c軸に垂直な電場による単結晶BiFeO3の抵抗メモリー効果2016

    • Author(s)
      河智史朗、伊藤利充、三宅厚志、徳永将史
    • Organizer
      日本物理学会2016年秋季大会
    • Place of Presentation
      金沢大学(石川県・金沢市)
    • Year and Date
      2016-09-13
    • Related Report
      2016 Research-status Report
  • [Presentation] 四面体磁性鎖を持つ Cu3Mo2O9 の「磁歪プラトー」2016

    • Author(s)
      黒江晴彦、江袋佑太、長谷正司、河智史朗、徳永将史、岡邦彦、伊藤利充、永崎洋
    • Organizer
      日本物理学会2016年秋季大会
    • Place of Presentation
      金沢大学(石川県・金沢市)
    • Year and Date
      2016-09-13
    • Related Report
      2016 Research-status Report
  • [Presentation] Magnetic and electric control of transverse electric polarization in BiFeO32016

    • Author(s)
      M. Tokunaga, S. Kawachi, A. Miyake, and T. Ito
    • Organizer
      Multiferroic & Magnetoelectric Materials, Gordon Research Conference
    • Place of Presentation
      Bates College, USA
    • Year and Date
      2016-08-07
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research

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Published: 2016-04-21   Modified: 2022-02-21  

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