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Experimental investigation of quantum phase transition on one-dimensional spin gapped system

Research Project

Project/Area Number 17540331
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Condensed matter physics II
Research InstitutionKYUSHU UNIVERCITY

Principal Investigator

HITAKA Masako  Kyushu University, Faculty of Engineering, Research Associate, 大学院工学研究院, 助手 (00264094)

Co-Investigator(Kenkyū-buntansha) KAWAE Tatsuya  Kyushu University, Faculty of Engineering, Associate Professor, 大学院工学研究院, 助教授 (30253503)
IDOGAKI Toshihiro  Kyushu University, Faculty of Engineering, Professor, 大学院工学研究院, 教授 (40038013)
Project Period (FY) 2005 – 2006
Project Status Completed (Fiscal Year 2006)
Budget Amount *help
¥3,500,000 (Direct Cost: ¥3,500,000)
Fiscal Year 2006: ¥1,100,000 (Direct Cost: ¥1,100,000)
Fiscal Year 2005: ¥2,400,000 (Direct Cost: ¥2,400,000)
Keywordsspin gap / one-dimensional Heisenberg spin / antiferromagnetic spin chain / low temperature and high field / field induced phase transition / Tomonaga-Luttinger liquid / F_5PNN / DMACuCl_3 / 一次元ハイゼンベルグ系 / 極低温・磁場中比熱測定
Research Abstract

We have studied a typical S=1/2 Heisenberg alternating spin chain system ; pentafulorophenyl nitronyl nitroxide (F_5PNN) and a novel magnetic system with two critical field regios ; (CH_3)_2NH_2CuCl_3 (DMACuCl_3) to investigate field induced phase transitions and Tomonaga-Luttinger liquid phase in spin-gapped system.
In F_5PNN, we found a field induced magnetic ordering between Hc1=3T and Hc2=6.5T below T=250mK. Characteristic behaviors are observed depending on the magnetic field up to above Hc2 outside of the H-T phase boundary for the field induced phase. The temperature and field dependence of the specific heat are qualitatively in good agreement with the theoretical calculation on an S=1/2 spin gapped system.
In DMACuCl_3,a spontaneous magnetic ordering is observed below Hc1=2T, while no magnetic ordering is in the 1/2 magnetization plateau field region from Hc1=2T to Hc2 =3.5T. A field induced magnetic ordering emerges above Hc2=3.5T, which grows with increasing magnetic field up to H=8T.

Report

(3 results)
  • 2006 Annual Research Report   Final Research Report Summary
  • 2005 Annual Research Report
  • Research Products

    (20 results)

All 2006 2005

All Journal Article (20 results)

  • [Journal Article] Possible Observation of the Quadrupolar Kondo Effect in Dilute Quadrupolar System Pr_xLa_<1-x>Pb_3 for x≦O.052006

    • Author(s)
      T.Kawae 他 6名
    • Journal Title

      Physical Review Letters 96

      Pages: 27210-27210

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Coexisting Ferromagnetic Order and Disorder in a Uniform System of Hydroxyhalide Co_2(OH)_3Cl2006

    • Author(s)
      X.G.Zheng, T.Kawae, 他3名
    • Journal Title

      Physical Review Letters 97

      Pages: 247204-247204

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Annual Research Report 2006 Final Research Report Summary
  • [Journal Article] Non-Fermi Liquid Behavior in Pr-based Dilute Quadrupolar System2006

    • Author(s)
      T.Kawae 他8名
    • Journal Title

      Journal of Alloys and Compounds 408

      Pages: 47-50

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Annual Research Report 2006 Final Research Report Summary
  • [Journal Article] Pressure-induced Valence Change in the Rare Earth Metals : The Case of Praseodymium2006

    • Author(s)
      N.Tateiwa, A.Nakagawa, K.Fujio, T.Kawae, K.Takeda
    • Journal Title

      Journal of Alloys and Compounds 408

      Pages: 244-247

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Annual Research Report 2006 Final Research Report Summary
  • [Journal Article] Single-crystal Growth of Layered Ce-Ni-Ge Ternary Compounds2006

    • Author(s)
      M.Ohashi, G.Oomi, K.Ishida, I.Satoh, T.Komatsubara, T.Kawae, K Takeda
    • Journal Title

      Journal of Alloys and Compounds 408

      Pages: 84-87

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Annual Research Report 2006 Final Research Report Summary
  • [Journal Article] Molecular Field and Monte Carlo Study for the Mixed-Spin Axial Next-Nearest- Neighbor Ising Model2006

