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A self-regenerable particulate matter sensor using active oxygen

Research Project

Project/Area Number 17H01895
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Environmental engineering and reduction of environmental burden
Research InstitutionNagoya University

Principal Investigator

Hibino Takashi  名古屋大学, 環境学研究科, 教授 (10238321)

Project Period (FY) 2017-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2020)
Budget Amount *help
¥17,030,000 (Direct Cost: ¥13,100,000、Indirect Cost: ¥3,930,000)
Fiscal Year 2020: ¥3,120,000 (Direct Cost: ¥2,400,000、Indirect Cost: ¥720,000)
Fiscal Year 2019: ¥3,120,000 (Direct Cost: ¥2,400,000、Indirect Cost: ¥720,000)
Fiscal Year 2018: ¥5,590,000 (Direct Cost: ¥4,300,000、Indirect Cost: ¥1,290,000)
Fiscal Year 2017: ¥5,200,000 (Direct Cost: ¥4,000,000、Indirect Cost: ¥1,200,000)
Keywordsパティキュレートマター / センシング / 排ガス浄化 / 環境浄化 / 環境分析 / 触媒プロセス / エネルギー / 環境技術 / 触媒・化学プロセス
Outline of Final Research Achievements

In the present technology, a small-sized all-solid-state sensor is installed in the exhaust manifold of a diesel vehicle to instantly measure the PM concentration in the exhaust gas. Specifically, an electrochemical device, consisting of a proton conducting electrolyte and an electrode catalyst, is operated through the following processes: (1) active oxygen species are electrochemically produced in the exhaust gas; (2) the PM is oxidized by the active oxygen with 100% efficiency; (3) a large electrical signal is generated in the process of (2). This sensor enables continuous monitoring of PM, which is not possible for sensors reported so far, because it has self-regeneration ability.

Academic Significance and Societal Importance of the Research Achievements

活性酸素を in-situ で生成し、積極的に活用する化学センサの開発は革新的であり、しかも検知極に自己浄化能力を付与する技術はこれまでにない発想である。それ故、その他の PM センサと異なり、被検物をリアルタイムで連続的にモニタすることが可能になった(独創的な点)。ディーゼル車は大型車を中心に普及しており、PM センサは排ガス制御システムに不可欠な部品である(経済的意義)。しかも、PM が人体に与える影響は大であるので、そのような PM を完全に除去できれば、大気・都市環境の改善にも貢献できる。

Report

(5 results)
  • 2020 Annual Research Report   Final Research Report ( PDF )
  • 2019 Annual Research Report
  • 2018 Annual Research Report
  • 2017 Annual Research Report
  • Research Products

    (21 results)

All 2021 2020 2019 2018 2017 Other

All Int'l Joint Research (2 results) Journal Article (12 results) (of which Int'l Joint Research: 3 results,  Peer Reviewed: 12 results,  Open Access: 6 results) Presentation (7 results) (of which Int'l Joint Research: 2 results,  Invited: 1 results)

  • [Int'l Joint Research] 中国海洋大学(中国)

    • Related Report
      2020 Annual Research Report
  • [Int'l Joint Research] 中国海洋大学(中国)

    • Related Report
      2019 Annual Research Report
  • [Journal Article] Solid oxide fuel cell using municipal solid waste directly as fuel: biomass, resin, plastic, and food waste2021

    • Author(s)
      Takashi Hibino, Kazuyo Kobayashi, Shinya Teranishi, Takuma Hitomi
    • Journal Title

      ACS Sustainable Chemistry & Engineering

      Volume: 9 Issue: 8 Pages: 3124-3136

    • DOI

      10.1021/acssuschemeng.0c07657

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Ionic conductive and photocatalytic properties of cementitious materials: calcium silicate hydrate and calcium aluminoferrite2020

    • Author(s)
      Masahiro Nagao, Kazuyo Kobayashi, Yongcheng Jin, Ippei Maruyama, Takashi Hibino
    • Journal Title

      Journal of Materials Chemistry A

      Volume: 8 Issue: 30 Pages: 15157-15166

    • DOI

      10.1039/d0ta04866f

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Fuel cell and electrolyzer using plastic waste directly as fuel2020

    • Author(s)
      Tetsuya Hori, Kazuyo Kobayashi, Shinya Teranishi, Masahiro Nagao, Takashi Hibino
    • Journal Title

      Waste Management

      Volume: 102 Pages: 30-39

    • DOI

      10.1016/j.wasman.2019.10.019

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] A cellulose electrolysis cell with metal-free carbon electrodes2020

    • Author(s)
      Yaorong Li, Masahiro Nagao, Kazuyo Kobayashi, Yongcheng Jin, Takashi Hibino
    • Journal Title

      Catalysts

      Volume: 10 Issue: 1 Pages: 106-106

    • DOI

      10.3390/catal10010106

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Humidity driven transition from insulator to ionic conductor in Portland cement2019

    • Author(s)
      Masahiro Nagao, Kazuyo Kobayashi, Tetsuya Hori, Yaorong Li, Takashi Hibino
    • Journal Title

