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Study on the transfer phenomena of gas, liquid, heat, and electron in a cell for the development of high performance PEM fuel cell available in low temperature conditions

Research Project

Project/Area Number 17360089
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Thermal engineering
Research InstitutionHokkaido University

Principal Investigator

CHIKAHISA Takemi  Hokkaido University, Graduate School of Engineering, Professor (00155300)

Co-Investigator(Kenkyū-buntansha) TABE Yutaka  Hokkaido University, Graduate School of Engineering, Associate Professor (80374578)
KIKUTA Kazushige  Hokkaido University, Graduate School of Engineering, Assistant Professor (90214741)
Project Period (FY) 2005 – 2007
Project Status Completed (Fiscal Year 2007)
Budget Amount *help
¥14,980,000 (Direct Cost: ¥14,200,000、Indirect Cost: ¥780,000)
Fiscal Year 2007: ¥3,380,000 (Direct Cost: ¥2,600,000、Indirect Cost: ¥780,000)
Fiscal Year 2006: ¥5,400,000 (Direct Cost: ¥5,400,000)
Fiscal Year 2005: ¥6,200,000 (Direct Cost: ¥6,200,000)
KeywordsFuel Cell / PEFC / Polymer Electric Membrane / Water / Freezing / Two Phase Flow / Observation / Gas Diffusion Layer
Research Abstract

This study has been conducted to clarify the mass, heat, electron transport phenomena in gas diffusion layers (GDLs) in fuel cell. Using an optical fuel cell, temperature distribution in cathode channel and current density distribution in anode channel was investigated. The experimental results showed that there is good correlation between the temperature distribution and the current density distribution, and uniformity of the contact pressure strongly influences the temperature and current density distributions. The observation result indicated that there is a condition when gas paths are established deep in the gas diffusion layer in flooded condition, suggesting a possibility to legalize good performance with utilizing this phenomenon.
In PEFC at low temperature, the freezing of produced water induces the extreme deterioration of cell performance. To clarify the freezing phenomenon and influencing factors of freezing in PEFC, experimental attempts were conducted. The results showed t … More hat the water initially diffuses back into the membrane, followed by water production in the surface of the cathode. The initial step is dependent on the water content in the membrane, and it must be controlled to an optimal value before lowering the temperature. It was also shown that the freezing characteristics are different for GDL characteristics. When temperature is lower than -20 deg. C, the frozen layer appears to be formed in catalysis layer.
The lattice Boltzmann method was applied and the two-phase flow in the separator-channels was simulated to understand the behavior of condensed water in PEMFC. The projection method was used for the large density difference between liquid and gas. Further, the wetting potential was introduced into the boundary conditions to consider the effect of wettability on the water behavior. It demonstrated the difference in the water removal motion for the different configurations and wettabilities of channels. The method can be a powerful tool for the simulation of two-phase flow in fuel cells. Less

Report

(4 results)
  • 2007 Annual Research Report   Final Research Report Summary
  • 2006 Annual Research Report
  • 2005 Annual Research Report
  • Research Products

    (44 results)

All 2008 2007 2006 2005

All Journal Article (12 results) (of which Peer Reviewed: 1 results) Presentation (32 results)

  • [Journal Article] 薄形セパレータを用いたPEM形燃料電池の性能影響因子評価2008

    • Author(s)
      高橋 浩, 関口 重幸, 近久 武美
    • Journal Title

      日本機械学会論文集(B編) 74-737

      Pages: 196-203

    • NAID

      110006571271

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Annual Research Report 2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Evaluation of Factors Influencing Performance of PEM Fuel Cell with Thin Separator Channels2008

    • Author(s)
      Takahasi, H., Sekiguchi, S., and Chikahisa, T.
    • Journal Title

      Trans. of JSME (B) 74-737

      Pages: 196-203

    • NAID

      130000303710

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Measurement of Water Production Phenomena, Temperature, and current Density Distributions in a Polymer Electrolyte Fuel Cell2006

