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Comparative studies on organic chemical composition of atmospheric aerosols from Chinese 14 cities, Jeju Island and Chichi-Jima Island and their hygroscopic properties

Research Project

Project/Area Number 17340166
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Geochemistry/Astrochemistry
Research InstitutionHokkaido University

Principal Investigator

KAWAMURA Kimitaka  Hokkaido University, Inst. Low Tem. Science, Professor (70201449)

Project Period (FY) 2005 – 2006
Project Status Completed (Fiscal Year 2006)
Budget Amount *help
¥15,600,000 (Direct Cost: ¥15,600,000)
Fiscal Year 2006: ¥3,700,000 (Direct Cost: ¥3,700,000)
Fiscal Year 2005: ¥11,900,000 (Direct Cost: ¥11,900,000)
KeywordsChinese-megacities / Chinese aerosols / Dicarboxylic acids / Levoglucosan / Normal alkanes / Photochemistry / Biomass burning / Fossil fuel combustion / シュウ酸 / 大気化学 / 化石燃料の燃焼 / 環境分析 / 地球化学 / 有機物
Research Abstract

Nation-wide studies of organic aerosols were conducted on a molecular level in 15 Chinese cities. The results showed strikingly high levels of organic compounds (e.g., annual concentrations of polycyclic aromatic hydrocarbons, phthalates, sugars and diacids are 110, 370, 400 and 830 ng m^3, respectively), especially in the midwest region during winter (up to 125 mg m^3 organic carbon). Fossil fuel combustion and/or biomass burning products are 3-30 times more abundant in winter than in summer. In contrast, significant quantity of phthalates (168-2200 ng m^3) was detected in summer. Concentrations of the pollutants are generally 1-3 orders of magnitude higher than those in developed countries. Their source strengths are characterized in winter by fossil fuel combustion, followed by secondary oxidation, plant wax emissions and biomass burning, whereas in summer they are characterized by secondary oxidation, followed by fossil fuel combustion and plastic emissions.

Report

(3 results)
  • 2006 Annual Research Report   Final Research Report Summary
  • 2005 Annual Research Report
  • Research Products

    (18 results)

All 2007 2006 2005

All Journal Article (15 results) Book (3 results)

  • [Journal Article] Identification, abundance and seasonal variation of anthropogenic organic aerosols from a mega-city in China2007

    • Author(s)
      Gehui Wang
    • Journal Title

      Atmospheric Environment 41

      Pages: 407-416

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Annual Research Report 2006 Final Research Report Summary
  • [Journal Article] Size distributions of dicarboxylic acids and inorganic ions in atmospheric aerosols collected during polar sunrise in the Canadian High Arctic2007

    • Author(s)
      Kimitaka Kawamura
    • Journal Title

      J. Geophys. Res. 112・D10307

    • NAID

      120000968610

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Chemical Closure Study on Hygroscopic Properties of Urban Aerosol Particles in Sapporo, Japan2007

    • Author(s)
      Shankar Gopala Aggarwal
    • Journal Title

      Environ. Sci. Technol. 41

      Pages: 6920-6925

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Size distributions of dicarboxylic acids and inorganic ions in atmospheric aerosols collected during polar sunrise in the Canadian High Arctic2007

    • Author(s)
      Kimitaka Kawamura
    • Journal Title

      J. Geophys. Res. 112, D10307

    • NAID

      120000968610

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Stable carbon isotopic composition of low-molecular-weight dicarboxylic acids and ketoacids in remote marine aerosols2006

    • Author(s)
      Haobo Wang
    • Journal Title

      J. Geophys. Res. 111, D07304

    • Related Report
      2006 Annual Research Report
  • [Journal Article] 大気中に存在する有機エアロゾルの組成分布と変質2006

    • Author(s)
      河村 公隆
    • Journal Title

      地球化学 40

      Pages: 65-82

    • NAID

      110008680115

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Molecular, seasonal and spatial distribution of organic aerosols from fourteen Chinese cities2006

    • Author(s)
      Gehui Wang
    • Journal Title

      Environ. Sci. and Technol. 40

      Pages: 4619-4625

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Determination of low molecular weight dicarboxylic acids in seawater samples2006

    • Author(s)
      Marc Tedetti
    • Journal Title

      Analytical Chemistry 78

      Pages: 6012-6018

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Relationship between hygroscopicity and cloud condensation nuclei activity for urban aerosols in Tokyo2006

    • Author(s)
      Michihiro Mochida
    • Journal Title

      J. Geophys. Res. 111, D23204

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Water-soluble dicarboxylic acids, ketoacids and dicarbonyls in the atmosphere over the Southern Ocean and western North Pacific2005

    • Author(s)
      Haobo Wang
    • Journal Title

      Journal of Atmospheric Chemistry (in press)

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Carbonaceous and ionic components in wintertime atmospheric aerosols from two New Zealand cities : Implication for solid fuel combustion2005

    • Author(s)
      Haobo Wang
    • Journal Title

      Atmospheric Environment Vol.39

      Pages: 5865-5875

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Diurnal changes in the distribution of dicarboxylic acids, ketocarboxylic acids and dicarbonyls in the urban atmosphere2005

    • Author(s)
      Kimitaka Kawamura
    • Journal Title

      Atmospheric Environment Vol.39

      Pages: 1945-1960

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Photochemical production and loss of organic acids in high Arctic aerosols during long range transport and polar sunrise ozone depletion events2005

    • Author(s)
      Kimitaka Kawamura
    • Journal Title

      Atmospheric Environment

      Pages: 599-614

    • NAID

      120000963994

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Molecular characteristics of of urban organic aerosols from Nanjing : A case study of a mega-city in China2005

    • Author(s)
      Gehui Wang
    • Journal Title

      Environmental Science and Technology Vol.39

      Pages: 7430-7438

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Age discrepancy between molecular biomarker and calcareous foraminifera isolated from same horizons from the Northwest Pacific sediments2005

    • Author(s)
      Masao Uchida
    • Journal Title

      Chemical Geology 218

      Pages: 73-89

    • Related Report
      2005 Annual Research Report
  • [Book] 第5版実験化学講座20-2 環境化学(日本化学会編)2007

    • Author(s)
      河村 公隆
    • Total Pages
      536
    • Publisher
      丸善
    • Related Report
      2006 Annual Research Report
  • [Book] エアロゾルの大気環境影響(笠原三紀夫・東野達編)2007

    • Author(s)
      河村 公隆
    • Total Pages
      361
    • Publisher
      京都大学学術出版会
    • Related Report
      2006 Annual Research Report
  • [Book] 大気・水圏の地球化学2005

    • Author(s)
      河村公隆
    • Total Pages
      336
    • Publisher
      培風館
    • Related Report
      2005 Annual Research Report

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Published: 2005-04-01   Modified: 2016-04-21  

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