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Development of an efficient purification process of low-grade waste cooking oil by melt crystallization

Research Project

Project/Area Number 16K06832
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Properties in chemical engineering process/Transfer operation/Unit operation
Research InstitutionUniversity of Hyogo

Principal Investigator

Yamamoto Takuji  兵庫県立大学, 工学研究科, 教授 (30358288)

Co-Investigator(Kenkyū-buntansha) 伊藤 和宏  兵庫県立大学, 工学研究科, 准教授 (80347525)
Research Collaborator MAEDA Kouji  
KURAMOCHI Hidetoshi  
TAYAKOUT-FAYOLLE Mélaz  
Project Period (FY) 2016-04-01 – 2019-03-31
Project Status Completed (Fiscal Year 2018)
Budget Amount *help
¥4,940,000 (Direct Cost: ¥3,800,000、Indirect Cost: ¥1,140,000)
Fiscal Year 2018: ¥520,000 (Direct Cost: ¥400,000、Indirect Cost: ¥120,000)
Fiscal Year 2017: ¥2,210,000 (Direct Cost: ¥1,700,000、Indirect Cost: ¥510,000)
Fiscal Year 2016: ¥2,210,000 (Direct Cost: ¥1,700,000、Indirect Cost: ¥510,000)
Keywordsモデル廃食油 / テーラー渦 / 溶質分配理論 / 晶析操作 / 脂肪酸混合物 / 有効分配因子 / テイラー渦
Outline of Final Research Achievements

To separate a saturated fatty acid from an unsaturated fatty acid contained in low-grade waste cooking oil (WGO), we performed melt crystallization employing an annular-cylindrical-type apparatus. In this study, we examined the following three items: (i) melt crystallization of binary mixture of fatty acids as model WGO, (ii) elucidation of formation mechanism of Taylor vortex in the annular space of a melt crystallization bath, (iii) building of a solute distribution theory using ternary mixture of fatty acids as model WGO.

Academic Significance and Societal Importance of the Research Achievements

本研究の実施によって,バイオ燃料精製を目的とした融液晶析における基幹技術と基盤となる理論を確立できた。また,本研究で確立した技術は低品位廃食油の再資源化のために不可欠な精製技術であるため,石油代替資源としての低品位廃食油のエネルギー利用に加えて,炭酸ガス排出量削減などの環境面での波及効果も期待される。

Report

(4 results)
  • 2018 Annual Research Report   Final Research Report ( PDF )
  • 2017 Research-status Report
  • 2016 Research-status Report
  • Research Products

    (32 results)

All 2019 2018 2017 2016 Other

All Int'l Joint Research (3 results) Journal Article (9 results) (of which Int'l Joint Research: 4 results,  Peer Reviewed: 9 results,  Acknowledgement Compliant: 1 results) Presentation (20 results) (of which Int'l Joint Research: 5 results)

  • [Int'l Joint Research] LAGEPP/Universite Claude Bernard Lyon 1(フランス)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] University of Claud Bernard Lyon 1(France)

    • Related Report
      2017 Research-status Report
  • [Int'l Joint Research] University of Claude Bernard Lyon 1(France)

    • Related Report
      2016 Research-status Report
  • [Journal Article] Effect of high pressure on growth of colloidal particles during sol-gel phase transition of resorcinol-formaldehyde solution2019

    • Author(s)
      T. Yamamoto, M. Tayakout-Fayolle, K. Iimura, H. Satone, T. Kakibe, K. Itoh, K. Maeda
    • Journal Title

      International Journal of Adsorption

      Volume: in publication Issue: 6 Pages: 1-6

    • DOI

      10.1007/s10450-019-00042-4

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Ozonation of aqueous phenol using high-silica zeolite in an aerated mixing vessel2018

    • Author(s)
      Yamamoto Takuji、Iimura Kenji、Satone Hiroshi、Itoh Kazuhiro、Maeda Kouji
    • Journal Title

      Asia-Pacific Journal of Chemical Engineering

      Volume: 13 Issue: 2

    • DOI

      10.1002/apj.2175

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Use of ethanol with triolein for fatty acid ethyl ester as biodiesel fuel in a Novozym fixed-bed reactor2018

    • Author(s)
      Y. Endo, T. Hatanaka, K. Maeda, K. Arafune, T. Yamamoto, K. Itoh, H. Kuramochi, Y. Kashino, K. Ifuku
    • Journal Title

      Biomass and Bioenergy

      Volume: 108 Pages: 433-438

    • DOI

      10.1016/j.biombioe.2017.11.023

    • Related Report
      2017 Research-status Report
    • Peer Reviewed
  • [Journal Article] Crystallizing Concentration of the Diatom <i>Chaetoceros gracilis</i> Cell Solutions2018

