Novel quantum spin liquid states on honeycomb lattice iridium oxides
Project/Area Number |
17H01140
|
Research Category |
Grant-in-Aid for Scientific Research (A)
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Allocation Type | Single-year Grants |
Section | 一般 |
Research Field |
Condensed matter physics II
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Research Institution | The University of Tokyo |
Principal Investigator |
Takagi Hidenori 東京大学, 大学院理学系研究科(理学部), 教授 (40187935)
|
Co-Investigator(Kenkyū-buntansha) |
平岡 奈緒香 (太田奈緒香) 東京大学, 大学院理学系研究科(理学部), 助教 (40758827)
北川 健太郎 東京大学, 大学院理学系研究科(理学部), 講師 (90567661)
|
Project Period (FY) |
2017-04-01 – 2020-03-31
|
Project Status |
Completed (Fiscal Year 2019)
|
Budget Amount *help |
¥44,980,000 (Direct Cost: ¥34,600,000、Indirect Cost: ¥10,380,000)
Fiscal Year 2019: ¥9,490,000 (Direct Cost: ¥7,300,000、Indirect Cost: ¥2,190,000)
Fiscal Year 2018: ¥18,460,000 (Direct Cost: ¥14,200,000、Indirect Cost: ¥4,260,000)
Fiscal Year 2017: ¥17,030,000 (Direct Cost: ¥13,100,000、Indirect Cost: ¥3,930,000)
|
Keywords | 量子スピン液体 / Kitaev模型 / 量子磁性 / Ir酸化物 / 強相関電子系 / キタエフ模型 / ハニカム構造 / キタエフ系 / イリジウム酸化物 / エキシトニック磁性 / 中性子回折 / 核磁気共鳴 |
Outline of Final Research Achievements |
Realization of quantum spin liquid is one of the grand challenges in condensed matter physics. A quantum spin liquid on honeycomb lattice theoretically discovered by Kitaev has been attracting considerable interests among the condensed matter scientists as it is obtained as the exact solution comprising of two kinds of Majorana fermions, itinerant and localized. In the honeycomb oxide H3LiIr2O6, we discovered that the interacting spin-orbital-entangled Jeff=1/2 moments do not show any signature of magnetic ordering, namely spontaneous symmetry breaking down to an extremely low temperature, which lead us to conclude the realization of a quantum spin liquid state.
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Academic Significance and Societal Importance of the Research Achievements |
Kitaevの理論模型に触発された量子スピン液体状態の実験的探索は世界的規模で研究が進んでいる。その舞台として当初提案された他のIr酸化物やRu塩化物では、いずれも量子スピン液体ではなく長距離磁気秩序の発現が観測されている。現実の物質での実現は不可能であるとも言われた。そのような状況の中でH3LiIr2O6に実験的に量子スピン液体の存在が確認されたことの意義は極めて大きい。さらに、この発見が液体状態発現の微視的起源、特にKitaev相互作用の役割や水素の役割など、新たな極めて挑戦的課題を投げかけていることも強調されるべきである。
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Report
(4 results)
Research Products
(127 results)
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[Journal Article] Lattice dynamics and structural transition of the hyperhoneycomb iridate $\ensuremath{\beta}\ensuremath{-}{\mathrm{Li}}_{2}{\mathrm{IrO}}_{3}$ investigated by high-pressure Raman scattering2020
Author(s)
S. Choi, H.-S. Kim, H.-H. Kim, A. Krajewska, G. Kim, M. Minola, T. Takayama, H. Takagi, K. Haule, D. Vanderbilt, B. Keimer
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Journal Title
Phys. Rev. B
Volume: 101
Issue: 5
DOI
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[Journal Article] Spin-orbit-controlled metal-insulator transition in Sr 2 IrO 42020
Author(s)
B. Zwartsenberg, R. P. Day, E. Razzoli, M. Michiardi, N. Xu, M. Shi, J. D. Denlinger, G. Cao, S. Calder, K. Ueda, J. Bertinshaw, H. Takagi, B. J. Kim, I. S. Elfimov, A. Damascelli
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Journal Title
Nat. Phys.
