• Search Research Projects
  • Search Researchers
  • How to Use
  1. Back to previous page

Development of terahertz-wave synthesizer using nonlinear-optical effect

Research Project

Project/Area Number 17206008
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field Applied optics/Quantum optical engineering
Research InstitutionTohoku University

Principal Investigator

TANIUCHI Tetsuo  Tohoku University, CENTER FOR INTERDISCIPLINARY RESEARCH, PROFESSOR (80260446)

Project Period (FY) 2005 – 2007
Project Status Completed (Fiscal Year 2007)
Budget Amount *help
¥48,490,000 (Direct Cost: ¥37,300,000、Indirect Cost: ¥11,190,000)
Fiscal Year 2007: ¥7,800,000 (Direct Cost: ¥6,000,000、Indirect Cost: ¥1,800,000)
Fiscal Year 2006: ¥14,690,000 (Direct Cost: ¥11,300,000、Indirect Cost: ¥3,390,000)
Fiscal Year 2005: ¥26,000,000 (Direct Cost: ¥20,000,000、Indirect Cost: ¥6,000,000)
Keywordsterahertz wave / nonlinear optics / organic crystal
Research Abstract

A coherent tunable terahertz (THz) source is a key device for applications such as THz frequency-domain spectroscopy and THz imaging. The purpose of this research project is to develop a THz-wave synthesizer based on difference-frequency generation (DFG) using nonlinear optical crystals. The n-conjugated organic crystals such as 4'-dimethylamino-N-methyl-4-stilbazolium tosylate (DAST) are promising materials for wideband THz-wave generation using DFG We synthesized a new organic crystal of 4'-dimethylamino-N- methyl-4-stilbazolium p-chlorobenzenesulfonate (DASC), which possessed p-chlorobenzenesulfonate instead of the tosylate of DAST. DASC crystals can be grown using a slow-cooling method in methanol solution, the same as DAST.
Widely tunable THz waves ranging from 2 to 30 THz were generated from DAST and DASC crystals using a dual-wavelength optical parametric oscillator (OPO) with two KTiOPO_4 crystals as the input light source. The OPO has a tunable range from 1340 to 1550 rim and is pumped by a frequency-doubled (532 rim), Q-switched Nd:YAG laser with a pulse duration of 12 ns. The THz output energy exceeding 500 nJ was obtained with a 0.5-mm-thick DAST and DASC crystal. Sub-THz waves in the range of 0.3-2 THz were also generated using an improved dual-wavelength OPO near 990 run with 2-mm-thick DAST crystals. The widely tunable -THz-wave synthesizer could potentially be used for real-time THz-imaging, THz-ranging, and spectroscopic applications.

Report

(4 results)
  • 2007 Annual Research Report   Final Research Report Summary
  • 2006 Annual Research Report
  • 2005 Annual Research Report
  • Research Products

    (52 results)

All 2007 2006 2005 Other

All Journal Article (35 results) (of which Peer Reviewed: 10 results) Presentation (10 results) Book (2 results) Remarks (2 results) Patent(Industrial Property Rights) (3 results)

  • [Journal Article] 有機結晶を用いたコヒーレントテラヘルツ波発生とその応用2007

    • Author(s)
      谷内 哲夫
    • Journal Title

      高分子 11

      Pages: 906-909

    • NAID

      10019763790

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Annual Research Report 2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Single crystal preparation of DAST for terahertz-wave generation2007

    • Author(s)
      Y. Mineno
    • Journal Title

      Mol. Cryst. Liq. Cryst. 463

      Pages: 55-61

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Annual Research Report 2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Synthesis and Teratertz-Wave Generation of Mixed Crystals of l-Methyl-4- {2-[4- (dimethylamino) phenyl]ethenyl} pyridinium p-Toluenesulfbnate and p-Chlorobenzenesulfonate2007

    • Author(s)
      T. Matsukawa
    • Journal Title

      J. Crystal Growth 299

      Pages: 344-348

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] 有機DAST結晶を用いた波長可変テラヘルツ波発生とその応用2007

    • Author(s)
      谷内 哲夫
    • Journal Title

      電子情報通信学会 信学技報 OME-142

      Pages: 13-18

    • NAID

      110006248834

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Coherent terahertz-wave generation in organic crystals and its applications2007

