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Preparation of capsule-like particles containing single-core and their application to medical analysis

Research Project

Project/Area Number 17310064
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Nanomaterials/Nanobioscience
Research InstitutionIbaraki University (2006-2007)
Tohoku University (2005)

Principal Investigator

KOBAYASHI Yoshio  Ibaraki University, College of Engineering, Professor (40250849)

Co-Investigator(Kenkyū-buntansha) TAKEDA Motohiro  Tohoku University, Graduate School of Engineering, Associate Professor (10333808)
OHUCHI Noriaki  Tohoku University, Graduate School of Medicine, Professor (90203710)
KASUYA Atsuo  Tohoku University, Center for Interdisciplinary Research, Professor (10005986)
Project Period (FY) 2005 – 2007
Project Status Completed (Fiscal Year 2007)
Budget Amount *help
¥15,490,000 (Direct Cost: ¥14,500,000、Indirect Cost: ¥990,000)
Fiscal Year 2007: ¥4,290,000 (Direct Cost: ¥3,300,000、Indirect Cost: ¥990,000)
Fiscal Year 2006: ¥3,000,000 (Direct Cost: ¥3,000,000)
Fiscal Year 2005: ¥8,200,000 (Direct Cost: ¥8,200,000)
KeywordsX-ray contrast agent / MRI / nanoparticle / encapsulation / Agl / Gd / silica / sol-gel method / 追添加 / MRI造影剤 / 粒子 / 蛍光ビーズ / コア-シェル型 / ゾル-ゲル法
Research Abstract

Iodine compounds and gadolinium compounds have been used as contrast agents for X-ray CT and magnetic resonance imaging, respectively. These existing compounds may provoke adverse events as allergic reactions in patients, so that they can not be administered to such people. Core-shell nanoparticles are good candidates for prevention of allergic reactions because the shell materials can keep the contrast agents from living systems. In present works, several methods for silica-coating of contrast agent nanoparticles are proposed.
Silica-coating of AgI nanoparticles with a Stober method was carried out to find out reaction conditions for control of the shell thickness. The AgI nanoparticles were prepared from AgCIO_4 and KI with the use of 3-mercaptopropyltrimethoxysilane (MPS) as a silane coupling agent and dimethylamine (DMA) catalyst for alkoxide hydrolysis. AgI-silica core-shell particles could be prepared with the use of 4.5×10^<-5> MMPS, 20M water, 0.01 MDMA and 1 mM AgI. Silica shell thickness could be varied from 15 to 28 nm with an increase in the TEOS concentration from 0.005 to 0.04M.
A preparation method for multilayered silica-Gd-silica core-shell particles is proposes. Silica particles with an average size of 30.9 nm were prepared by the Stober method. Silica-Gd core-shell particles with a size of 57.4 nm were synthesized by a homogeneous precipitation method at 80℃ in water/propanol solution with 27.7 M H_2O, 0.001 M Gd (NO_3)_3, 0.5 M urea and 1 g/l polyvinylpyrrolidone in the presence of 0.001 vol% suspension of the silica particles. Succeeding silica-coating of the silica-Gd core-shell particles was performed with 0.0133 MTEOS and 0.002 M NaOH in the presence of a suspension of silica-Gd core-shell particles. Consequently, multilayered silica-Gd-silica core-shell particles with an average size of 71.2 nm could be obtained. These particles exhibited clear enhancement in magnetic resonance images.

