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Room temperature spin-dependent single-electron-tunneling in nanostructures with controlled Fermi levels

Research Project

Project/Area Number 17360003
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Applied materials science/Crystal engineering
Research InstitutionTohoku University

Principal Investigator

MITANI Seiji  Tohoku University, Tohoku University, IMR, Associate Professor (20250813)

Co-Investigator(Kenkyū-buntansha) SHIMA Toshiyuki  Tohoku Gakuin University, Faculty of Engineering, Associate Professor (50261508)
TAKANASHI Koki  Tohoku University, IMR, Professor (00187981)
薬師寺 啓  東北大学, 金属材料研究所, 助手 (10361172)
Project Period (FY) 2005 – 2007
Project Status Completed (Fiscal Year 2007)
Budget Amount *help
¥15,060,000 (Direct Cost: ¥14,400,000、Indirect Cost: ¥660,000)
Fiscal Year 2007: ¥2,860,000 (Direct Cost: ¥2,200,000、Indirect Cost: ¥660,000)
Fiscal Year 2006: ¥2,600,000 (Direct Cost: ¥2,600,000)
Fiscal Year 2005: ¥9,600,000 (Direct Cost: ¥9,600,000)
KeywordsNanomaterials / Tunnel effect / Quantum dot / Spin electronics / Electron device / Coulomb blockade / 電子デバイス・機器 / フェルミ準位 / 帯電効果 / 磁気抵抗効果
Research Abstract

Aiming at the observation of spin dependent single electron tunneling phenomena at room temperature, experimental and theoretical studies were carried out on material properties, including Fermi levels, and device structures etc. In this study, the key issues were low resistive and low capacitive tunnel barriers and optimization of the whole device structures for the clear observation of spin dependent single electron tunneling.
In the experiments using MgO barriers, fairly good MgO barriers with the barrier height of ~ 1 eV were obtained, with good reproducibility and suitability for device applications, by choosing appropriate growth conditions. The obtained barrier height for MgO barrier layers is much lower than a half of the band gap for bulk MgO, and this suggests that the Fermi level shifts upward by about 2 eV, compared to that for bulk. While relatively low barrier heights were obtained, we found a problem for MgO barriers with a very low barrier height (typically < ~ 0.5 eV). Although low resistive barriers with a very low barrier height is useful for high temperature operation of single electron devices, their resistance ratio between on and off states for the devices is too small to be used for practical applications. In the experiments using AlO barriers, it was found that a multiple oxidation process is useful for preparation of flat tunnel barriers.
In addition, large tunnel magnetoresistance was observed for Fe and FeCo nanopartices embedded in a monocrystalline MgO matrix. This is almost the first observation of large tunnel magnetoresistance in monocrystalline granular systems, and the magnitude is consistent with the value predicted from spin polarization in Fe and FeCo.

Report

(4 results)
  • 2007 Annual Research Report   Final Research Report Summary
  • 2006 Annual Research Report
  • 2005 Annual Research Report
  • Research Products

    (25 results)

All 2007 2006 2005

All Journal Article (19 results) (of which Peer Reviewed: 6 results) Presentation (6 results)

  • [Journal Article] Preparation and magnetotransport properties of MgO-barrier-based magnetic doubletunnel junctions including nonmagnetic nanoparticles2007

    • Author(s)
      Y. Nogi
    • Journal Title

      Journal of Physics D 40

      Pages: 1242-1246

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Spin-accumulation in metallic nanoparticles2007

    • Author(s)
      F. Ernult
    • Journal Title

      Journal of Physics: Condensed Matter 19

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Spin-dependent tunneling and Coulomb blockade in ferromagnetic nanoparticles2007

    • Author(s)
      K. Yakushiji
    • Journal Title

      Phys. Rep. 451

      Pages: 1-35

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Annual Research Report 2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Spin dependent single electron tunneling and spin accumulation in metallic nanoparticles2007

    • Author(s)
      S. Mitani
    • Journal Title

      Proc. Northeastern Asian Symp. Adv. Mater.

      Pages: 96-99

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Annual Research Report 2007 Final Research Report Summary
  • [Journal Article] Preparation and magnetotransport properties of MgO-barrier-based magnetic double tunnel junctions including nonmagnetic nanoparticles2007

    • Author(s)
      Y. Nogi et. al.
    • Journal Title

      Journal of Physics D 40

      Pages: 1242-1246

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Spin-accumulation in metallic nanoparticles2007

    • Author(s)
      F. Ernult et. al.
    • Journal Title

      Journal of Physics: Condensed Matter 19

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Spin-dependent tunneling and Coulomb blockade in ferromagnetic nanoparticles2007

    • Author(s)
      K. Yakushiji et. al.
    • Journal Title

      Phys. Rep. 451

      Pages: 1-35

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Spin dependent single electron tunneling and spin accumulation in metallic nanoparitcles2007

    • Author(s)
      S. Mitani et. al.
    • Journal Title

      Proc. Northeastern Asican Symp. Adv. Mater.

