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Development of an integrated numerical tool to predict fate and transport of contaminants in groundwater based on a DNAPL migration model wi10008881th entrapment and residual effect of droplets

Research Project

Project/Area Number 17560483
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Civil and environmental engineering
Research InstitutionSaitama University

Principal Investigator

SATO Kuniaki  Saitama University, Geosphere Research Institute, Professor Emeritus, 地圏科学研究センター, 名誉教授 (10008881)

Co-Investigator(Kenkyū-buntansha) KOMATSU Toshiko  Saitama University, Graduate school of Science and Engineering, Professor, 理工学研究科, 教授 (80034396)
Project Period (FY) 2005 – 2006
Project Status Completed (Fiscal Year 2006)
Budget Amount *help
¥2,600,000 (Direct Cost: ¥2,600,000)
Fiscal Year 2006: ¥1,100,000 (Direct Cost: ¥1,100,000)
Fiscal Year 2005: ¥1,500,000 (Direct Cost: ¥1,500,000)
KeywordsDNAPL / migration model / fingering / Invasion Percolation Theory / soil colloid mobility / diffusion coefficient / air permeability / predictive model of gas transport parameters / groundwater resource management / 土壌コロイド粒子 / コロイド粒子移動特性
Research Abstract

The following five major subjects were investigated in this research
(1) Study on characteristics of parameters governing the entrapment and residual effect of DNAPL droplets in pores
(2) Improvement of prediction accuracy of the DNAPL migration model for contaminant source area in aquifer
(3) Identification of the entrapment and residual parameters in contaminated layers
(4) Development of a numerical simulation tool based on the DNAPL migration model for both saturated and unsaturated areas
(5) Application of the simulation tool with the entrapment and residual parameters to field sites
(1) : It was shown that a parameter for residual DNAPL in soil was related to a macroscopic capillary number and a bond number. The following parameters associated with transport, prediction and remediation of contaminants in soils were obtained. 1) Colloid diffusion in water films was a limiting factor in leaching of soil colloids, which enhance the transport of contaminants. 2) Around 50% of the supplied … More colloids were captured in soil. 3) The velocity of colloids was three to four times higher than that of tracer (Br-). 4) The adsorption of pesticides onto colloids was significantly higher (3x10^3 times higher) than that onto soil. 5) For the gas transport in soils, new prediction models for gas transport parameters that consider soil structure such as air content or pore size distribution were developed. These new models enabled to predict the transport of gaseous contaminants in soils.
(2) : The fingering model based on Invasion Percolation (IP) theory and the random walk model of the DNAPL liquid drop developed in this study were compared and the prediction accuracy of the DNAPL migration model was improved based on the understanding of characteristic of parameter λ.
(3): It was confirmed that the dissolution rate became low even in high velocity condition based on column experiments assuming heterogeneous contaminated soil.
(4): The stochastic model represented by Diffusion Limited Aggregation (DLA) or IP theory and the finite difference method for convection dispersion equation were investigated at void, laboratory and field scale, respectively. The stability of difference scheme and the grid dependency of solution and mass-balance were clarified.
(5): The application of the developed model to field sites was conducted. From the view point of conservation and utilization of healthy groundwater environment, a framework of the groundwater resource management was established. The problems with the numerical methods and its application to groundwater flow analysis based on small- and large-scale hydraulic models were clarified. Less

Report

(3 results)
  • 2006 Annual Research Report   Final Research Report Summary
  • 2005 Annual Research Report
  • Research Products

    (34 results)

All 2007 2006 2005

All Journal Article (34 results)

  • [Journal Article] Gas Transport Parameters Along Field Transects of a Volcanic Ash Soil2007

    • Author(s)
      Resurreccion, A.C., K.Kawamoto, T.Komatsu, P.Moldrup, N.Ozaki, D.E.Rolston
    • Journal Title

      Soil Science Vol.172, No.1

      Pages: 3-16

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Annual Research Report 2006 Final Research Report Summary
  • [Journal Article] Gas Diffusivity and Air Permeability in a Volcanic Ash Soil Profile : Effects of Organic Matter and Water Retention2007

    • Author(s)
      Augustus C.Resurreccion, Ken Kawamoto, Toshiko Komatsu, Per Moldrup, Kuniaki Sato, Dennis E.Rolston
    • Journal Title

      Soil Science (Accepted: Feb.2,2007)

      Pages: 11-11

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] 地下水資源マネージメント2007

    • Author(s)
      佐藤邦明
    • Journal Title

      水循環 貯留と浸透 第63号

      Pages: 5-9

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Annual Research Report 2006 Final Research Report Summary
  • [Journal Article] IP理論にもとづく空隙中DNAPL残存特性の基礎的研究2007

    • Author(s)
      佐々木孝, 佐藤邦明
    • Journal Title

      土木学会水工学論文集 第51巻

      Pages: 505-510

    • NAID

      130003842495

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Annual Research Report 2006 Final Research Report Summary
  • [Journal Article] 地下水中難水溶性物質移行モデルの現地適用における数値手法の課題2007