      Materials

      Volume: 12 Issue: 22 Pages: 3701-3701

    • DOI

      10.3390/ma12223701

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Electrolysis of humidified methane to hydrogen and carbon dioxide at low temperatures and voltages2019

    • Author(s)
      Tetsuya Hori, Qiang Ma, Kazuyo Kobayashi, Masahiro Nagao, Shinya Teranishi, Takashi Hibino
    • Journal Title

      International Journal of Hydrogen Energy

      Volume: 44 Issue: 5 Pages: 2454-2460

    • DOI

      10.1016/j.ijhydene.2018.12.044

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Efficient Hydrogen Production by Direct Electrolysis of Waste Biomass at Intermediate Temperatures2018

    • Author(s)
      Takashi Hibino, Kazuyo Kobayashi, Masaya Ito, Qiang Ma, Masahiro Nagao, Mai Fukui, Shinya Teranishi
    • Journal Title

      ACS Sustainable Chemistry & Engineering

      Volume: 6 Issue: 7 Pages: 9360-9368

    • DOI

      10.1021/acssuschemeng.8b01701

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Direct electrolysis of waste newspaper for sustainable hydrogen production: an oxygen-functionalized porous carbon anode2018

    • Author(s)
      Takashi Hibino, Kazuyo Kobayashi, Masaya Ito, Masahiro Nagao, Mai Fukui, Shinya Teranishi
    • Journal Title

      Applied Catalysis B : Environmental

      Volume: 231 Pages: 191-199

    • DOI

      10.1016/j.apcatb.2018.03.021

    • Related Report
      2018 Annual Research Report 2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Intermediate-temperature electrolysis of energy grass Miscanthus sinensis for sustainable hydrogen production2018

    • Author(s)
      Masaya Ito, Tetsuya Hori, Shinya Teranishi, Masahiro Nagao, Takashi Hibino
    • Journal Title

      Scientific Reports

      Volume: 8 Issue: 1 Pages: 16186-16186

    • DOI

      10.1038/s41598-018-34544-y

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] NOx sensing characteristics of semiconductor gas sensors under controlled oxygen activity conditions using a proton-conducting electrolyte2017

    • Author(s)
      Masahiro Nagao, Kazuyo Kobayashi, Peiling Lv, Shinya Teranishi, Takashi Hibino
    • Journal Title

      Journal of The Electrochemical Society

      Volume: 164 Issue: 9 Pages: B397-B402

    • DOI

      10.1149/2.0361709jes

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Hydrogen production by direct Lignin electrolysis at intermediate temperatures2017

    • Author(s)
      Takashi Hibino, Kazuyo Kobayashi, Masahiro Nagao, Shinya Teranishi
    • Journal Title

      ChemElectroChem

      Volume: 4 Issue: 9 Pages: 3032-3036

    • DOI

      10.1246/bcsj.20170163

    • NAID

      130006077916

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Hydrogen production by direct Lignin electrolysis at intermediate temperatures2017

    • Author(s)
      Takashi Hibino, Kazuyo Kobayashi, Masahiro Nagao, Shinya Teranishi
    • Journal Title

      ChemElectroChem

      Volume: 4 Issue: 12 Pages: 3032-3036

    • DOI

      10.1002/celc.201700917

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Presentation] Direct conversion of plastic wastes into electricity in an intermediate-temperature fuel cell2019

    • Author(s)
      Tetsuya Hori, Shiya Teranishi, Masahiro Nagao, Takashi Hibino
    • Organizer
      APCChE 2019
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 廃棄プラスチックを直接使用した燃料電池発電2019

    • Author(s)
      堀 哲也,伊藤雅哉,寺西真哉,長尾征洋,日比野高士
    • Organizer
      電気化学会第86回大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 廃棄バイオマスの直接電解による水素生成2019

    • Author(s)
      寺西真哉,堀 哲也,伊藤雅哉,長尾征洋,日比野高士
    • Organizer
      電気化学会第86回大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 草本およびその構成成分の直接電解による水素生成と電気化学特性評価2018

    • Author(s)
      伊藤雅哉,堀 哲也,寺西真哉,長尾征洋,日比野高士
    • Organizer
      第49回中部化学関係学協会支部連合秋季大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] バイオマスの電解による水素生成2018

    • Author(s)
      長尾征洋、伊藤雅哉、呂佩玲、小林和代、福井舞、日比野高士
    • Organizer
      電気化学会第85回大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Direct biomass fuel cell using wood sawdust and pulp as fuels at intermediate temperature2017

    • Author(s)
      Masahiro Nagao, Takashi Hibino, Kazuyo Kobayashi, Peiling Lv, Shinya Teranishi, Toshiyuki Mori
    • Organizer
      IUMRS-LCAM2017
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Electrochemical Reaction of Nano-Carbons for PM Monitoring in Diesel Engine Exhaust2017

    • Author(s)
      Masaya Ito, Peiling Lv, Masahiro Nagao, Kazuyo Kobayashi, Yanbai Shen, Takashi Hibino
    • Organizer
      ICMaSS2017
    • Related Report
      2017 Annual Research Report

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Published: 2017-04-28   Modified: 2022-01-27  

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