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Investigations on morphology effect and quantum properties of single luminescent nanomaterial

Research Project

Project/Area Number 16K17483
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeMulti-year Fund
Research Field Nanostructural physics
Research InstitutionNational Institute of Information and Communications Technology (2017)
Kyoto University (2016)

Principal Investigator

Ihara Toshiyuki  国立研究開発法人情報通信研究機構, 未来ICT研究所フロンティア創造総合研究室, 研究員 (10619860)

Project Period (FY) 2016-04-01 – 2018-03-31
Project Status Completed (Fiscal Year 2017)
Budget Amount *help
¥4,290,000 (Direct Cost: ¥3,300,000、Indirect Cost: ¥990,000)
Fiscal Year 2017: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2016: ¥3,250,000 (Direct Cost: ¥2,500,000、Indirect Cost: ¥750,000)
Keywordsナノ発光材料 / 半導体ナノ粒子 / コロイド量子ドット / 強度相関 / 発光寿命 / カスケード発光 / 光吸収断面積 / スペクトル拡散 / ナノ粒子 / 量子ドット / 単一ドット / 励起子分子 / 単一光子 / イオン化 / 吸収断面積 / モルフォロジー / 光子相関 / 発光効率 / ナノ材料 / 半導体物性
Outline of Final Research Achievements

We studied the effect of size, shape, and composition, to the properties of luminescent nanomaterial such as semiconductor nanocrystals. We developed new techniques for revealing optical properties of single nano objects by combining microscopy and time-correlated single photon counting methods. Using the developed techniques, we studied the cascade emission process, where two photons are sequentially emitted from a single nano object. We elucidated that, by analysing the cascade emission process, one can deteremine the optical properties of single nano objects, such as absorption cross section and the ratio of radiative recombination rate of the two-photon emission process.

Report

(3 results)
  • 2017 Annual Research Report   Final Research Report ( PDF )
  • 2016 Research-status Report
  • Research Products

    (19 results)

All 2018 2017 2016 Other

All Int'l Joint Research (2 results) Journal Article (7 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 7 results,  Acknowledgement Compliant: 3 results) Presentation (10 results) (of which Int'l Joint Research: 3 results,  Invited: 1 results)

  • [Int'l Joint Research] National (Taiwan) University/National Taipei University of Technology(Taiwan)

    • Related Report
      2017 Annual Research Report
  • [Int'l Joint Research] Southern University of Science and Tech.(China)

    • Related Report
      2017 Annual Research Report
  • [Journal Article] Simultaneously measured photoluminescence lifetime and quantum yield of two-photon cascade emission on single CdSe/ZnS nanocrystals2017

    • Author(s)
      Hiroshige Nao、Ihara Toshiyuki、Kanemitsu Yoshihiko
    • Journal Title

      Physical Review B

      Volume: 95 Issue: 24

    • DOI

      10.1103/physrevb.95.245307

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] High-Performance CsPb1xSnxBr3 Perovskite Quantum Dots for Light-Emitting Diodes2017

    • Author(s)
      Wang Hung-Chia、Wang Weigao、Tang An-Cih、Tsai Hsin-Yu、Bao Zhen、Ihara Toshiyuki、Yarita Naoki、Tahara Hirokazu、Kanemitsu Yoshihiko、Chen Shuming、Liu Ru-Shi
    • Journal Title

      Angewandte Chemie International Edition

      Volume: 56 Issue: 44 Pages: 13650-13654

    • DOI

      10.1002/anie.201706860

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Enhanced radiative recombination rate for electron-hole droplets in a silicon photonic crystal nanocavity2017

    • Author(s)
      Toshiyuki Ihara, Yasushi Takahashi, Susumu Noda, and Yoshihiko Kanemitsu
    • Journal Title

      Physical Review B

      Volume: 96 Issue: 3 Pages: 035303-035303

    • DOI

      10.1103/physrevb.96.035303

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Coulomb-Enhanced Radiative Recombination of Biexcitons in Single Giant-Shell CdSe/CdS Core/Shell Nanocrystals2017

    • Author(s)
      Nao Hiroshige, Toshiyuki Ihara, Masaki Saruyama, Toshiharu Teranishi, and Yoshihiro Kanemitsu
    • Journal Title

      Journal of Physical Chemistry Letters

      Volume: 8 Issue: 9 Pages: 1961-1966

    • DOI

      10.1021/acs.jpclett.7b00547

    • Related Report
      2016 Research-status Report
    • Peer Reviewed
  • [Journal Article] Dynamics of Charged Excitons and Biexcitons in CsPbBr2 Perovskite Nanocrystals Revealed by Femtosecond Transient-absorption and Single-dot Luminescence Spectroscopy2017

