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Solid phase film formation of polymer/ceramic compound particles by hetero-structure control and comprehensive analysis of film formation mechanisms

Research Project

Project/Area Number 17H01235
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field Materials/Mechanics of materials
Research InstitutionTohoku University

Principal Investigator

OGAWA Kazuhiro  東北大学, 工学研究科, 教授 (50312616)

Co-Investigator(Kenkyū-buntansha) 鈴木 研  東北大学, 工学研究科, 准教授 (40396461)
CAVAILLE JY  東北大学, 高等研究機構等, 客員教授 (40794623)
市川 裕士  東北大学, 工学研究科, 准教授 (80451540)
Project Period (FY) 2017-04-01 – 2020-03-31
Project Status Completed (Fiscal Year 2019)
Budget Amount *help
¥44,720,000 (Direct Cost: ¥34,400,000、Indirect Cost: ¥10,320,000)
Fiscal Year 2019: ¥9,360,000 (Direct Cost: ¥7,200,000、Indirect Cost: ¥2,160,000)
Fiscal Year 2018: ¥14,170,000 (Direct Cost: ¥10,900,000、Indirect Cost: ¥3,270,000)
Fiscal Year 2017: ¥21,190,000 (Direct Cost: ¥16,300,000、Indirect Cost: ¥4,890,000)
Keywordsコールドスプレー / ヘテロ構造制御 / ポリマー / ナノセラミック / 固相成膜 / 成膜メカニズム / セラミックス / 超高分子量ポリエチレン / ナノセラミックス / 複合粒子 / フッ素系樹脂 / 成膜 / ヘテロ構造
Outline of Final Research Achievements

By combining active nano-ceramic particles with a polymer, we succeeded in forming a solid state coatings by cold spray technique without melting the particles. The particle deposition mechanism was elucidated and its interfacial strength was evaluated by experimental approach and numerical simulation, and it was clarified that the hydroxyl groups on the surface of nano-ceramic particles are effective. Regarding this mechanism, it is considered that the hydroxyl groups on the particle surface promote hydrogen bonding and are chemically bonded.

Academic Significance and Societal Importance of the Research Achievements

これまでに固相成膜が困難であったポリマー材料に関し,金属成膜が主であったコールドスプレー法と呼ばれる成膜技術および活性なナノセラミックス粒子を応用することで,大気中で簡便に厚膜の形成に成功した.ポリマー材料は熱により,酸化等の劣化が考えられるが,このような劣化を回避し,厚膜形成できることは,耐食性,耐摩耗性,絶縁性の付与を必要とする多くの機器・構造物への応用が期待できる.また,粒子付着メカニズムの検討から,水酸基を表面に有するナノセラミックスが水素結合を促し,ポリマー同士の接合を可能にした点は極めて新しい知見である.

Report

(4 results)
  • 2019 Annual Research Report   Final Research Report ( PDF )
  • 2018 Annual Research Report
  • 2017 Annual Research Report

Research Products

(29 results)

All 2019 2018 2017 Other

All Int'l Joint Research (4 results) Journal Article (6 results) (of which Int'l Joint Research: 4 results,  Peer Reviewed: 6 results,  Open Access: 1 results) Presentation (17 results) (of which Int'l Joint Research: 13 results,  Invited: 5 results) Book (2 results)

  • [Int'l Joint Research] INSA-Lyon(フランス)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] 西安交通大学(中国)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] INSA-Lyon(フランス)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] INSA-Lyon/Ecole Centrale de Lyon(フランス)

    • Related Report
      2017 Annual Research Report
  • [Journal Article] Fabrication of micro-/nano-structured super-hydrophobic fluorinated polymer coatings by cold-spray2019

    • Author(s)
      Ravi Kesavan、Sulen Wesley Lock、Bernard Chrystelle、Ichikawa Yuji、Ogawa Kazuhiro
    • Journal Title

