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Site selective ion desorption induced by positron-annihilation

Research Project

Project/Area Number 16K21424
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeMulti-year Fund
Research Field Physical chemistry
Thin film/Surface and interfacial physical properties
Research InstitutionTokyo University of Science (2017-2018)
Rikkyo University (2016)

Principal Investigator

Tachibana Takayuki  東京理科大学, 理学部第二部物理学科, 研究員 (90449306)

Project Period (FY) 2016-04-01 – 2019-03-31
Project Status Completed (Fiscal Year 2018)
Budget Amount *help
¥4,290,000 (Direct Cost: ¥3,300,000、Indirect Cost: ¥990,000)
Fiscal Year 2018: ¥650,000 (Direct Cost: ¥500,000、Indirect Cost: ¥150,000)
Fiscal Year 2017: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Fiscal Year 2016: ¥2,210,000 (Direct Cost: ¥1,700,000、Indirect Cost: ¥510,000)
Keywords陽電子 / 電子遷移誘起脱離 / 原子分子 / 量子ビーム / 表面物理 / 陽電子対消滅 / 陽電子消滅 / 表面・界面物性 / 化学物理 / 原子・分子物理
Outline of Final Research Achievements

Positron- and electron-stimulated desorption of positive ions from a titania surface have been investigated. The results indicate that positron-stimulated desorption of O+ ions is predominantly caused by pair annihilation of surface-trapped positrons with inner-shell electrons. The ion desorption from water chemisorbed on the titania surface was also obserbed. It found that the desorption of specific ions was enhanced by positron annihilation, above the ion yield with electron bombardment. This finding indicates that annihilation-site selectivity of positrons results in site-selective ion desorption from a bombarded surface.

Academic Significance and Societal Importance of the Research Achievements

これまで測定の困難さ故に陽電子ビームに誘起される表面の動的過程を対象とした実験的研究は皆無であった。本研究は「陽電子対消滅によるイオン脱離の観測実験」を発展させて,この未開拓の分野に本格的な実験的研究を展開することを試みた。その結果、陽電子ビーム入射に特有の脱離現象の観測に成功した。これらの成果や知見は、陽電子ビームを利用した新たな表面分析法や表面改質法の開発に繋がる重要なものである。

Report

(4 results)
  • 2018 Annual Research Report   Final Research Report ( PDF )
  • 2017 Research-status Report
  • 2016 Research-status Report
  • Research Products

    (16 results)

All 2019 2018 2017 2016

All Journal Article (7 results) (of which Peer Reviewed: 7 results,  Open Access: 3 results,  Acknowledgement Compliant: 2 results) Presentation (8 results) (of which Int'l Joint Research: 1 results,  Invited: 1 results) Book (1 results)

  • [Journal Article] Efficient and surface site-selective ion desorption by positron annihilation2018

    • Author(s)
      Tachibana Takayuki、Yamashita Takashi、Nagira Masaru、Yabuki Hisakuni、Nagashima Yasuyuki
    • Journal Title

      Scientific Reports

      Volume: 8 Issue: 1 Pages: 7197-7197

    • DOI

      10.1038/s41598-018-25506-5

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Positron-Annihilation-Induced Desorption Spectroscopy2018

    • Author(s)
      Takayuki Tachibana、Yasuyuki Nagashima
    • Journal Title

      Compendium of Surface and Interface Analysis

      Volume: - Pages: 497-500

    • DOI

      10.1007/978-981-10-6156-1_81

    • ISBN
      9789811061554, 9789811061561
    • Related Report
      2017 Research-status Report
    • Peer Reviewed
  • [Journal Article] Experimental and computational studies of positron-stimulated ion desorption from TiO2(1?1?0) surface2017

    • Author(s)
      Yamashita T、Hagiwara S、Tachibana T、Watanabe K、Nagashima Y
    • Journal Title

      MATERIALS RESEARCH EXPRESS

      Volume: 4 Issue: 11 Pages: 116303-116303

    • DOI

      10.1088/2053-1591/aa9454

    • Related Report
      2017 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] 陽電子消滅誘起イオン脱離2017

    • Author(s)
      立花隆行、長嶋泰之
    • Journal Title

      しょうとつ

      Volume: 14 Pages: 44-50

    • Related Report
      2017 Research-status Report
    • Peer Reviewed
  • [Journal Article] Photon-stimulated desorption of Ne metastable atoms from Ar adsorbed on Ne solid2017

    • Author(s)
      A. Iwabuchi, T. Tachibana, and H. Hirayama
    • Journal Title

      Journal of Electron Spectroscopy and Related Phenomena

      Volume: 印刷中 Pages: 25-27

    • DOI

      10.1016/j.elspec.2017.03.017

    • Related Report
      2017 Research-status Report 2016 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Development of a UHV-compatible Low-energy Electron Gun using the Photoelectric Effect2017