      Pages: 96-99

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Preparation and magnetotransport properties of MgO-barrier-based magnetic double tunnel junctions including nonmagnetic nanoparticles2007

    • Author(s)
      Y.Nogi
    • Journal Title

      Journal of Physics D 40

      Pages: 1242-1246

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Spin-accumulation in metallic nanoparticles2007

    • Author(s)
      F.Ernult
    • Journal Title

      Journal of Physics : Condensed Matter (in press)

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Self-assembled metallic nanoparticles for spin dependent single electron tunneling2006

    • Author(s)
      F. Ernult
    • Journal Title

      Phase Transition 79

      Pages: 717-726

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Self-assembled metallic nanoparticles for spin dependent single electron tunneling2006

    • Author(s)
      F. Ernult et. al.
    • Journal Title

      Phase Transition 79

      Pages: 717-726

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Self-assembled metallic nanoparticles for spin dependent single electron tunneling2006

    • Author(s)
      F.Ernult
    • Journal Title

      Phase Transition 79

      Pages: 717-726

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Fabrication and characterization of L10-ordered FePt/AlO/FeComagnetic tunnel junctions2005

    • Author(s)
      S. Mitani
    • Journal Title

      IEEE Transaction on Magnetics 41

      Pages: 2602-2608

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Electrical transport and magnetoresistance in Co-Al-O granularfilms under high pressure2005

    • Author(s)
      S. Kaji
    • Journal Title

      Journal of Physical Society of Japan 74

      Pages: 2783-2790

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Fabrication and characterization of L10-ordered FePt/AlO/FeCo magnetic tunnel junctions2005

    • Author(s)
      S. Mitani et. al.
    • Journal Title

      IEEE Transaction on Magnetics 41

      Pages: 2602-2608

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Electrical transport and magnetoresistance in Co-Al-O granular films under high pressure2005

    • Author(s)
      S. Kaji et. al.
    • Journal Title

      Journal of Physical Society of Japan 74

      Pages: 2783-2790

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Fabrication and characterization of LlO-ordered FePt/AlO/FeCo magnetic tunnel junctions2005

    • Author(s)
      S.Mitani
    • Journal Title

      IEEE Transaction on Magnetics 41

      Pages: 2602-2608

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Electrical transport and magnetoresistance in Co-Al-O granular films under high pressure2005

    • Author(s)
      S.Kaji
    • Journal Title

      Journal of Physical Society of Japan 74

      Pages: 2783-2790

    • Related Report
      2005 Annual Research Report
  • [Presentation] Spin-dependent single electron tunneling and spin accumulation in nonmagnetic nanoparticles2007

    • Author(s)
      S. Mitani
    • Organizer
      lst International Symposium on Advanced Magnetic Materials and Application
    • Place of Presentation
      Jeju, Korea
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Spin-dependent single electron tunneling in nonmagnetic nanoparticles: Effect of spinaccumulation2007

    • Author(s)
      S. Mitani
    • Organizer
      Northern Asia Symposium on Advanced Materials
    • Place of Presentation
      Beijing, China
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Spin-dependent single electron tunneling and spin accumulation in nonmagnetic nanoparticles2007

    • Author(s)
      S. Mitani ed. al.
    • Organizer
      1^st International Symposium on Advanced Magnetic Materials and Application
    • Place of Presentation
      Jeju, Korea
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Spin-dependent single electron tunneling in nonmagnetic nanoparticles: Effect of spin accumulation2007

    • Author(s)
      S. Mitani ed. al.
    • Organizer
      Northern Asia Symposium on Advanced Materials
    • Place of Presentation
      Beijing, China
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Spin-dependent single electron tunneling and spin accumulation in nonmagnetic nanoparticles2007

    • Author(s)
      S. Mitani
    • Organizer
      1st International Symposium on Advanced Magnet ic Materials and Application
    • Place of Presentation
      Jeju, Korea
    • Related Report
      2007 Annual Research Report
  • [Presentation] Spin-dependent single electron tunneling in nonmagnetic nanoparticles: Effct of spin accumulation2007

    • Author(s)
      S. Mitani
    • Organizer
      Northern Asia Symposium on Advanced Materials
    • Place of Presentation
      Beijing, China
    • Related Report
      2007 Annual Research Report

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Published: 2005-04-01   Modified: 2016-04-21  

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