Report

(4 results)
  • 2007 Annual Research Report   Final Research Report Summary
  • 2006 Annual Research Report
  • 2005 Annual Research Report
  • Research Products

    (58 results)

All 2008 2007 2006 2005 Other

All Journal Article (45 results) (of which Peer Reviewed: 17 results) Presentation (12 results) Remarks (1 results)

  • [Journal Article] Synthesis of Spherical Submicron-Sized Magnetite/Silica Nanocomposite Particles2008

    • Author(s)
      Y., Kobayashi, et. al.
    • Journal Title

      Journal of Sol-Gel Science and Technology 45

      Pages: 35-41

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Silica-Coating of Metallic Copper Nanoparticles in Aqueous Solution2008

    • Author(s)
      Y., Kobayashi・T., Sakuraba
    • Journal Title

      Colloids and Surfaces A: Physiochemical and Engineering Aspects 317

      Pages: 756-759

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Synthesis and Properties of Co-Pt Alloy-Silica Core-Shell Particles2008

    • Author(s)
      Y., Kobayashi, et. al.
    • Journal Title

      Journal of Sol-Gel Science and Technology 47

      Pages: 16-22

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Synthesis of Spherical Submicron-Sized Magnetite/Silica Nanocomposite Particles2008

    • Author(s)
      Y. Kobayashi, et. al.
    • Journal Title

      Journal of Sol-Gel Science and Technology 45

      Pages: 35-41

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Silica-Coating of Metallic Copper Nanoparticles in Aqueous Solution2008

    • Author(s)
      Y. Kobayashi and T. Sakuraba
    • Journal Title

      Colloids and Surfaces A : Physiochemical and Engineering Aspects 317

      Pages: 756-759

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Synthesis and Properties of Co-Pt Alloy-Silica Core-Shell Particles2008

    • Author(s)
      Y. Kobayashi, et. al.
    • Journal Title

      Journal of Sol-Gel Science and Technology 47

      Pages: 16-22

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Photoluminescence of CdSe and CdSe/CdO・nH_2O Core/Shell Nanoparticles Prepared in Aqueous Solution2007

    • Author(s)
      X., Zhou, et. al.
    • Journal Title

      Optical Materials 29

      Pages: 1048-1054

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Synthesis of SiO_2-Coated Magnetite Nanoparticles and Immobilization of Proteins on Them2007

    • Author(s)
      Y., Kobayashi, et. al.
    • Journal Title

      Ceramic Transactions 198

      Pages: 135-141

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Direct Coating of Particles by a Liquid Phase Process2007

    • Author(s)
      Y., Kobayashi , et. al.
    • Journal Title

      Current Nanoscience 3

      Pages: 222-240

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Preparation of Multilayered Silica-Gd-Silica Core-Shell Particles and Their Magnetic Resonance Images2007

    • Author(s)
      Y., Kobayashi, et al.
    • Journal Title

      Colloids and Surfaces A: Physiochemical and Engineering Aspects 308

      Pages: 14-17

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Control of Shell Thickness in Silica-Coating of AgI Nanoparticles2007

    • Author(s)
      Y., Kobayashi, et. al.
    • Journal Title

      Advanced Materials Research 29-30

      Pages: 191-194

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Photoluminescence of CdSe and CdSe/CdO・nH2O Core/Shell Nanoparticles Prepared in Aqueous Solution2007

    • Author(s)
      X. Zhou, et. al.
    • Journal Title

      Optical Materials 29

      Pages: 1048-1054

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Synthesis of Si0_2-Coated Magnetite Nanoparticles and Immobilization of Proteins on Them2007

    • Author(s)
      Y. Kobayashi, et. al.
    • Journal Title

      Ceramic Transactions 198

      Pages: 135-141

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Direct Coating of Particles by a Liquid Phase Process2007

    • Author(s)
      Y. Kobayashi, et. al.
    • Journal Title

      Current Nanoscience 3

      Pages: 222-240

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Preparation of Multilayered Silica-Gd-Silica Core-Shell Particles and Their Magnetic Resonance Images2007

    • Author(s)
      Y. Kobayashi, et. al.
    • Journal Title

      Colloids and Surfaces A 303

      Pages: 14-19

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Control of Shell Thickness in Silica-Coating of AgI Nanoparticles2007

