Elucidation of the mechanism of the new superconductivity without doping in T'-type cuprates
Project/Area Number |
16K05458
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Research Category |
Grant-in-Aid for Scientific Research (C)
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Allocation Type | Multi-year Fund |
Section | 一般 |
Research Field |
Condensed matter physics II
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Research Institution | Sophia University |
Principal Investigator |
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Research Collaborator |
SUMURA takuya
KAWABATA koki
PARK sangeun
BAQIYA malik anjelh
KURASHIMA koshi
ONISHI shusei
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Project Period (FY) |
2016-04-01 – 2019-03-31
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Project Status |
Completed (Fiscal Year 2018)
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Budget Amount *help |
¥4,550,000 (Direct Cost: ¥3,500,000、Indirect Cost: ¥1,050,000)
Fiscal Year 2018: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2017: ¥1,300,000 (Direct Cost: ¥1,000,000、Indirect Cost: ¥300,000)
Fiscal Year 2016: ¥2,210,000 (Direct Cost: ¥1,700,000、Indirect Cost: ¥510,000)
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Keywords | 高温超伝導体 / 電子ドープ型銅酸化物 / 母物質ノンドープ超伝導 / 還元処理 / ミュオンスピン緩和 / X線吸収分光 / 単結晶 / マイスナー反磁性 / 光学反射率 / 単結晶育成 / 強相関電子系 / 超伝導材料・素子 / 低温物性 / 粒子線 / 磁性 |
Outline of Final Research Achievements |
In order to elucidate the mechanism of superconductivity in the parent compounds of the electron-doped high-Tc cuprate superconductors with the T'-structure, we have investigated detailed changes of the electronic states through the reduction annealing from the electrical resistivity, muon spin relaxation etc. using single crystals of the T'-cuprates. By improving the reduction annealing, we have succeeded in removing effectively the excess oxygen from the single crystals of the T'-cuprates. It has been clarified that not only electrons but also holes are generated through the reduction annealing in the T'-cuprates, suggesting that holes are related to the appearance of superconductivity. Moreover, it has been clarified that the Cu-spin correlation and superconductivity are in intimate relation with each other in the T'-cuprates.
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Academic Significance and Societal Importance of the Research Achievements |
本研究の結果、電子ドープ型T'銅酸化物から過剰な酸素を効果的に取り除く方法を確立した。これは、他の遷移金属酸化物に対しても利用できる技術なので、様々な機能性酸化物の開発に貢献するだろう。 本研究から、T'銅酸化物において還元とともに電子状態がどのように変化するのかが明らかになった。特に、超伝導が発現する試料におけるホールキャリアの存在とCuスピン相関の発達を結論できたことは特筆に値する。今後は、元素置換によらない新たなキャリアドープ法による新規高温超伝導体の創製が発展するだろう。
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Report
(4 results)
Research Products
(72 results)
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[Journal Article] Undoped high-Tc superconductivity in T'-La1.8Eu0.2CuO4+δ revealed by 63,65Cu and 139La NMR: Bulk superconductivity and antiferromagnetic fluctuations2017
Author(s)
H. Fukazawa, S. Ishiyama, M. Goto, S. Kanamaru, K. Ohashi, T. Kawamata, T. Adachi, M. Hirata, T. Sasaki, Y. Koike and Y. Kohori
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Journal Title
Physica C
Volume: 541
Pages: 30-35
DOI
Related Report
Peer Reviewed
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[Journal Article] Pressure tuning of structure, superconductivity, and novel magnetic order in the Ce-underdoped electron-doped cuprate T'-Pr1.3-xLa0.7CexCuO4 (x=0.1)2017
Author(s)
Z. Guguchia, T. Adachi, Z. Shermadini, T. Ohgi, J. Chang, E. S. Bozin, F. von Rohr, A. M. dos Santos, J. J. Molaison, R. Boehler, Y. Koike, A. R. Wieteska, B. A. Frandsen, E. Morenzoni, A. Amato, S. J. L. Billinge, Y. J. Uemura and R. Khasanov
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Journal Title
Physical Review B
Volume: 96
Issue: 9
DOI
Related Report
Peer Reviewed / Int'l Joint Research
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[Journal Article] Strong electron correlation behind the superconductivity in Ce-free and Ce-underdoped high-Tc T'-cuprates2016
Author(s)
T. Adachi, A. Takahashi, K. M. Suzuki, M. A. Baqiya, T. Konno, T. Takamatsu, M. Kato, I. Watanabe, A. Koda, M. Miyazaki, R. Kadono, Y. Koike
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Journal Title
Journal of the Physical Society of Japan
Volume: 85
Issue: 11
Pages: 114716-114716
DOI
NAID
Related Report
Peer Reviewed
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[Presentation] 電子ドープ型高温超伝導体T'-Pr1.3-xLa0.7CexCuO4+δの63,65Cu,139La-NMR2019
Author(s)
金丸周平, Lee Yongsun, 後藤雅人, 深澤英人, 小堀洋, 高橋晶, 川股隆行, 川端公貴, 田島一輝, 足立匡, 小池洋二
Organizer
日本物理学会第74回年次大会
Related Report
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[Presentation] Reduction and electron-doping effects on the Cu-spin correlation in electron-doped high-Tc cuprates Pr2-x-yLayCexCuO4+δ2018
Author(s)
T. Adachi, T. Sumura, M. A. Baqiya, T. Ishimoto, H. Kuwahara, K. Kurashima, I. Watanabe, A. Koda, M. Miyazaki, R. Kadono, Y. Koike
Organizer
