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Membrane filtration with rapid pretreatment using adsorbent of submicron particle size

Research Project

Project/Area Number 17360255
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Civil and environmental engineering
Research InstitutionHokkaido University

Principal Investigator

MATSUI Yoshihiko  Hokkaido University, Graduate School of Engineering, Professor, 大学院工学研究科, 教授 (00173790)

Co-Investigator(Kenkyū-buntansha) MATSUSHIMA Taku  Hokkaido University, Graduate School of Engineering, Associate Professor, 大学院工学研究科, 助教授 (30283401)
Project Period (FY) 2005 – 2006
Project Status Completed (Fiscal Year 2006)
Budget Amount *help
¥11,900,000 (Direct Cost: ¥11,900,000)
Fiscal Year 2006: ¥2,800,000 (Direct Cost: ¥2,800,000)
Fiscal Year 2005: ¥9,100,000 (Direct Cost: ¥9,100,000)
Keywordsadsorption / powdered activated carbon / MF membrane / membrane separation / drinking water treatment
Research Abstract

Normal manufacturer-supplied powdered activated carbon (PAC) was pulverized to reduce the PAC particle size to less than 1 μm; we call the pulverized PAC super-powdered activated carbon (S-PAC). Advantages of S-PAC over normal PAC, mainly in terms of adsorptive removal of natural organic matter (NOM) and geosmin (musty-earthy taste and odor compund), were studied. Batch adsorption kinetic tests and tubular flow reactor tests revealed that S-PAC rapidly adsorbed NOM from water samples. NOM concentration rapidly decreased after S-PAC addition and reached a plateau of practically attainable removal in a contact time of 5 s. Next, S-PAC adsorption as a pretreatment for microfiltration (MF) was studied by using laboratory-scale and bench-scale pilot plants. Use of S-PAC could decrease significantly the detention time for adsorption pretreatment before MF. A detention time of 2.4 s yielded the same NOM concentration in the MF permeate as a detention of 15 min. Use of S-PAC could also decrease the dosage compared with normal PAC by a factor of 1/4. The dosing sequence, PAC followed by coagulant and then MF, showed slightly better NOM removal than the sequence, coagulant followed by PAC and then MF, suggesting that flocculation of PAC particles somewhat hinders adsorbate uptake into PAC particles. Adsorption pretreatment by using this S-PAC removed the geosmin with vastly greater efficiency than by normal PAC. Removal was attained in a much shorter contact time and at a much lower dosage. The S-PAC was also beneficial in attenuating the trans-membrane pressure rises that occurred between both physical backwashings and chemical cleanings. No membrane fouling effect was observed as a result of S-PAC addition before MF.

Report

(3 results)
  • 2006 Annual Research Report   Final Research Report Summary
  • 2005 Annual Research Report
  • Research Products

    (16 results)

All 2006 2005

All Journal Article (16 results)

  • [Journal Article] Evaluating submicron-sized activated carbon adsorption for microfiltration pretreatment2006

    • Author(s)
      Yoshihiko Matsui et al.
    • Journal Title

      Water Sci. Technol : Water Supply 6(1)

      Pages: 149-155

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Evaluating submicron-sized activated carbon adsorption for microfiltration pretreatment.2006

    • Author(s)
      Matsui, Y., Sanogawa, T., Aoki, N., Mima, S., Matsushita
    • Journal Title

      Water Sci. Technol : Water Supply 6(1)

      Pages: 149-155

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Evaluating submicron-sized activated carbon adsorption for microfiltration pretreatment2006

    • Author(s)
      Matsui, Y., Sanogawa, T., Aoki, N., Mima, S., Matsushita
    • Journal Title

      Water Sci. Technol : Water Supply 6(1)

      Pages: 149-155

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Adsorptive removal of geosmin by ceramic membrane filtration with super-powdered activated carbon adsorption2006

    • Author(s)
      Matsui, Y., Aizawa, T., Suzuki, M., Kawase, Y.
    • Journal Title

      Proc. 7th International Symposium on Water Supply Technology 2006

      Pages: 462-469

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Characteristics of submicron activated carbon adsorption : experiments and a branched -pore model analysis2006

