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Research for Hyperfine Nuclear Magnetism of PrPba in the Antiferro-Quadrupoinr Ordered State

Research Project

Project/Area Number 17540321
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Condensed matter physics II
Research InstitutionKanazawa University

Principal Investigator

ABE Satoshi  Kanazawa University, Graduate School of Natural Science and Technology, Lecturer (60251914)

Co-Investigator(Kenkyū-buntansha) MATSUMOTO Koichi  Kanazawa University, Graduate School of NaturalScience and Technoology, Associate Professor (10219496)
鈴木 治彦  金沢大学, 自然科学研究科, 教授 (50004370)
Project Period (FY) 2005 – 2007
Project Status Completed (Fiscal Year 2007)
Budget Amount *help
¥3,640,000 (Direct Cost: ¥3,400,000、Indirect Cost: ¥240,000)
Fiscal Year 2007: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2006: ¥900,000 (Direct Cost: ¥900,000)
Fiscal Year 2005: ¥1,700,000 (Direct Cost: ¥1,700,000)
KeywordsQuadrupole ordering / Enhanced nuclear magnetism / Nuclear magnetic ordering / Ultra low temperatures / 反強四極子秩序 / 反強四重極子秩序
Research Abstract

We have investigated the hyperfine enhanced nuclear magnetic properties of PrPb3 at the antiferro quadrupole (AFQ) ordered state at ultra low temperatures. The static magnetization and the ac susceptibility of PrPb3 single crystals in the magnetic fields up 6.21 mT parallel to [100] and [110] directions were simultaneously measured down to below 1 mK by an ac impedance bridge using a SQUID magnetometer. In the AFQ ordered state, the hyperfine enhanced nuclear magnetic susceptibility increased below 40 mK according to the Curie Weiss law, and showed a peak at 5 mK. The enhancement factor obtained from the Curie constant was 1+K=30. The peak height at 5 mK was only 10^<3> of the expected saturated nuclear magnetization. These results suggest that the hyperfine enhanced nuclear magnetic moments of <141>^Pr antiferromagnetically order below 5 mK. The ac susceptibility in the magnetic field and the static magnetization around the zero magnetic field have a different temperature dependence from the static magnetization in the magnetic field. The ac susceptibility and the static magnetization show the superconductive diamagnetism at 35.7 mK, and the critical magnetic field at zero temperature is 0.568 mT.
In order to measure the magnetic susceptibility in higher magnetic fields, we have developed a new ac susceptibility measurement system without a SQUID magnetometer which is assembled from five pick up coils and a modulation coil for mutual inductance measurement, a small superconducting solenoid for applying static magnetic filed, and the magnetic shield of niobium and it-metal cylinders. Furthermore, cooperating with Metoki group in Japan Atomic Energy Agency, we have developed a nuclear adiabatic demagnetization refrigerator for a neutron diffraction measurement at sub milikelvin temperatures for the purpose of direct observation of nuclear ordered spin structures.

Report

(4 results)
  • 2007 Annual Research Report   Final Research Report Summary
  • 2006 Annual Research Report
  • 2005 Annual Research Report
  • Research Products

    (30 results)

All 2008 2007 2006 2005

All Journal Article (7 results) (of which Peer Reviewed: 2 results) Presentation (23 results)

  • [Journal Article] 金沢大学極低温研究室と物性研究2008

    • Author(s)
      阿部聡
    • Journal Title

      低温工学 43

      Pages: 29-29

    • NAID

      10019913483

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Solid state physics research at Ultra low temperature Laboratory in Kanazawa University2008

    • Author(s)
      S. Abe
    • Journal Title

      J. Cyro. Soc. Jpn(Unrefereed) 43

      Pages: 28-29

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Hyperfine Nuclear Magnetism of PrPb_3 in the Antiferro-Quadrupolar Ordered State2006

    • Author(s)
      S. Abe, (他5名)
    • Journal Title

      AIP Conf. Proc. 850

      Pages: 1293-1294

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Magnetic properties of CeRu_2Si_2 at small magnetic fields and ultra low temperatures2006