12th International Conference on Materials and Mechanisms of Superconductivity and High Temperature Superconductors (M2S-HTSC-XII)
Related Report
Int'l Joint Research
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[Presentation] Direct observation of symmetry-distinct states with nontrivial doping evolution in a high-Tc cuprate family by polarization-dependent ARPES2018
Author(s)
R.-H. He, M. Hashimoto, K. Tanaka, S.-K. Mo, A. Sorini, T. Sasagawa, M. Fujita, T. Adachi, M. Enoki, S. Iikubo, Y. He, M. Yi, N. Mannella, H. Yao, W. Meevasana, T. P. Devereaux, Y. Koike, K. Yamada, Z.Hussain, Z.-X. Shen
Organizer
12th International Conference on Materials and Mechanisms of Superconductivity and High Temperature Superconductors (M2S-HTSC-XII)
Related Report
Int'l Joint Research
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[Presentation] 63,65CuNMR studies of superconducting T'-La1.8Eu0.2CuO4+δ with Nd2CuO4 structure2018
Author(s)
Y. Kohori, H. Fukazawa, S. Ishiyama, M. Goto, S. Kanamaru, K. Ohashi, T. Kawamata, T. Adachi, M. Hirata, T. Sasaki, Y. Koike
Organizer
12th International Conference on Materials and Mechanisms of Superconductivity and High Temperature Superconductors (M2S-HTSC-XII)
Related Report
Int'l Joint Research
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[Presentation] Transport and muon spin relaxation studies of the novel electronic state in the electron-doped high-Tc T'-cuprates2017
Author(s)
T. Adachi, A. Takahashi, M. A. Baqiya, T. Konno, T. Ohgi, T. Sumura, K. Kurashima, K. M. Suzuki, T. Takamatsu, T. Kawamata, M. Kato, I. Watanabe, A. Koda, M. Miyazaki, R. Kadono, H. Oguro, S. Awaji, Y. Koike
Organizer
The 37th REIMEI Workshop on Frontiers of Correlated Quantum Matters and Spintronics
Place of Presentation
Tokai (Japan)
Year and Date
2017-01-14
Related Report
Int'l Joint Research / Invited
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[Presentation] Coincident disappearance of superconductivity in La2-xSrxCu1-yMyO4 (M = Fe, Al)2017
Author(s)
K. M. Suzuki, T. Adachi, M. A. Baqiya, H. Guo, I. Kawasaki, M. Abdel-Jawad, S. Yoon, I. Watanabe, Y. Koike
Organizer
The 14th International Conference on Muon Spin Rotation, Relaxation and Resonance (μSR2017)
Related Report
Int'l Joint Research
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[Presentation] Over-reduction effects on the Cu-spin correlation in the electron-doped T'-cuprate Pr1.3-xLa0.7CexCuO4+δ (x = 0.10)2017
Author(s)
T. Sumura, T. Ishimoto, H. Kuwahara, K. Kurashima, Y. Koike, I. Watanabe, M. Miyazaki, A. Koda, R. Kadono, T. Adachi
Organizer
The 14th International Conference on Muon Spin Rotation, Relaxation and Resonance (μSR2017)
Related Report
Int'l Joint Research
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[Presentation] Cu-spin correlation and novel electronic state in the electron-doped high-Tc cuprates2017
Author(s)
T. Adachi, T. Sumura, M. A. Baqiya, A. Takahashi, T. Konno, T. Ohgi, K. Kurashima, T. Kawamata, T. Ishimoto, H. Kuwahara, I. Watanabe, A. Koda, M. Miyazaki, R. Kadono, S. Awaji and Y. Koike
Organizer
28th International Conference on Low Temperature Physics (LT28)
Related Report
Int'l Joint Research
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[Presentation] Cu-spin correlation and novel electronic state in the electron-doped high-Tc T'-superconductors2017
Author(s)
T. Adachi, T. Sumura, M. A. Baqiya, A. Takahashi, T. Konno, T. Ohgi, K. Kurashima, T. Kawamata, T. Ishimoto, H. Kuwahara, I. Watanabe, A. Koda, M. Miyazaki, R. Kadono, S. Awaji and Y. Koike
Organizer
International Conference Electron Correlation in Superconductors and Nanostructures (ECSN-2017)
Related Report
Int'l Joint Research / Invited
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[Presentation] Undoped superconductivity and the novel electronic state in the high-Tc T'-cuprates2017
Author(s)
T. Adachi, T. Sumura, M. A. Baqiya, A. Takahashi, T. Konno, T. Ohgi, K. Ohashi, K. Kurashima, T. Kawamata, T. Ishimoto, H. Kuwahara, I. Watanabe, A. Koda, M. Miyazaki, R. Kadono, S. Awaji and Y. Koike
Organizer
The 2017 European Materials Research Society Fall Meeting
Related Report
Int'l Joint Research / Invited
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[Presentation] 過剰に還元された電子ドープ型T'銅酸化物の電子状態2017
Author(s)
足立匡, 洲村拓哉, M. A. Baqiya, 高橋晶, 今野巧也, 扇太郎, 倉嶋晃士, 川股隆行, 石本奨, 桑原英樹, 渡邊功雄, 幸田章宏, 宮崎正範, 門野良典, 小池洋二
Organizer
高温超伝導フォーラム第5回会合
Related Report
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[Presentation] Muon spin relaxation and transport studies in the electron-doped high-Tc T'-superconductors revealing the novel electronic state2016
Author(s)
T. Adachi, A. Takahashi, T. Konno, T. Ohgi, M. A. Baqiya, K. Kurashima, K. M. Suzuki, T. Takamatsu, T. Kawamata, M. Kato, I. Watanabe, A. Koda, M. Miyazaki, R. Kadono, H. Oguro, S. Awaji, Y. Koike
Organizer
International Conference on Superstirpes 2016
Place of Presentation
Ischia (Italy)
Year and Date
2016-06-23
Related Report
Int'l Joint Research / Invited
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