    • Author(s)
      佐々木孝, 佐藤邦明
    • Journal Title

      日本地下水学会地下水流動解析とモデル化に関するシンポジウム

      Pages: 35-42

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Annual Research Report 2006 Final Research Report Summary
  • [Journal Article] Gas Diffusivity and Air Permeability in a Volcanic Ash Soil Profile : Effects of Organic Matter and Water Retention2007

    • Author(s)
      Augustus C.Resurreccion, Ken Kawamoto, Toshiko Komatsu Per Moldrup, Kuniaki Sato, Dennis E.Rolston
    • Journal Title

      Soil Science (Accepted : Feb.2, 2007)

      Pages: 11-11

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Groundwater resource management2007

    • Author(s)
      SATO, K.
    • Journal Title

      Journal of Hydrological System, Association for rainwater storage and infiltration technology (in Japanese) Vol.63

      Pages: 5-9

    • NAID

      40015357993

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Fundamental study on characteristics of entrapped DNAPL droplets in pores based on Invasion Percolation Theory2007

    • Author(s)
      SASAKI, T., SATO, K.
    • Journal Title

      Annual Journal of Hydraulic Engineering, JSCE (in Japanese) Vol.51

      Pages: 505-510

    • NAID

      130003842495

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Topics on numerical methods in laboratory and field scale of DNAPL migration model in groundwater2007

    • Author(s)
      SASAKI, T., SATO, K.
    • Journal Title

      Proceedings of the symposium on Groundwater hydraulics and modeling, Japanese Association of Groundwater Hydrology (in Japanese)

      Pages: 35-42

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Gas Diffusivity and Air Permeability in a Volcanic Ash Soil Profile : Effects of Organic Matter and Water Retention2007

    • Author(s)
      Augustus C.Resurreccion, Ken Kawamoto, Toshiko Komatsu, Per Moldrup, Kuniaki Sato, Dennis E.Rolston
    • Journal Title

      Soil Science (Accepted : Feb. 2, 2007)

      Pages: 11-11

    • Related Report
      2006 Annual Research Report
  • [Journal Article] 地球化学的モデリングを利用した地下水質解析の紹介-地下水中のヒ素濃度変化の解析を例として-2006

    • Author(s)
      小林滋, 伊藤一正, 佐藤邦明
    • Journal Title

      地下水技術 第48巻・第2号

      Pages: 27-32

    • NAID

      40007176284

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary 2005 Annual Research Report
  • [Journal Article] Colloid and Bromide Transport in Undisturbed Soil Columns : Application of Two-region Model2006

    • Author(s)
      Poulsen, T., P.Moldrup, L.W.de Jonge, T.Komatsu
    • Journal Title

      Vadose Zone Journal No.5

      Pages: 649-656

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Bi-modal probability law model for unified description of water retention, air and water permeability, and gas diffusivity in variably saturated soil2006

    • Author(s)
      Poulsen, T.G., P.Moldrup, S.Yoshikawa, T.Komatsu
    • Journal Title

      Vadose Zone Journal No.5

      Pages: 1119-1128

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Gas Transport Parameters in the Vadose Zone : Gas Diffusivity in Field and Lysimeter Soil Profiles2006

    • Author(s)
      Kawamoto, K., P.Moldrup, P.Schjonning, B.V.Iversen, D.E.Rolston, T.Komatsu
    • Journal Title

      Vadose Zone Journal No.5

      Pages: 1194-1204

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Annual Research Report 2006 Final Research Report Summary
  • [Journal Article] Gas Transport Parameters in the Vadose Zone : Development and Tests of Power-Law Models for Air Permeability2006

    • Author(s)
      Kawamoto, K., P.Moldrup, P.Schjonning, B.V.Iversen, T.Komatsu, D.E.Rolston
    • Journal Title

      Vadose Zone Journal No.5

      Pages: 1205-1215

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] 都市における地下水有効利用の方向性について2006

    • Author(s)
      蛯原雅之, 渡邉暁人, 佐藤邦明
    • Journal Title

      地下水技術 第48巻、第12号

      Pages: 23-30

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Annual Research Report 2006 Final Research Report Summary
  • [Journal Article] IP理論にもとづくDNAPL残存モデルの検証と応用2006

    • Author(s)
      佐々木孝, 佐藤邦明
    • Journal Title

      第12回地下水・土壌汚染とその防止対策に関する研究集会

      Pages: 191-194

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Annual Research Report 2006 Final Research Report Summary
  • [Journal Article] TCE原液の混在する地盤における溶出速度に関する実験的研究2006

    • Author(s)
      増岡健太郎, 下村雅則, 樋口雄一
    • Journal Title

      第12回地下水・土壌汚染とその防止対策に関する研究集会

      Pages: 328-331

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Annual Research Report 2006 Final Research Report Summary
  • [Journal Article] 不均質地盤中での残留DNAPLの溶出モデルに関する研究2006