    • Author(s)
      前田光治,伊藤和宏,菓子野康浩,伊福健太郎,新船幸二,山本拓司
    • Journal Title

      KAGAKU KOGAKU RONBUNSHU

      Volume: 44 Issue: 1 Pages: 18-22

    • DOI

      10.1252/kakoronbunshu.44.18

    • NAID

      130006316108

    • ISSN
      0386-216X, 1349-9203
    • Related Report
      2017 Research-status Report
    • Peer Reviewed
  • [Journal Article] 微小蒸気泡の安定性に関する分子動力学解析2018

    • Author(s)
      伊藤和宏,木佐悠人,山本拓司,前田光治
    • Journal Title

      混相流

      Volume: 32 Pages: 43-48

    • NAID

      130006731299

    • Related Report
      2017 Research-status Report
    • Peer Reviewed
  • [Journal Article] Transesterification of Triolein and Methanol by Novozym 435 with Dimethyl Ether2017

    • Author(s)
      K. Maeda, H. Kuramochi, K. Arafune, K. Itoh, T. Yamamoto
    • Journal Title

      JOURNAL OF CHEMICAL ENGINEERING OF JAPAN

      Volume: 50 Issue: 12 Pages: 924-928

    • DOI

      10.1252/jcej.17we123

    • NAID

      130006258897

    • ISSN
      0021-9592, 1881-1299
    • Related Report
      2017 Research-status Report
    • Peer Reviewed
  • [Journal Article] Melt crystallization of binary mixture of fatty acids as model biofuel2017

    • Author(s)
      Takuji YAMAMOTO, Takuto FUJIKAWA, Nobuyoshi OKAMOTO, Kazuhiro ITOH, Kouji MAEDA, Keisuke FUKUI, Hidetoshi KURAMOCHI
    • Journal Title

      Crystal Research and Technology

      Volume: 52 Issue: 2 Pages: 1600316-1600316

    • DOI

      10.1002/crat.201600316

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Molecular dynamics study on phase equilibriumaround vapor bubbles in low-density liquid argon2017

    • Author(s)
      Kazuhiro ITOH, Yuto KISA, Takuji YAMAMOTO, Kouji MAEDA
    • Journal Title

      Journal of Molecular Liquids

      Volume: 230 Pages: 322-328

    • DOI

      10.1016/j.molliq.2016.12.118

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Consecutive Vacuum Degassing and Steam Treatment of Sewage Sludge using a Steam Ejector2017

    • Author(s)
      伊藤和宏, 山本拓司, 前田光治, 立川浩史
    • Journal Title

      KAGAKU KOGAKU RONBUNSHU

      Volume: 43 Issue: 1 Pages: 57-62

    • DOI

      10.1252/kakoronbunshu.43.57

    • NAID

      130005290196

    • ISSN
      0386-216X, 1349-9203
    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Presentation] 融液晶析による脂肪酸混合物の分離・精製2019

    • Author(s)
      大西沙季,伊藤和宏,前田光治,山本拓司
    • Organizer
      第21回化学工学会学生発表会(京都大会)
    • Related Report
      2018 Annual Research Report
  • [Presentation] オレイン酸+リノール酸2成分系の高圧固液平衡の測定2019

    • Author(s)
      内藤洋輔,前田光治,新船幸二,伊藤和宏,山本拓司,倉持秀敏
    • Organizer
      第21回化学工学会学生発表会(京都大会)
    • Related Report
      2018 Annual Research Report
  • [Presentation] 珪藻細胞のマイクロバブル濃縮に対する気泡径の寄与2019

    • Author(s)
      中筋 智樹,伊藤 和宏,菓子野 康浩,伊福 健太郎,前田 光治,山本 拓司
    • Organizer
      第21回化学工学会学生発表会(京都大会)
    • Related Report
      2018 Annual Research Report
  • [Presentation] Effect of Taylor Vortex in Melt Crystallization of Fatty Acids2018

    • Author(s)
      T. Yamamoto, T. Inoue, Y. Hayashi, K. Itoh, K. Fukui, K. Maeda
    • Organizer
      Asian Crystallization Technology Symposium 2018
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Distribution of Hydrogen in Electroless Nickel-Phosphorus Plating under High Pressure2018

    • Author(s)
      H. Yokohama, Y. Yoshida, N. Fukumuro, S. Yae, K. Itoh, K. Maeda, T. Yamamoto
    • Organizer
      Asian Crystallization Technology Symposium 2018
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Effect of High Pressure on Growth of Colloidal Particles during Sol-Gel Phase Transition of Resorcinol-Formaldehyde Solution2018

    • Author(s)
      T. Yamamoto, M. Tayakout-Fayolle, T. Kakibe, H. Satone, K. Iimura, K. Itoh, K. Maeda
    • Organizer
      8th Pacific Basin Conference on Adsorption Science and Technology
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Kinetic Modelling of Electroless Nickel-Phosphorus Plating under High Pressure2018

    • Author(s)
      H. Yokohama, M. Tayakout-Fayolle, N. Fukumuro, S. Yae, K. Itoh, K. Maeda, T. Yamamoto
    • Organizer
      8th Pacific Basin Conference on Adsorption Science and Technology
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 高速空気注入型エアレーターの効率評価に関する研究2018