      Surface and Coatings Technology

      Volume: 373 Pages: 17-24

    • DOI

      10.1016/j.surfcoat.2019.05.078

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Influence of nanoceramic interlayer on polymer consolidation during cold-spray coating formation2019

    • Author(s)
      Ravi Kesavan、Deplancke Tiana、Lame Olivier、Ogawa Kazuhiro、Cavaill? Jean-Yves、Dalmas Florent
    • Journal Title

      Journal of Materials Processing Technology

      Volume: 273 Pages: 116254-116254

    • DOI

      10.1016/j.jmatprotec.2019.116254

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Effects of nano-ceramic particle addition for cold sprayed fluoropolymer coatings2019

    • Author(s)
      Lock Sulen, W., Ravi, K., Bernard, C., Mary, N., Ichikawa, Y., Ogawa, K.
    • Journal Title

      Key Engineering Materials

      Volume: 813 Pages: 141-146

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Elucidation of cold-spray deposition mechanism by auger electron spectroscopic evaluation of bonding interface oxide film2019

    • Author(s)
      Ichikawa Yuji、Tokoro Ryotaro、Tanno Masatoshi、Ogawa Kazuhiro
    • Journal Title

      Acta Materialia

      Volume: 164 Pages: 39-49

    • DOI

      10.1016/j.actamat.2018.09.041

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Understanding deposition mechanism in cold sprayed ultra high molecular weight polyethylene coatings on metals by isolated particle deposition method2018

    • Author(s)
      Kesavan Ravi, Tiana Deplancke, Kazuhiro Ogawa, Jean-Yves Cavaille, Olivier Lame
    • Journal Title

      Additive Manufacturing

      Volume: 21 Pages: 191-200

    • DOI

      10.1016/j.addma.2018.02.022

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] コールドスプレー法によるポリマー皮膜におけるマイクロ・ナノ接合2017

    • Author(s)
      小川和洋
    • Journal Title

      Journal of the Vacuum Society of Japan

      Volume: 60 Pages: 187-192

    • NAID

      130005118503

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Presentation] The Role of the Interfacial Oxide film on Cold Spayed Particle Deposition at the Interface Between an Aluminum Particle and an YSZ Ceramic Substrate2019

    • Author(s)
      Kazuhiro OGAWA
    • Organizer
      2nd Global Forum on Advanced Materials and Technologies for Sustainable Development (GFMAT-2)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Possibility of Repair and Preventive Coatings Using Cold Spray Technique2019

    • Author(s)
      Kazuhiro OGAWA
    • Organizer
      International Symposium on Material Service Performance in Nuclear Power Plants 2019
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Influence of Surface Oxide Film on Surface Activate Bonding for Dissimilar Metallic Materials2019

    • Author(s)
      Kazuhiro OGAWA
    • Organizer
      Visual-JW 2019 & WSE 2019
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Development of fluoropolymer coating using low pressure cold spray2019

    • Author(s)
      W.L.Sulen, K.Ravi, Y.Ichikawa, K.Ogawa
    • Organizer
      International Thermal Spray Conference 2019
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Effects of Nano-Ceramic Particle Addition for Cold Sprayed Fluoropolymer Coatings2019

    • Author(s)
      W.L.Sulen, K.Ravi, C.Bernard, N.Mary, Y.Ichikawa, K.Ogawa
    • Organizer
      33rd Conference on Surface Modification Technologies
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Nano-ceramic particle effect on Flourinated Ethylene Propylene (FEP) coating using Low Pressure Cold Spray2019

    • Author(s)
      LOCK SULENWESLEY ANAK, Kazuhiro Ogawa, Yuji Ichikawa, Kesavan Ravi
    • Organizer
      未踏科学技術協会 第28回インテリジェント・ナノ材料シンポジウム
    • Related Report
      2018 Annual Research Report
  • [Presentation] Ceramic and Polymer Coatings by Cold Spray Technique2018

