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圧力誘起磁気量子相転移と重い電子系超伝導の極低温高圧下NMR/NQR法による研究

Research Project

Project/Area Number 17740225
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeSingle-year Grants
Research Field Condensed matter physics II
Research InstitutionOkayama University (2006-2007)
Osaka University (2005)

Principal Investigator

川崎 慎司  Okayama University, 大学院・自然科学研究科, 講師 (80397645)

Project Period (FY) 2005 – 2007
Project Status Completed (Fiscal Year 2007)
Budget Amount *help
¥3,500,000 (Direct Cost: ¥3,500,000)
Fiscal Year 2007: ¥800,000 (Direct Cost: ¥800,000)
Fiscal Year 2006: ¥800,000 (Direct Cost: ¥800,000)
Fiscal Year 2005: ¥1,900,000 (Direct Cost: ¥1,900,000)
Keywords核磁気共鳴 / 重い電子系 / 異方的超伝導 / 低温 / 高圧 / 量子相転移 / 超伝導
Research Abstract

・重い電子系充填スクッテルダィト化合物PrOs_<4>Sb_<12>の超伝導相図の確立
PrOs_<4>Sb_<12>の超伝導はその4f電子の結晶場励起と密接に関連していることが多くの実験事実から示唆されていた。この結晶場を実験的に制御(加圧)し、超伝導との関連を調べることが期待される。本研究では、インデンター型圧力セルを核磁気共鳴測定に新たに導入し、これまでは微視的測定では到達が困難であった3GPa以上でのSb-NQR測定に成功し、3GPaを超える圧力下でこの物質の結晶場励起に関する情報を世界で初めて報告した。またPrOs_<4>Sb_<12>の超伝導と、結晶場の関係について微視的視点から圧力相図を明らかにした。
・重い電子系反強磁性体Celn_3の圧力相図の確立。
重い電子系超伝導はいわゆる量子臨界点近傍(絶対零度での二次相転移点近傍)で発現することが広く信じられている。本研究では詳細な低温高圧下NQR測定から、重い電子系化合物Celn_3の反強磁性一常磁性量子相転移は一次相転移であることを明らかにし、圧力誘起超伝導はその一次相転移点近傍で誘起される新奇な量子臨界現象を媒介として発現するという、これまでの常識を覆す全く新しい事実を見出した。
・Na_<x>CoO_2・yH_2O超伝導の圧力効果。
層状Co酸化物超伝導体Na_<x>CoO_2・yH_2Oは、同じ3d電子を舞台とする銅酸化物高温超伝導体との系統性からも世界的に注目されている。本研究では低温高圧下NMR/NQR測定からNa_<x>CoO_2・yH_2Oの超伝導の圧力相図を確立し、圧力下におけるこの物質の異方的超伝導と電子相関の関連を世界で初めて明らかにした。

Report

(3 results)
  • 2007 Annual Research Report
  • 2006 Annual Research Report
  • 2005 Annual Research Report
  • Research Products

    (19 results)

All 2008 2007 2006 2005

All Journal Article (16 results) (of which Peer Reviewed: 5 results) Presentation (3 results)

  • [Journal Article] Pressure-induced unconventional superconductivity in the heavy-fermion antiferromagnet CeIn_3: An <115>^In-NQR study under pressure2008

    • Author(s)
      川崎慎司
    • Journal Title

      Physical Review B 77

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Unconventional superconductivity and antiferromagnetic Quantum phase transition in CeRhin_5: <115>^In-NQR study under pewssure2008

    • Author(s)
      八島光晴
    • Journal Title

      Physica B 403

      Pages: 914-916

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Pressure dependence of the superconducting transition and electron correlations in Na_xCoO_2・1.3H_2O2007

    • Author(s)
      草野江里
    • Journal Title

      Phycical Review B 76

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Quantum phase diagram of antiferromagnetism and superconductivity with a tetracritical point in CeRhIn_5 in zero magnetic field2007

    • Author(s)
      八島光晴
    • Journal Title

      Phycical Review B 76

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Experimental evidence for ferromagnetic spin-pairing superconductivity emerging in UGe_2: A <73>^Ge-nuclear-quadrupole study under pressure2007