    • Author(s)
      T.Kasama, Y.Muraoka, T.Idogaki
    • Journal Title

      Physical Review B73

      Pages: 214411-214411

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Possible Observation of the Quadrupolar Kondo Effect in Dilute Quadrupolar System Pr_xLa_<1-x>Pb_3 for x≦0.052006

    • Author(s)
      T.Kawae, K.Kinoshita, Y.Nakaie, N.Tateiwa, K.Takeda, H.S.Suzuki, T.Kitai.
    • Journal Title

      Phys.Rev.Lett. 96

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Coexisting Ferromagnetic Order and Disorder in a Uniform System of Hydroxyhalide Co_2(OH)_3Cl2006

    • Author(s)
      X.G.Zheng, T.Kawae, H.Yamada, K.Nishiyama, C.N.Xu
    • Journal Title

      Phys.Rev.Lett. 97

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Non-Fermi Liquid Behavior in Pr-based Dilute Quadrupolar System2006

    • Author(s)
      T.Kawae, K.Kinoshita, CS.Li, Y.Nakaie, Y.Yoshida, M.Hitaka, N.Tateiwa, K.Takeda, T.Kitai
    • Journal Title

      Journal of Alloys and Compounds 408

      Pages: 47-50

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Pressure-induced Valence Change in the Rare Earth Metals : The Case of raseodymium2006

    • Author(s)
      N.Tateiwa, A.Nakagawa, K.Fujio, T.Kawae, K.Takeda
    • Journal Title

      Journal of Alloys and Compounds 408

      Pages: 244-247

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Single-crystal Growth of Layered Ce-Ni-Ge Ternary Compounds2006

    • Author(s)
      M.Ohashi, G.Oomi, K.Ishida, I.Satoh, T.Komatsubara, T.Kawae, K Takeda
    • Journal Title

      Journal of Alloys and Compounds 480

      Pages: 84-87

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Molecular Field and Monte Carlo Study for the Mixed-Spin Axial Next-Nearest-Neighbor Ising Model2006

    • Author(s)
      T.Kasama, Y.Muraoka, T.Idogaki
    • Journal Title

      Phys.Rev.B 73

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Possible Observation of the Quadrupolar Kondo Effect in Dilute Quadrupolar System Pr_xLa_<1-x>Pb_3 for x≦0.052006

    • Author(s)
      T.Kawae 他 6名
    • Journal Title

      Physical Review Letters 96

      Pages: 27210-27210

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Molecular Field and Monte Carlo Study for the Mixed-Spin Axial Next-Nearest-Neighbor Ising Model2006

    • Author(s)
      T.Kasama, Y.Muraoka, T.Idogaki
    • Journal Title

      Physical Review B73

      Pages: 214411-214411

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Specific Heat Study of an S=1/2 Alternating Heisenberg Spin Chain System : F5PNN in a Magnetic Field,2005

    • Author(s)
      Y.Yoshida et al.
    • Journal Title

      Physical Review Letters 94巻・3号

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Unconventional magnetic transitions in the mineral clinoatacamite Cu2Cl(OH)32005

    • Author(s)
      X.G.Zheng et al.
    • Journal Title

      Physical Review B 71巻・5号

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Magnetic ordering in a genuine organic crystal with triangular antiferromagnetic spin units2005

    • Author(s)
      K.Takeda et al.
    • Journal Title

      Physical Review B 72巻・2号

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Coexistence of Long Range Order and Spin Fluctuation in Geometrically Frustrated Clinoatacamite Cu2Cl(OH)32005

    • Author(s)
      X.G.Zheng et al.
    • Journal Title

      Physical Review Letters 95巻・5号

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Low-Temperature Properties in Dilute Quadrupolar Compound PrxLa1-xInAg22005

    • Author(s)
      T.Kawae et al.
    • Journal Title

      Journal of the Physical Society of Japan 74巻・8号

      Pages: 2332-2337

    • NAID

      130004539377

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Specific Heat Study on a Novel Spin-Gapped System : (CH3)2NH2CuCl32005

    • Author(s)
      Y.Yoshida et al.
    • Journal Title

      Journal of the Physical Society of Japan 74巻・11号

      Pages: 2917-2920

    • Related Report
      2005 Annual Research Report

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Published: 2005-04-01   Modified: 2020-05-15  

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