    • Author(s)
      T. Taniuchi
    • Journal Title

      Kobunshi High Polymers 11

      Pages: 906-909

    • NAID

      10019763790

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Synthesis and teratertz-wave generation of mixed crystals of 1-methy1-4-{2-[4-(dimethylamino)phenyl]ethenyl}pyridinium p-toluenesulfonate and p-chlorobenzenesulfonate2007

    • Author(s)
      T. Matsukawa
    • Journal Title

      J. Crystal Growth 299

      Pages: 344-348

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Tunable terahertz-wave generation in organic crystals and its application2007

    • Author(s)
      T. Taniuchi
    • Journal Title

      IEICE Technical Report OME-142

      Pages: 13-18

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Synthesis and Teratertz-Wave Generation of Mixed Crystals of 1-Methyl-4-{2-[4-(dimethylamino)phenyl]ethenyl}pyridinium p-Toluenesulfonate and p-Chlorobenzenesulfonate2007

    • Author(s)
      T. Matsukawa
    • Journal Title

      J. Crystal Growth 299

      Pages: 344-348

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Synthesis and Teratertz-Wave Generation of Mixed Crystals of 1-Methyl-4-{2-[4-dimethylamino)phenyl]ethenyl}pyridinium p-Toluenesulfonate and p-Chlorobenzenesulfonate2007

    • Author(s)
      Takeshi Matsukawa
    • Journal Title

      J. Crystal Growth 299

      Pages: 344-348

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Organic nonlinear optical DAST crystals for electro-optic measurement and terahertz wave generation2006

    • Author(s)
      Y. Takahashi
    • Journal Title

      J. Photochemistry and photobiology A: Chemistry 183

      Pages: 247-252

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] テラヘルツ波応用に向けた有機結晶材料の開発2006

    • Author(s)
      谷内 哲夫
    • Journal Title

      機械の研究 58

      Pages: 823-829

    • NAID

      40007404233

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] 有機結晶からの未踏光の発生2006

    • Author(s)
      岡田 修司
    • Journal Title

      光アライアンス 17

      Pages: 213-218

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Organic materials for terahertz-wave applications2006

    • Author(s)
      T. Taniuchi
    • Journal Title

      Science of Machine 58-8

      Pages: 823-829

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Terahertz-wave generation from organic crystals2006

    • Author(s)
      S. Okada
    • Journal Title

      Optical Alliance 17

      Pages: 213-218

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Widely tunable terahertz-wave source using organic DAST crystal2006

    • Author(s)
      T. Taniuchi
    • Journal Title

      Optical Sensing Technology 6

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Organic nonlinear optical DAST crystals for electro-optic measurement and terahertz wave generation2006

    • Author(s)
      Yoshinori Takahashi
    • Journal Title

      J. Photochemistry and photobiology A : Chemistry 183

      Pages: 247-252

    • Related Report
      2006 Annual Research Report
  • [Journal Article] π-Conjugated Organic Ionic Crystals for Terahertz-Wave Generation2006

    • Author(s)
      Shuji Okada
    • Journal Title

      The International Conference on Science and Technology of Synthetic Metals 2006 1

      Pages: 47-47

    • Related Report
      2006 Annual Research Report
  • [Journal Article] テラヘルツ波応用に向けた有機結晶材料の開発2006

    • Author(s)
      谷内 哲夫
    • Journal Title

      機械の研究 58・8

      Pages: 823-829

    • NAID

      40007404233

    • Related Report
      2006 Annual Research Report
  • [Journal Article] 有機結晶からの未踏光の発生2006

    • Author(s)
      岡田 修司
    • Journal Title

      光アライアンス 17・4

      Pages: 213-218

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Advanced growth technology of DAST crystals for THz wave generation2006

    • Author(s)
      Yoshinori Takahashi
    • Journal Title

      International Symposium on Frontiers in Organic Photonics, I-2

      Pages: 3-4

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Widely tunable terahertz-wave source with an organic DAST crystal2005

    • Author(s)
      T. Taniuchi
    • Journal Title

      Nonlinear Optics, Quantum Optics 34

      Pages: 57-60

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Crystal growth of DAST and its derivative for THz-wave gen eration2005