    • Author(s)
      Y. Kobayashi, et. al.
    • Journal Title

      Advanced Materials Research 29-30

      Pages: 191-194

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Annual Research Report 2007 Final Research Report Summary
  • [Journal Article] Photoluminescence of CdSe/CdO-nH_2O Core/Shell Nanoparticles Prepared in Aqueous Solution2007

    • Author(s)
      X.Zhou
    • Journal Title

      Optical Materials 29

      Pages: 1048-1054

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Synthesis of SiO_2-Coated Magnetite Nanoparticles and Immobilization of Proteins on Them2007

    • Author(s)
      Y.Kobayashi
    • Journal Title

      Transactions of the American Ceramic Society 印刷中

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Control of Shell Thickness in Silica-Coating of AgI Nanoparticles2007

    • Author(s)
      Y.Kobayashi
    • Journal Title

      Materials Science Forum 印刷中

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Preparation of Highly Monodisperse Poly (methyl methacrylate) Particles Incorporating Fluorescent Rhodamine 6G for Colloidal Crystals2006

    • Author(s)
      D., Nagao, et. al.
    • Journal Title

      Journal of Colloid and Interface Science 298

      Pages: 232-237

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Preparation of Silica-Coated Co-Pt Alloy Nanoparticles2006

    • Author(s)
      Y., Kobayash, et. al.
    • Journal Title

      Materials Letters 60

      Pages: 2046-2049

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] X-ray Absorption of Gold Nanoparticles with Thin Silica Shell2006

    • Author(s)
      Y.-S., Park, et. al.
    • Journal Title

      Journal of Nanoscience and Nanotechnology 6

      Pages: 3503-3506

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Preparation of Highly Monodisperse Poly(methyl methacrylate)Particles Incorporating Fluorescent Rhodamine 6G for Colloidal Crystals2006

    • Author(s)
      D. Nagao, et. al.
    • Journal Title

      Journal of Colloid and Interface Science 298

      Pages: 232-237

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Preparation of Silica-Coated Co-Pt Alloy Nanoparticles2006

    • Author(s)
      Y. Kobayashi, et. al.
    • Journal Title

      Materials Letters 60

      Pages: 2046-2049

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] X-ray Absorption of the Gold Nanoparticles with Thin Silica Shell2006

    • Author(s)
      Y.-S. Park, et. al.
    • Journal Title

      Journal of Nanoscience and Nanotechnology 6

      Pages: 3503-3506

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Nanosized Silver Iodide Beads as New Contrast Media for Sentinel Lymph Node Navigation Surgery2006

    • Author(s)
      Y.Sakurai
    • Journal Title

      Breast Disease 25

      Pages: 55-56

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Detection of Sentinel Lymph Nodes by Novel MR Contrast Media2006

    • Author(s)
      M.Takeda
    • Journal Title

      Breast Disease 25

      Pages: 47-47

    • Related Report
      2006 Annual Research Report
  • [Journal Article] X-ray Absorption of the Gold Nanoparticles with Thin Silica Shell2006

    • Author(s)
      Y.-S.Park
    • Journal Title

      Journal of Nanoscience and Nanotechnology 6

      Pages: 3503-3506

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Preparation of Silica-Coated Co-Pt Alloy Nanoparticles2006

    • Author(s)
      Y.Kobayashi
    • Journal Title

      Materials Letters (印刷中)

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Silica Coating of Silver Nanoparticles Using a Modified Stober Method2005

    • Author(s)
      Y., Kobayashi, et. al.
    • Journal Title

      Journal of Colloid and Interface Science 283

      Pages: 392-396

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Preparation of Silica Encapsulated CdSe Quantum Dots in Aqueous Solution with the Improved Optical Properties2005

    • Author(s)
      X., Zhou, et. al.
    • Journal Title

      Applied Surface Science 242

      Pages: 281-286

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Strong Luminescing CdSe Nanoparticles by Surface Modification with Cadmium (II ) Hydrous Oxide2005