    • Author(s)
      原田淳之
    • Journal Title

      Physical Review B 75

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Evidence for Point Nodes in the Superconducting Gap Function in the Filled Skutterudite Heavy-Fermion Compound PrOs_4Sb_<12>:^<123>Sb-NQR Study under Pressure2007

    • Author(s)
      片山功多
    • Journal Title

      Journal of the Physical Society of Japan 76

    • Related Report
      2006 Annual Research Report
  • [Journal Article] ^<73>Ge-NQR study of heavy-fermion compound CeNi_2Ge_22007

    • Author(s)
      川崎慎司
    • Journal Title

      Journal of Magnetism and Magnetic Materials 310

      Pages: 590-592

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Novel phase diagram of antiferromagnetism and superconductivity in CeRhIn_52007

    • Author(s)
      八島光晴
    • Journal Title

      Journal of Magnetism and Magnetic Materials 310

      Pages: 322-324

    • Related Report
      2006 Annual Research Report
  • [Journal Article] ^<115>In-NQR study of CeRh_<1-x>Ir_xIn_5 under pressure2007

    • Author(s)
      麦野遥一
    • Journal Title

      Journal of Magnetism and Magnetic Materials 310

      Pages: 584-586

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Enhancing the Superconducting Transition Temperature of CeRh_<1-x>Ir_xln_5 due to the Strong-Coupling Effects of Antiferromagnetic Spin Fluctuations : An ^<115>In Nuclear Quadrupole Resonance Study2006

    • Author(s)
      川崎慎司
    • Journal Title

      Physical Review Letters 96

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Evidence for unconventional superconducting fluctuations in heavy-fermion compound CeNi_2Ge_22006

    • Author(s)
      川崎慎司
    • Journal Title

      Journal of the Physical Society of Japan 75

    • Related Report
      2006 Annual Research Report
  • [Journal Article] ^<115>In-NQR study of antiferromagnetism and superconductivity in CeRhIn_5 and CeIn_3 under pressure2006

    • Author(s)
      川崎慎司
    • Journal Title

      Journal of Physics and Chemistry of Solids (印刷中)

    • Related Report
      2005 Annual Research Report
  • [Journal Article] NMR/NQR experiments on heavy-fermion systems and superconductors2005

    • Author(s)
      北岡良雄
    • Journal Title

      Physica B 359-361

      Pages: 341-341

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Unconventional superconductivity near the antiferromagnetic criticality in CeCoIn_5 : a study of ^<115>In-NQR under pressure2005

    • Author(s)
      八島光晴
    • Journal Title

      Physica B 359-361

      Pages: 404-404

    • Related Report
      2005 Annual Research Report
  • [Journal Article] ^<115>In-NQR study of antiferromagnetism and superconductivity near magnetic criticality in CeIn_32005

    • Author(s)
      川崎慎司
    • Journal Title

      Physica B 359-361

      Pages: 413-413

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Cooperative Phenomenon of Ferromagnetism and Unconventional Superconductivity in UGe_2 : A ^<73>Ge-NQR Study under Pressure2005

    • Author(s)
      原田淳之
    • Journal Title

      Journal of the Physical Society of Japan 74

      Pages: 2675-2675

    • Related Report
      2005 Annual Research Report
  • [Presentation] Bi_2Sr_<2-x>La_xCuO_6における擬ギャップの基底状態の研究(強磁場NMR)2008

    • Author(s)
      川崎慎司
    • Organizer
      日本物理学会 2008年年次大会
    • Place of Presentation
      近畿大学
    • Year and Date
      2008-03-26
    • Related Report
      2007 Annual Research Report
  • [Presentation] Sb-NQR study of PrOs_4Sb_<12> under high pressure2007

    • Author(s)
      川崎慎司
    • Organizer
      International Conference on "New Quantum Phenomena in Skutterudite and Related Systems"
    • Place of Presentation
      神戸大学
    • Year and Date
      2007-09-27
    • Related Report
      2007 Annual Research Report
  • [Presentation] 重い電子系超伝導体PrOs_4Sb_<12>の圧力下Sb-NQRによる研究2007

    • Author(s)
      川崎慎司
    • Organizer
      日本物理学会 中国支部・四国支部 2007 年度 支部学術講演会
    • Place of Presentation
      岡山大学
    • Year and Date
      2007-08-04
    • Related Report
      2007 Annual Research Report

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Published: 2005-04-01   Modified: 2020-05-15  

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