    • Author(s)
      Y. Mineno
    • Journal Title

      Nonlinear Optics, Quantum Optics 34

      Pages: 53-56

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Terahertz properties of a new organic crystal, 4'-dimethylamino-N-methy1-4-stilbazolium p-chlorobenzenesulfonate2005

    • Author(s)
      T. Taniuchi
    • Journal Title

      Jpn. J. Appl. Phys. 44

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Tunable Sub-Terahertz Wave Generation from an Organic DAST Crystal2005

    • Author(s)
      T. Taniuchi
    • Journal Title

      Jpn. J. Appl. Phys. 44

    • NAID

      10016150702

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Synthesis and properties of 1-methyl-4-{2-[4-(dimethylamino)phenyl]ethenyl} pyridiniump-toluenesulfonate derivatives with isomorphous crys tal structure2005

    • Author(s)
      Z. Glavcheva
    • Journal Title

      Jpn. J. Appl. Phys. 44

      Pages: 5231-5235

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Crystal growth of DAST and its derivative for THZ-wave generation2005

    • Author(s)
      Y. Mineno
    • Journal Title

      Nonlinear Optics, Quantum Optics 34

      Pages: 53-56

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Terahertz properties of a new organic crystal, 4'' -dimethylamino-N-methy1-4 Stibazolium p-chlorobenzenesulfonate2005

    • Author(s)
      T. Taniuchi
    • Journal Title

      Jpn. J. Appl. Phys. 44-29

      Pages: 932-934

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Tunable sub-terahertz wave generation from an organic DAST crystal2005

    • Author(s)
      T. Taniuchi
    • Journal Title

      Jpn. J. Appl. Phys. 44-21

      Pages: 652-654

    • NAID

      10016150702

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Syntesis and properties of 1-methy1-4-{2-[4-(Dimethylamino) phenyl]ethenyl}pyridiniump-toluenesulfonate derivatives with isomorphous crystal structure2005

    • Author(s)
      Z. Glavcheva
    • Journal Title

      Jpn. J. Appl. Phys. 44-7A

      Pages: 5231-5235

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Widely tunable terahertz-wave generation from organic DAST crystal2005

    • Author(s)
      T. Taniuchi
    • Journal Title

      Terahertz Technology 9

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Widely tunable terahertz-wave source with an organic DAST crystal2005

    • Author(s)
      Tetsuo Taniuchi
    • Journal Title

      Nonlinear Optics, Quantum Optics 34

      Pages: 57-60

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Crystal growth of DAST and its derivative for THz-wave generation2005

    • Author(s)
      Shuji Okada
    • Journal Title

      Nonlinear Optics, Quantum Optics 34

      Pages: 53-56

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Tunable sub-terahertz wave generation from an organic DAST crystal2005

    • Author(s)
      Tetsuo Taniuchi
    • Journal Title

      Jpn.J.Appl.Phys. 44・21

    • NAID

      10016150702

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Synthesis and properties of 1-methyl-4-{2-[4-(dimethylamino)phenyl]ethenyl}pyridiniump-toluenesulfonate derivatives with isomorphous crystal structure2005

    • Author(s)
      Zornitza Glavcheva
    • Journal Title

      Jpn.J.Appl.Phys. 44・7A

      Pages: 5231-5235

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Terahertz-wave generation in a new organic crystal,4'-dimethylamino-N-methyl-4-stilbazolium p-chlorobenzenesulfonate2005

    • Author(s)
      Tetsuo Taniuchi
    • Journal Title

      The 12th International Conference on Unconventional Photoactive Systems

      Pages: 114-114

    • Related Report
      2005 Annual Research Report
  • [Presentation] π-Conjugated Organic Ionic Crystals for Terahertz-Wave Generation2006

    • Author(s)
      S. Okada
    • Organizer
      The International Conference on Science and Technology of Synthetic Metals 2006
    • Place of Presentation
      アイルランド
    • Year and Date
      2006-07-05
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] π-Conjugated Organic Ionic Crystals for Terahertz-Wave Generation2006

    • Author(s)
      S. Okada
    • Organizer
      The International Conference on Science and Technology of Synthetic Metals (ICSM2006)
    • Place of Presentation
      Ireland
    • Year and Date
      2006-07-05
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] 新有機結晶DAST/DASC混晶における波長可変テラヘルツ波発生特性2006