    • Author(s)
      小松大祐,伊藤和宏,吉田憲史,山本拓司,前田光治
    • Organizer
      化学工学会学生発表会2018
    • Related Report
      2017 Research-status Report
  • [Presentation] 微小蒸気泡の安定性に関する分子動力学解析2017

    • Author(s)
      伊藤和宏,木佐悠人,山本拓司,前田光治
    • Organizer
      日本混相流学会 混相流シンポジウム2017
    • Related Report
      2017 Research-status Report
  • [Presentation] Growth of colloidal particles during sol-gel phase transition of resorcinol-formaldehyde solution under high pressure2017

    • Author(s)
      T. Yamamoto, M. Tayakout-Fayolle, T. Kakibe, H. Satone, K. Iimura, K. Itoh, K. Maeda
    • Organizer
      The 20th International Symposium on Industrial Crystallization
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research
  • [Presentation] 高圧力下における無電解ニッケル-リンめっきの反応機構2017

    • Author(s)
      横濱大空,Tayakout-Fayolle Melaz,福室直樹,八重真治,伊藤和宏,前田光治,山本拓司
    • Organizer
      化学工学会第49回秋季大会
    • Related Report
      2017 Research-status Report
  • [Presentation] 高圧力が無電解ニッケル-リンめっきに与える効果 -泡のでないめっき-2017

    • Author(s)
      横濱大空,福室直樹,八重真治,伊藤和宏,前田光治,山本拓司
    • Organizer
      兵庫県立大学知の交流シンポジウム2017
    • Related Report
      2017 Research-status Report
  • [Presentation] 高圧力下での無電解ニッケル-リンめっきにおける水素の分配2017

    • Author(s)
      横濱大空,吉田悠一郎,福室直樹,八重真治,伊藤和宏,前田光治,山本拓司
    • Organizer
      化学工学会金沢大会2017
    • Related Report
      2017 Research-status Report
  • [Presentation] モデルバイオ燃料としての脂肪酸の2成分系混合物の融液晶析2017

    • Author(s)
      山本拓司, 前田光治, 伊藤和宏, 福井啓介, 倉持秀敏
    • Organizer
      化学工学会第82年会
    • Place of Presentation
      芝浦工業大学豊洲キャンパス
    • Related Report
      2016 Research-status Report
  • [Presentation] モデルバイオ燃料としての脂肪酸の2成分系混合物の融液晶析2017

    • Author(s)
      山本拓司
    • Organizer
      兵庫県立大学大学院工学研究科次世代分散型エネルギー研究センターシンポジウム
    • Place of Presentation
      兵庫県立大学姫路工学キャンパス書写紀念会館
    • Related Report
      2016 Research-status Report
  • [Presentation] 高圧力下での無電解ニッケル-リンめっき2017

    • Author(s)
      横濱大空, 山本拓司, 前田光治, 八重真治, 福室直樹
    • Organizer
      第19回化学工学会学生発表会(豊中大会)
    • Place of Presentation
      大阪大学豊中キャンパス
    • Related Report
      2016 Research-status Report
  • [Presentation] ベンチュリ管式マイクロバブル発生装置が珪藻細胞の破壊と濃縮に及ぼす影響2017

    • Author(s)
      都筑功, 伊藤和宏, 菓子野康浩, 伊福健太郎, 山本拓司, 前田光治
    • Organizer
      第19回化学工学会学生発表会(豊中大会)
    • Place of Presentation
      大阪大学豊中キャンパス
    • Related Report
      2016 Research-status Report
  • [Presentation] Nucleation and growth of nano-particles during sol-gel reaction of resorcinol-formaldehyde solution under high pressure2016

    • Author(s)
      Takuji YAMAMOTO, Melaz TAYAKOUT-FAYOLLE, Hiroshi SATONE, Tadashi NAKAZAWA, Asaki TANABE, Kenji IIMURA, Kouji MAEDA
    • Organizer
      The 20th International Drying Symposium (IDS2016)
    • Place of Presentation
      長良川コンベンションセンター
    • Year and Date
      2016-08-07
    • Related Report
      2016 Research-status Report
  • [Presentation] 融液晶析を利用した物質の分離・精製2016

    • Author(s)
      山本拓司, 林保典, 井上貴博, 伊藤和宏, 前田光治
    • Organizer
      企業・大学・学生マッチング in HIMEJI 2016
    • Place of Presentation
      兵庫県立大学姫路工学キャンパス体育館
    • Related Report
      2016 Research-status Report
  • [Presentation] 相互貧溶媒晶析法の分子動力学による検討2016

    • Author(s)
      市川遥雄, 前田光治, 新船幸二, 伊藤和宏, 山本拓司
    • Organizer
      化学工学会第48回秋季大会
    • Place of Presentation
      徳島大学常三島キャンパス
    • Related Report
      2016 Research-status Report

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Published: 2016-04-21   Modified: 2020-03-30  

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