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Development of isotope analysis method using supersonic plasma wind tunnel and spectral resolution enhancement by low-temperature plasma

Research Project

Project/Area Number 16K14542
Research Category

Grant-in-Aid for Challenging Exploratory Research

Allocation TypeMulti-year Fund
Research Field Nuclear engineering
Research InstitutionJapan Atomic Energy Agency

Principal Investigator

Kuwahara Akira  国立研究開発法人日本原子力研究開発機構, 原子力科学研究部門 原子力科学研究所 バックエンド技術部, 技術・技能職 (50732418)

Project Period (FY) 2016-04-01 – 2018-03-31
Project Status Completed (Fiscal Year 2017)
Budget Amount *help
¥3,640,000 (Direct Cost: ¥2,800,000、Indirect Cost: ¥840,000)
Fiscal Year 2017: ¥1,690,000 (Direct Cost: ¥1,300,000、Indirect Cost: ¥390,000)
Fiscal Year 2016: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Keywords同位体分析 / レーザー吸収分光 / 同位体シフト / 超音速プラズマ / プラズマ風洞 / ドップラー広がり / レーザー分光 / 同位体比分析 / プラズマ分光 / 原子力工学
Outline of Final Research Achievements

An isotope analysis method based on diode laser absorption spectroscopy using supersonic plasma jet has been developed. First, the translation temperature and flow velocity downstream of a supersonic nozzle are measured using an atomic argon transition of 826.45 nm from an excited state.
Next, the trace gas measurement capability is verified injecting natural xenon in the argon plasma, and optical measurements are carried out at an atomic xenon transition to 823.16 nm. The detection limit of xenon over the argon molar ratio is estimated to be 140 parts per million downstream.
Finally, in order to enhance spectral resolution drastically by supersonic plasma jet, a demonstration was carried out using natural stable xenon isotopes. As a result, the temperature was found to be about 180 K and the spectral resolution was about one order of magnitude higher than that of the conventional high-temperature source such as laser ablation plasma plume.

Report

(3 results)
  • 2017 Annual Research Report   Final Research Report ( PDF )
  • 2016 Research-status Report
  • Research Products

    (11 results)

All 2018 2017 2016

All Journal Article (1 results) (of which Peer Reviewed: 1 results) Presentation (9 results) (of which Int'l Joint Research: 3 results) Patent(Industrial Property Rights) (1 results)

  • [Journal Article] Development of an isotope analysis method based on diode laser absorption spectroscopy using an arc-jet plasma wind tunnel2018

    • Author(s)
      Kuwahara Akira、Aiba Yasuaki、Nankawa Takuya、Matsui Makoto
    • Journal Title

      Journal of Analytical Atomic Spectrometry

      Volume: 印刷中 Issue: 5 Pages: 893-896

    • DOI

      10.1039/c8ja00040a

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Presentation] Development of Isotope Analytical Method Based on Diode Laser Absorption Spectroscopy Using Arc-Jet Plasma Wind Tunnel2018

    • Author(s)
      Akira Kuwahara, Aiba Yasuaki, Takuya Nankawa, Makoto Matsui
    • Organizer
      2018 Winter Conference on Plasma Spectrochemistry
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Atomization of Strontium Powders Using Arcjet for Isotope Detection System2018

    • Author(s)
      Aiba Yasuaki, Akira Kuwahara, Makoto Matsui
    • Organizer
      11st International Workshop on Hybrid Functionally Materials
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 同位体分析のための光共振器を用いた 高感度レーザー吸収分光システムの開発2018

    • Author(s)
      桑原彬、南川卓也、松井信
    • Organizer
      日本原子力学会2018年春の年会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 塩化ストロンチウム粉末を混合したアルゴンアークジェットの発光スペクトルの相対強度測定2018

    • Author(s)
      相羽祇亮、桑原彬、松井信
    • Organizer
      第65回応用物理学会春季学術講演会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Investigation of Al2O3 plasma reduction by liquid phase samples using laser absorption spectroscopy2017

    • Author(s)
      Akira Kuwahara, Yasuaki Aiba and Makoto Matsui
    • Organizer
      2017 International Symposium Toward the Future of Advanced Researches in Shizuoka University
    • Place of Presentation
      静岡大学(静岡県静岡市)
    • Year and Date
      2017-02-27
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research
  • [Presentation] 半導体レーザーを用いた同位体分析における圧力広がりの影響2017

    • Author(s)
      桑原彬、南川卓也、相羽祇亮、松井信
    • Organizer
      平成29年度北関東支部原子力学会若手研究発表会
    • Related Report
      2017 Annual Research Report
  • [Presentation] アークジェットプラズマを用いたレーザー分光分析の特性評価2017

    • Author(s)
      桑原彬、相羽祇亮、南川卓也、松井信
    • Organizer
      日本原子力学会2017年秋の大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 同位体分析のためのアークプラズマ風洞を用いたストロンチウム粉末試料の原子化2017

    • Author(s)
      相羽祇亮、桑原彬、松井信
    • Organizer
      第78回応用物理学会秋季学術講演会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 飽和吸収分光におけるスペクトル形状の評価2016

    • Author(s)
      桑原彬、相羽祇亮、松井信、南川卓也
    • Organizer
      平成28年度北関東支部原子力学会若手研究発表会
    • Place of Presentation
      東海会館(茨城県東海村)
    • Year and Date
      2016-04-15
    • Related Report
      2016 Research-status Report
  • [Patent(Industrial Property Rights)] 同位体分析装置及び同位体分析方法2017

    • Inventor(s)
      桑原彬、南川卓也、藤平俊夫、松井信
    • Industrial Property Rights Holder
      桑原彬、南川卓也、藤平俊夫、松井信
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      2017-064440
    • Filing Date
      2017-03-29
    • Related Report
      2016 Research-status Report

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Published: 2016-04-21   Modified: 2019-03-29  

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