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Research for the magnetic and electronic states of the quaternary Heusler alloys with high spin polarization

Research Project

Project/Area Number 16K14370
Research Category

Grant-in-Aid for Challenging Exploratory Research

Allocation TypeMulti-year Fund
Research Field Physical properties of metals/Metal-base materials
Research InstitutionTohoku University

Principal Investigator

Umetsu Rie  東北大学, 金属材料研究所, 准教授 (60422086)

Project Period (FY) 2016-04-01 – 2018-03-31
Project Status Completed (Fiscal Year 2017)
Budget Amount *help
¥3,640,000 (Direct Cost: ¥2,800,000、Indirect Cost: ¥840,000)
Fiscal Year 2017: ¥1,820,000 (Direct Cost: ¥1,400,000、Indirect Cost: ¥420,000)
Fiscal Year 2016: ¥1,820,000 (Direct Cost: ¥1,400,000、Indirect Cost: ¥420,000)
Keywordsホイスラー合金 / ハーフメタル型電子状態 / 原子配列 / 磁気モーメント / 粉末中性子回折 / 磁性・電子・情報材料
Outline of Final Research Achievements

The objective of the present study is to search new quaternary Heuseler alloys with high spin polarization and to experimentally confirm the half-metallic electronic state. CoVMnAl and CrTiVAl alloys were fabricated and powder neutron diffraction experiments were performed in order to decide the atomic configuration. It is cleared that both alloys include a part of disordering and the results are different to the previous report. Furthermore, absorption x-ray spectroscopy and resonant inelastic x-ray scattering in magnetic field were experienced in SPring-8 with using Mn2VAl and Co2MnSi single crystals, that are typical materials as the half-metallic ferro-(ferri-)magnets. Obtained spectra are well reproduced by the simulated ones based on the density functional theory. It is said that these experiments are powerful tool to confirm the characteristic electronic state of the half-metallic materials.

Report

(3 results)
  • 2017 Annual Research Report   Final Research Report ( PDF )
  • 2016 Research-status Report
  • Research Products

    (26 results)

All 2018 2017 2016 Other

All Int'l Joint Research (1 results) Journal Article (5 results) (of which Peer Reviewed: 5 results,  Open Access: 3 results) Presentation (19 results) (of which Int'l Joint Research: 4 results,  Invited: 2 results) Remarks (1 results)

  • [Int'l Joint Research] Nat. Univ. Science and Technology(ロシア連邦)

    • Related Report
      2017 Annual Research Report
  • [Journal Article] Pressure effect on the magnetic properties of the half-metallic Heusler alloy Co2TiSn2018

    • Author(s)
      Shigeta Iduru、Fujimoto Yutaro、Ooka Ryutaro、Nishisako Yuya、Tsujikawa Masahito、Umetsu Rie Y.、Nomura Akiko、Yubuta Kunio、Miura Yoshio、Kanomata Takeshi、Shirai Masafumi、Gouchi Jun、Uwatoko Yoshiya、Hiroi Masahiko
    • Journal Title

      Physical Review B

      Volume: 97 Issue: 10 Pages: 104414-104414

    • DOI

      10.1103/physrevb.97.104414

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Electronic structure and magnetic properties of the half-metallic ferrimagnet Mn2VAl probed by soft x-ray spectroscopies2018

    • Author(s)
      Nagai K.、Fujiwara H.、Aratani H.、Fujioka S.、Yomosa H.、Nakatani Y.、Kiss T.、Sekiyama A.、Kuroda F.、Fujii H.、Oguchi T.、Tanaka A.、Miyawaki J.、Harada Y.、Takeda Y.、Saitoh Y.、Suga S.、Umetsu R. Y.
    • Journal Title

      Physical Review B

      Volume: 97 Issue: 3 Pages: 035143-035143

    • DOI

      10.1103/physrevb.97.035143

    • NAID

      120006731610

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Temperature dependences of the electrical resistivity on the Heusler alloy system Ni2MnGa1-xFex2017

    • Author(s)
      Y. Adachi, Y. Ogi, N. Kobayashi, Y. Hayasaka, T. Kanomata, Rie Y. Umetsu, X. Xu and R. Kainuma
    • Journal Title

      Metals

      Volume: 7 Issue: 10 Pages: 413-413

    • DOI

      10.3390/met7100413

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Evidence of the change in the density of states during the martensitic transformation of Ni-Mn-In metamagnetic shape memory alloys2017