Volume: 16
Issue: 3
Pages: 290-294
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[Journal Article] Black Current: Structure, Characterization, and Optoelectronic Properties of Ce3Cl3[MoO6]2019
Author(s)
K. V. Dorn, B. Blaschkowski, H. Bamberger, J. van Slageren, K. Doll, R. Claus, Y. Matsumoto, H. Takagi, I. Hartenbach
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Journal Title
Chemistry - A European Journal
Volume: 25
Issue: 33
Pages: 7921-7926
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[Journal Article] Giant thermal Hall conductivity in the pseudogap phase of cuprate superconductors2019
Author(s)
G. Grissonnanche, A. Legros, S. Badoux, E. Lefrancois, V. Zatko, M. Lizaire, F. Laliberte, A. Gourgout, J.-S. Zhou, S. Pyon, T. Takayama, H. Takagi, S. Ono, N. Doiron-Leyraud, L. Taillefer
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Journal Title
Nature
Volume: 571
Issue: 7765
Pages: 376-380
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[Journal Article] Superconductivity at 4.8 K and Violation of Pauli Limit in La2IRu2 Comprising Ru Honeycomb Layer2019
Author(s)
H. Ishikawa, U. Wedig, J. Nuss, R. K. Kremer, R. Dinnebier, M. Blankenhorn, M. Pakdaman, Y. Matsumoto, T. Takayama, K. Kitagawa, H. Takagi
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Journal Title
Inorg. Chem.
Volume: 58
Issue: 19
Pages: 12888-12894
DOI
NAID
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[Journal Article] Valence-bond insulator in proximity to excitonic instability2019
Author(s)
Y. Chiba, T. Mitsuoka, N. L. Saini, K. Horiba, M. Kobayashi, K. Ono, H. Kumigashira, N. Katayama, H. Sawa, M. Nohara, Y. F. Lu, H. Takagi, T. Mizokawa
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Journal Title
Physical Review B
Volume: 100
Issue: 24
Pages: 245129-245129
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[Journal Article] Inverse-perovskites A3BO (A = Sr, Ca, Eu/B = Pb, Sn): A platform for control of Dirac and Weyl Fermions2019
Author(s)
A. W. Rost, J. Kim, S. Suetsugu, V. Abdolazimi, K. Hayama, J. A. N. Bruin, C. Muehle, K. Kitagawa, A. Yaresko, J. Nuss, H. Takagi
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Journal Title
APL Materials
Volume: 7
Issue: 12
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[Journal Article] Three-Dimensional Fermi Surface of Overdoped La-Based Cuprates2018
Author(s)
Horio M.、Hauser K.、Sassa Y.、Mingazheva Z.、Sutter D.、Kramer K.、Cook A.、Nocerino E.、Forslund O.K.、Tjernberg O.、Kobayashi M.、Chikina A.、Schroeter N.B.M.、Krieger J.A.、Schmitt T.、Strocov V.N.、Pyon S.、Takayama T.、Takagi H.、et al.