    • Author(s)
      谷内 哲夫
    • Organizer
      平成18年第53回応用物理学関係連合講演会
    • Place of Presentation
      日本
    • Year and Date
      2006-03-25
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Tunable THz-wave generation from new organic DAST/DASC mixed crystal2006

    • Author(s)
      T. Taniuchi
    • Organizer
      The 53th Spring Meeting of Japan Society of Applied Physics
    • Place of Presentation
      Japan
    • Year and Date
      2006-03-25
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Terahertz properties of a new organic crystal, 4'-dimethylamino-N-methyl-4-stilbazolium p-chlorobenzenesulfonate2005

    • Author(s)
      T. Taniuchi
    • Organizer
      The 12th International Conference on Unconvent ional Photoactive Systems
    • Place of Presentation
      日本
    • Year and Date
      2005-10-04
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Terahertz-wave generation in a new organic crystal, 4''-dimethylamino-N-methyl-4-stilbazolium-chlorobenzenesulfonate2005

    • Author(s)
      T. Taniuchi
    • Organizer
      The 12th International Conference on Unconventional Photoactive Systems
    • Place of Presentation
      Japan
    • Year and Date
      2005-10-04
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] 新有機結晶DASCを用いた波長可変テラヘルツ波発生2005

    • Author(s)
      谷内 哲夫
    • Organizer
      平成17年第66回応用物理学会学術講演会
    • Place of Presentation
      日本
    • Year and Date
      2005-09-09
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Tunable THz-wave generation from new organic DASC crystal2005

    • Author(s)
      T. Taniuchi
    • Organizer
      The 66th Autumn Meeting of the Japan Society of Applied Physics
    • Place of Presentation
      Japan
    • Year and Date
      2005-09-09
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] テラヘルツ波発生のためのDAST類縁体単結晶の作製2005

    • Author(s)
      松川 健
    • Organizer
      平成17年第66回応用物理学会学術講演会
    • Place of Presentation
      日本
    • Year and Date
      2005-09-08
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Single crystal preparaton of DAST analogues for THz-wave generation2005

    • Author(s)
      T. Matsukawa
    • Organizer
      The 66th Autumn Meeting of the Japan Society of Applied Physics
    • Place of Presentation
      Japan
    • Year and Date
      2005-09-08
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Book] 光センシング技術資料集2006

    • Author(s)
      谷内 哲夫
    • Total Pages
      6
    • Publisher
      オプトロニクス社
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary 2006 Annual Research Report
  • [Book] テラヘルツテクノロジー2005

    • Author(s)
      谷内 哲夫
    • Total Pages
      9
    • Publisher
      NTS出版
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary 2005 Annual Research Report
  • [Remarks] 「研究成果報告書概要(和文)」より

    • URL

      http://www.cir.tohoku.ac.jp/taniuchi/

    • Related Report
      2007 Final Research Report Summary
  • [Remarks]

    • URL

      http://www.cir.tohoku.ac.jp/taniuchi/

    • Related Report
      2007 Annual Research Report
  • [Patent(Industrial Property Rights)] テラヘルツ波発生用有機材料2006

    • Inventor(s)
      谷内哲夫他
    • Industrial Property Rights Holder
      東北大学 他
    • Patent Publication Number
      2007-328145
    • Filing Date
      2006-06-08
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Patent(Industrial Property Rights)] 有機光学結晶, 差周波発生素子, テラヘルツ波発生装置2006

    • Inventor(s)
      高橋義典他
    • Industrial Property Rights Holder
      大阪大学, 東北大学 他
    • Patent Publication Number
      2007-232936
    • Filing Date
      2006-02-28
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Patent(Industrial Property Rights)] テラヘルツ波発生用有機材料2006

    • Inventor(s)
      谷内哲夫他
    • Industrial Property Rights Holder
      東北大学他
    • Industrial Property Number
      2006-159424
    • Filing Date
      2006-06-08
    • Related Report
      2006 Annual Research Report

URL: 

Published: 2005-04-01   Modified: 2016-04-21  

Information User Guide FAQ News Terms of Use Attribution of KAKENHI

Powered by NII kakenhi