    • Author(s)
      R.Y. Umetsu, X. Xu, W. Ito and R. Kainuma
    • Journal Title

      Metals

      Volume: 7 Issue: 10 Pages: 414-414

    • DOI

      10.3390/met7100414

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] High Field X-ray diffraction study for Ni46.4Mn38.8In12.8Co2.0 metamagnetic shape memory film2017

    • Author(s)
      Y. Mitsui, K. Koyama, M. Ohtsuka, R.Y. Umetsu, R. Kainuma, and K. Watanabe
    • Journal Title

      Metals

      Volume: 7 Issue: 9 Pages: 364-364

    • DOI

      10.3390/met7090364

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Presentation] 磁場中軟X線共鳴発光分光によるハーフメタル型ホイスラー合金Mn2VAlの電子構造研究2018

    • Author(s)
      藤原秀紀, 梅津理恵, 永井浩大, 中谷泰博, 川田萌樹, 関山明, 黒田文彬, 藤井将, 小口多美夫, 原田慈久, 宮脇淳, 菅滋正
    • Organizer
      第30回日本放射光学会年会・放射光科学合同シンポジウム
    • Related Report
      2017 Annual Research Report
  • [Presentation] Pd基ホイスラー合金PdMnSnの相転移温度の圧力効果2018

    • Author(s)
      福本拓実、安達 義也、相澤直輝、鹿又武、梅津理恵、宍戸統悦、小原和夫、許キョウ、貝沼亮介
    • Organizer
      日本金属学会2018年春期講演大会(第162回)
    • Related Report
      2017 Annual Research Report
  • [Presentation] ハーフメタル型ホイスラー合金Mn2VAlの磁場中における共鳴非弾性X線散乱測定2017

    • Author(s)
      梅津理恵、永井浩大, 藤原秀紀、中谷泰博、川田萌樹、右衛門佐寛、関山明、宮脇淳、原田慈久、菅滋正、鹿又武
    • Organizer
      日本物理学会第75回年次大会
    • Place of Presentation
      大阪大学
    • Year and Date
      2017-03-17
    • Related Report
      2016 Research-status Report
  • [Presentation] 軟X線吸収磁気円二色性によるフェリ磁性体Mn2VAl単結晶の磁性・電子構造研究2017

    • Author(s)
      永井浩大, 藤原秀紀, 荒谷秀和, 藤岡修平, 右衛門佐寛, 木須孝幸, 関山明, 菅滋正, 黒田文彬, 藤井将, 小口多美夫, 田中新, 竹田幸治, 斎藤祐児, 鹿又武, 梅津理恵
    • Organizer
      日本物理学会第75回年次大会
    • Place of Presentation
      大阪大学
    • Year and Date
      2017-03-17
    • Related Report
      2016 Research-status Report
  • [Presentation] L21構造を有するMn2VAlホイスラー合金の磁場中共鳴非弾性X線散乱測定2017

    • Author(s)
      梅津理恵、永井浩大、藤原秀紀、中谷泰博、川田萌樹、右衛門佐寛、関山明、宮脇淳、原田慈久、菅滋正、鹿又武
    • Organizer
      日本金属学会2017年春期(第160回)講演大会
    • Place of Presentation
      首都大学東京
    • Year and Date
      2017-03-15
    • Related Report
      2016 Research-status Report
  • [Presentation] 軟X線磁気円二色性によるハーフメタルホイスラー合金Mn2VAlの電子構造研究2017

    • Author(s)
      永井浩大, 藤原秀紀, 荒谷秀和, 藤岡修平, 右衛門佐寛, 木須孝幸, 黒田文彬, 藤井将, 小口多美夫, 田中新, 梅津理恵, 菅滋正, 竹田幸治, 斎藤祐児, 関山明
    • Organizer
      第30回日本放射光学会年会・放射光科学合同シンポジウム
    • Place of Presentation
      神戸芸術センター
    • Year and Date
      2017-01-07
    • Related Report
      2016 Research-status Report
  • [Presentation] Atomic configuration and magnetic properties of Co- and Mn-based Heusler alloys2017

    • Author(s)
      R.Y. Umetsu
    • Organizer
      Frontiers in Materials Processing Applications, Research and Technology
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Effect of annealing temperature on the degree of order and magnetic properties of CoVMnAl alloy2017

    • Author(s)
      R.Y. Umetsu, K. Saito, K. Ono, T. Ishigaki
    • Organizer
      Yamada Science Foundation, Junjiro Kanamori Memorial International Symposium, New Horizon of Magnetism
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Anisotropic Magnetic Properties and Cr Substitution Effects on the Curie Temperature of MnAlGe Layered Compounds2017