    • Author(s)
      増岡健太郎, 下村雅則
    • Journal Title

      日本地下水学会2006年秋季講演会講演要旨

      Pages: 156-161

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Annual Research Report 2006 Final Research Report Summary
  • [Journal Article] Application of geochemical modeling method to groundwater quality analysis - Change of arsenic concentration -2006

    • Author(s)
      Kobayashi, S., Ito, K., Sato, K.
    • Journal Title

      Journal of ground water technology (in Japanese) Vol.48 No.2

      Pages: 27-32

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Proposal on new good use of groundwater resource in urban areas2006

    • Author(s)
      Ebihara M., Watanabe, A., Sato, K.
    • Journal Title

      Journal of ground water technology (in Japanese) Vol.48, No.12

      Pages: 23-30

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] On validation and application of an entrapped DNAPL model based on the Invasion Percolation Theory2006

    • Author(s)
      SASAKI, T., SATO, K.
    • Journal Title

      Proceedings of the 12th Symposium on Soil and Groundwater Contamination and Remediation (in Japanese)

      Pages: 191-194

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] An experimental study of DNAPL dissolution in saturated porous media2006

    • Author(s)
      Masuoka, K., Shimomura, M., Higuchi, Y.
    • Journal Title

      Proceedings of the 12th Symposium on Soil and Groundwater Contamination and Remediation (in Japanese)

      Pages: 328-331

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] A study of modeling for residual DNAPL dissolution in heterogeneous porous media2006

    • Author(s)
      Masuoka, K., Shimomura, M.
    • Journal Title

      Proceedings of Autumn Symposium 2006, Japanese Association of Groundwater Hydrology (in Japanese)

      Pages: 156-161

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Golloid and Bromide Transport in Undisturbed Soil Columns : Application of Two-region Model2006

    • Author(s)
      Poulsen, T., P.Moldrup, L.W.de Jonge, T.Komatsu
    • Journal Title

      Vadose Zone Journal No.5

      Pages: 649-656

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Bi-modal probability law model for unified description of water retention, air and water permeability, and gas diffusivity in variably saturate soil2006

    • Author(s)
      Poulsen, T.G., P.Moldrup, S.Yoshikawa, T.Komatsu
    • Journal Title

      Vadose Zone Journal No.5

      Pages: 1119-1128

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Gas Transport Parameters in the Vadose Zone : Development and Tests of Power-Law Models for Air Permeability2006

    • Author(s)
      Kawamoto K., P.Moldrup, P.Schjonning, B.V.Iversen, T.Komatsu, D.E.Rolston
    • Journal Title

      Vadise Zone Journal No.5

      Pages: 1205-1215

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Colloid and Bromide Transport in Undisturbed Soil Columns : Application of Two-region Model2006

    • Author(s)
      Poulsen, T., P.Moldrup, L.W.de Jonge, T.Komatsu
    • Journal Title

      Vadose Zone Journal No.2(in press)

    • Related Report
      2005 Annual Research Report
  • [Journal Article] DNAPL migration analysis by means of a coupled TVD finite difference method with random walk process2005

    • Author(s)
      Sasaki, T., Sato, K., Wada, A., Giri, R.R.
    • Journal Title

      Proceedings of 31th IAHR Congress, Seoul, Korea Vol."Theme C"

      Pages: 2284-2293

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] 差分連成ランダムウォーク法による難水溶性物質の地下水汚染解析2005

    • Author(s)
      佐々木孝, 佐藤邦明, 鈴山宏, 木野由也
    • Journal Title

      第19回数値流体力学シンポジウム

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary 2005 Annual Research Report
  • [Journal Article] Colloid Transport in a Volcanic Ash Soil : A Laboratory Column Experiment2005

    • Author(s)
      Zaman Md.M., K.Kawamoto, T.Komatsu
    • Journal Title

      Proceedings of the Seventh International Summer Symposium, Japan Society of Civil Engineers

      Pages: 161-164

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary 2005 Annual Research Report
  • [Journal Article] DNAPL migration analysis by means of a coupled TVD finite difference method with random walk process2005

    • Author(s)
      Sasaki, T., Sato, K., Wada, A., Giri, R.R.
    • Journal Title

      Proceedings of 31th IAHR Congress (Seoul, Korea) Vol. "Theme C"

      Pages: 2284-2293

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] A coupled TVD finite difference method with random walk model for DNAPL transport in groundwater2005

    • Author(s)
      SASAKI, T., SATO, K., SUZUYAMA, H., KINO, Y.
    • Journal Title

      Proceedings of the 19th Computational Fluid Dynamics Symposium (in Japanese) c4-1

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] DNAPL migration analysis by means of a coupled TVD finite difference method with random walk process2005

    • Author(s)
      Sasaki, T., Sato, K., Wada, A., Giri, R.R.
    • Journal Title

      Proceedings of 31th IAHR Congress, Seoul, Korea, Vol."Theme C"

      Pages: 2284-2293

    • Related Report
      2005 Annual Research Report

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Published: 2005-04-01   Modified: 2016-04-21  

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