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Journal Title
Physical Review Letters
Volume: 121
Issue: 7
Pages: 077004-077004
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[Journal Article] Photo-induced semimetallic states realised in electron-hole coupled insulators2018
Author(s)
Kozo Okazaki, Yu Ogawa, Takeshi Suzuki, Takashi Yamamoto, Takashi Someya, Shoya Michimae, Mari Watanabe, Yangfan Lu, Minoru Nohara, Hidenori Takagi, Naoyuki Katayama, Hiroshi Sawa, Masami Fujisawa, Teruto Kanai, Nobuhisa Ishii, Jiro Itatani, Takashi Mizokawa, Shik Shin
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Journal Title
Nature Communications
Volume: 9:4322
Issue: 1
Pages: 1-6
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[Journal Article] Pseudogap temperature T* of cuprate superconductors from the Nernst effect2018
Author(s)
O. Cyr-Choiniere, R. Daou, F. Laliberte, C. Collignon, S. Badoux, D. LeBoeuf, J. Chang, B. J. Ramshaw, D. A. Bonn, W. N. Hardy, R. Liang, J.-Q. Yan, J.-G. Cheng, J.-S. Zhou, J. B. Goodenough, S. Pyon, T. Takayama, H. Takagi, N. Doiron-Leyraud, L. Taillefer
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Journal Title
Phys. Rev. B
Volume: 97
Issue: 6
DOI
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[Journal Article] Long-range interactions in the effective low-energy Hamiltonian of Sr2IrO4: A core-to-core resonant inelastic x-ray scattering study2017
Author(s)
S. Agrestini, C.-Y. Kuo, M. Moretti Sala, Z. Hu, D. Kasinathan, K.-T. Ko, P. Glatzel, M. Rossi, J.-D. Cafun, K. O. Kvashnina, A. Matsumoto, T. Takayama, H. Takagi, L. H. Tjeng, M. W. Haverkort
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Phys. Rev. B
Volume: 95
Issue: 20
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[Journal Article] Pulsed laser deposition for the synthesis of monolayer WSe22017
Author(s)
A. Mohammed, H. Nakamura, P. Wochner, S. Ibrahimkutty, A. Schulz, K. Mueller, U. Starke, B. Stuhlhofer, G. Cristiani, G. Logvenov, H. Takagi
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Journal Title
Appl. Phys. Lett.
Volume: 111
Issue: 7
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[Journal Article] Ultrafast Electronic Band Gap Control in an Excitonic Insulator2017
Author(s)
S. Mor, M. Herzog, D. Golez, P. Werner, M. Eckstein, N. Katayama, M. Nohara, H. Takagi, T. Mizokawa, C. Monney, J. Staehler
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Journal Title
Phys. Rev. Lett.
Volume: 119
Issue: 8
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[Journal Article] Pressure tuning of bond-directional exchange interactions and magnetic frustration in the hyperhoneycomb iridate β-Li2IrO32017
Author(s)
L. S. I. Veiga, M. Etter, K. Glazyrin, F. Sun, C. A. Escanhoela, G. Fabbris, J. R. L. Mardegan, P. S. Malavi, Y. Deng, P. P. Stavropoulos, H.-Y. Kee, W. G. Yang, M. van Veenendaal, J. S. Schilling, T. Takayama, H. Takagi, D. Haskel
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Phys. Rev. B
Volume: 96
Issue: 14
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[Journal Article] Pseudogap phase of cuprate superconductors confined by Fermi surface topology2017
Author(s)
N. Doiron-Leyraud, O. Cyr-Choiniere, S. Badoux, A. Ataei, C. Collignon, A. Gourgout, S. Dufour-Beausejour, F. F. Tafti, F. Laliberte, M.-E. Boulanger, M. Matusiak, D. Graf, M. Kim, J.-S. Zhou, N. Momono, T. Kurosawa, H. Takagi, L. Taillefer
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Nat. Commun.
Volume: 8
Issue: 1
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[Presentation] 周波数領域角度分解光電子分光法によるTa2NiSe5における光誘起絶縁体金属転移の研究(理論)2019
Author(s)
篠原康, 鈴木剛, 魯楊帆, 渡邉真莉, 徐佳笛, 高木英典, 野原実, 片山尚幸, 澤博, 藤澤正美, 金井輝人, 石井順久, 板谷治郎, 溝川貴司, 岡﨑浩三, 辛埴, 石川顕一
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日本物理学会2019年秋季大会
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[Presentation] 周波数領域角度分解光電子分光法によるTa2NiSe5における光誘起絶縁体金属転移の研究(実験)2019
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[Presentation] 励起子絶縁体Ta2Ni1-xCoxSe5の時間分解光電子分光2019
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