    • Author(s)
      Chikahisa, Tabe, Kikuta, Nohara, Shinohara
    • Journal Title

      Proceedings of International Conference on Fuel Cell Science, Engineering and Technology (CD-ROM)

      Pages: 1-6

    • Related Report
      2006 Annual Research Report
  • [Journal Article] STUDY ON FREEZING PHENOMENA IN PEM FUEL CELL BLOW FREEZING2006

    • Author(s)
      Tabe, Nakamiya, Kikuta, Chikahisa, Kagami, Yoshizawa
    • Journal Title

      Proceedings of International Heat Transfer Conference (CD-ROM)

      Pages: 1-8

    • Related Report
      2006 Annual Research Report
  • [Journal Article] 氷点下起動時における固体高分子形燃料電池内凍結現象の温度分布画像計測2006

    • Author(s)
      田部, 中宮, 菊田, 近久, 各務, 吉澤
    • Journal Title

      日本伝熱シンポジウム講演論文集 Vol II

      Pages: 367-368

    • Related Report
      2006 Annual Research Report
  • [Journal Article] PEFC内の気液流動現象および電流密度分布と電池性能2006

    • Author(s)
      安田, 野原, 田部, 菊田, 近久, 篠原
    • Journal Title

      日本伝熱シンポジウム講演論文集 Vol II

      Pages: 377-378

    • Related Report
      2006 Annual Research Report
  • [Journal Article] PEFCにおけるガス拡散層およびセパレータチャネル内の気液流動特性と電池性能2006

    • Author(s)
      安田, 田部, 菊田, 近久, 小境
    • Journal Title

      電池討論会講演要旨集

      Pages: 208-209

    • Related Report
      2006 Annual Research Report
  • [Journal Article] 格子ボルツマン法によるセパレータチャネル内の液滴挙動シミュレーション2006

    • Author(s)
      木保, 田部, 菊田, 近久, 小境
    • Journal Title

      電池討論会講演要旨集

      Pages: 206-207

    • Related Report
      2006 Annual Research Report
  • [Journal Article] PEFCにおける物質・熱・電流移動の三次元数値シミュレーション2005

    • Author(s)
      石川, 菊田, 田部, 近久
    • Journal Title

      日本伝熱シンポジウム講演論文集 Vol.II

      Pages: 245-246

    • Related Report
      2005 Annual Research Report
  • [Journal Article] 固体高分子形燃料電池内現象の可視化と電流密度分布の同時計測2005

    • Author(s)
      野原, 菊田, 田部, 近久
    • Journal Title

      日本機械学会年次大会講演論文集 Vol.3

      Pages: 273-274

    • Related Report
      2005 Annual Research Report
  • [Journal Article] 氷点下起動時における固体高分子形燃料電池内凍結現象に関する研究2005

    • Author(s)
      中宮, 菊田, 田部, 近久, 各務, 吉澤
    • Journal Title

      日本機械学会年次大会講演論文集 Vol.3

      Pages: 275-276

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Numerical simulation of liquid water behavior in separator-channels in PEMFC using LBM2005

    • Author(s)
      Y.Tabe, T.Ochi, K.Kikuta, T.Chikahisa
    • Journal Title

      Proceeding of 3rd International Conference on Fuel Cell Science, Engineering and Technology (CD-ROM) 74172

      Pages: 1-6

    • Related Report
      2005 Annual Research Report
  • [Presentation] Numerical Simulation of Liquid Water and Air Flow in Separator-Channels in PEM Fuel Cell using LBM2007

    • Author(s)
      Tabe, Y., Kibo, K., Kikuta, K., Chikahisa, T. and Kozakai, M.
    • Organizer
      Proceedings of 7th ASME-JSME Thermal Engineering Summer Heat Transfer Conference
    • Place of Presentation
      Vancouver, Canada (Westin Bayshore)
    • Year and Date
      2007-07-10
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Simulation of Liquid Water and Air Flow in Separator-Channels in PEM Fuel Cell using LBMProceedings of 7th ASME-JSME Thermal Engineering Summer2007