    • Author(s)
      Naoki Yarita, Hirokazu Tahara, Toshiyuki Ihara, Tokuhisa Kawawaki, Ryota Sato, Masaki Saruyama, Toshiharu Teranishi, Yoshihiko Kanemitsu
    • Journal Title

      J. Phys. Chem. Lett.

      Volume: 8 Issue: 7 Pages: 1413-1418

    • DOI

      10.1021/acs.jpclett.7b00326

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Biexciton cascade emission reveals absolute absorption cross section of single semiconductor nanocrystals2016

    • Author(s)
      Toshiyuki Ihara
    • Journal Title

      Physical Review B

      Volume: 93 Issue: 23

    • DOI

      10.1103/physrevb.93.235442

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Spectral Diffusion of Emissions of Excitons and Trions in Single CdSe/ ZnS Nanocrystals: Charge Fluctuations in and around Nanocrystals2016

    • Author(s)
      Hiroto Ibuki, Toshiyuki Ihara, and Yoshihiko Kanemitsu
    • Journal Title

      The Journal of Physical Chemistry C

      Volume: 120 Issue: 41 Pages: 23772-23779

    • DOI

      10.1021/acs.jpcc.6b06220

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Presentation] Advanced time-resolving analysis of room-temperature cascade emission from single quantum dots2018

    • Author(s)
      T. Ihara, T. Kaji, T. Yamada, and A. Otomo
    • Organizer
      SPIE photonics west
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 単一ドット発光の強度相関に対する2パルス励起子分子生成過程の影響2018

    • Author(s)
      井原章之, 梶貴博, 山田俊樹, 大友明
    • Organizer
      日本物理学会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 励起分光法を活用した単一低次元系の量子光物性の研究2017

    • Author(s)
      井原章之
    • Organizer
      日本物理学会
    • Place of Presentation
      大阪大学
    • Year and Date
      2017-03-17
    • Related Report
      2016 Research-status Report
    • Invited
  • [Presentation] タイムタグ計測を活用した単一ナノ粒子の2光子カスケード発光の研究2017

    • Author(s)
      井原章之, 広重直
    • Organizer
      応用物理学会
    • Place of Presentation
      パシフィコ横浜
    • Year and Date
      2017-03-14
    • Related Report
      2016 Research-status Report
  • [Presentation] タイムゲートを活用した単一ドット発光の強度相関解析2017

    • Author(s)
      井原章之, 梶貴博, 山田俊樹, 大友明
    • Organizer
      応用物理学会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Quantitative study on photoluminescence properties of single nanocrystals using advanced time-resolved measurement techniques2016

    • Author(s)
      Toshiyuki Ihara
    • Organizer
      Workshop on solid-state chemistry for oxide and mixed-anion systems
    • Place of Presentation
      Kyoto, Japan
    • Year and Date
      2016-12-05
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research
  • [Presentation] 単一CdSe/ZnSナノ粒子の励起子分子カスケード発光分光:寿命と量子効率の関係2016

    • Author(s)
      井原章之, 広重直
    • Organizer
      日本物理学会
    • Place of Presentation
      金沢大学
    • Year and Date
      2016-09-13
    • Related Report
      2016 Research-status Report
  • [Presentation] 分光実験自動化ソフトウェアの開発と顕微発光計測への活用2016

    • Author(s)
      井原章之
    • Organizer
      日本物理学会
    • Place of Presentation
      金沢大学
    • Year and Date
      2016-09-13
    • Related Report
      2016 Research-status Report
  • [Presentation] 発光励起分光法による単一CdSe/CdS dot-in-rodの光吸収の研究2016

    • Author(s)
      井原章之, 佐藤良太, 寺西利治, 金光義彦
    • Organizer
      日本物理学会
    • Place of Presentation
      金沢大学
    • Year and Date
      2016-09-13
    • Related Report
      2016 Research-status Report
  • [Presentation] Quantitative Determination of Absorption Cross Section of Single Colloidal Quantum Dots Using a Hanbury-Brown Twiss Interferometer2016

    • Author(s)
      Toshiyuki Ihara and Yoshihiko Kanemitsu
    • Organizer
      The 9th International Conference on Quantum Dots (QD2016)
    • Place of Presentation
      Jeju, Korea
    • Year and Date
      2016-05-22
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research

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Published: 2016-04-21   Modified: 2022-08-18  

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