    • Author(s)
      X., Zhou, et. al.
    • Journal Title

      International Journal of Modern Physics B 19

      Pages: 2835-2840

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Silica-coationg of Fluorescent Polystyrene Microspheres by a Modified Stober Method and their Stability against Photo-Bleaching2005

    • Author(s)
      Y., Kobayashi, et. al.
    • Journal Title

      e-Polymers no. 052

      Pages: 1-8

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Preparation of Fluorescent Polymer Particles by Emulsion Polymerization2005

    • Author(s)
      S., Gu, et. al.
    • Journal Title

      e-Polymers no. 064

      Pages: 1-5

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Preparation and Colloidal Stability of Monodisperse Magnetic Polymer Particles2005

    • Author(s)
      S., Gu, et. al.
    • Journal Title

      Journal of Colloid and Interface Science 2005

      Pages: 419-426

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Silica Coating of Silver Nanoparticles Using a Modified Stober Method2005

    • Author(s)
      Y. Kobayashi, et. al.
    • Journal Title

      Journal of Colloid and Interface Science 283

      Pages: 392-396

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Preparation of Silica Encapsulated CdSe Quantum Dots in Aqueous Solution with the Improved Optical Properties2005

    • Author(s)
      X. Zhou, et. al.
    • Journal Title

      Applied Surface Science 242

      Pages: 281-286

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Strong Luminescing CdSe Nanoparticles by Surface Modification with Cadmium(II)Hydrous Oxide2005

    • Author(s)
      X. Zhou, et. al.
    • Journal Title

      International Journal of Modern physics B 19

      Pages: 2835-2840

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Silica-coating of Fluorescent Polystyrene Microspheres by a Modified Stober Method and their Stability against Photo-Bleaching2005

    • Author(s)
      Y. Kobayashi, et. al.
    • Journal Title

      e-Polymers no.052

      Pages: 1-8

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Preparation of Fluorescent Polymer Particles by Emulsion Polymerization2005

    • Author(s)
      S. Gu, et. al.
    • Journal Title

      e-Polymers no.064

      Pages: 1-5

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Preparation and Colloidal Stability of Monodisperse Magnetic Polymer Particles2005

    • Author(s)
      S. Gu, et. al.
    • Journal Title

      Journal of Colloid and Interface Science 289

      Pages: 419-426

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Preparation of Silica Encapsulated CdSe Quantum Dots in Aqueous Solution with the Improved Optical Properties2005

    • Author(s)
      X.Zhou
    • Journal Title

      Applied Surface Science 242

      Pages: 281-286

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Strong Luminescing CdSe Nanoparticles by Surface Modification with Cadmium (II) Hydrous Oxide2005

    • Author(s)
      X.Zhou
    • Journal Title

      International Journal of Modern Physics B 19

      Pages: 2835-2840

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Silica-Coating of Fluorescent Polystyrene Microspheres by a Modified Stober Method and Their Stability against Photo-Bleaching2005

    • Author(s)
      Y.Kobayashi
    • Journal Title

      e-Polymers no.052

      Pages: 1-8

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Preparation of Fluorescent Polymer Particles by Emulsion Polymerization2005

    • Author(s)
      S.Gu
    • Journal Title

      e-Polymers no.064

      Pages: 1-5

    • Related Report
      2005 Annual Research Report
  • [Presentation] Preparation and Properties of Silica-Coated AgI Nanoparticles with a Modified Stober Method.2008

    • Author(s)
      Y., Kobayashi, et al.
    • Organizer
      2008 MRS Spring Meeting
    • Place of Presentation
      San Francisco,USA
    • Year and Date
      2008-03-27
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Preparation and Properties of Silica-Coated AgI Nanoparticles with a Modified Stober Method2008