    • Author(s)
      Kazuhiro Ogawa
    • Organizer
      THERMEC 2018
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Thermomechanical modelling of cold-spray process: Application to Ultra-High Molecular Polyethylene2018

    • Author(s)
      C.A. Bernard, K. Ogawa, J.-Y. Cavaille, O. Lame, K. Ravi, T. Deplancke
    • Organizer
      International Thermal Spray Conference ITSC2018
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Investigation of the Flow Field Dynamics during Polymer Coating by Cold-Spray2018

    • Author(s)
      C.A. Bernard, H. Takana, K. Ravi, O. Lame, K. Ogawa, J.-Y. Cavaille
    • Organizer
      ICFD2018
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] High Strain Rate Sensitivity of Ultra-High Molecular Weight Polyethylene and its Consequence on Cold-Spray Deposition Behavior2018

    • Author(s)
      Kesavan Ravi, Kazuhiro Ogawa, Tiana Deplancke, Olivier Lame, Jean-Yves Cavaille
    • Organizer
      International Thermal Spray Conference ITSC2018
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] レーザーテクスチャリング処理による コールドスプレー皮膜の成膜効率改善2018

    • Author(s)
      高思源,市川裕士,小川和洋
    • Organizer
      日本溶射学会2018年度春季全国講演大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Development of Cold Sprayed GaN Coatings2018

    • Author(s)
      S.Zhou, B.Chrystelle, K.Ravi, Y.Ichikawa, K.Ogawa
    • Organizer
      日本溶射学会2018年度秋季全国講演大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Development of High Functional Polymer Metal Integrated Systems2018

    • Author(s)
      Wesley Anak Lock Sulen, Siyuan Gao, Kesavan Ravi, Kazuhiro Ogawa
    • Organizer
      The 15th Challenge Cup National Undergraduate Extracurricular Academic Science and Technology Contest、The Belt and Road International Special Event Contest of CEFC CHINA ENERGY COMPANY LIMITED
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] コールドスプレー法を利用した高耐熱高分子皮膜の開発2018

    • Author(s)
      高橋 迪大,市川 裕士,小川和洋
    • Organizer
      日本機械学会東北学生会 第48回学生員卒業研究発表講演会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Thermomechanical modelling of High Molecular Weight semi-crystalline polymers2018

    • Author(s)
      C. A. Bernard, T. Deplancke, O. Lame, K. Ogawa, J.-Y. Cavaille
    • Organizer
      ELyT Workshop 2018
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Inter-Particle Sintering of UHMWPE-FNA Nano-Composites Under Different Interfacial Loading Conditions2017

    • Author(s)
      Kesavan Ravi, Olivier Lame, Kazuhiro Ogawa, Jean-Yves Cavaille, Tiana Deplancke, Chrystelle Bernard
    • Organizer
      Fourth International Symposium on Smart Layered Materials and Structures for Energy Saving
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Molecular Simulation Analysis for Adhesion Mechanisms Involved in Polyethylene Processed by Cold Spray2017

    • Author(s)
      Yukie Ishizawa, Kenji Inaba, Ryuji Miura, Ai Suzuki, Naoto Miyamoto, Nozomu Hatakeyama, Akira Miyamoto , Kazuhiro Ogawa, Chrystelle Bernard, Jean-Yves Cavaille, Olivier Lame, Kesavan Ravi
    • Organizer
      Fourth International Symposium on Smart Layered Materials and Structures for Energy Saving
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Book] 多次元アディティブ・マニュファクチャリング2018

    • Author(s)
      小川和洋,他
    • Total Pages
      188
    • Publisher
      日本溶接協会
    • ISBN
      9784907200084
    • Related Report
      2018 Annual Research Report
  • [Book] 多次元アディティブ・マニュファクチャリング2018

    • Author(s)
      小川和洋 他13名
    • Total Pages
      188
    • Publisher
      日本溶接協会
    • Related Report
      2017 Annual Research Report

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Published: 2017-04-28   Modified: 2022-01-27  

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