    • Author(s)
      R.Y. Umetsu, Y. Mitsui, J. Xia, H. Katsui, Y. Nozaki, I. Yuitoo, T. Takeuchi, T. Taniyama, H. Kawarada
    • Organizer
      2nd International Symposium on Creation of Life Innovation Materials for Interdisciplinary and International Researcher Development (iLIM-2)
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Atomic configuration and magnetic properties of CoVMnAl alloy2017

    • Author(s)
      R.Y. Umetsu, K. Saito, K. Ono, T. Ishigaki
    • Organizer
      62nd Annunal Conference on Magnetism and Magnetic Materials
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Co2NbSn1-xGaxの磁化と相転移温度の圧力効果2017

    • Author(s)
      小木雄貴、安達義也、佐々木達治、鹿又武、梅津理恵、湯蓋邦夫、許キョウ、貝沼亮介、郷地順、上床美也
    • Organizer
      日本金属学会2017 年秋期講演大会(第161回)
    • Related Report
      2017 Annual Research Report
  • [Presentation] Co 基ホイスラー合金の相安定性と特異なマルテンサイト変態(基調講演)2017

    • Author(s)
      貝沼亮介、許皛、梅津理恵
    • Organizer
      日本金属学会2017 年秋期講演大会(第161回)
    • Related Report
      2017 Annual Research Report
  • [Presentation] 円偏光放射光分光を用いたホイスラー型高スピン偏極材料の電子状態の研究(基調講演)2017

    • Author(s)
      梅津理恵、藤原秀紀、宮脇淳、菅滋正
    • Organizer
      日本金属学会2017 年秋期講演大会(第161回)
    • Related Report
      2017 Annual Research Report
  • [Presentation] 強磁性ホイスラー合金 Mn2VAl の中性子回折2017

    • Author(s)
      小野寛太、斉藤耕太郎、梅津理恵、土屋朋生、窪田崇秀、大原高志、中尾朗子、高梨弘毅
    • Organizer
      日本金属学会2017 年秋期講演大会(第161回)
    • Related Report
      2017 Annual Research Report
  • [Presentation] 圧力下におけるCo基ホイスラー合金Co2TiGaの磁気特性2017

    • Author(s)
      大岡隆太郎、重田出、梅津理恵、野村明子、湯蓋邦夫、上床美也、鹿又武、廣井政彦
    • Organizer
      日本物理学会2017年秋季大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] ハーフメタル型ホイスラー合金Co2TiSnの磁化の圧力効果とスピンゆらぎ理論の解析2017

    • Author(s)
      重田出, 大岡隆太郎, 梅津理恵, 野村明子, 湯葢邦夫, 鹿又武, 上床美也, 廣井政彦
    • Organizer
      日本物理学会2017年秋季大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 高スピン分極ホイスラー合金Co2TiGa1-xSnxと超伝導体Pbのアンドレーエフ反射接合における微分コンダクタンスの温度依存性2017

    • Author(s)
      大岡隆太郎, 重田出, 梅津理恵, 野村明子, 湯蓋邦夫, 山内徹, 鹿又武, 廣井政彦
    • Organizer
      日本物理学会2017年秋季大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] ホイスラー合金Co2TiSnの磁化の圧力効果とスピンゆらぎ理論の解析2016

    • Author(s)
      大岡隆太朗、藤本祐太郎、重田出、梅津理恵、野村明子、湯葢邦夫、鹿又武、上床美也、廣井政彦
    • Organizer
      日本物理学会2016年秋季大会
    • Place of Presentation
      金沢大学
    • Year and Date
      2016-09-13
    • Related Report
      2016 Research-status Report
  • [Presentation] ホイスラー合金Co2TiGa1-xSnxの磁化とスピン分極率2016

    • Author(s)
      大岡隆太朗、鋤野好美、藤本祐太郎、重田出、梅津理恵、三浦良雄、野村明子、湯葢邦夫、山内恭彦、鹿又武、廣井政彦
    • Organizer
      日本物理学会2016年秋季大会
    • Place of Presentation
      金沢大学
    • Year and Date
      2016-09-13
    • Related Report
      2016 Research-status Report
  • [Remarks] 東北大学研究者紹介

    • URL

      http://db.tohoku.ac.jp/whois/detail/b51713d5148969420b77255b303f0d00.html

    • Related Report
      2016 Research-status Report

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Published: 2016-04-21   Modified: 2022-07-19  

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