    • Author(s)
      J. Yoshida, S. Abe, (他3名)
    • Journal Title

      AIP Conf. Proc. 850

      Pages: 1171-1173

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Hyperfine Nuclear Magnetism of PrPb3 in the Antiferro-Quadrupolar Ordered State2006

    • Author(s)
      S. Abe, D. Takahashi, J. Yoshida, K. Matsumoto, H. Suzuki, T. Kitai
    • Journal Title

      AIP Conf. Proc(Refereed) 850

      Pages: 1293-1294

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Magnetic properties of CeRu2Si2 at small magnetic fields and ultra low temperatures2006

    • Author(s)
      J. Yoshida, S. Abe, D. Takahashi, K. Matsumoto, H. Suzuki
    • Journal Title

      AIP Conf. Proc(Refereed) 850

      Pages: 1171-1173

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Hyperfine Nuclear Magnetism of PrPb_3 in the Antiferro-Quadrupolar Ordered State2006

    • Author(s)
      S.Abe
    • Journal Title

      AIP Conf. Proc. 850

      Pages: 1293-1294

    • Related Report
      2006 Annual Research Report
  • [Presentation] 熱膨張測定による重い電子系CeRu2Si2の量子臨界現象の研究2007

    • Author(s)
      瀬川芳紀, 阿部聡, (他6名)
    • Organizer
      日本物理学会年次大会
    • Place of Presentation
      北海道大学札幌キャンパス
    • Year and Date
      2007-09-21
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] PrMg3の核磁気秩序状態の探索2007

    • Author(s)
      吉田潤, 阿部聡, (他4名)
    • Organizer
      日本物理学会年次大会
    • Place of Presentation
      北海道大学札幌キャンパス
    • Year and Date
      2007-09-21
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] JRR-3の多目的単色熱中性子実験ビームポート「武蔵」における超低温中性子散乱実験2007

    • Author(s)
      目時直人, 阿部聡, (他4名)
    • Organizer
      日本物理学会年次大会
    • Place of Presentation
      北海道大学札幌キャンパス
    • Year and Date
      2007-09-21
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] 中性子散乱実験用核断熱消磁ステージの開発2007

    • Author(s)
      阿部聡, (他7名)
    • Organizer
      日本物理学会年次大会
    • Place of Presentation
      北海道大学札幌キャンパス
    • Year and Date
      2007-09-21
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Study of the Quantum Critical Phenomena of Heavy-Fermion CeRu2Si2 by Thermal Expansion Measurements2007

    • Author(s)
      Y. Segawa
    • Organizer
      Meeting of the Physical Society of Japan
    • Place of Presentation
      Hokkaido University
    • Year and Date
      2007-09-21
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Search for Nuclear Magnetic Ordered State in PrMg32007

    • Author(s)
      J. Yoshida
    • Organizer
      Meeting of the Physical Society of Japan
    • Place of Presentation
      Hokkaido University
    • Year and Date
      2007-09-21
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Instrumentation for neutron scattering experiments at ultra-low temperature at MUSASI beam port in JRR-32007

    • Author(s)
      N. Metoki
    • Organizer
      Meeting of the Physical Society of Japan
    • Place of Presentation
      Hokkaido University
    • Year and Date
      2007-09-21
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Development of the nuclear demagnetization cryostat for neutron diffraction experiments2007

    • Author(s)
      S. Abe
    • Organizer
      Meeting of the Physical Society of Japan
    • Place of Presentation
      Hokkaido University
    • Year and Date
      2007-09-21
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] 中性子散乱実験用核断熱消磁ステージの開発2007

    • Author(s)
      阿部 聡(他8名)
    • Organizer
      日本物理学会
    • Place of Presentation
      北海道大学札幌キャンパス
    • Year and Date
      2007-09-21
    • Related Report
      2007 Annual Research Report
  • [Presentation] JRR-3の多目的単色熱中性子実験ビームポート「武蔵」における超低温中性子散乱実験2007

    • Author(s)
      目時 直人(他5名)
    • Organizer
      日本物理学会
    • Place of Presentation
      北海道大学札幌キャンパス
    • Year and Date
      2007-09-21
    • Related Report
      2007 Annual Research Report
  • [Presentation] 超低温領域における重い電子系CeRu_2Si_2の熱膨張測定2007

