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Nanoscale Observation of Liquid-Gas Phase Change Using Transmission Electron Microscopy

Research Project

Project/Area Number 16K14174
Research Category

Grant-in-Aid for Challenging Exploratory Research

Allocation TypeMulti-year Fund
Research Field Thermal engineering
Research InstitutionKyushu University

Principal Investigator

Takahashi Koji  九州大学, 工学研究院, 教授 (10243924)

Co-Investigator(Kenkyū-buntansha) 生田 竜也  九州大学, 工学研究院, 技術専門職員 (70532331)
Project Period (FY) 2016-04-01 – 2018-03-31
Project Status Completed (Fiscal Year 2017)
Budget Amount *help
¥3,770,000 (Direct Cost: ¥2,900,000、Indirect Cost: ¥870,000)
Fiscal Year 2017: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Fiscal Year 2016: ¥2,340,000 (Direct Cost: ¥1,800,000、Indirect Cost: ¥540,000)
Keywordsナノバブル / 不均質核生成 / ナノマイクロ熱工学 / 透過電子顕微鏡 / カーボンナノチューブ / 透過型電子顕微鏡
Outline of Final Research Achievements

This study investigated the generation and growth of nanobubbles using liquid cell electron microscopy. We developed the Fresnel fringe method, which enables us to determine the location of bubble interface in transmission electron microscopy (TEM) observation. It was found that heterogeneous nucleation is the major mechanism even in the thin water of 600 nm thickness. Hydrophilized carbon nanotubes were also tested and water film adhering to most of the inner wall surface was observed. Also, suspended ultrathin water films were found inside the CNT. The stability of these water films is attributed to the additional molecular interactions in the carbon nanotubes.

Report

(3 results)
  • 2017 Annual Research Report   Final Research Report ( PDF )
  • 2016 Research-status Report
  • Research Products

    (12 results)

All 2018 2017 2016 Other

All Int'l Joint Research (1 results) Journal Article (2 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 2 results,  Acknowledgement Compliant: 1 results) Presentation (9 results) (of which Int'l Joint Research: 6 results,  Invited: 2 results)

  • [Int'l Joint Research] エジンバラ大学(英国)

    • Related Report
      2017 Annual Research Report
  • [Journal Article] Superstable Ultrathin Water Film Confined in a Hydrophilized Carbon Nanotube2018

    • Author(s)
      Tomo Yoko、Askounis Alexandros、Ikuta Tatsuya、Takata Yasuyuki、Sefiane Khellil、Takahashi Koji
    • Journal Title

      Nano Letters

      Volume: 18 Issue: 3 Pages: 1869-1874

    • DOI

      10.1021/acs.nanolett.7b05169

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Nanobubble nucleation studied using Fresnel fringes in liquid cell electron microscopy2017

    • Author(s)
      Yoko TOMO, Koji TAKAHASHI, Takashi NISHIYAMA, Tatsuya IKUTA, Yasuyuki TAKATA
    • Journal Title

      International Journal of Heat and Mass Transfer

      Volume: 108 Pages: 1460-1465

    • DOI

      10.1016/j.ijheatmasstransfer.2017.01.013

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Presentation] Bubble Generation and Growth in a Nano Liquid Cell and a Carbon Nanotube2018

    • Author(s)
      Yoko Tomo, Alexandros Askounis, Yasuyuki Takata, Koji Takahashi
    • Organizer
      5th European Conference on MicroFluidics 2018
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Three dimensional investigation of bubble formation in liquid cell electron microscopy2017

    • Author(s)
      Yoko Tomo, Koji Takahashi, Takashi Nishiyama, Tatsuya Ikuta, Yasuyuki Takata
    • Organizer
      the 6th International Symposium on Micro and Nano Technology, ISMNT-6
    • Place of Presentation
      Fukuoka, Japan
    • Year and Date
      2017-03-19
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research
  • [Presentation] AFM and TEM studies on nanobubbles2017

    • Author(s)
      Koji Takahashi
    • Organizer
      9th NFS-JSPS US-Japan Joint Seminar on Nanoscale Transport Phenomena
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Direct Observation of Heterogeneous Bubble Nucleation in Nanoscale2017

    • Author(s)
      Yoko Tomo, Koji Takahashi, Tatsuya Ikuta, Yasuyuki Takata
    • Organizer
      International conference on nanochannels, microchannels, and minichannels
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 透過型電子顕微鏡を用いた気液界面挙動の観察2017

    • Author(s)
      塘陽子、高橋厚史、西山貴史、生田竜也、高田保之
    • Organizer
      第54回日本伝熱シンポジウム
    • Related Report
      2017 Annual Research Report
  • [Presentation] 固液界面ナノバブルの実験について2017

    • Author(s)
      高橋厚史
    • Organizer
      相変化界面研究会2017沖縄
    • Related Report
      2017 Annual Research Report
  • [Presentation] ナノスケールの気相生成に関する実験的研究2016

    • Author(s)
      塘陽子、高橋厚史、西山貴史、生田竜也、高田保之
    • Organizer
      日本機械学会熱工学コンファレンス
    • Place of Presentation
      松山市
    • Year and Date
      2016-10-22
    • Related Report
      2016 Research-status Report
  • [Presentation] TEM Study on Phase Change in a Nano Liquid Cell2016

    • Author(s)
      Yoko TOMO, Koji TAKAHASHI, Takashi NISHIYAMA, Tatsuya IKUTA, Yasuyuki TAKATA
    • Organizer
      5th Micro and Nano Flows Conference
    • Place of Presentation
      Milan, Italy
    • Year and Date
      2016-09-11
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research
  • [Presentation] Experimental Study of Nanobubbles and Nanodroplets on Hydrophilic/Hydrophobic Combined Surfaces2016

    • Author(s)
      Takahashi K., Nishiyama T., Yamada Y. and Takata Y.
    • Organizer
      12th International Conference on Heat Transfer, Fluid Mechanics and Thermodynamics
    • Place of Presentation
      Costa del Sol, Spain
    • Year and Date
      2016-07-11
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research / Invited

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Published: 2016-04-21   Modified: 2022-06-16  

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