    • Author(s)
      SAWA Hiroyoshi、ANZAI Mao、KONISHI Tatsuya、TACHIBANA Takayuki、HIRAYAMA Takato
    • Journal Title

      Journal of the Vacuum Society of Japan

      Volume: 60 Issue: 12 Pages: 467-470

    • DOI

      10.3131/jvsj2.60.467

    • NAID

      130006252427

    • ISSN
      1882-2398, 1882-4749
    • Related Report
      2017 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] Ion desorption from TiO2(110) by low energy positron impact2016

    • Author(s)
      Takayuki Tachibana, Luca Chiari, Masaru Nagira, Takato Hirayama and Yasuyuki Nagashima
    • Journal Title

      Defect and Diffusion Forum

      Volume: 373 Pages: 324-327

    • DOI

      10.4028/www.scientific.net/ddf.373.324

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Presentation] 陽電子消滅誘起イオン脱離の機構解明に向けた新たな装置開発2019

    • Author(s)
      立花隆行、新井智哉、草苅知花、長嶋泰之
    • Organizer
      日本物理学会大74回年次大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 陽電子入射によるLiF表面からの分子イオン脱離2018

    • Author(s)
      立花 隆行
    • Organizer
      原子衝突学会第43回年会
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] Observation of positron stimulated ion desorption from LiF surfaces2018

    • Author(s)
      T. Tachibana, D. Hoshi, R. Gladen, Y. Nagashima
    • Organizer
      18th International Conference on Positron Annihilation
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] TiO2(110)表面における陽電子刺激イオン脱離と表面捕獲陽電子2017

    • Author(s)
      山下貴志, 立花隆行, Luca Chiari, 柳楽勝, 矢吹壽国, 萩原聡, 渡辺一之, 平山孝人, 長嶋泰之
    • Organizer
      日本物理学会第72回年次大会
    • Place of Presentation
      大阪大学豊中キャンパス(大阪府吹田市)
    • Year and Date
      2017-03-17
    • Related Report
      2016 Research-status Report
  • [Presentation] TiO2(110)表面からの陽電子刺激イオン脱離と 電子刺激イオン脱離の比較2016

    • Author(s)
      山下貴志,立花隆行,柳楽勝,矢吹壽国,Luca Chiari,平山孝人,長嶋泰之
    • Organizer
      原子衝突学会第41回年会
    • Place of Presentation
      富山大学五福キャンパス(富山県富山市)
    • Year and Date
      2016-12-10
    • Related Report
      2016 Research-status Report
  • [Presentation] 二酸化チタン表面における陽電子刺激イオン脱離収率とS-parameterの入射エネルギー依存性2016

    • Author(s)
      山下貴志,立花隆行,ルカ・チアリ,柳楽勝,矢吹壽国,平山孝人,長嶋泰之
    • Organizer
      平成28年度京都大学原子炉実験所専門研究会「陽電子科学とその理工学への応用」
    • Place of Presentation
      京都大学原子炉実験所(大阪府泉南郡)
    • Year and Date
      2016-12-08
    • Related Report
      2016 Research-status Report
  • [Presentation] TiO2(110)およびH2O/TiO2表面上における陽電子刺激イオン脱離2016

    • Author(s)
      立花隆行, 山下貴志, 柳楽勝, 矢吹壽国, Luca Chiari, 平山孝人, 長嶋泰之
    • Organizer
      日本物理学会2016年秋季大会
    • Place of Presentation
      金沢大学角間キャンパス(石川県金沢市)
    • Year and Date
      2016-09-21
    • Related Report
      2016 Research-status Report
  • [Presentation] TiO2(110)表面における陽電子刺激イオン脱離収量とS-parameterの比較2016

    • Author(s)
      山下貴志, 立花隆行, 柳楽勝, 矢吹壽国, 平山孝人, 長嶋泰之
    • Organizer
      日本物理学会2016年秋季大会
    • Place of Presentation
      金沢大学角間キャンパス(石川県金沢市)
    • Year and Date
      2016-09-21
    • Related Report
      2016 Research-status Report
  • [Book] Compendium of Surface and Interface Analysis, Chapter: Positron-annihilation-induced desorption2018

    • Author(s)
      T. Tachibana, Y. Nagashima
    • Total Pages
      4
    • Publisher
      Springer
    • ISBN
      9789811061554
    • Related Report
      2018 Annual Research Report

URL: 

Published: 2016-04-21   Modified: 2023-03-16  

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