    • Author(s)
      Y. Kobayashi, et. al.
    • Organizer
      2008 MRS Spring Meeting
    • Place of Presentation
      San Francisco, USA
    • Year and Date
      2008-03-27
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Annual Research Report 2007 Final Research Report Summary
  • [Presentation] AgI/SiO_2複合粒子コロイドの調製法の開発2008

    • Author(s)
      湊真理絵, ら
    • Organizer
      化学工学会第73年会
    • Place of Presentation
      浜松
    • Year and Date
      2008-03-17
    • Related Report
      2007 Annual Research Report
  • [Presentation] 液相法によるAgI/SiO_2複合粒子の作製法の開発の研究2007

    • Author(s)
      湊真理絵, ら
    • Organizer
      第18回日本化学会関東支部茨城地区研究交流会
    • Place of Presentation
      水戸
    • Year and Date
      2007-11-30
    • Related Report
      2007 Annual Research Report
  • [Presentation] Prep.aration of Aniine-Free Silipa-Coated AgI Nanoparticles with a Modified Stober Method2007

    • Author(s)
      Y., Kobayashi, et al.
    • Organizer
      The 9th Annual Conference of the Yugoslav Materials Research Society
    • Place of Presentation
      Herceg Novi,Montenegro
    • Year and Date
      2007-09-13
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Preparation of Amine-Free Silica-Coated AgI Nanoparticles with a Modified Stober Method2007

    • Author(s)
      Y. Kobayashi, et. al.
    • Organizer
      The 9th Annual Conference of the Yugoslav Materials Research Society
    • Place of Presentation
      Herceg Novi, Montenegro
    • Year and Date
      2007-09-13
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Annual Research Report 2007 Final Research Report Summary
  • [Presentation] Control of Shell Thickness in Silica-Coatjng of Agl Nanoparticles2006

    • Author(s)
      Y., Kobayashi, et al.
    • Organizer
      The 4th International Conference en Advanced Materials
    • Place of Presentation
      Hamilton,New Zealand
    • Year and Date
      2006-12-11
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Control of Shell Thickness in Silica-Coating of AgI Nanoparticles2006

    • Author(s)
      Y. Kobayashi, et. al.
    • Organizer
      The 4th International Conference on Advanced Materials
    • Place of Presentation
      Hamilton, New Zealand
    • Year and Date
      2006-12-11
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Direct Ceating of Magnetite Nanobarticles with Silica by a Seeded Polymerization Technique and Immobilization of Proteins on the Silica-Coated Particles2006

    • Author(s)
      Y., Kobayashi, et al.
    • Organizer
      The Second lntemational Conference on the Characterization and Control of Interfaces
    • Place of Presentation
      Kurashiki,Japan
    • Year and Date
      2006-09-07
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Direct Coating of Magnetite Nanoparticles with Silica by a Seeded Polymerization Technique Immobilization of Proteins on the Silica-Coated Particles2006

    • Author(s)
      Y. Kobayashi, et. al.
    • Organizer
      The Second International Conference on the Characterization and Control of Interfaces
    • Place of Presentation
      Kurashiki, Japan
    • Year and Date
      2006-09-07
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Silica-Coating of Agl Nanopartiicles Using a Modified Stober Method2005

    • Author(s)
      Y., Kobayashi, et. al.
    • Organizer
      Twelfth International Confcrence on Composites/Nano Epgineering
    • Place of Presentation
      Tenerife,Spain
    • Year and Date
      2005-08-02
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Silica-Coating of Agl Nanopartiicles Using a Modified Stober Method2005

    • Author(s)
      Y. Kobayashi, et. al.
    • Organizer
      Twelfth International Conference on Composites/Nano Engineering
    • Place of Presentation
      Tenerife, Spain
    • Year and Date
      2005-08-02
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Remarks] 茨城大学研究者情報総覧

    • URL

      http://info.ibaraki.ac.jp/scripts/websearch/index.htm

    • Related Report
      2007 Annual Research Report

URL: 

Published: 2005-04-01   Modified: 2016-04-21  

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