    • Author(s)
      Tabe, Y., Kibo, K., Kikuta, K., Chikahisa, T. and Kozakai, M, Numerical
    • Organizer
      Heat Transfer Conference, CD-ROM
    • Place of Presentation
      Vancouver, Canada
    • Year and Date
      2007-07-10
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Numerical Simulation of Liquid Water and Air Flow in Separator-Channels in PEM Fuel Cell using LBM2007

    • Author(s)
      Tabe, Y., Kibo, K., Kikuta, K., Chikahisa, T. and Kozakai, M.
    • Organizer
      Proceedings of 7th ASME-JSME Thermal Engineering Summer Heat Transfer Conference
    • Place of Presentation
      Vancouver, Canada(Hotel; Westin Bayshore)
    • Year and Date
      2007-07-10
    • Related Report
      2007 Annual Research Report
  • [Presentation] PEFC内気液流動特性とその電流密度分布および電池性能に及ぼす影響2007

    • Author(s)
      吉田大輪, 安田陽介, 田部豊, 菊田和重, 近久武美, 小境正也.
    • Organizer
      第12回動力・エネルギー技術シンポジウム講演論文集、
    • Place of Presentation
      東京(東京海洋大学)
    • Year and Date
      2007-06-15
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Characteristics of Gas-Liquid Flow in PEM Fuel Cell and its Effect on Current Density Distribution and Cell Performance2007

    • Author(s)
      Yoshida, Yasuda, Tabe, Kikuta, Chikahisa, Kozakai
    • Organizer
      Power and Energy Conference
    • Place of Presentation
      Tokyo
    • Year and Date
      2007-06-15
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] PEFC内気液流動特性とその電流密度分布および電池性能に及ぼす影響2007

    • Author(s)
      吉田大輪, 安田陽介, 田部豊, 菊田和重, 近久武美, 小境正也.
    • Organizer
      第12回動力・エネルギー技術シンポジウム講演論文集
    • Place of Presentation
      東京(東京海洋大学)
    • Year and Date
      2007-06-15
    • Related Report
      2007 Annual Research Report
  • [Presentation] 氷点下における固体高分子形燃料電池の低温起動特性と凍結挙動2007

    • Author(s)
      福井、中宮、田部、近久、高橋、吉澤
    • Organizer
      第44回日本伝熱シンポジウム講演論文集Vol.I、2007.
    • Place of Presentation
      長崎(長崎ブリックホール)
    • Year and Date
      2007-05-23
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] 格子ボルツマン法によるPEFCセパレータチャネル内の気液二相流シミュレーション2007

    • Author(s)
      田部、木保、菊田、近久、小境
    • Organizer
      第44回日本伝熱シンポジウム講演論文集Vol.I、2007.
    • Place of Presentation
      長崎(長崎ブリックホール)
    • Year and Date
      2007-05-23
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Cold Start Characteristics and Freezing Phenomena in PEM fuel Cell below Freezing2007

    • Author(s)
      Fukui, Nakamiya, Tabe, Chikahisa, Takahashi, Yoshizawa
    • Organizer
      Heat Transfer Conference
    • Place of Presentation
      Nagasaki
    • Year and Date
      2007-05-23
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Simulation in Separator-Channel of PEM Fuel Cell using Lattice Boltzmann Method2007

    • Author(s)
      Tabe, Kibo, Kikuta, Chikahisa, Kozakai, Two-Phase Gas-Liquid Flow
    • Organizer
      Heat Transfer Conference
    • Place of Presentation
      Nagasaki
    • Year and Date
      2007-05-23
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] 氷点下における固体高分子形燃料電池の低温起動特性と凍結挙動2007