    • Author(s)
      Matsui, Y., Kurihara, S., Sanogawa, T., Murai, K., Sawaoka, D., Ohno, K.
    • Journal Title

      Proceedings IWA 5th World Water Congress 2006(CR-ROM)

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Enhancing an Adsorption-Membrane Hybrid System with Microground Activated Carbon.2005

    • Author(s)
      Yoshihiko Matsui et al.
    • Journal Title

      Water Sci. & Tech. : Water Supply 4

      Pages: 189-197

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Rapid Adsorption Pretreatment with Submicron Powdered Activated Carbon Particles before Microfiltration.2005

    • Author(s)
      Yoshihiko Matsui et al.
    • Journal Title

      Water Sci. & Tech. 51

      Pages: 249-256

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Ceramic MF with Submicron-sized Activated Carbon Adsorption and Coagulation Pretreatments for Rapid and Effective NOM Removal.2005

    • Author(s)
      Yoshihiko Matsui et al.
    • Journal Title

      Water and Environmental Management Series (WEMS), 2nd IWA Leading-Edge on Water and Wastewater Treatment Technologies 8

      Pages: 23-32

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Enhancing an Adsorption-Membrane Hybrid System with Microground Activated Carbon.2005

    • Author(s)
      Yoshihiko Matsui, Yoshitaka Fukuda, Takanobu Inoue, Taku Matsushita, Nobuhiro Aoki, Satoru Mima
    • Journal Title

      Water Sci. & Tech. : Water Supply 4(5-6)

      Pages: 189-197

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Rapid Adsorption Pretreatment with Submicron Powdered Activated Carbon Particles before Microfiltration.2005

    • Author(s)
      Yoshihiko Matsui, Ryota Murase, Takahiro Sanogawa, Nobuhiro Aoki, Satoru Mima, Takanobu, Inoue, Taku Matsushita
    • Journal Title

      Water Sci. & Tech. 51(6-7)

      Pages: 249-256

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Ceramic MF with Submicron-sized Activated Carbon Adsorption and Coagulation Pretreatments for Rapid and Effective NOM Removal.2005

    • Author(s)
      Yoshihiko Matsui, Yoshitaka Fukuda, Ryota Murase, Nobuhiro Aoki, Satoru Mima, Takanobu Inoue, Taku Matsushita
    • Journal Title

      Water and Environmental Management Series (WEMS) 2ndIWA Leading-Edge on Water and Wastewater Treatment Technologies No.8

      Pages: 23-32

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Micro-ground Powdered Activated Carbon for Effective Removal of Nat ural Organic Matter during Water Treatment2005

    • Author(s)
      Yoshihiko Matsui et al.
    • Journal Title

      Water Sci.& Tech.:Water Supply 4

      Pages: 155-163

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Enhancing an Adsorption-Membrane Hybrid System with Microground Activated Carbon.2005

    • Author(s)
      Yoshihiko Matsui et al.
    • Journal Title

      Water Sci.& Tech.:Water Supply 4

      Pages: 189-197

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Rapid Adsorption Pretreatment with Submicron Powdered Activated Carbon Particles before Microfiltration.2005

    • Author(s)
      Yoshihiko Matsui et al.
    • Journal Title

      Water Sci.& Tech. 51

      Pages: 249-256

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Ceramic MF with Submicron-sized Activated Carbon Adsorption and Coagulation Pretreatments for Rapid and Effective NOM Removal.2005

    • Author(s)
      Yoshihiko Matsui et al.
    • Journal Title

      Water and Environmental Management Series (WEMS), 2nd IWA Leading-Edge on Water and Wastewater Treatment Technologies, 8

      Pages: 23-32

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Evaluating submicron-sized activated carbon adsorption for microfiltration pretreatment.2005

    • Author(s)
      Yoshihiko Matsui et al.
    • Journal Title

      Proceedings of IWA International Conference on Particle Separation, Seoul, Korea

      Pages: 553-560

    • Related Report
      2005 Annual Research Report

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Published: 2005-04-01   Modified: 2016-04-21  

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