    • Author(s)
      吉田潤, 阿部聡, (他5名)
    • Organizer
      日本物理学会春季大会
    • Place of Presentation
      鹿児島大学郡元キャンパス
    • Year and Date
      2007-03-18
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Thermal Expansion Measurement of Heavy-Fermion CeRu2Si2 at Ultra Low Temperatures2007

    • Author(s)
      J. Yoshida
    • Organizer
      Meeting of the Physical Society of Japan
    • Place of Presentation
      Kagoshima University
    • Year and Date
      2007-03-18
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] 超低温領域における重い電子系CeRu2Si2の熱膨張測定II2006

    • Author(s)
      吉田潤, 阿部聡, (他5名)
    • Organizer
      日本物理学会年次大会
    • Place of Presentation
      愛媛大学・松山大学
    • Year and Date
      2006-03-29
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Thermal Expansion Measurement of Heavy-Fermion CeRu2Si2 at Ultra Low Temperatures II2006

    • Author(s)
      J. Yoshida
    • Organizer
      Meeting of the Physical Society of Japan
    • Place of Presentation
      Ehime University and Matsuyama Universit
    • Year and Date
      2006-03-29
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] 超低温領域における重い電子系CeRu_2Si_2の熱膨張測定2005

    • Author(s)
      吉田潤, 阿部聡, (他5名)
    • Organizer
      日本物理学会秋期大会
    • Place of Presentation
      同志社大学京田辺キャンパス
    • Year and Date
      2005-09-19
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Thermal Expansion Measurement of Heavy-Fermion CeRu2Si2 at Ultra Low Temperatures2005

    • Author(s)
      J. Yoshida
    • Organizer
      Meeting of the Physical Society of Japan
    • Place of Presentation
      Doshisya University
    • Year and Date
      2005-09-19
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Thermal Expansion Measurement of Heavy-Fermion CeRu2Si2 at Ultra Low Temperatures2005

    • Author(s)
      J. Yoshida
    • Organizer
      Meeting of the Physical Society of Japan
    • Place of Presentation
      Tokyo University of Science
    • Year and Date
      2005-03-25
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Hyperfine Nuclear Magnetism of PrPb_3 in the Antiferro-Quadrupolar Orderde State2005

    • Author(s)
      S. Abe, (他5名)
    • Organizer
      24th International Conference on Low Temperature Physics
    • Place of Presentation
      Orlando, Florida, U. S. A.
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Magnetic properties of CeRu_2Si_2 at small magnetic fields and ultra low temperatures2005

    • Author(s)
      J. Yoshida, S. Abe, (他3名)
    • Organizer
      24th International Conference on Low Temperature Physics
    • Place of Presentation
      Orlando, Florida, U. S. A.
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Hyperfine Nuclear Magnetism of PrPb_3 in the Antiferro-Quadrupolar Ordered State2005

    • Author(s)
      S. Abe, (他5名)
    • Organizer
      International Conference on Ultra Low Temperature Physics 2005
    • Place of Presentation
      Gainesville, Florida, U. S. A
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Hyperfine Nuclear Magnetism of PrPb3 in the Antiferro-Quadrupolar Ordered State2005

    • Author(s)
      S. Abe
    • Organizer
      24th International Conference on Low Temperature Physics
    • Place of Presentation
      Orlando, Florida, U.S.A
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Magnetic properties of CeRu2Si2 at small magnetic fields and ultra low temperatures2005

    • Author(s)
      J. Yoshida
    • Organizer
      24th International Conference on Low Temperature Physics
    • Place of Presentation
      Orlando, Florida. U.S.A
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Hyperfine Nuclear Magnetism of PrPb3 in the Antiferro-Quadrupolar Ordered State2005

    • Author(s)
      S. Abe
    • Organizer
      International Conference on Ultra Low Temperature Physics 2005
    • Place of Presentation
      Gainesville. Florida. U.S.A
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary

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Published: 2005-04-01   Modified: 2020-05-15  

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