    • Author(s)
      福井薫, 中宮弘満, 田部豊, 近久武美, 高橋真一, 吉澤幸大
    • Organizer
      第44回日本伝熱シンポジウム講演論文集Vol. I
    • Place of Presentation
      長崎(長崎ブリックホール)
    • Year and Date
      2007-05-23
    • Related Report
      2007 Annual Research Report
  • [Presentation] 格子ボルツマン法によりるPEFCセパレータチャネル内気液二相流シミュレーション2007

    • Author(s)
      田部豊, 木保康介, 菊田和重, 近久武美, 小境正也
    • Organizer
      第44回日本伝熱シンポジウム講演論文集Vol. I
    • Place of Presentation
      長崎(長崎ブリックホール)
    • Year and Date
      2007-05-23
    • Related Report
      2007 Annual Research Report
  • [Presentation] PEFCにおけるガス拡散層およびセパレータチャネル内の気液流動特性と電池性能2006

    • Author(s)
      安田、田部、菊田、近久、小境.
    • Organizer
      電池討論会講演要旨集、2006、208-209
    • Place of Presentation
      東京(江戸川区総合区民ホール)
    • Year and Date
      2006-11-22
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] 格子ボルツマン法によるセパレータチャネル内の液滴挙動シミュレーション2006

    • Author(s)
      木保、田部、菊田、近久、小境
    • Organizer
      電池討論会講演要旨集、2006、206-207
    • Place of Presentation
      東京(江戸川区総合区民ホール)
    • Year and Date
      2006-11-22
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Relationship among Gas and Water Flow Behavior in Gas Diffusion Layer and Separator Channel, and Cell Performance in Polymer Electrolyte Fuel Cell2006

    • Author(s)
      Yasuda, Tabe, Kikuta, Chikahisa, Kozakai
    • Organizer
      Battery conference
    • Place of Presentation
      Tokyo
    • Year and Date
      2006-11-22
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Numerical simulation of liquid water behavior in separator-channels using LBM2006

    • Author(s)
      Kibo, Tabe, Kikuta, Chikahisa, Kozakai
    • Organizer
      Battery conference
    • Place of Presentation
      Tokyo
    • Year and Date
      2006-11-22
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Measurement of Water Production Phenomena, Temperature, and current Density Distributions in a Polymer Electrolyte Fuel Cell2006

    • Author(s)
      Chikahisa, Tabe, Kikuta, Nohara, Shinohara
    • Organizer
      Proceedings of 4th International Conference on Fuel Cell Science, Engineering and Technology
    • Place of Presentation
      Irvine, California (Hyatt Regency Irvine Hotel)
    • Year and Date
      2006-06-19
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Study on Freezing Phenomena in PEM Fuel Cell blow Freezing2006

    • Author(s)
      Tabe, Nakamiya, Kikuta, Chikahisa, Kagami, Yoshizawa
    • Organizer
      Proceedings of International Heat Transfer Conference、 CD-ROM、 2006、 1-8
    • Place of Presentation
      Sydney, Australia (Sydney Convention and Exhibition Centre)
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] 氷点下起動時における固体高分子形燃料電池内凍結現象の温度分布画像計測2006

    • Author(s)
      田部、中宮、菊田、近久、各務、吉澤.
    • Organizer
      日本伝熱シンポジウム講演論文集Vol II、2006、367-368
    • Place of Presentation
      名古屋(名古屋国際会議場)
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] PEFC内の気液流動現象および電流密度分布と電池性能2006

    • Author(s)
      安田、野原、田部、菊田、近久、篠原
    • Organizer
      日本伝熱シンポジウム講演論文集、Vol II、2006、377-378
    • Place of Presentation
      名古屋(名古屋国際会議場)
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Study on Freezing Pheomena in PEM Fuel Cell blow Freezing2006

    • Author(s)
      Tabe, Nakamiya, Kikuta, Chikahisa, Kagami, Yoshizawa
    • Organizer
      Proceedings of International Heat Transfer Conference
    • Place of Presentation
      Sydney, Australia
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Visualization of Freezing Phenomenon in Polymer Electrolyte Fuel Cell by Temperature Distribution Measurement2006

    • Author(s)
      Tabe, Nakamiya, Kikuta, Chikahisa, Kagami, Yoshizawa
    • Organizer
      Heat Transfer Conference
    • Place of Presentation
      Nagoya
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Relationship among Gas and Water Flow Behavior, Local Current Density Distribution and Cell Performance in Polymer Electrolyte Fuel Cell2006

    • Author(s)
      Yasuda, Nohara, Tabe, Kikuta, Chikahisa, Shinohara
    • Organizer
      Heat Transfer Conference
    • Place of Presentation
      Nagoya
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] 固体高分子形燃料電池内現象の可視化と電流密度分布の同時計測2005

    • Author(s)
      野原、菊田、田部、近久
    • Organizer
      日本機械学会年次大会講演論文集、Vol.3、2005、273-274
    • Place of Presentation
      調布(電気通信大学)
    • Year and Date
      2005-09-19
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] 氷点下起動時における固体高分子形燃料電池内凍結現象に関する研究2005

    • Author(s)
      中宮、菊田、田部、近久、各務、吉澤
    • Organizer
      日本機械学会年次大会講演論文集、Vol.3、2005、275-276
    • Place of Presentation
      調布(電気通信大学)
    • Year and Date
      2005-09-19
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Simultaneous Measurement of Mass and Heat Transfer Phenomena and Current Density Distribution in PEFC2005

    • Author(s)
      Nohara, Kikuta, Tabe, Chikahisa
    • Organizer
      JSME Conference
    • Place of Presentation
      Chofu
    • Year and Date
      2005-09-19
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Study on Freezing Phenomenon in Polymer Electrolyte Fuel Cell2005

    • Author(s)
      Nakamiya, Kikuta, Tabe, Chikahisa
    • Organizer
      JSME Conference
    • Place of Presentation
      Chofu
    • Year and Date
      2005-09-19
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Numerical simulation of liquid water behavior in separator-channels in PEMFC using LBM2005

    • Author(s)
      Y. Tabe, T. Ochi, K. Kikuta, and T. Chikahisa
    • Organizer
      Proceedings of 3rd International Conference on Fuel Cell Science, Engineering and Technology
    • Place of Presentation
      Ypsilanti, Michigan (Ypsilanti Marriott Hotel)
    • Year and Date
      2005-05-23
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Numerical simulation of liquid water behavior in separator- channels in PEMFC using LBM2005

    • Author(s)
      Y. Tabe, T. Ochi, K. Kikuta, and T. Chikahisa
    • Organizer
      Proceedings of 3rd International Conference on Fuel Cell Science, Engineering and Techology
    • Place of Presentation
      Ypsilanti, Michigan
    • Year and Date
      2005-05-23
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Temperatrue, and current Density Distributions in a Polymer electrolyte Fuel Cell2005

    • Author(s)
      Chikahisa, Tabe, Kikuta, Nohara, Shinohara, Measurement of Water Production Phenomena
    • Organizer
      Proceedings of International Conference on Fuel Cell Science, Engineering and Technology
    • Place of Presentation
      Ypsilanti, Michigan
    • Year and Date
      2005-02-23
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] PEFCにおける物質・熱・電流移動の三次元数値シミュレーション2005

    • Author(s)
      石川、菊田、田部、近久
    • Organizer
      P日本伝熱シンポジウム講演論文集、Vol.II、2005、245-246
    • Place of Presentation
      仙台(仙台国際センター)
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] 3D numerical simulation of mass, heat and electron transfer in OEM fuel cells2005

    • Author(s)
      Ishikawa, Kikuta, Tabe, Chikahisa
    • Organizer
      Heat Transfer Conference
    • Place of Presentation
      Sendai
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary

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Published: 2005-04-01   Modified: 2016-04-21  

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